arXiv subjects

Qihuang Gong

Publications and source records attributed to Qihuang Gong.

At least 19 recordsLinked to original sources

arXiv2026

Power-Bandwidth Scaling of Resonantly Coupled Soliton Microcombs

A soliton microcomb requires increasing pump power as its optical bandwidth is broadened. Resonant pumping through an auxiliary microresonator can reduce the power required to sustain a soliton, but simultaneously increases the power required for soliton formation. We show that this competition leads to optimal inter-resonator coupling, and the predicted minimum input pump power scales as the two-thirds power of the comb bandwidth, in contrast to the quadratic scaling under direct pumping. Experiments support the opposing power trends, providing a design rule for power-efficient, ultra-broadband soliton microcombs.

physics.optics↗

arXiv2026

High-efficiency loading of 2,400 Ytterbium atoms in optical tweezer arrays

Neutral atom arrays have emerged as a powerful platform for quantum computation, simulation, and metrology.Among them, alkaline-earth-like atoms exhibit distinct advantages, including long coherence time, high-fidelity Rydberg gates, and erasure correction for efficient quantum error correction. However, their scalability has lagged behind that of the alkali atoms. Here, we report 2400 ytterbium-174 atoms trapped in an optical tweezer array with enhanced loading efficiency of 83.5(1)\% via blue-detuned light-assisted collisions. We develop a quantitative model of the collision dynamics and find good agreement between the calculated inelastic collision rates and the experimentally measured loading efficiencies.Notably, the loading efficiency is largely maintained for array sizes ranging from dozens to thousands, exhibiting excellent scalability. We further demonstrate that the enhancement exists robustly across a range of interatomic potentials, suggesting its utility for other atomic species. To establish the capability of the $^{174}$Yb arrays toward universal quantum computation, we propose to encode the qubit in the ground-clock state manifold and estimate a 99.9\% two-qubit gate fidelity with experimentally feasible parameters. Our work advances the prospects for realizing large-scale quantum computers using alkaline-earth-like atoms.

quant-ph↗

arXiv2026

A universal framework for nonlinear frequency combs under electro-optic modulation

Nonlinear frequency combs, including electro-optic and Kerr combs, have become central platforms for chip-scale frequency synthesis. Recent breakthroughs in strong-coupling electro-optic modulation further expanded their accessible nonlinear dynamics, unlocking new phenomena and functionalities, but the underlying foundation remains largely unexplored. Here we establish a universal theoretical and experimental framework for nonlinear combs under arbitrary electro-optic modulation by introducing a general evolution equation (GEE) that transcends the mean-field Lugiato-Lefever equation. The GEE reduces to a discrete-time Integration Hamiltonian that provides a frequency-domain formalism unifying strong-coupling electro-optic modulation with photonic synthetic dimensions. Together with a band-wave correspondence linking modulation waveforms to synthetic band structures, the formalism enables programmable spectral control. We further show compatibility between Kerr nonlinearity and strong-coupling electro-optic modulation, highlighting their cooperative dynamics. Our work provides a foundational model for strong-coupling electro-optics in nonlinear combs, opening a route toward chip-integrated, microwave-programmable comb sources for metrology, spectroscopy, and emerging photonic technologies.

physics.optics↗

arXiv2026

Program gain and loss for broadband soliton microcombs

Soliton microcombs provide compact, broadband, coherent light sources for precision metrology, spectroscopy, communications, and microwave photonics. Extending their spectral span while retaining useful output power remains challenging and often requires impractically high pump power. Existing approaches mainly tailor the dispersion and pumping conditions, but they do not exploit the coupling spectrum as a programmable aspect of soliton operation. Here we introduce a meta-coupler whose lithographically programmed coupling spectrum concentrates strong pump access near the pumped resonance while leaving most comb lines close to the intrinsic loss rate. Si$_3$N$_4$ microresonators incorporating a meta-coupler exhibit broader circulating soliton spectra, nearly twofold larger 3 dB soliton bandwidths, up to about 12 dB higher central comb-line power, and up to about fivefold greater emitted comb power, without an additional pump-power penalty. Our work unlocks gain and loss as simultaneous programmable knobs for realizing high-performance soliton microcombs.

