arXiv subjects

Qiangwei Yin

Publications and source records attributed to Qiangwei Yin.

33 records · Page 2Linked to original sources

arXiv2021

Quantum transport evidence of topological band structures of kagome superconductor CsV3Sb5

We report the transport properties of kagome superconductor CsV$_{3}$Sb$_{5}$ single crystals at magnetic field up to 32 T. The Shubnikov de Haas (SdH) oscillations emerge at low temperature and four frequencies of $F_α=$ 27 T, $F_β=$ 73 T, $F_ε=$ 727 T, and $F_η=$ 786 T with relatively small cyclotron masses are observed. For $F_β$ and $F_ε$, the Berry phases are close to $π$, providing a clear evidence of nontrivial topological band structures of CsV$_{3}$Sb$_{5}$. Furthermore, the consistence between theoretical calculations and experimental results implies that these frequencies can be assigned to the Fermi surfaces locating near the boundary of Brillouin zone and confirms that the structure with an inverse Star of David distortion could be the most stable structure at charge density wave state. These results will shed light on the nature of correlated topological physics in kagome material CsV$_{3}$Sb$_{5}$.

cond-mat.supr-con↗

arXiv2021

Pressure-induced superconductivity in itinerant antiferromagnet CrB2

The recent discovery of superconductivity up to 32 K in the pressurized MoB2 revives the interests in exploring novel superconductors in transition-metal diborides isostructural to MgB2. Although the Mo 4d-electrons participate in Cooper pairing, the electron-phonon coupling remains the dominant mechanism for the emergence of superconductivity in MoB2. To explore possible superconductivity driven by unconventional pairing mechanism, we turn our attention to an itinerant antiferromagnet CrB2. Here we report on the discovery of superconductivity up to 7 K in CrB2 via the application of external pressure. Superconductivity is observed after the antiferromagnetic transition at TN ~ 88 K under ambient pressure is completely suppressed. Then, the superconducting Tc increases monotonically with pressure and this evolution takes place without a structural transition in the sample. Since the proximity of superconductivity to an antiferromagnetic order, the quantum criticality and unconventional superconductivity may exist in CrB2. Current study would promote further studies and explorations of novel superconductors in other transition-metal diborides.

cond-mat.supr-con↗

arXiv2021

Roton pair density wave and unconventional strong-coupling superconductivity in a topological kagome metal

The transition-metal kagome lattice materials host frustrated, correlated, and topological quantum states of matter. Recently, a new family of vanadium-based kagome metals AV3Sb5 (A=K, Rb, and Cs) with topological band structures has been discovered. These layered compounds are nonmagnetic and undergo charge density wave transitions before developing superconductivity at low temperatures. Here we report the observation of unconventional superconductivity and pair density wave (PDW) in CsV3Sb5 using scanning tunneling microscope/spectroscopy (STM/STS) and Josephson STS. We find that CsV3Sb5 exhibits a V-shaped pairing gap Δ~0.5 meV and is a strong-coupling superconductor (2Δ/kBTc~5) that coexists with 4a0 unidirectional and 2a0X2a0 charge order. Remarkably, we discover a 3Q PDW accompanied by bidirectional 4a0/3 spatial modulations of the superconducting gap, coherence peak and gap-depth in the tunneling conductance. We term this novel quantum state a roton-PDW associated with an underlying vortex-antivortex lattice that can account for the observed conductance modulations. Probing the electronic states in the vortex halo in an applied magnetic field, in strong-field that suppresses superconductivity, and in zero-field above Tc reveals that the PDW is a primary state responsible for an emergent pseudogap and intertwined electronic order. Our findings show striking analogies and distinctions to the phenomenology of high-Tc cuprate superconductors, and provide groundwork for understanding the microscopic origin of correlated electronic states and superconductivity in vanadium-based kagome metals.

cond-mat.supr-con↗

arXiv2021

Evolution of electronic structure in pristine and hole-doped kagome metal RbV$_3$Sb$_5$

