arXiv subjects

Qing Ai

Publications and source records attributed to Qing Ai.

At least 73 records · Page 4Linked to original sources

arXiv2016

Transitionless intra-cavity quantum state transfer in optomechanical systems

Quantum state transfer between cavities is crucial for quantum information processing and quantum computation in optomechanical systems. Here, we present the first scheme for the transitionless intra-cavity quantum state transfer based on transitionless quantum driving (TQD) algorithm in optomechanical systems. We also present a physically feasible system for the TQD process based on largely detuned optomechanical cavity. With the Gaussian time-dependence coupling strengths, our scheme can achieve the perfect quantum state transfer with no undesired transition and reduce the dependence of accurately controlling evolution time and interval of coupling strengths. Our computational results show that the TQD process can be accomplished with no need of the mechanical oscillator in its ground state and is also robust to the mechanical dissipation.

quant-ph↗

arXiv2016

Negative Refraction Induced by Möbius Topology

We theoretically show the negative refraction existing in Möbius molecules. The negative refractive index is induced by the non-trivial topology of the molecules. With the Möbius boundary condition, the effective electromagnetic fields felt by the electron in a Möbius ring is spatially inhomogeneous. In this regard, the $D_{N}$ symmetry is broken in Möbius molecules and thus the magnetic response is induced through the effective magnetic field. Our findings open up a new architecture for negative refractive index materials based on the non-trivial topology of Möbius molecules.

quant-ph↗

arXiv2016

Proposal for probing energy transfer pathway by single-molecule pump-dump experiment

The structure of Fenna-Matthews-Olson (FMO) light-harvesting complex has long been recognized as containing seven bacteriochlorophyll (BChl) molecules. Recently, an additional BChl molecule was discovered in the crystal structure of the FMO complex, which may serve as a link between baseplate and the remaining seven molecules. Here, we investigate excitation energy transfer (EET) process by simulating single-molecule pump-dump experiment in the eight-molecules complex. We adopt the coherent modified Redfield theory and non-Markovian quantum jump method to simulate EET dynamics. This scheme provides a practical approach of detecting the realistic EET pathway in BChl complexes with currently available experimental technology. And it may assist optimizing design of artificial light-harvesting devices.

physics.chem-ph↗

arXiv2016

Quantum Zeno effect in a nitrogen-vacancy center embedded in a spin bath

We study the longitudinal relaxation of a nitrogen-vacancy (NV) center surrounded by a $^{13}$C nuclear spin bath in diamond. By means of cluster-correlation expansion (CCE), we numerically demonstrate the decay process of electronic state induced by cross relaxation at low temperature. It is shown that the CCE method is not only capable of describing pure-dephasing effect at large-detuning regime, but it can also simulate the quantum dynamics of populations in the nearly resonant regime. We present a proposal to slow down the decay of NV center via implementing quantum Zeno effect (QZE). The numerical result shows that QZE can effectively inhibit the decay of NV center.

quant-ph↗

arXiv2016

Physically feasible three-level transitionless quantum driving with multiple Schrödinger dynamics

Three-level quantum systems, which possess some unique characteristics beyond two-level ones, such as electromagnetically induced transparency, coherent trapping, and Raman scatting, play important roles in solid-state quantum information processing. Here, we introduce an approach to implement the physically feasible three-level transitionless quantum driving with multiple Schrödinger dynamics (MSDs). It can be used to control accurately population transfer and entanglement generation for three-level quantum systems in a nonadiabatic way. Moreover, we propose an experimentally realizable hybrid architecture, based on two nitrogen-vacancy-center ensembles coupled to a transmission line resonator, to realize our transitionless scheme which requires fewer physical resources and simple procedures, and it is more robust against environmental noises and control parameter variations than conventional adiabatic passage techniques. All these features inspire the further application of MSDs on robust quantum information processing in experiment.

quant-ph↗

arXiv2016

Complete nondestructive analysis of two-photon six-qubit hyperentangled Bell states assisted by cross-Kerr nonlinearity