physics.optics↗

arXiv2026

Attosecond quantum spectroscopy with entangled photon pairs

Bright squeezed light from parametric down-conversion in the infrared (IR) frequency range has triggered the emergence of attosecond quantum optics -- a new research field at the interface of quantum optics, strong-field physics, and attosecond technology. Two challenges arise at this interface: transferring quantum features of the IR light sources to the ultraviolet (UV) and extreme ultraviolet (XUV) frequency range via strong-field nonlinearities, and exploiting quantum optical properties of the nonlinear optical response as a new probe in ultrafast dynamics. Here, we address both by driving high-harmonic generation (HHG) in solids with entangled photon pairs either in degenerate or non-degenerate frequency modes. In the degenerate mode, single-shot measurements of harmonics up to the 10th order reveal strong photon bunching whose $g^{(2)}$ first grows and then decreases with the harmonic order. We show that this behavior tracks different microscopic mechanisms responsible for harmonic emission, demonstrating the potential of attosecond quantum optical spectroscopy. In the non-degenerate case, the harmonics retain quantum-induced correlations, verified by wavelength-resolved second-order cross-correlation maps. Our findings demonstrate transfer of quantum photon correlations into the XUV domain and open a pathway toward quantum-enhanced attosecond spectroscopy and control of ultrafast dynamics in solids.

physics.optics↗

arXiv2026

Electrical detection of high-order optical orbital angular momentum

The orbital angular momentum (OAM) of light provides an unbounded set of orthogonal modes for ultrahigh-capacity optical information processing. However, current OAM detection schemes typically rely on light interference or diffraction, which require bulky optical components and pose a major obstacle to on-chip integration. Here, we demonstrate a fully integrated silicon-based photodetector that enables direct electrical detection of light OAM. This photodetector can resolve vortex beams with topological charges from m = -9 to 9, achieving a record-high mode number resolution among on-chip devices. By integrating plasmonic gratings onto the device electrodes, incident vortex beams can be converted into surface plasmon polaritons with OAM-dependent splitting angles, which in turn produce photocurrents that vary monotonically with the OAM order. Further incorporation of a surface dielectric lens can enhance mode resolution, and a split-electrode architecture enables OAM chirality discrimination. Owing to its CMOS-compatibility and spectral scalability, this platform provides a compact and robust solution for integrated OAM detection, opening new opportunities for on-chip optical communication and computing systems based on structured light.

physics.optics↗

arXiv2025

Perfect continuous-variable quantum microcombs

Quantum microcombs generated in high-Q microresonators provide compact, multiplexed sources of entangled modes for continuous-variable (CV) quantum information processing. While deterministic generation of CV states via Kerr-induced two-mode squeezing has been demonstrated, achieving spectrally uniform squeezing remains challenging because of asymmetry and anomalies in the dispersion profile. Here we overcome these limitations by combining a microresonator with an engineered mode spectrum and optimized pump conditions. We realize a CV quantum microcomb comprising 14 independent two-mode squeezed states, each exhibiting more than 4 dB of raw squeezing (up to 4.3 dB) across a 0.7 THz bandwidth. This uniform, high-performance quantum resource represents a key step toward scalable, integrated CV quantum technologies operating beyond classical limits.

quant-ph↗

arXiv2025

Communication-ready high-power soliton microcombs in highly-dispersive Fabry-Perot-microresonators

Microcombs generated in optical microresonators are widely regarded as promising light sources for next-generation communication systems, but the optical power available per comb line has so far fallen short of practical requirements. Here we introduce an integrated Fabry-Pérot microresonator platform that overcomes fundamental dispersion-engineering constraints and enables bright soliton microcombs with unprecedented power per line. The resonator is defined by chirped Bragg gratings that provide exceptionally large anomalous group-velocity dispersion, allowing more than ten comb lines to reach the milliwatt level. These combs can be used directly in coherent communication systems without additional amplification, achieving an aggregate data rate of 2 Tb/s. Once integrated, our high-power soliton microcombs could be instantly ready for communications as well as a broad range of practical comb-based applications.

