Searcharxiv⌕ Search

arXiv subjects

Qihuang Gong

Publications and source records attributed to Qihuang Gong.

At least 91 records · Page 5Linked to original sources

Topologically Enabled Ultralarge Purcell Enhancement Robust to Photon Scattering

Micro/nanoscale single photon source is a building block of on-chip quantum information devices. Owing to possessing ultrasmall optical mode volume, plasmon structures can provide large Purcell enhancement, however scattering and absorption are two barriers to prevent them from being used in practice. To overcome these barriers, we propose the topological photonic structure containing resonant plasmon nanoantenna, where nanoantenna provides large Purcell enhancement while topological photonic crystal guides all scattering light into its edge state. Through the optical mode design, the rate of single photons emitted into the edge state reaches more than 104γ0 simultaneously accompanied with an obvious reduction of absorption. This kind of nonscattering large Purcell enhancement will provide new sight for on-chip quantum light sources such as a single photon source and nanolaser.

physics.optics↗

Discrete time symmetry breaking in quantum circuits: exact solutions and tunneling

We discuss general properties of discrete time quantum symmetry breaking in degenerate parametric oscillators. Recent experiments in superconducting quantum circuit with Josephson junction nonlinearities give rise to new properties of strong parametric coupling and nonlinearities. Exact analytic solutions are obtained for the steady-state of this single-mode case of subharmonic generation. We also obtain analytic solutions for the tunneling time over which the time symmetry-breaking is lost above threshold. We find that additional anharmonic terms found in the superconducting case increase the tunneling rate, and can also lead to new regimes of tristability as well as bistability. Our analytic results are confirmed by number state calculations.

quant-ph↗

Schrödinger cats and steady states in subharmonic generation with Kerr nonlinearities

We discuss general properties of the equilibrium state of parametric down-conversion in superconducting quantum circuits with detunings and Kerr anharmonicities, in the strongly nonlinear regime. By comparing moments of the steady state and those of a Schrödinger cat, we show that true Schrödinger cats cannot survive in the steady state if there is any single-photon loss. A delta-function 'cat-like' steady-state distribution can be formed, but this only exists in the limit of an extremely large nonlinearity. The steady state is a mixed state, which is more complex than a mixture or linear combination of delta-functions, and whose purity is reduced by driving. We expect this general behaviour to occur in other driven, dissipative quantum subharmonic non-equilibrium open systems.

quant-ph↗

Engineering asymmetric steady-state Einstein-Podolsky-Rosen steering in macroscopic hybrid systems

Generation of quantum correlations between separate objects is of significance both in fundamental physics and in quantum networks. One important challenge is to create the directional "spooky action-at-a-distanc" effects that Schrödinger called "steering" between two macroscopic and massive objects. Here, we analyze a generic scheme for generating steering correlations in cascaded hybrid systems in which two distant oscillators with effective masses of opposite signs are coupled to a unidirectional light field, a setup which is known to build up quantum correlations by means of quantum back-action evasion. The unidirectional coupling of the first to the second oscillator via the light field can be engineered to enhance steering in both directions and provides an active method for controlling the asymmetry of steering. We show that the resulting scheme can efficiently generate unconditional steady-state Einstein-Podolsky-Rosen steering between the two subsystems, even in the presence of thermal noise and optical losses. As a scenario of particular technological interest in quantum networks, we use our scheme to engineer enhanced steering from an untrusted node with limited tunability (in terms of interaction strength and type with the light field) to a trusted, highly tunable node, hence offering a path to implementing one-sided device-independent quantum tasks.

quant-ph↗

Synchronization and temporal nonreciprocity of optical microresonators via spontaneous symmetry breaking

