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Qing-Feng Sun

Publications and source records attributed to Qing-Feng Sun.

At least 109 records · Page 6Linked to original sources

Molecular Collapse States in Elliptical Graphene/WSe2 Heterostructure Quantum Dots

In relativistic physics, both atomic collapse in heavy nucleus and Hawking radiation in black hole are predicted to occur through Klein tunneling process that couples particles and antiparticles. Recently, atomic collapse states (ACSs) were explicitly realized in graphene because of its relativistic Dirac excitation with large fine structure constant. However, essential role of the Klein tunneling on the ACSs remains elusive in experiment. Here we systematically study the quasibound states in elliptical graphene quantum dots (GQDs). Bonding and antibonding molecular collapse states formed by two coupled ACSs are observed in the elliptical GQDs. Our experiments, supported by theoretical calculations, indicate that the antibonding state of the ACSs will change into a Klein-tunneling-induced quasibound state, revealing deep connection between the ACSs and the Klein tunneling.

cond-mat.mes-hall↗

Magnetic field-tunable valley-contrasting pseudomagnetic confinement in graphene

Introducing quantum confinement has uncovered a rich set of interesting quantum phenomena and allows one to directly probe the physics of confined (quasi-)particles. In most experiments, however, electrostatic potential is the only available method to generate the quantum confinement in a continuous system. Here, we demonstrated experimentally that inhomogeneous pseudomagnetic fields in strained graphene can introduce exotic quantum confinement of massless Dirac fermions. The pseudomagnetic fields have opposite directions in the two distinct valleys of graphene. By tuning real magnetic field, the total effective magnetic fields in the two valleys are imbalanced. Then, we realized valley-contrasting spatial confinement, which lifts the valley degeneracy and results in field-tunable valley-polarized confined states in graphene. Our results provide a new avenue to manipulate the valley degree of freedom.

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Transport Theory of Half-quantized Hall Conductance in a Semi-magnetic Topological Insulator

Recently,a half-quantized Hall conductance (HQHC) plateau is experimentally observed in a semi-magnetic topological insulator heterostructure. However,the heterostructure is metallic with a nonzero longitudinal conductance, which contradicts the common belief that quantized Hall conductance is usually observed in insulators.In this work,we systematically study the surface transport of the semi-magnetic topological insulator with both gapped and gapless Dirac surfaces in the presence of dephasing process.In particular, we reveal that the HQHC is directly related to the half-quantized chiral current along the edge of a strongly dephasing metal. The Hall conductance keeps a half-quantized value for large dephasing strengths, while the longitudinal conductance varies with Fermi energies and dephasing strengths. Furthermore, we evaluate both the conductance and resistance as a function of the temperature, which is consistent with the experimental results.Our results not only provide the microscopic transport mechanism of the HQHC,but also are instructive for the probe of the HQHC in future experiments.

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Resonant tunneling in disordered borophene nanoribbons with line defects

Very recently, borophene has been attracting extensive and ongoing interest as the new wonder material with structural polymorphism and superior attributes, showing that the structural imperfection of line defects (LDs) occurs widely at the interface between $ν_{1/5}$ ($χ_3$) and $ν_{1/6}$ ($β_{12}$) boron sheets. Motivated by these experiments, here we present a theoretical study of electron transport through two-terminal disordered borophene nanoribbons (BNRs) with random distribution of LDs. Our results indicate that LDs could strongly affect the electron transport properties of BNRs. In the absence of LDs, both $ν_{1/5}$ and $ν_{1/6}$ BNRs exhibit metallic behavior, in agreement with experiments. While in the presence of LDs, the overall electron transport ability is dramatically decreased, but some resonant peaks of conductance quantum can be found in the transmission spectrum of any disordered BNR with arbitrary arrangement of LDs. These disordered BNRs exhibit metal-insulator transition by varying nanoribbon width with tunable transmission gap in the insulating regime. Furthermore, the bond currents present fringe patterns and two evolution phenomena of resonant peaks are revealed for disordered BNRs with different widths. These results may help for understanding structure-property relationships and designing LD-based nanodevices.