physics.optics↗

arXiv2025

Integrated soliton microcombs beyond the turnkey limit

Soliton microcombs generated in optical microresonators are accelerating the transition of optical frequency combs from laboratory instruments to industrial platforms. Self injection locking (SIL) enables direct driving of soliton microcombs by integrated lasers, providing turnkey initiation and improved coherence, but it also pins the pump close to resonance, limiting both spectral span and tuning flexibility. Here we theoretically and experimentally demonstrate that introducing a thermally tunable auxiliary microresonator extends the bandwidth of SIL soliton microcombs. By engineering hybridization of the pumped resonance, we achieve deterministic access to single soliton states and then push operation into a far detuned regime inaccessible to direct initiation. The resulting combs reach a near 200 nm span at a 25 GHz repetition rate, while preserving the SIL-enabled noise suppression throughout. Moreover, the added degree of freedom afforded by the coupled resonator architecture enables orthogonal control of the comb's repetition rate and center frequency. These advances expand the spectral reach and controllability of integrated soliton microcombs for information processing and precision metrology.

physics.optics↗

arXiv2025

Raman-induced dynamics of ultrafast microresonator solitons

Soliton microcombs are evolving towards octave-spanning for $f$-$2f$ self-referencing and expanding applications in spectroscopy and timekeeping. As spectra broaden and pulses shorten, the Raman-induced soliton self-frequency shift (SSFS) becomes a principal limitation: it reduces pump-to-comb conversion efficiency, constrains achievable span, and can, in extremes, preclude stationary operation. We develop a complementary theory of SSFS in microresonators that remains valid when the soliton duration $τ_s$ is shorter than the Raman response timescale. The theory predicts a reduced dependence of the SSFS on $τ_s$ which also expands the soliton existence range. Such predictions are validated by numerical simulations and by experiments on Si$_3$N$_4$ microresonators. Our results provide practical guidelines for engineering efficient and broadband soliton microcombs.

physics.optics↗

arXiv2025

Transfer learning discovery of molecular modulators for perovskite solar cells

The discovery of effective molecular modulators is essential for advancing perovskite solar cells (PSCs), but the research process is hindered by the vastness of chemical space and the time-consuming and expensive trial-and-error experimental screening. Concurrently, machine learning (ML) offers significant potential for accelerating materials discovery. However, applying ML to PSCs remains a major challenge due to data scarcity and limitations of traditional quantitative structure-property relationship (QSPR) models. Here, we apply a chemical informed transfer learning framework based on pre-trained deep neural networks, which achieves high accuracy in predicting the molecular modulator's effect on the power conversion efficiency (PCE) of PSCs. This framework is established through systematical benchmarking of diverse molecular representations, enabling lowcost and high-throughput virtual screening over 79,043 commercially available molecules. Furthermore, we leverage interpretability techniques to visualize the learned chemical representation and experimentally characterize the resulting modulator-perovskite interactions. The top molecular modulators identified by the framework are subsequently validated experimentally, delivering a remarkably improved champion PCE of 26.91% in PSCs.

cond-mat.mtrl-sci↗

arXiv2025

Electrically-pumped soliton microcombs on thin-film lithium niobate

Thin-film lithium niobate (TFLN) has enabled efficient on-chip electro-optic modulation and frequency conversion for information processing and precision measurement. Extending these capabilities with optical frequency combs unlocks massively parallel operations and coherent optical-to-microwave transduction, which are achievable in TFLN microresonators via Kerr microcombs. However, fully integrated Kerr microcombs directly driven by semiconductor lasers remain elusive, which has delayed integration of these technologies. Here we demonstrate electrically pumped TFLN Kerr microcombs without optical amplification. With optimized laser-to-chip coupling and optical quality factors, we generate soliton microcombs at a 200 GHz repetition frequency with an optical span of 180 nm using only 25 mW of pump power. Moreover, self-injection locking enables turnkey initiation and substantially narrows the laser linewidth. Our work provides integrated comb sources for TFLN-based communicational, computational, and metrological applications.