Synchronization is of importance in both fundamental and applied physics, but their demonstration at the micro/nanoscale is mainly limited to low-frequency oscillations like mechanical resonators. Here, we report the synchronization of two coupled optical microresonators, in which the high-frequency resonances in optical domain are aligned with reduced noise. It is found that two types of synchronization emerge with either the first- or second-order transition, both presenting a process of spontaneous symmetry breaking. In the second-order regime, the synchronization happens with an invariant topological character number and a larger detuning than that of the first-order case. Furthermore, an unconventional hysteresis behavior is revealed for a time-dependent coupling strength, breaking the static limitation and the temporal reciprocity. The synchronization of optical microresonators offers great potential in reconfigurable simulations of many-body physics and scalable photonic devices on a chip.

physics.optics↗

Michelson Interferometry of High-order Harmonic Generation in Solids

For the high-order harmonic generation in solids, we find a distinct and clean interference pattern in the high-energy end of the spectrum which can be interpreted as a Michelson interferometer of the Bloch electron. Our results are achieved by a numerical solution to the time-dependent Schrödinger equation of the quasi-electron in solids and can be explained by an analytical model based on the principle of the Michelson interferometry. The present study deepens our understanding of the HHG mechanism in crystalline materials and may find potential applications in imaging of the dispersion relation or topological structure of the energy bands in solids.

physics.atom-ph↗

Manipulation and enhancement of asymmetric steering via interference effects induced by closed-loop coupling

We present a phase control method for a general three-mode system with closed-loop in coupling that drives the system into an entangled steady state and produces directional steering between two completely symmetric modes via quantum interference effects. In the scheme, two modes are coupled with each other both by a direct binary interaction and by an indirect interaction through a third intermediate damping mode, creating interference effects determined by the relative phase between the two physical interaction paths. By calculating the populations and correlations of the two modes, we show that depending on the phase, two modes can be prepared into an entangled steady state with asymmetric and directional steering even if they possess completely symmetric decoherence properties. Meanwhile, entanglement and steering can be significantly enhanced due to constructive interference, and thus more robust to thermal noises. This provides an active method to manipulate the asymmetry of steering instead of adding asymmetric losses or noises on subsystems at the cost of reducing steerability. Moreover, we show that the interference effects can also enhance and control the correlations between other pair of modes in the loop with opposite phase dependent behavior, indicating monogamy constraints for distributing correlations among multipartite. The present model could be applied in cavity optomechanical systems or in antiferromagnets where all components can mutually interact.

quant-ph↗

Photon-momentum transfer in diatomic molecules: an ab initio study

For a molecule, the two-center interference and the molecular scattering phase of the electron are important for almost all the processes that may occur in a laser field. In this study, we investigate their effects in the transfer of linear photon momentum to the ionized electron by absorbing a single photon. The time-dependent Schrödinger equation of H$_2^+$ is numerically solved in {the multipolar} gauge in which the electric quadrupole term and the magnetic dipole term are explicitly expressed. This allows us to separate the contributions of the two terms in the momentum transfer. For different configurations of the molecular and the laser orientation, the transferred momentum to the electron is evaluated at different internuclear distances with various photon energies { and two-center interferences are identified in the whole region. At small electron energies and small internuclear distances, we find significant deviations from the prediction of the classical double-slit model due to the strong mediation of the Coulomb potential.} Finally, even for a large internuclear distance, our results show that a varying molecular scattering phase is important at all electron energies, which is beyond the simple prediction of the linear combination of the atomical orbitals.

physics.atom-ph↗

Accurate in situ Measurement of Ellipticity Based on Sub-cycle Ionization Dynamics

Elliptically polarized laser pulses (EPLPs) are widely applied in many fields of ultrafast sciences, but the ellipticity~($\varepsilon$) has never been in situ measured in the interaction zone of the laser focus. In this work, we propose and realize a robust scheme to retrieve the $\varepsilon$ by temporally overlapping two identical counter-rotating EPLPs. The combined linearly electric field is coherently controlled to ionize Xe atoms by varying the phase delay between the two EPLPs. The electron spectra of the above-threshold ionization and the ion yield are sensitively modulated by the phase delay. We demonstrate that these modulations can be used to accurately determine $\varepsilon$ of the EPLP. We show that the present method is highly reliable and is applicable in a wide range of laser parameters. The accurate retrieval of $\varepsilon$ offers a better characterization of a laser pulse, promising a more delicate and quantitative control of the sub-cycle dynamics in many strong field processes.