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Evidence for anisotropic spin-triplet Andreev reflection at the 2D van der Waals ferromagnet/superconductor interface

Fundamental symmetry breaking and relativistic spin-orbit coupling give rise to fascinating phenomena in quantum materials. Of particular interest are the interfaces between ferromagnets and common s-wave superconductors, where the emergent spin-orbit fields support elusive spin-triplet superconductivity, crucial for superconducting spintronics and topologically-protected Majorana bound states. Here, we report the observation of large magnetoresistances at the interface between a quasi-two-dimensional van der Waals ferromagnet Fe0.29TaS2 and a conventional s-wave superconductor NbN, which provides the possible experimental evidence for the spin triplet Andreev reflection and induced spin-triplet superconductivity at ferromagnet/superconductor interface arising from Rashba spin-orbit coupling. The temperature, voltage, and interfacial barrier dependences of the magnetoresistance further support the induced spin-triplet superconductivity and spin-triplet Andreev reflection. This discovery, together with the impressive advances in two-dimensional van der Waals ferromagnets, opens an important opportunity to design and probe superconducting interfaces with exotic properties.

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Spin-triplet superconductor$-$quantum anomalous Hall insulator$-$spin-triplet superconductor Josephson junctions: $0$-$π$ transition, $ϕ_{0}$ phase and switch effects

We study the Josephson effect in spin-triplet superconductor$-$quantum anomalous Hall insulator$-$spin-triplet superconductor junctions using the nonequilibrium Green function method. The current-phase difference relations show strong dependence on the orientations of the $\bf{d}$-vectors in superconductors. We focus on two $\bf{d}$-vector configurations, the parallel one with the left and right ${\bf{d}}$-vectors being in the same direction, and the nonparallel one with the left ${\bf{d}}$-vector fixed at the $z$-axis. For the parallel configuration, the $0$-$π$ transition can be realized when one rotates the ${\bf{d}}$-vectors from the parallel to the junction plane to the perpendicular direction. The $ϕ_{0}$ phase with nonzero Josephson current at zero phase difference can be obtained as long as ${d_{x}}{d_{z}}\ne0$. For the nonparallel configuration, the $0$-$π$ transition and the $ϕ_{0}$ phase still exist. The condition for the formation of the $ϕ_{0}$ phase becomes $d_{Rx}\ne0$. The switch effects of the Josephson current are found in both configurations when the ${\bf{d}}$-vectors are rotated in the $xy$ plane. Furthermore, the symmetries satisfied by the current-phase difference relations are analysed in details by the operations of the time-reversal, mirror-reflections, the spin-rotation and the gauge transformation, which can well explain the above selection rules for the $ϕ_{0}$ phase. Our results reveal the peculiar Josephson effect between spin-triplet superconductors and the quantum anomalous Hall insulator, which provide helpful phases and effects for the device designs. The distinct current-phase difference relations for different orientations may be used to determine the direction of the ${\bf{d}}$-vector in the spin-triplet superconductor.

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Coexistence of electron whispering-gallery modes and atomic collapse states in graphene WSe2 heterostructure quantum dots

The relativistic massless charge carriers with a Fermi velocity of about c300 in graphene enable us to realize two distinct types of resonances (c, the speed of light in vacuum). One is electron whispering-gallery mode in graphene quantum dots arising from the Klein tunneling of the massless Dirac fermions. The other is atomic collapse state, which has never been observed in experiment with real atoms due to the difficulty of producing heavy nuclei with charge Z 170, however, can be realized near a Coulomb impurity in graphene with a charge Z 1 because of the small velocity of the Dirac excitations. Here, unexpectedly, we demonstrate that both the electron whispering-gallery modes and atomic collapse states coexist in grapheneWSe2 heterostructure quantum dots due to the Coulomb-like potential near their edges. By applying a perpendicular magnetic field, evolution from the atomic collapse states to unusual Landau levels in the collapse regime are explored for the first time.