We report on in situ low-temperature (4 K) scanning tunneling microscope measurements of atomic and electronic structures of the cleaved surfaces of an alkali-based kagome metal RbV$_3$Sb$_5$ single crystals. We find that the dominant pristine surface exhibits Rb-1x1 structure, in which a unique unidirectional $\sqrt{3}a_0$ charge order is discovered. As the sample temperature slightly rises, Rb-$\sqrt{3}$x1 and Rb-$\sqrt{3}$x$\sqrt{3}$ reconstructions form due to desorption of surface Rb atoms. Our conductance mapping results demonstrate that Rb desorption not only gives rise to hole doping, but also renormalizes the electronic band structures. Surprisingly, we find a ubiquitous gap opening near the Fermi level in tunneling spectra on all the surfaces despite their large differences of hole-carrier concentration, indicating an orbital-selective band reconstruction in RbV$_3$Sb$_5$.

cond-mat.supr-con↗

arXiv2021

Charge density wave orders and enhanced superconductivity under pressure in the kagome metal CsV3Sb5

Superconductivity in topological kagome metals has recently received great research interests. Here, charge density wave (CDW) orders and the evolution of superconductivity under various pressures in CsV3Sb5 single crystal with V kagome lattice are investigated. By using high-resolution scanning tunnelling microscopy /spectroscopy (STM/STS), two CDW orders in CsV3Sb5 are observed which correspond to 4a*1a and 2a*2a superlattices. By applying pressure, the superconducting transition temperature Tc is significantly enhanced and reaches a maximum value of 8.2 K at around 1 GPa. Accordingly, CDW state is gradually declined as increasing the pressure, which indicates the competing interplay between CDW and superconducting state in this material. The broad superconducting transitions around 0.4 - 0.8 GPa can be related to the strong competition relation among two CDW states and superconductivity. These results demonstrate that CsV3Sb5 is a new platform for exploring the interplay between superconductivity and CDW in topological kagome metals.

cond-mat.supr-con↗

arXiv2021

Charge-density-wave-induced bands renormalization and energy gaps in a kagome superconductor RbV3Sb5

Recently discovered Z2 topological kagome metals AV3Sb5 (A = K, Rb, and Cs) exhibit charge density wave (CDW) phases and novel superconducting paring states, providing a versatile platform for studying the interplay between electron correlation and quantum orders. Here we directly visualize CDW-induced bands renormalization and energy gaps in RbV3Sb5 using angle-resolved photoemission spectroscopy, pointing to the key role of tuning van Hove singularities to the Fermi energy in mechanisms of ordering phases. Near the CDW transition temperature, the bands around the Brillouin zone (BZ) boundary are shifted to high-binding energy, forming an "M"-shape band with singularities near the Fermi energy. The Fermi surfaces are partially gapped and the electronic states on the residual ones should be possibly dedicated to the superconductivity. Our findings are significant in understanding CDW formation and its associated superconductivity.

cond-mat.supr-con↗

arXiv2021

Spin excitations in metallic kagome lattice FeSn and CoSn

In two-dimensional (2D) metallic kagome lattice materials, destructive interference of electronic hopping pathways around the kagome bracket can produce nearly localized electrons, and thus electronic bands that are flat in momentum space. When ferromagnetic order breaks the degeneracy of the electronic bands and splits them into the spin-up majority and spin-down minority electronic bands, quasiparticle excitations between the spin-up and spin-down flat bands should form a narrow localized spin-excitation Stoner continuum coexisting with well-defined spin waves in the long wavelengths. Here we report inelastic neutron scattering studies of spin excitations in 2D metallic Kagome lattice antiferromagnetic FeSn and paramagnetic CoSn, where angle resolved photoemission spectroscopy experiments found spin-polarized and nonpolarized flat bands, respectively, below the Fermi level. Although our initial measurements on FeSn indeed reveal well-defined spin waves extending well above 140 meV coexisting with a flat excitation at 170 meV, subsequent experiments on CoSn indicate that the flat mode actually arises mostly from hydrocarbon scattering of the CYTOP-M commonly used to glue the samples to aluminum holder. Therefore, our results established the evolution of spin excitations in FeSn and CoSn, and identified an anomalous flat mode that has been overlooked by the neutron scattering community for the past 20 years.

