Shedding Light on (Anti-)nuclei Production with Pion-Nucleus Femtoscopy
High-energy nuclear collisions provide a unique environment for synthesizing both nuclei and antinuclei (such as $\bar{d}$ and $^4\overline{\text{He}}$) at temperatures ($k_BT\sim100$ MeV) much higher than their binding energies per nucleon of a few MeV. The underlying production mechanism, whether through statistical hadronization, nucleon coalescence, or dynamical regeneration and disintegration, remains unsettled. Here we address this question using pion-nucleus femtoscopy. By solving relativistic kinetic equations for pion-catalyzed reactions ($πNN \leftrightarrow πd$) for deuteron production and including final-state $p-$wave scatterings derived from an established effective interaction, we successfully reproduce the resonance peaks of both $π^+-p$ and $π^+-d$ femtoscopic correlations observed in $pp$ collisions at $\sqrt{s} = 13~\mathrm{TeV}$. The interplay between $Δ$ resonance and $p$-wave scatterings shifts both correlation peaks downward by about $70\text{ MeV}$ relative to vacuum $Δ$ decay. Conversely, both the nucleon coalescence model and the statistical hadronization model significantly underestimate the data and produce additional dips that are absent from the data. These results provide compelling evidence that pion-catalyzed reactions play a dominant role in the production of light (anti-)nuclei in high-energy nuclear collisions and cosmic rays.