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Qiong Qin

Publications and source records attributed to Qiong Qin.

9 recordsLinked to original sources

Response tensor for the superconducting (Josephson) diode effect

We propose a response tensor $\mathbf{\hat χ}$ to characterize the non-reciprocal critical current response of the superconducting (Josephson) diode effect. It describes the coupling between the dipole component of the angular distribution of the critical current and the applied magnetic field -- an analogue to the Hall response in the normal state. In quasi-2D systems with Rashba spin-orbit coupling and point group symmetries $C_{3v}$, $C_{4v}$ or $C_{6v}$, this tensor takes a fully antisymmetric form. When nematicity is present, a symmetric contribution emerges, providing an indicator of the nematic order in the superconducting state. In contrast, for systems exhibiting Dresselhaus spin-orbit coupling with the $D_{2d}$ symmetry, the tensor becomes diagonal traceless, and nematicity brings in a trace part. Our analysis not only accounts for the superconducting diode effect under external applied or intrinsic effective magnetic fields, but also predicts the symmetry conditions for realizing the diode effect when the magnetic field is aligned with the current. Beyond this, the proposed tensor provides a promising tool for detecting nematicity and potential nematic transitions deep within the superconducting phase. It may also encode additional information about the underlying electronic structure and symmetry-breaking orders, warranting further experimental investigation.

cond-mat.supr-con

Chiral finite-momentum superconductivity in the tetralayer graphene

Motivated by the recent experimental discovery of superconductivity in rhombohedral tetralayer graphene, we investigate the pairing mechanism arising from the density-density interactions within the random-phase approximation. This approach successfully highlights the dominance of the chiral $p$-wave pairing between electrons with the same spin and valley index at low densities, while also predicting the superconducting range in agreement with experimental findings. Furthermore, we examine the characteristics of distinct superconducting regions: SC1 and SC2 exhibit chiral finite-momentum superconductivity with pronounced phase fluctuations, whereas SC4 displays zero-momentum spin-singlet superconductivity.

cond-mat.supr-con

Nonvolatile electric switching of critical current in cross-bar superconducting junctions

Superconducting (SC) diodes are key passive building blocks for future SC electronics. However, realizing their active counterparts is essential for functional logic. Here, we demonstrate deterministic nonvolatile electrical switching of the critical current ($I_\text{c}$) in overlap crossbar SC junctions. By applying a minimal perpendicular magnetic field ($H_\text{z}$), $I_\text{c}$ is modulated by a factor of four with a large switching efficiency of 60\%, achieved at a significantly reduced excitation current density of $5\times10^5$~A/cm$^2$. We also uncover anomalous behaviors: an electrically switchable critical temperature and a non-monotonic $I_\text{c}$-$H_\textit{z}$ response. These observations are interpreted in terms of unique asymmetry involving isolated vortex injection, configuration and repulsion inherent to the junction geometry. Our device provides a scalable, low-power alternative to complex SQUID-based architectures, paving the way for high-density SC integrated circuits.

cond-mat.supr-con

Revealing altermagnetic Fermi surfaces with two Kondo impurities

Motivated by recent advances in the study of altermagnetism, or unconventional magnetism, and in the realization and manipulation of two-impurity Kondo physics in real materials, we propose a phase-sensitive method to explore unconventional magnetic symmetries. Our method can be implemented with spin-resolved scanning tunneling microscopy to study two-impurity Kondo phenomena on altermagnetic metals by varying the distance and orientation between magnetic impurities. Using quantum Monte Carlo simulations, we analyze the spin splitting of the Kondo resonance, whose spatial distribution sensitively captures the symmetry of the underlying altermagnetic order. Furthermore, the impurity spin correlations reflects the anisotropy of the RKKY interaction due to the altermagnetic Fermi surface splitting. This work provides a framework for studying the competition between the Kondo effect, the RKKY interaction and altermagnetism, in the simplest possible system.

cond-mat.str-el

Emergent superconducting stripes in two-orbital superconductors

Motivated by recent experiments in KTaO$_3$/EuO interface, we propose an intrinsic mechanism where superconducting stripes emerge naturally without involving disorder, charge inhomogeneity, or competing orders. Our theory is based on a two-orbital model of superconductivity, where one orbital displays a quasi-one-dimensional dispersion and the other orbital is more localized and contributes pairing interactions along the perpendicular direction. Our auxiliary-field Monte Carlo simulations demonstrate that the pairing amplitude exhibits spatial modulation such that the superconductivity naturally disaggregates into two-leg or three-leg superconducting stripes separated by non-superconducting blocks. Our work provides a promising scenario of emergent superconducting stripes in homogeneous two-dimensional systems and reveals unexpectedly rich physics in two-orbital superconductors for future materials design.