physics.optics↗

arXiv2025

Universal dynamics and microwave control of programmable cavity electro-optic frequency combs

Electro-optic (EO) frequency combs are foundational for metrology and spectroscopy. Specifically, microresonator-based cavity EO combs are distinguished by efficient sideband generation, precisely controlled by microwave signals, enabling high-performance integrated frequency references and pulse sources. However, the apparent simplicity of these devices, often described by the EO modulation-induced coupling of nearest-neighbor cavity modes, has limited investigations of their fundamental physics, thereby restricting their full potential. Here, we uncover the universal dynamics and complete frequency lattice connectivity underpinning cavity EO microcombs, as well as characterize the full space of nonlinear optical states, controlled by modulation depth and optical detuning, using the thin-film lithium niobate photonic platform. Leveraging this understanding, we design complex long-range couplings between cavity modes to realize programmable spectro-temporal shaping of the generated combs and pulses. We achieve three technological advances, including repetition-rate flexibility, substantial comb bandwidth extension beyond traditional scaling laws, and resonantly-enhanced flat-top spectrum. Our results provide physical insights for synchronously driven cavity-based EO systems, broadly defined, paving the way for electrically controlled and electrically enhanced comb generators for next-generation photonic applications.

physics.optics↗

arXiv2025

Strong-coupling and high-bandwidth cavity electro-optic modulation for advanced pulse-comb synthesis

Cavity electro-optic (EO) modulation plays a pivotal role in optical pulse and frequency comb synthesis, supporting a wide range of applications including communication, computing, ranging, and quantum information. The ever-growing demand for these applications has driven efforts in enhancing modulation coupling strength and bandwidth towards advanced pulse-comb synthesis. However, the effects of strong-coupling and high-bandwidth cavity EO modulation remain underexplored, due to the lack of a general, unified model that captures this extreme condition. In this work, we present a universal framework for pulse-comb synthesis under cavity EO modulation, where coupling strength and modulation bandwidth far exceed the cavity's free spectral range (FSR). We show that, under such intense and ultrafast driving conditions, EO-driven frequency combs and pulses exhibit rich higher-order nonlinear dynamics, including temporal pulse compression and comb generation with arbitrary pump detuning. Leveraging this framework, we reveal a direct link between the higher-order dynamics of EO pulse-comb generation and the band structure of synthetic dimension. Furthermore, we demonstrate arbitrary comb shaping via machine-learning-based inverse microwave drive design, achieving a tenfold enhancement in cavity electro-optic comb flatness by exploring the synergistic effects of high-bandwidth driving and detuning-induced frequency boundaries. Our findings push cavity electro-optic modulation into a new frontier, unlocking significant potential for universal and machine-learning-programmable electro-optic frequency combs, topological photonics, as well as photonic quantum computing in the strong-coupling and high-bandwidth regimes.

physics.optics↗

arXiv2025

Power-efficient ultra-broadband soliton microcombs in resonantly-coupled microresonators

The drive to miniaturize optical frequency combs for practical deployment has spotlighted microresonator solitons as a promising chip-scale candidate. However, these soliton microcombs could be very power-hungry when their span increases, especially with fine comb spacings. As a result, realizing an octave-spanning comb at microwave repetition rates for direct optical-microwave linkage is considered not possible for photonic integration due to the high power requirements. Here, we introduce the concept of resonant-coupling to soliton microcombs to reduce pump consumption significantly. Compared to conventional waveguide-coupled designs, we demonstrate (i) a threefold increase in spectral span for high-power combs and (ii) up to a tenfold reduction in repetition frequency for octave-spanning operation. This configuration is compatible with laser integration and yields reliable, turnkey soliton generation. By eliminating the long-standing pump-power bottleneck, microcombs will soon become readily available for portable optical clocks, massively parallel data links, and field-deployable spectrometers.

