arXiv subjects

Qiuyu Shang

Publications and source records attributed to Qiuyu Shang.

9 recordsLinked to original sources

arXiv2026

Cavity-enhanced superconductivity in the two-dimensional limit of NbSe2

Vacuum electromagnetic fluctuations have emerged as a means of controlling collective quantum phases without external driving. Cavity-induced modification of superconductivity has been widely predicted. What sets the size of the effect, and which microscopic channel carries it, remain open. Here we couple few-layer NbSe2 to a terahertz complementary split-ring resonator (CSRR) and show that the enhancement grows sharply on approaching the two-dimensional limit. In bilayer NbSe2 the superconducting transition temperature rises by 10%, from 3.02 K to 3.41 K, on a cavity resonant at 0.92 THz - roughly four times the shift measured in a ten-layer device at the same resonance. Within a single device the shift maps onto the simulated cavity field profile, falling from 0.39 K at the field maximum to zero outside the resonator, with the lower critical field following the same spatial ordering; because all regions are measured on one continuous flake in a single cooldown, sample-to-sample variation is excluded by construction. The frequency dependence is non-monotonic, with suppression below resonance and maximal enhancement near 0.96 THz. Quantum electrodynamical density functional theory calculations show that cavity coupling redistributes spectral weight in the Eliashberg function, weakening the total electron-phonon coupling while hardening the logarithmic average phonon frequency; competition between the two reproduces a sign change in Tc. These results identify dimensionality, local field amplitude and detuning as the control parameters of cavity-enhanced superconductivity, and point to electron-phonon reweighting as its microscopic origin.

cond-mat.supr-con↗

arXiv2025

Electronic Phonons in a Moiré Electron Crystal

Collective quantum phenomena, such as the excitation of composite fermions1, spin waves2, and exciton condensation3,4, can emerge in strongly correlated systems like the fractional quantum Hall states5, spin liquids6, or excitonic insulators7. Two-dimensional (2D) moiré superlattices have emerged as a powerful platform for exploring such correlated phases and their associated collective excitations8,9. Specifically, electron crystals stabilized by longrange Coulomb interactions may host collective vibrational excitations emerging from electron correlations10, termed electronic phonons, which are fundamentally distinct from atomic lattice phonons. Despite theoretical prediction of their existence in moiré electron crystals11, direct experimental evidence has remained elusive. Here we report the observation of electronic phonons in the Mott insulating and stripe phases of a WS2/WSe2 moiré superlattice, achieved through light scattering measurements. The phonon energies, temperature and filling factor dependencies, along with theoretical modeling, corroborate their origin as collective vibrations of a correlated electron crystal. Polarization-resolved measurements further indicate rotational symmetry breaking in the Mott state. Notably, these electronic phonons exhibit strong tunability in energy, intensity, and polarization under external electric or magnetic fields, highlighting rich and controllable lattice dynamics of the electron crystal. These findings provide direct spectroscopic evidence for the electronic crystalline nature of correlated phases, opening avenues for probing and manipulating collective excitations in correlated electron systems.

cond-mat.str-el↗

arXiv2024

Room temperature spin-layer locking of exciton-polariton nonlinearities

Recent advancements in transition metal dichalcogenides (TMDs) have unveiled exceptional optical and electronic characteristics, opened up new opportunities, and provided a unique platform for exploring light-matter interactions under the strong coupling regime. The exploitation of exciton-polaritons, with their peculiar hybrid light-matter properties, for the development of spintronic customizable devices that enhance both the information capacity and functionality at ambient temperatures is often suggested as a promising route. However, although TMD polaritons have shown promising potential, the microscopic mechanisms leading to nonlinearities in TMD polaritons are complex and their spin-anisotropy, a crucial requirement for many proposed polaritonic devices, has been missing. Here, we demonstrate the absence of spin-anisotropic interaction in a monolayer WS2 microcavity (at room temperature) and show how spin-dependent interactions can be controlled and spin anisotropy recovered by engineering double WS2 layer structures with varied interlayer spacing. We attribute this phenomenon to a distinctive feature in exciton-polariton physics: layer-dependent polariton-phonon coupling. We use theoretical calculations of the phonon electrostatic potentials finding a drastically different coupling strength for single and double monolayer samples and discuss qualitatively how this explains the observed spin-anisotropic response. This is further consistent with experiments on multi WS2 layer samples and the identification of a critical separation distance, above which an effective single monolayer spin-anisotropic response is recovered, both in experiment and theory. Our work lays the groundwork for the development of spin-optronic polaritonic devices at room temperature.

physics.optics↗

arXiv2024

Observation of Ferromagnetic Phase in the Second Moiré Band of Twisted MoTe2

Flat bands and electron correlation in moiré lattices give rise to many exotic phases, including Mott insulators, superconductivity, and topological states. Within the first moiré band, integer and fractional quantum anomalous Hall effects have been observed in twisted bilayer MoTe2 (tMoTe2) at one hole doping and fractional doping per moiré unit cell, respectively. When the second moiré band is fully hole doped, quantum spin Hall insulator has also been reported in tMoTe2 at a certain twist angle. Exotic topological states together with ferromagnetic (FM) states in the high moiré band can potentially exist as well. In this study, we report the observation of a FM phase in the second moiré band in tMoTe2. The FM phase can be tuned by both the doping level and displacement field. At filling around 2.58 holes per moiré unit cell, the FM phase reaches a Curie temperature of 3.5 K. A large displacement field can suppress the FM phase, like the FM phase at the filling of -1. Our results demonstrate the realization of time-reversal symmetry-breaking states in the higher moiré bands in tMoTe2.

cond-mat.mes-hall↗

arXiv2024

Room-temperature continuous-wave pumped exciton polariton condensation in a perovskite microcavity