Hyperentanglement, the entanglement in several degrees of freedom (DOFs) of a quantum system, has attracted much attention as it can be used to increase both the channel capacity of quantum communication and its security largely. Here, we present the first scheme to completely distinguish the hyperentangled Bell states of two-photon systems in three DOFs with the help of cross-Kerr nonlinearity without destruction, including two longitudinal momentum DOFs and the polarization DOF. We use cross-Kerr nonlinearity to construct quantum nondemolition detectors which can be used to make a parity-check measurement and analyze Bell states of two-photon systems in different DOFs. Our complete scheme for two-photon six-qubit hyperentangled Bell-state analysis may be useful for the practical applications in quantum information, especially in long-distance high-capacity quantum communication.

quant-ph↗

arXiv2016

Shortcuts to adiabatic holonomic quantum computation in decoherence-free subspace with transitionless quantum driving algorithm

By using transitionless quantum driving algorithm (TQDA), we present an efficient scheme for the shortcuts to the holonomic quantum computation (HQC). It works in decoherence-free subspace (DFS) and the adiabatic process can be speeded up in the shortest possible time. More interestingly, we give a physical implementation for our shortcuts to HQC with nitrogen-vacancy centers in diamonds dispersively coupled to a whispering-gallery mode microsphere cavity. It can be efficiently realized by controlling appropriately the frequencies of the external laser pulses. Also, our scheme has good scalability with more qubits. Different from previous works, we first use TQDA to realize a universal HQC in DFS, including not only two noncommuting accelerated single-qubit holonomic gates but also a accelerated two-qubit holonomic controlled-phase gate, which provides the necessary shortcuts for the complete set of gates required for universal quantum computation. Moreover, our experimentally realizable shortcuts require only two-body interactions, not four-body ones, and they work in the dispersive regime, which relax greatly the difficulty of their physical implementation in experiment. Our numerical calculations show that the present scheme is robust against decoherence with current experimental parameters.

quant-ph↗

arXiv2015

Quantum Zeno and Zeno-like effects in nitrogen vacancy centers

We present a proposal to realize the quantum Zeno effect (QZE) and quantum Zeno-like effect (QZLE) in a proximal $\mathrm{^{13}C}$ nuclear spin by controlling a proximal electron spin of a nitrogen vacancy (NV) center. The measurement is performed by applying a microwave pulse to induce the transition between different electronic spin states. Under the practical experimental conditions, our calculations show that there exist both QZE and QZLE in a $^{13}$C nuclear spin in the vicinity of an NV center.

quant-ph↗

arXiv2015

Optical Properties of Drug Metabolites in Latent Fingermarks

Drug metabolites usually have structures of split-ring resonators (SRRs), which might lead to negative permittivity and permeability in electromagnetic field. As a result, in the UV-vis region, the latent fingermarks images of drug addicts and non drug users are inverse. The optical properties of latent fingermarks are quite different between drug addicts and non-drug users. This is a technic superiority for crime scene investigation to distinguish them. In this paper, we calculate the permittivity and permeability of drug metabolites using tight-binding model. The latent fingermarks of smokers and non-smokers are given as an example.

physics.med-ph↗

arXiv2015

Stability and phase transition of localized modes in Bose-Einstein condensates with both two- and three-body interactions

We investigate the stability and phase transition of localized modes in Bose-Einstein Condensates (BECs) in an optical lattice with the discrete nonlinear Schrödinger model by considering both two- and three-body interactions. We find that there are three types of localized modes, bright discrete breather (DB), discrete kink (DK), and multi-breather (MUB). Moreover, both two- and three-body on-site repulsive interactions can stabilize DB, while on-site attractive three-body interactions destabilize it. There is a critical value for the three-body interaction with which both DK and MUB become the most stable ones. We give analytically the energy thresholds for the destabilization of localized states and find that they are unstable (stable) when the total energy of the system is higher (lower) than the thresholds. The stability and dynamics characters of DB and MUB are general for extended lattice systems. Our result is useful for the blocking, filtering, and transfer of the norm in nonlinear lattices for BECs with both two- and three-body interactions.