physics.optics↗

arXiv2025

Universal Quantum Computational Spectroscopy on a Quantum Chip

Spectroscopy underpins modern scientific discovery across diverse disciplines. While experimental spectroscopy probes material properties through scattering or radiation measurements, computational spectroscopy combines theoretical models with experimental data to predict spectral properties, essential for advancements in physics, chemistry, and materials science. However, quantum systems present unique challenges for computational spectroscopy due to their inherent complexity, and current quantum algorithms remain largely limited to static and closed quantum systems. Here, we present and demonstrate a universal quantum computational spectroscopy framework that lifts these limitations. Through leveraging coherently controlled quantum dynamics, our method efficiently reconstructs the spectral information for both closed and open systems, furtherly for time-dependent driven systems. We experimentally validate this approach using a programmable silicon-photonic quantum processing chip, capable of high-fidelity time-evolution simulations. The versatility of our framework is demonstrated through spectroscopic computations for diverse quantum systems -- including spin systems, non-Hermitian systems, and quantum Floquet systems -- revealing novel phenomena such as parity-time symmetry breaking and topological holonomy that are inaccessible to conventional spectroscopy or quantum eigenstate algorithms. {Furthermore, systematic benchmarking of UQCS against existing quantum algorithms is numerically performed to demonstrate its unprecedented capabilities and superior performance. This work establishes a noise-robust and transformative paradigm for quantum spectral analysis.

quant-ph↗

arXiv2025

Full Polarization Control of Photons with Evanescent Wave Coupling in the Ultra Subwavelength Gap of Photonic Molecules

Polarization of photons plays a key role in quantum optics and light-matter interactions, however, it is difficult to control in nanosystems since the eigenstate of a nanophotonic cavity is usually fixed and linearly polarized. Here we reveal polarization control of photons using photonic molecules (PMs) that host supermodes of two coupled nanobeam cavities. In contrast to conventional PMs in a 2D photonic crystal slab, for the two 1D photonic crystal nanobeam cavities the shift and gap between them can be tuned continuously. With an ultra subwavelength gap, the coupling between the two cavities is dominated by the evanescent wave coupling in the surrounding environment, rather not the emission wave coupling for conventional PMs. As such, non-Hermiticity of the system becomes pronounced, and the supermodes consist of a non-trivial phase difference between bare eigenstates that supports elliptical polarization. We observe that both the polarization degree and polarization angle of the antisymmetric mode strongly depend on the shift and gap between the two cavities, exhibiting polarization states from linear to circular. This full polarization control indicates great potential of PMs in quantum optical devices and spin-resolved cavity quantum electrodynamics.

physics.optics↗

arXiv2025

Compact Turnkey Soliton Microcombs at Microwave Rates via Wafer-Scale Fabrication

Soliton microcombs generated in nonlinear microresonators facilitate the photonic integration of timing, frequency synthesis, and astronomical calibration functionalities. For these applications, low-repetition-rate soliton microcombs are essential as they establish a coherent link between optical and microwave signals. However, the required pump power typically scales with the inverse of the repetition rate, and the device footprint scales with the inverse of square of the repetition rate, rendering low-repetition-rate soliton microcombs challenging to integrate within photonic circuits. This study designs and fabricates silicon nitride microresonators on 4-inch wafers with highly compact form factors. The resonator geometries are engineered from ring to finger and spiral shapes to enhance integration density while attaining quality factors over 10^7. Driven directly by an integrated laser, soliton microcombs with repetition rates below 10 GHz are demonstrated via turnkey initiation. The phase noise performance of the synthesized microwave signals reaches -130 dBc/Hz at 100 kHz offset frequency for 10 GHz carrier frequencies. This work enables the high-density integration of soliton microcombs for chip-based microwave photonics and spectroscopy applications.

physics.optics↗