cond-mat.str-el↗

arXiv2021

Intrinsic nature of chiral charge order in the kagome superconductor RbV3Sb5

Superconductors with kagome lattices have been identified for over 40 years, with a superconducting transition temperature TC up to 7K. Recently, certain kagome superconductors have been found to exhibit an exotic charge order, which intertwines with superconductivity and persists to a temperature being one order of magnitude higher than TC. In this work, we use scanning tunneling microscopy (STM) to study the charge order in kagome superconductor RbV3Sb5. We observe both a 2x2 chiral charge order and nematic surface superlattices (predominantly 1x4). We find that the 2x2 charge order exhibits intrinsic chirality with magnetic field tunability. Defects can scatter electrons to introduce standing waves, which couple with the charge order to cause extrinsic effects. While the chiral charge order resembles that discovered in KV3Sb5, it further interacts with the nematic surface superlattices that are absent in KV3Sb5 but exist in CsV3Sb5.

cond-mat.str-el↗

arXiv2021

s-wave superconductivity in kagome metal CsV$_{3}$Sb$_{5}$ revealed by $^{121/123}$Sb NQR and $^{51}$V NMR measurements

We report $^{121/123}$Sb nuclear quadrupole resonance (NQR) and $^{51}$V nuclear magnetic resonance (NMR) measurements on kagome metal CsV$_3$Sb$_5$ with $T_{\rm c}=2.5$ K. Both $^{51}$V NMR spectra and $^{121/123}$Sb NQR spectra split after a charge density wave (CDW) transition, which demonstrates a commensurate CDW state. The coexistence of the high temperature phase and the CDW phase between $91$ K and $94$ K manifests that it is a first order phase transition. At low temperature, electric-field-gradient fluctuations diminish and magnetic fluctuations become dominant. Superconductivity emerges in the charge order state. Knight shift decreases and $1/T_{1}T$ shows a Hebel--Slichter coherence peak just below $T_{\rm c}$, indicating that CsV$_3$Sb$_5$ is an s-wave superconductor.

cond-mat.supr-con↗

arXiv2021

Superconductivity and normal-state properties of kagome metal RbV3Sb5 single crystals

We report the discovery of superconductivity and detailed normal-state physical properties of RbV3Sb5 single crystals with V kagome lattice. RbV3Sb5 single crystals show a superconducting transition at Tc ~ 0.92 K. Meanwhile, resistivity, magnetization and heat capacity measurements indicate that it exhibits anomalies of properties at T* ~ 102 - 103 K, possibly related to the formation of charge ordering state. When T is lower than T*, the Hall coefficient RH undergoes a drastic change and sign reversal from negative to positive, which can be partially explained by the enhanced mobility of hole-type carriers. In addition, the results of quantum oscillations show that there are some very small Fermi surfaces with low effective mass, consistent with the existence of multiple highly dispersive Dirac band near the Fermi energy level.

cond-mat.supr-con↗

arXiv2020

Electronic correlations and flattened band in magnetic Weyl semimetal candidate Co3Sn2S2

The interplay between electronic correlations and topological protection may offer a rich avenue for discovering emergent quantum phenomena in condensed matter. However, electronic correlations have so far been little investigated in Weyl semimetals (WSMs) by experiments. Here, we report a combined optical spectroscopy and theoretical calculation study on the strength of electronic correlations in a kagome magnet Co3Sn2S2 and the influence of electronic correlations on its WSM state expected within a single-particle picture. The electronic kinetic energy estimated from our optical data is about half of that obtained from single-particle ab initio calculations, which indicates intermediate-strength electronic correlations in this system. Furthermore, comparing the energy ratios between the interband-transition peaks at high energies in the experimental and single-particle-ab-initio-calculation derived optical conductivity spectra with the electronic bandwidth renormalization factors obtained by many-body calculations enables us to estimate the Coulomb-interaction strength (U ~ 4 eV) of electronic correlations in Co3Sn2S2. Our many-body calculations with U ~ 4 eV show that a WSM state, which is characterized by bulk Weyl cones and surface Fermi arcs, survives in this correlated electron system. Besides, a sharp experimental optical conductivity peak at low energy, which is absent in the single-particle-ab-initio-calculation-derived optical conductivity spectrum but is consistent with the optical conductivity peaks obtained by many-body calculations, indicates that an electronic band connecting the two Weyl cones is flattened by electronic correlations and emerges near the Fermi energy in Co3Sn2S2. Our work paves the way for exploring flat-band-generated quantum phenomena in WSMs.