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Multi-orbital model reveals second-order topological insulator in 1H-transition metal dichalcogenide

Recently, a new class of second-order topological insulators (SOTIs) characterized by an electronic dipole has been theoretically introduced and proposed to host topological corner states. As a novel topological state, it has been attracting great interest and experimentally realized in artificial systems of various fields of physics based on multi-sublattice models, e.g., breathing kagome lattice. In order to realize such kind of SOTI in natural materials, we proposed a symmetry-faithful multi-orbital model. Then, we reveal several familiar transition metal dichalcogenide (TMD) monolayers as a material family of two-dimensional SOTI with large bulk gaps. The topologically protected corner state with fractional charge is pinned at Fermi level due to the charge neutrality and filling anomaly. Additionally, we propose that the zero-energy corner state preserves in the heterostructure composed of a topological nontrivial flake embedded in a trivial material. The novel second-order corner states in familiar TMD materials hold promise for revealing unexpected quantum properties and applications.

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Continuously Tunable Berry Phase and Valley-Polarized Energy Spectra in Bilayer Graphene Quantum Dots

Berry phase plays an important role in determining many physical properties of quantum systems. However, a Berry phase altering energy spectrum of a quantum system is comparatively rare. Here, we report an unusual tunable valley polarized energy spectra induced by continuously tunable Berry phase in Bernal-stacked bilayer graphene quantum dots. In our experiment, the Berry phase of electron orbital states is continuously tuned from about pi to 2pi by perpendicular magnetic fields. When the Berry phase equals pi or 2pi, the electron states in the two inequivalent valleys are energetically degenerate. By altering the Berry phase to noninteger multiples of pi, large and continuously tunable valley polarized energy spectra are detected in our experiment. The observed Berry phase-induced valley splitting, on the order of 10 meV at a magnetic field of 1 T, is about 100 times larger than Zeeman splitting for spin, shedding light on graphene-based valleytronics.

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Charge transport in a multi-terminal DNA tetrahedron: Interplay among contact position, disorder, and base-pair mismatch

As a secondary structure of DNA, DNA tetrahedra exhibit intriguing charge transport phenomena and provide a promising platform for wide applications like biosensors, as shown in recent electrochemical experiments. Here, we study charge transport in a multi-terminal DNA tetrahedron, finding that its charge transport properties strongly depend upon the interplay among contact position, on-site energy disorder, and base-pair mismatch. Our results indicate that the charge transport efficiency is nearly independent of contact position in the weak disorder regime, and is dramatically declined by the occurrence of a single base-pair mismatch between the source and the drain, in accordance with experimental results [J. Am. Chem. Soc. {\bf 134}, 13148 (2012); Chem. Sci. {\bf 9}, 979 (2018)]. By contrast, the charge transport efficiency could be enhanced monotonically by shifting the source toward the drain in the strong disorder regime, and be increased when the base-pair mismatch takes place exactly at the contact position. In particular, when the source moves successively from the top vertex to the drain, the charge transport through the tetrahedral DNA device can be separated into three regimes, ranging from disorder-induced linear decrement of charge transport to disorder-insensitive charge transport, and to disorder-enhanced charge transport. Finally, we predict that the DNA tetrahedron functions as a more efficient spin filter compared to double-stranded DNA and opposite spin polarization could be observed at different drains, which may be used to separate spin-unpolarized electrons into spin-up ones and spin-down ones. These results could be readily checked by electrochemical measurements and may help for designing novel DNA tetrahedron-based molecular nanodevices.

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Specular Andreev reflection and its detection

We propose a universal method to detect the specular Andreev reflection taking the simple two dimensional Weyl nodal-line semimetal-superconductor double-junction structure as an example. The quasiclassical quantization conditions are established for the energy levels of bound states formed in the middle semimetal along a closed path. The establishment of the conditions is completely based on the intrinsic character of the specularly reflected hole which has the same sign relation of its wave vector and group velocity with the incident electron. This brings about the periodic oscillation of conductance with the length of the middle semimetal, which is lack for the retro-Andreev reflected hole having the opposite sign relation with the incident electron. The positions of the conductance peaks and the oscillation period can be precisely predicted by the quantization conditions. Our detection method is irrespective of the details of the materials, which may promote the experimental detection of and further researches on the specular Andreev reflection as well as its applications in superconducting electronics.