physics.atom-ph↗

A photonic interface of chiral cavity quantum electrodynamics

Cavity quantum electrodynamics studies light-matter interactions at single quanta level. Chiral photon-emitter coupling in photonic structures is characterized as unidirectional propagation locked by the local polarization of light. However, to realize the strong interaction of photon-emitter with direction-locked propagation, which will bring novel applications in nonreciprocal quantum devices, has not been reported yet. Here, we propose the coupled photonic crystal and metallic nanoparticle structure, where through strong local field with high helicity, the rate of circularly polarized photons emitting into photonic crystal waveguide is one order larger than that without the nanoparticle and the linewidth of Rabi splitting spectra is about one-tenth of that with only the nanoparticle, both with $\sim$ 95$\%$ photons propagating unidirectionally, which can be utilized in directional quantum light sources.

physics.optics↗

Spontaneous $\mathcal{T}$-symmetry breaking and exceptional points in cavity quantum electrodynamics systems

Spontaneous symmetry breaking has revolutionized the understanding in numerous fields of modern physics. Here, we theoretically demonstrate the spontaneous time-reversal symmetry breaking in a cavity quantum electrodynamics system in which an atomic ensemble interacts coherently with a single resonant cavity mode. The interacting system can be effectively described by two coupled oscillators with positive and negative mass when the two-level atoms are prepared in their excited states. The occurrence of symmetry breaking is controlled by the atomic detuning and the coupling to the cavity mode, which naturally divides the parameter space into the symmetry broken and symmetry unbroken phases. The two phases are separated by a spectral singularity, a so-called exceptional point, where the eigenstates of the Hamiltonian coalesce. When encircling the singularity in the parameter space, the quasi-adiabatic dynamics shows chiral mode switching which enables topological manipulation of quantum states.

quant-ph↗

Coherent control of superradiance from nitrogen ions pumped with femtosecond pulses

Singly ionized nitrogen molecules in ambient air pumped by near-infrared femtosecond laser give rise to superradiant emission. Here we demonstrate coherent control of this superradiance by injecting a pair of resonant seeding pulses inside the nitrogen gas plasma. Strong modulation of the 391.4 nm superradiance with a period of 1.3 fs is observed when the delay between the two seeding pulses are finely tuned, pinpointing the essential role of macroscopic coherence in this lasing process. Based on this time-resolved method, the complex temporal evolution of the macroscopic coherence between two involved energy levels has been experimentally revealed, which is found to last for around 10 picoseconds in the low gas pressure range. These observations provide a new level of control on the "air lasing" based on nitrogen ions, which can find potential applications in optical remote sensing.

physics.optics↗

Generalized spatial differentiation from spin Hall effect of light

Optics naturally provides us with some powerful mathematical operations. Here we experimentally demonstrate that during reflection or refraction at a single optical planar interface, the optical computing of spatial differentiation can be realized by analyzing specific orthogonal polarization states of light. We show that the spatial differentiation is intrinsically due to the spin Hall effect of light and generally accompanies light reflection and refraction at any planar interface, regardless of material composition or incident angles. The proposed spin-optical method takes advantages of a simple and common structure to enable vectorial-field computation and perform edge detection for ultra-fast and energy-efficient image processing.