cond-mat.quant-gas↗

arXiv2015

Quantum information processing on nitrogen-vacancy ensembles with the local resonance assisted by circuit QED

With the local resonant interaction between a nitrogen-vacancy-center ensemble (NVE) and a superconducting coplanar resonator, and the single-qubit operation, we propose two protocols for the state transfer between two remote NVEs and for fast controlled-phase (c-phase) on these NVEs, respectively. This hybrid quantum system is composed of two distant NVEs coupled to separated high-Q transmission line resonators (TLRs), which are interconnected by a current-biased Josephsonjunction superconducting phase qubit. The fidelity of our state-transfer protocol is about 99.65% within the operation time of 70.60 ns. The fidelity of our c-phase gate is about 98.23% within the operation time of 93.87 ns. Furthermore, using the c-phase gate, we construct a two-dimensional cluster state on NVEs in n*n square grid based on the hybrid quantum system for the one-way quantum computation. Our protocol may be more robust, compared with the one based on the superconducting resonators, due to the long coherence time of NVEs at room temperature.

quant-ph↗

arXiv2014

An Efficient Quantum Jump Method for Coherent Energy Transfer Dynamics in Photosynthetic Systems under the Influence of Laser Fields

We present a non-Markovian quantum jump approach for simulating coherent energy transfer dynamics in molecular systems in the presence of laser fields. By combining a coherent modified Redfield theory (CMRT) and a non-Markovian quantum jump (NMQJ) method, this new approach inherits the broad-range validity from the CMRT and highly efficient propagation from the NMQJ. To implement NMQJ propagation of CMRT, we show that the CMRT master equation can be casted into a generalized Lindblad form. Moreover, we extend the NMQJ approach to treat time-dependent Hamiltonian, enabling the description of excitonic systems under coherent laser fields. As a benchmark of the validity of this new method, we show that the CMRT-NMQJ method accurately describes the energy transfer dynamics in a prototypical photosynthetic complex. Finally, we apply this new approach to simulate the quantum dynamics of a dimer system coherently excited to coupled single-excitation states under the influence of laser fields, which allows us to investigate the interplay between the photoexcitation process and ultrafast energy transfer dynamics in the system. We demonstrate that laser-field parameters significantly affect coherence dynamics of photoexcitations in excitonic systems, which indicates that the photoexcitation process must be explicitly considered in order to properly describe photon-induced dynamics in photosynthetic systems. This work should provide a valuable tool for efficient simulations of coherent control of energy flow in photosynthetic systems and artificial optoelectronic materials.

quant-ph↗

arXiv2014

Molecular Split-Ring Resonators Based on Metal String Complexes

Metal string complexes or extended metal atom chains (EMACs) belong to a family of molecules that consist of a linear chain of directly bonded metal atoms embraced helically by four multidentate organic ligands. These four organic ligands are usually made up of repeating pyridyl units, single-nitrogen-substituted heterocyclic annulenes, bridged by independent amido groups. Here, in this paper, we show that these heterocyclic annulenes are actually nanoscale molecular split-ring resonators (SRRs) that can exhibit simultaneous negative electric permittivity and magnetic permeability in the UV-Vis region. Moreover, a monolayer of self-assembled EMACs is a periodic array of molecular SRRs which can be considered as a negative refractive index material. In the molecular scale, where the quantum-size effect is significant, we apply the tight-binding method to obtain the frequency-dependent permittivity and permeability of these molecular SRRs with their tensorial properties carefully considered.

physics.optics↗

arXiv2013

Clustered Geometries Exploiting Quantum Coherence Effects for Efficient Energy Transfer in Light Harvesting

Elucidating quantum coherence effects and geometrical factors for efficient energy transfer in photosynthesis has the potential to uncover non-classical design principles for advanced organic materials. We study energy transfer in a linear light-harvesting model to reveal that dimerized geometries with strong electronic coherences within donor and acceptor pairs exhibit significantly improved efficiency, which is in marked contrast to predictions of the classical Förster theory. We reveal that energy tuning due to coherent delocalization of photoexcitations is mainly responsible for the efficiency optimization. This coherence-assisted energy-tuning mechanism also explains the energetics and chlorophyll arrangements in the widely-studied Fenna-Matthews-Olson complex. We argue that a clustered network with rapid energy relaxation among donors and resonant energy transfer from donor to acceptor states provides a basic formula for constructing efficient light-harvesting systems, and the general principles revealed here can be generalized to larger systems and benefit future innovation of efficient molecular light-harvesting materials.