Microcavity exciton polaritons (polaritons) as part-light part-matter quasiparticles, garner significant attention for non-equilibrium Bose-Einstein condensation at elevated temperatures. Recently, halide perovskites have emerged as promising room-temperature polaritonic platforms thanks to their large exciton binding energies and superior optical properties. However, currently, inducing room-temperature non-equilibrium polariton condensation in perovskite microcavities requires optical pulsed excitations with high excitation densities. Herein, we demonstrate continuous-wave optically pumped polariton condensation with an exceptionally low threshold of ~0.6 W cm-2 and a narrow linewidth of ~1 meV. Polariton condensation is unambiguously demonstrated by characterizing the nonlinear behavior and coherence properties. We also identify a microscopic mechanism involving the potential landscape in the perovskite microcavity, where numerous discretized energy levels arising from the hybridization of adjacent potential minima enhance the polariton relaxation, facilitating polariton condensate formation. Our findings lay the foundation for the next-generation energy-efficient polaritonic devices operating at room temperature.

physics.optics↗

arXiv2022

Antiphase boundary in CH$_3$NH$_3$PbI$_3$ repels charge carriers while promotes fast ion migrations

Defects in organic-inorganic hybrid perovskites (OIHPs) greatly influence their optoelectronic properties. Identification and better understanding of defects existing in OIHPs is an essential step towards fabricating high-performance perovskite solar cells. However, direct visualizing the defects is still a challenge for OIHPs due to their sensitivity during electron microscopy characterizations. Here, by using low dose scanning transmission electron microscopy techniques, we observe the common existence of antiphase boundary (APB) in CH$_3$NH$_3$PbI$_3$ (MAPbI$_3$), resolve its atomic structure, and correlate it to the electrical/ionic activities and structural instabilities. Such an APB is caused by the half-unit-cell shift of [PbI$_6$]$_4$-octahedron along the [100]/[010] direction, leading to the transformation from corner-sharing [PbI$_6$]$_4$-octahedron in bulk MAPbI$_3$ into edge-sharing ones at the APB. Based on the identified atomic-scale configuration, we further carry out density functional theory calculations and reveal that the APB in MAPbI$_3$ repels both electrons and holes while serves as a fast ion-migration channel, causing a rapid decomposition into PbI$_2$ that is detrimental to optoelectronic performance. These findings provide valuable insights into the relationships between structures and optoelectronic properties of OIHPs and suggest that controlling the APB is essential for their stability.

physics.app-ph↗

arXiv2018

Room Temperature Continuous-wave Excited Biexciton Emission in CsPbBr3 Nanocrystals

Biexcitons are a manifestation of many-body excitonic interactions crucial for quantum information and quantum computation in the construction of coherent combinations of quantum states. However, due to their small binding energy and low transition efficiency, most biexcitons in conventional semiconductors exist either at cryogenic temperature or under femtosecond pulse laser excitation. Here we demonstrate room temperature, continuous wave driven biexciton states in CsPbBr3 perovskite nanocrystals through coupling with a plasmonic nanogap. The room temperature CsPbBr3 biexciton excitation fluence (~100 mW/cm2) is reduced by ~10^13 times in the Ag nanowire-film nanogaps. The giant enhancement of biexciton emission is driven by coherent biexciton-plasmon Fano interference. These results provide new pathways to develop high efficiency non-blinking single photon sources, entangled light sources and lasers based on biexciton states.

cond-mat.mes-hall↗

arXiv2017

Surface Plasmon Enhanced Strong Exciton-Photon Coupling in Hybrid Inorganic-Organic Perovskites Nanowires

Manipulating strong light-matter interaction in semiconductor microcavities is crucial for developing high-performance exciton polariton devices with great potentials in next-generation all-solid state quantum technologies. In this work, we report surface plasmon enhanced strong exciton-photon interaction in CH3NH3PbBr3 perovskite nanowires. Characteristic anti-crossing behaviors, indicating Rabi splitting energy up to ~ 560 meV, are observed near exciton resonance in hybrid semiconductor-insulator-metallic waveguide cavity at room temperature. An exciton-photon coupling strength enhancement factor of ~ 1.4 times is evaluated, which is mainly attributed to surface plasmon induced localized excitation field redistribution. Further, systematic studies on nanowires and insulator dimension dependence of exciton-photon interaction are presented. These results provide new avenues to achieve extremely high coupling strengths and push forward the development of electrically pumped and ultra-low threshold small lasers.

cond-mat.mes-hall↗

arXiv2017

Exciton-Polaritons in Hybrid Inorganic-organic Perovskite Fabry-Pérot Microcavity

Exciton-polaritons in semiconductor microcavities generate fascinating effects such as long-range spatial coherence and Bose-Einstein Condensation (BEC), which are attractive for their potential use in low threshold lasers, vortices and slowing light, etc. However, currently most of exciton-polariton effects either occur at cryogenic temperature or rely on expensive cavity fabrication procedures. Further exploring new semiconductor microcavities with stronger exciton photon interaction strength is extensively needed. Herein, we demonstrate room temperature photon exciton strong coupling in hybrid inorganic-organic CH3NH3PbBr3 Fabry-Pérot microcavities for the first time. The vacuum Rabi splitting energy is up to ~390 meV, which is ascribed to large oscillator strength and photon confinement in reduced dimension of optical microcavities. With increasing pumping energy, exciton-photon coupling strength is weakened due to carrier screening effect, leading to occurrence of photonic lasing instead of polartion lasing. The demonstrated strong coupling between photons and excitons in perovskite microcavities would be helpful for development of high performance polariton-based incoherent and coherent light sources, nonlinear optics, and slow light applications.

cond-mat.mes-hall↗