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Qinxin Shen

Publications and source records attributed to Qinxin Shen.

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Universal Magnetocaloric Effect near Quantum Critical Point of Magnon Bose-Einstein Condensation

Bose-Einstein condensation (BEC), a macroscopic quantum phenomenon arising from phase coherence and bosonic statistics, has been realized in quantum magnets. Here, we report the observation of a universal magnetocaloric effect (MCE) near a BEC quantum critical point (QCP) in copper sulfate crystal ($CuSO_4 \cdot 5H_2O$). By conducting magnetocaloric and nuclear magnetic resonance measurements, we uncover a field-driven BEC QCP, evidenced by the universal scaling law $T_c \propto (B_c - B)^{2/3}$ and the perfect data collapse of the magnetic Gr\"uneisen ratio. Thermal excitation triggers a dimensional crossover to a 1D quantum-critical regime, where the MCE scaling strictly matches the universality class of 1D Fermi gases. Notably, the quantum-critical MCE enables cooling down to 12.8 mK without helium-3, with very fast thermal relaxation rate that is critical for high cooling power. This work demonstrates the universal MCE in magnon BEC systems, using a common copper sulfate compound as a paradigmatic example, and paves the way for next-generation sub-Kelvin cooling.

cond-mat.str-el

Magnetic ground states in kagome YCu$_3$(OH)$_6$[(Cl$_x$Br$_{1-x}$)$_{3-y}$(OH)$_{y}$]

Quantum spin liquids represent exotic states of spin systems characterized by long-range entanglement and emergent fractionalized quasiparticles. It is generally believed that disorder is hostile to quantum spin liquids. In our study, we investigated the magnetic properties of a kagome system, YCu$_3$(OH)$_6$[(Cl$_x$Br$_{1-x}$)$_{3-y}$(OH)$_{y}$]. Within this system, some of the hexagons exhibit alternate bonds along the Cu-O-Cu exchange paths, while others remain uniform. We found that a long-range antiferromagnetic order emerges when uniform hexagons dominate. Conversely, a possible quantum-spin-liquid state arises when the number of alternate-bond hexagons exceeds about 2/3. Therefore, the alternate-bond hexagons, typically considered as disorders, actually serve as the building blocks of the quantum spin liquid in this system. Notably, the low-temperature properties of the quantum spin liquid are directly associated with the height of the out-of-plane yttrium ions, which may be linked to changes in superexchange energies. Our results suggest that understanding the magnetic ground states in this system lies beyond the theoretical framework of the Heisenberg model constructed on the kagome lattice.

cond-mat.str-el