physics.bio-ph↗

arXiv2012

The transition from Quantum Zeno to anti-Zeno effects for a qubit in a cavity by modulating the cavity frequency

We propose a strategy to demonstrate the transition from the quantum Zeno effect (QZE) to the anti-Zeno effect (AZE) by modulating the central frequency of the cavity mode. Our results are obtained without using the rotating wave approximation (RWA), and the initial state (a dressed state) is easy to prepare. When the central frequency of the cavity mode is resonant with the qubit energy level spacing, the normalized decay rate of the qubit is lower than 1, which manifests the QZE. However, when the cavity frequency is detuned from resonance, the normalized decay rate becomes larger than 1, which corresponds to the AZE. The change from the QZE to the AZE, by just varying the central frequency of the cavity mode, should allow to distinguish these two different effects. Moreover, we find that in the presence of both qubit's intrinsic bath and the cavity bath, the emergence of the QZE and the AZE behaviors relies not only on the match between the qubit energy level spacing and the central frequency of the cavity mode, but also on the coupling strength between the qubit and the cavity mode.

quant-ph↗

arXiv2012

Quantum statistics of the collective excitations of an atomic ensemble inside a cavity

We study the quantum statistical properties of the collective excitations of an atomic ensemble inside a high-finesse cavity. In the large-detuning regime, it is found that the virtual photon exchange can induce a long-range interaction between atoms, which results in correlated excitations. In particular, the atomic blockade phenomenon occurs when the induced long-range interaction effectively suppresses the double atomic excitation, when the average photon number takes certain values, which makes the two nearest energy levels degenerate. We also show that quantum phase transitions occur in the indirectly-interacting atomic ensemble when the average photon number reaches several critical points. In this sense, the quantum statistical properties of the collective excitations are very sensitive to the change of the average photon number. Our model exhibits quantum phase transitions similar to the ones in the Lipkin-Meshkov-Glick model. Our proposal could be implemented in a variety of systems including cavity quantum electrodynamics (QED), Bose-Einstein condensates, and circuit QED.

quant-ph↗

arXiv2011

Generalized Holstein model for spin-dependent electron transfer reaction

Some chemical reactions are described by electron transfer (ET) processes. The underlying mechanism could be modeled as a polaron motion in the molecular crystal-the Holstein model. By taking spin degrees of freedom into consideration, we generalize the Holstein model (molecular crystal model) to microscopically describe an ET chemical reaction. In our model, the electron spins in the radical pair simultaneously interact with a magnetic field and their nuclear-spin environments. By virtue of the perturbation approach, we obtain the chemical reaction rates for different initial states. It is discovered that the chemical reaction rate of the triplet state demonstrates its dependence on the direction of the magnetic field while the counterpart of the singlet state does not. This difference is attributed to the explicit dependence of the triplet state on the direction when the axis is rotated. Our model may provide a possible candidate for the microscopic origin of avian compass.

quant-ph↗

arXiv2011

Sensitive Chemical Compass Assisted by Quantum Criticality

The radical-pair-based chemical reaction could be used by birds for the navigation via the geomagnetic direction. An inherent physical mechanism is that the quantum coherent transition from a singlet state to triplet states of the radical pair could response to the weak magnetic field and be sensitive to the direction of such a field and then results in different photopigments in the avian eyes to be sensed. Here, we propose a quantum bionic setup for the ultra-sensitive probe of a weak magnetic field based on the quantum phase transition of the environments of the two electrons in the radical pair. We prove that the yield of the chemical products via the recombination from the singlet state is determined by the Loschmidt echo of the environments with interacting nuclear spins. Thus quantum criticality of environments could enhance the sensitivity of the detection of the weak magnetic field.

quant-ph↗