cond-mat.supr-con↗

Spatial and Magnetic Confinement of Massless Dirac Fermions

The massless Dirac fermions and the ease to introduce spatial and magnetic confinement in graphene provide us unprecedented opportunity to explore confined relativistic matter in this condensed-matter system. Here we report the interplay between the confinement induced by external electric fields and magnetic fields of the massless Dirac fermions in graphene. When the magnetic length lB is larger than the characteristic length of the confined electric potential lV, the spatial confinement dominates and a relatively small critical magnetic field splits the spatial-confinement-induced atomic-like shell states by switching on a pi Berry phase of the quasiparticles. When the lB becomes smaller than the lV, the transition from spatial confinement to magnetic confinement occurs and the atomic-like shell states condense into Landau levels (LLs) of the Fock-Darwin states in graphene. Our experiment demonstrates that the spatial confinement dramatically changes the energy spacing between the LLs and generates large electron-hole asymmetry of the energy spacing between the LLs. These results shed light on puzzling observations in previous experiments, which hitherto remained unaddressed.

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Noise signatures for determining chiral Majorana fermion modes

The conductance measurement of a half quantized plateau in a quantum anomalous Hall insulator-superconductor structure is reported by a recent experiment [Q. L. He \textit{et al.}, Science 357, 294-299 (2017)], which suggests the existence of the chiral Majorana fermion modes. However, such half quantized conductance plateau may also originates from a disorder-induced metallic phase. To identify the exact mechanism, we study the transport properties of such a system in the presence of strong disorders. Our results show that the local current density distributions of these two mechanisms are different. In particular, the current noises measurement can be used to distinguish them without any further fabrication of current experimental setup.

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Spin-dependent electron transport along hairpin-like DNA molecules

The chirality-induced spin selectivity (CISS), demonstrated in diverse chiral molecules by numerous experimental and theoretical groups, has been attracting extensive and ongoing interest in recent years. As the secondary structure of DNA, the charge transfer along DNA hairpins has been widely studied for more than two decades, finding that DNA hairpins exhibit spin-related effects as reported in recent experiments. Here, we propose a setup to demonstrate directly the CISS effect in DNA hairpins contacted by two nonmagnetic leads at both ends of the stem. Our results indicate that DNA hairpins present pronounced CISS effect and the spin polarization could be enhanced by using conducting molecules as the loop. In particular, DNA hairpins show several intriguing features, which are different from other chiral molecules. First, the local spin currents can flow circularly and assemble into a number of vortex clusters when the electron energy locates in the left/right electronic band of the stem. The chirality of vortex clusters in each band is the same and will be reversed by switching the electron energy from the left band to the right one, inducing the sign reversal of the spin polarization. Interestingly, the local spin currents can be greater than the corresponding spin component of the source-drain current. Second, both the conductance and the spin polarization can increase with molecular length as well as dephasing strength, contrary to the physical intuition that the transmission ability of molecular wires should be poorer when suffering from stronger scattering. Third, we unveil the optimal contact configuration of efficient electron transport and that of the CISS effect, which are distinct from each other and can be controlled by dephasing strength. The underlying physical mechanism is illustrated.

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Ferromagnetic induced Kondo effect in graphene with a magnetic impurity

We investigate the many-body effects of a magnetic adatom in ferromagnetic graphene by using the numerical renormalization group method. The nontrivial band dispersion of ferromagnetic graphene gives rise to interesting Kondo physics different from that in conventional ferromagnetic materials. For a half-filled impurity in undoped graphene, the presence of ferromagnetism can bring forth Kondo correlations, yielding two kink structures in the local spectral function near the Fermi energy. When the spin splitting of local occupations is compensated by an external magnetic field, the two Kondo kinks merge into a full Kondo resonance characterizing the fully screened ground state. Strikingly, we find the resulting Kondo temperature monotonically increases with the spin polarization of Dirac electrons, which violates the common sense that ferromagnetic bands are usually detrimental to Kondo correlations. Doped ferromagnetic graphene can behave as half metals, where its density of states at the Fermi energy linearly vanishes for one spin direction but keeps finite for the opposite direction. In this regime, we demonstrate an abnormal Kondo resonance that occurs in the first spin direction, while completely absent in the other one.