cond-mat.supr-con

Intrinsic constraint on $T_c$ for unconventional superconductivity

Can room temperature superconductivity be achieved in correlated materials under ambient pressure? Our answer to this billion-dollar question is probably no, at least for realistic models within the current theoretical framework. This is shown by our systematic simulations on the pairing instability of some effective models for two-dimensional superconductivity. For a square lattice model with nearest-neighbour pairing, we find a plaquette state formed of weakly-connected $2\times2$ blocks for sufficiently large pairing interaction. The superconductivity is suppressed on both sides away from its melting quantum critical point. Thus, the magnitude of $T_c$ is constrained by the plaquette state for the $d$-wave superconductivity, in resemblance of other competing orders. We then extend our simulations to a variety of effective models covering nearest-neighbour or onsite pairings, single layer or two-layer structures, intralayer or interlayer pairings, and find an intrinsic maximum of the ratio $T_c/J\approx 0.04-0.07$, where $J$ is the pairing interaction. Comparison with existing experiments supports this constraint in cuprate, iron-based, nickelate, and heavy fermion superconductors, despite that these compounds are so complicated well beyond our simplified models. As a result, the known families of unconventional superconductivity, possibly except the infinite-layer nickelates, seem to almost exhaust their potentials in reaching the maximal $T_c$ allowed by their respective $J$, while achieving room temperature superconductor would require a much larger $J$ beyond 400-700 meV, which seems unrealistic in existing correlated materials and hence demands novel pairing mechanisms. The agreement also implies some deep underlying principles of the constraint that urge for a more rigorous theoretical understanding.

cond-mat.supr-con

Frustrated superconductivity and intrinsic reduction of $T_c$ in trilayer nickelate

Identifying the key factors controlling the magnitude of $T_c$ is of critical importance in the pursuit of high-temperature superconductivity. In cuprates, $T_c$ reaches its maximal value in trilayer structure, leading to the belief that interlayer coupling may help promote the pairing. In contrast, for the recently discovered nickelate superconductors under high pressure, the maximum $T_c$ is reduced from about 80 K in the bilayer La$_3$Ni$_2$O$_{7}$ to 30 K in the trilayer La$_4$Ni$_3$O$_{10}$. Motivated by this opposite trend, we propose an interlayer pairing scenario for the superconductivity of La$_4$Ni$_3$O$_{10}$. Our theory reveals intrinsic frustration in the spin-singlet pairing that the inner layer tends to form with both of the two outer layers respectively, leading to strong superconducting fluctuations between layers. This explains the reduction of its maximum $T_c$ compared to that of the bilayer La$_3$Ni$_2$O$_{7}$. Our findings support a fundamental distinction between multilayer nickelate and cuprate superconductors, and ascribe it to their different (interlayer versus intralayer) pairing mechanisms. Furthermore, our theory predicts extended $s^\pm$-wave gap structures in La$_4$Ni$_3$O$_{10}$, with varying signs and possible nodes on different Fermi pockets. We also find an intrinsic Josephson coupling with potentially interesting consequences that may be examined in future experiments. Our work reveals the possibility of rich novel physics in multilayer superconductors with interlayer pairing.

cond-mat.supr-con

High-$T_c$ superconductivity by mobilizing local spin singlets and possible route to higher $T_c$ in pressurized La$_3$Ni$_2$O$_7$

We clarify the pairing mechanism of high-$T_c$ superconductivity in bilayer La$_3$Ni$_2$O$_7$ under high pressure by employing the static auxiliary field Monte Carlo approach to simulate a minimal effective model that contains local $d_{z^2}$ interlayer spin singlets and metallic $d_{x^2-y^2}$ bands. Superconductivity is induced when the local spin singlet pairs are mobilized and attain long-distance phase coherence by hybridization with the metallic bands. When projected onto realistic Fermi surfaces, it yields a nodeless $s$-wave gap on the $γ$ Fermi surface, and extended $s$-wave gaps of the same (opposite) sign on the $α$ ($β$) Fermi surface due to its bonding (antibonding) character, with nodes or gap minima along the diagonal direction of the two-dimensional Brillouin zone. We find a dual role of the hybridization that not only induces global phase coherence but also competes with the spin singlet formation. This lead to a tentative phase diagram where $T_c$ varies nonmonotonically with the hybridization, in good correspondence with experimental observations. A roughly linear relation is obtained for realistic hopping and hybridization parameters: $T_c\approx 0.04-0.05 J$, where $J$ is the interlayer superexchange interaction. We emphasize the peculiar tunability of the bilayer structure and propose that $T_c$ may be further enhanced by hole doping or applying uniaxial pressure along the $c$ axis on superconducting La$_3$Ni$_2$O$_7$. Our work provides reliable numerical evidence for the pairing mechanism of high-$T_c$ superconductivity in La$_3$Ni$_2$O$_7$ and points out a potential route to achieve even higher $T_c$.

cond-mat.supr-con

Superconducting fluctuations and charge-4$e$ plaquette state at strong coupling

We apply the static auxiliary field Monte Carlo approach to study phase correlations of the pairing fields in a microscopic model with spin-singlet pairing interaction. We find that the short- and long-range phase correlations are well captured by the phase mutual information, which allows us to construct a theoretical phase diagram containing the uniform $d$-wave superconducting region, the phase fluctuating region, the local pairing region, and the disordered region. We show that the gradual development of phase coherence has a number of consequences on spectroscopic measurements, such as the development of the Fermi arc and the anisotropy in the angle-resolved spectra, scattering rate, entropy, specific heat, and quasiparticle dispersion, in good agreement with experimental observations. For strong coupling, our Monte Carlo simulation reveals an unexpected charge-4$e$ plaquette state with $d$-wave bonds, which competes with the uniform $d$-wave superconductivity and exhibits a U-shaped density of states.

cond-mat.supr-con