physics.optics↗

Multidimensional quantum entanglement with large-scale integrated optics

The ability to control multidimensional quantum systems is key for the investigation of fundamental science and for the development of advanced quantum technologies. Here we demonstrate a multidimensional integrated quantum photonic platform able to robustly generate, control and analyze high-dimensional entanglement. We realize a programmable bipartite entangled system with dimension up to $15 \times 15$ on a large-scale silicon-photonics quantum circuit. The device integrates more than 550 photonic components on a single chip, including 16 identical photon-pair sources. We verify the high precision, generality and controllability of our multidimensional technology, and further exploit these abilities to demonstrate key quantum applications experimentally unexplored before, such as quantum randomness expansion and self-testing on multidimensional states. Our work provides a prominent experimental platform for the development of multidimensional quantum technologies.

quant-ph↗

Demonstration of monogamy relations for Einstein-Podolsky-Rosen steering in Gaussian cluster states

Understanding how quantum resources can be quantified and distributed over many parties has profound applications in quantum communication. As one of the most intriguing features of quantum mechanics, Einstein-Podolsky-Rosen (EPR) steering is a useful resource for secure quantum networks. By reconstructing the covariance matrix of a continuous variable four-mode square Gaussian cluster state subject to asymmetric loss, we quantify the amount of bipartite steering with a variable number of modes per party, and verify recently introduced monogamy relations for Gaussian steerability, which establish quantitative constraints on the security of information shared among different parties. We observe a very rich structure for the steering distribution, and demonstrate one-way EPR steering of the cluster state under Gaussian measurements, as well as one-to-multi-mode steering. Our experiment paves the way for exploiting EPR steering in Gaussian cluster states as a valuable resource for multiparty quantum information tasks.

quant-ph↗

Microcavity-engineered plasmonic resonances for radiation enhancement and strong coupling of a quantum emitter

Localized-surface plasmon resonance is of importance in both fundamental and applied physics for the subwavelength confinement of optical field, but realization of quantum coherent processes is confronted with challenges due to strong dissipation. Here we propose to engineer the electromagnetic environment of metallic nanoparticles (MNPs) using optical microcavities. An analytical quantum model is built to describe the MNP-microcavity interaction, revealing the significantly enhanced dipolar radiation and consequentially reduced Ohmic dissipation of the plasmonic modes. As a result, when interacting with a quantum emitter, the microcavity-engineered MNP enhances the quantum yield over 40 folds and the radiative power over one order of magnitude. Moreover, the system can enter the strong coupling regime of cavity quantum electrodynamics, providing a promising platform for the study of plasmonic quantum electrodynamics, quantum information processing, precise sensing and spectroscopy.

quant-ph↗

Revealing two heat-annealing related photoproduct systems and widely existed subgrain domains in organolead perovskite

For highly interested organolead perovskite based solar cells, the photoproducts are regarded as the co-existed exciton and free carriers. In this study, we carefully re-examined this conclusion with our recently developed density-resolved spectroscopic method. Heat-annealing related two photoproduct systems are observed. We found that the widely accepted model is only true for single crystal and freshly made films without heat-annealing. For those sufficiently heat-annealed films, another system presenting significant emissive exciton-carrier collision (ECC) is discovered. In addition, the appearing of ECC indicates the emerging of an internal morphology after heat annealing, which is assigned to a recently discussed twinning subgrain structure. We proved that such subgrain structures broadly exist in perovskite films. This finding could prove the morphological basis for high performance of perovskite working layers.

cond-mat.mtrl-sci↗

Mutually enhancing light emission between plasmonic nanostructures and fluorescent emitters

We demonstrate that the fluorescent emitters can increase light emission from the plasmonic nanostructures in turn. With the help of atomic force microscopy, a hybrid system consisting of a fluorescent nanodiamond and a gold nanoparticle was assembled step-by-step for in situ optical measurements. We found that the emission from the nanoparticle increased compared with that before coupling. The interaction between plasmonic nanostructures and fluorescent emitter was understood as an entity based on the concept of a quantized optical cavity by considering the nanodiamond and the nanoparticle as a two-level energy system and a nanoresonator, respectively. The theoretical calculations reveal that both the plasmonic coupling effect and the dielectric nanoantenna effect contribute to the enhancement of light emission from the gold nanoparticles.

physics.optics↗