cond-mat.str-el↗

Topological phase transitions of Thouless charge pumping realized in helical organic molecules with long-range hoppings

Recent studies indicated that helical organic molecules, such as DNA and $α$-helical protein, can behave as Thouless quantum pumps when a rotating electric field is applied perpendicularly to their helical axes. Here we investigate the influence of long-range hoppings on this topological pumping of electrons in single-helical organic molecules. Under variation of the long-range hoppings governed by a decay exponent $μ$, we find an energy gap in the molecular band structure closes at a critical value $μ_c$ of the decay exponent and reopens for $μ$ deviating from $μ_c$. The relevant bulk bands in a pumping cycle acquire different Chern numbers in the strong ($μ<μ_c$) and weak ($μ>μ_c$) long-range hopping regimes, with a sudden jump at criticality. This topological phase transition is also shown to separate two distinct behaviors of the midgap end states in the pumping process. The end states carry quantized current pumped by the rotating electric field and the current forms a plateau by sweeping the Fermi energy over the gap. In the strong hopping phase, the quantized current plateau is positive, which is reversed to a negative one with smaller amplitude in the weak hopping phase. However, the reversal is a smooth crossover, not a sharp transition, due to the finite sizes of the molecules. We show that these transport characteristics of the topological phase transition could also be observed at finite temperatures.

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Transport study of the wormhole effect in three-dimensional topological insulators

Inside a three-dimensional strong topological insulator, a tube with $h/2e$ magnetic flux carries a pair of protected one-dimensional linear fermionic modes. This phenomenon is known as the "wormhole effect". In this work, we find that the "wormhole effect", as a unique degree of freedom, introduces exotic transport phenomena and thus manipulates the transport properties of topological insulators. Our numerical results demonstrate that the transport properties of a double-wormhole system can be manipulated by the wormhole interference. Specifically, the conductance and local density of states both oscillate with the Fermi energy due to the interference between the wormholes. Furthermore, by studying the multi-wormhole systems, we find that the number of wormholes can also modulate the differential conductance through a $\mathbb{Z}$$_{2}$ mechanism. Finally, we propose two types of topological devices in real applications, the "wormhole switch" device and the "traversable wormhole" device, which can be finely tuned by controlling the wormhole degree of freedom.

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Enhancement of electron transport and bandgap opening in graphene induced by adsorbates

Impurities are unavoidable during the preparation of graphene samples and play an important role in graphene's electronic properties when they are adsorbed on graphene surface. In this work, we study the electronic structures and transport properties of a two-terminal zigzag graphene nanoribbon (ZGNR) device whose scattering region is covered by various adsorbates within the framework of the tight-binding approximation, by taking into account the coupling strength $γ$ between adsorbates and carbon atoms, the adsorbate concentration $n_i$, and the on-site energy disorder of adsorbates. Our results indicate that when the scattering region is fully covered by homogeneous adsorbates, i.e., $n_i=1$, a transmission gap opens around the Dirac point and its width is almost proportional to $γ^2$. In particular, two conductance plateaus of $G=2e^2/h$ appear in the vicinity of the electron energy $E=\pm γ$. When the scattering region is partially covered by homogeneous adsorbates ($0<n_i<1$), the transmission gap still survives around the Dirac point even at low $n_i$, and its width is firstly increased by $n_i$ and then declined by further increasing $n_i$; whereas the conductance decreases with $n_i$ in the regime of low $n_i$ and increases with $n_i$ in the regime of high $n_i$. While in the presence of disordered adsorbates whose on-site energies are random variables characterized by the disorder degree, the transmission gap disappears at low $n_i$ and reappears at relatively high $n_i$. Furthermore, the transmission ability of the ZGNR device can be enhanced by the adsorbate disorder when the disorder degree surpasses a critical value, contrary to the localization picture that the conduction of a nanowire becomes poorer with increasing the disorder degree. The physics underlying these transport characteristics is discussed. Our results are in good agreement with experiments.

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