cond-mat.mtrl-sci↗

arXiv2020

Localized spin-orbit polaron in magnetic Weyl semimetal Co$_3$Sn$_2$S$_2$

The kagome lattice Co$_3$Sn$_2$S$_2$ exhibits the quintessential topological phenomena of a magnetic Weyl semimetal such as the chiral anomaly and Fermi-arc surface states. Probing its magnetic properties is crucial for understanding this correlated topological state. Here, using spin-polarized scanning tunneling microscopy/spectroscopy (STM/S), we report the discovery of localized spin-orbit polarons (SOPs) with three-fold rotation symmetry nucleated around single-S vacancies in Co$_3$Sn$_2$S$_2$. The SOPs carry a spin-polarized magnetic moment and a large orbital magnetization of a topological origin associated with the Berry phase and the persistent circulating current. Appreciable magneto-elastic coupling of the SOP is detected by atomic force microscope and STM. Our findings suggest that the SOPs can enhance magnetism and stability of the magnetic Weyl nodes for more robust time-reversal-symmetry-breaking topological phenomena. Controlled engineering of the SOPs may pave the way toward practical applications in functional quantum devices.

cond-mat.mtrl-sci↗

arXiv2020

Novel Superstructure-Phase Two-Dimensional Material 1$\textit{T}$-VSe$_2$ at High Pressure

A superstructure can elicit versatile new properties of materials by breaking their original geometrical symmetries. It is an important topic in the layered graphene-like two-dimensional transition-metal dichalcogenides (TMDs), but its origin remains unclear. Using diamond-anvil cell techniques, synchrotron x-ray diffraction, x-ray absorption, and the first-principles calculations, we show that the evolution from the weak Van der Waals bonding to the Heisenberg covalent bonding between layers induces an isostructural transition in quasi-two-dimensional 1$\textit{T}$-type VSe$_2$ at high pressure. Furthermore, our results show that high-pressure induce a novel superstructure at 15.5 GPa, rather than suppress as it would normally, which is unexpected. It is driven by the Fermi surface nesting, enhanced by the pressure-induced distortion. The results suggest that the superstructure not only appears in the two-dimensional structure but also can emerge in the pressure-tuned three-dimensional structure with new symmetry and develop superconductivity.

cond-mat.mtrl-sci↗

arXiv2019

Intrinsic anomalous Nernst effect amplified by disorder in a half-metallic semimetal

Intrinsic anomalous Nernst effect (ANE), like its Hall counterpart, is generated by Berry curvature of electrons in solids. Little is known about its response to disorder. In contrast, the link between the amplitude of the ordinary Nernst coefficient and the mean-free-path is extensively documented. Here, by studying Co$_3$Sn$_2$S$_2$, a topological half-metallic semimetal hosting sizable and recognizable ordinary and anomalous Nernst responses, we demonstrate an anti-correlation between the amplitude of ANE and carrier mobility. We argue that the observation, paradoxically, establishes the intrinsic origin of the ANE in this system. We conclude that various intrinsic off-diagonal coefficients are set by the way the Berry curvature is averaged on a grid involving the mean-free-path, the Fermi wavelength and the de Broglie thermal length.

cond-mat.mtrl-sci↗

arXiv2019

Near-room-temperature giant topological Hall effect in antiferromagnetic kagome metal YMn6Sn6

The kagome lattice, consisting of interconnected triangles and hexagons uniquely, is an excellent model system for study frustrated magnetism, electronic correlation and topological electronic structure. After an intensive investigation on frustrated magnetism in insulating magnetic kagome lattices, the interplay between charge and spin degrees of freedom via spin-orbital coupling in metallic systems (kagome metals) has become an attractive topic recently. Here, we study centrosymmetric YMn6Sn6 with Mn kagome lattice. We discover that it exhibits giant topological Hall effect near room temperature, ascribed to the field-induced non-collinear spin texture, possibly a skyrmion lattice (SkL) state. Combined with the large intrinsic anomalous Hall effect, YMn6Sn6 shows a synergic effect of real- and momentum-space Berry phase on physical properties. Since the features of tunable magnetic interaction and flexible structure in this large homologous series, it provides a novel platform for understanding the influence of electronic correlations on topological quantum states in both real and momentum spaces.

cond-mat.str-el↗