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Qiwen Tan

Publications and source records attributed to Qiwen Tan.

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Modulation of Spin Angular Momentum of Emission in Symmetric 1D Plasmonic Crystals by Cathodoluminescence

The spin angular momentum (SAM) of light has become a cornerstone of numerous photonic applications, including optical communication and chiral photonics. Because SAM is inherently associated with circularly polarized light (CPL), the ability to modulate CPL in a controlled and efficient manner is essential not only for advancing fundamental studies of light-matter interactions but also for enabling next-generation photonic technologies. However, such modulation is commonly realized by structurally chiral systems, which inherently limits the feasibility of dynamic tuning. Here, we demonstrate that one-dimensional plasmonic crystals (1D PlCs), despite their structural symmetry, can serve as a platform for controllable CPL generation. By employing an electron beam in scanning transmission electron microscopy (STEM), we coherently excite transition radiation and emission from 1D PlC modes. Their interference produces energy- and momentum- (emission angle-) resolved CPL, which clearly reveals its dispersion and spatial dependence at the nanoscale, providing direct guidance for its manipulation and offering insights into the design of plasmonic devices including the phase information. Furthermore, interference with surface plasmon polariton scattering at the structural boundary enables the efficiency modulation of CPL generation via the excitation position along the terrace.

physics.optics

Drift Correction of Scan Images by Snapshot Referencing

Reliable quantitative analysis in scanning (transmission) electron microscopy (S(T)EM) is often hindered by image drift during long-duration spectral mapping for elemental analysis or for various material functions. We here present snapshot-referencing (SSR) drift correction, a retrospective approach to eliminate spatial distortion based on the temporal nature of the scanning process. A continuous drift vector for every pixel is calculated for a normalized time-field of the scan pattern (e.g., serpentine or raster) utilizing a high-signal, fast-scan "snapshot" as a drift-free reference to guide the correction of simultaneously acquired analytical maps. To describe the drift, we employed Bezier basis functions to model smooth thermal or mechanical drifts and piece-wise linear basis for high-frequency "spiky" shifts such as those caused by charging. We demonstrate the efficacy of this approach on experimental cathodoluminescence (CL) datasets, showing that it effectively restores spatial integrity to hyperspectral data cubes without the need for specialized hardware. This flexible, software-based solution is broadly applicable to any probe-based analytical technique where a fast imaging signal can be recorded alongside slow spectroscopic data.

physics.ins-det

Room Temperature Collective Blinking and Photon Bunching from CsPbBr3 Quantum Dot Superlattice

Development of quantum light sources and search for quantum systems capable of supporting collective many-body states are crucial for further progress of modern quantum technologies. Metal halide perovskite quantum dots (QDs) have emerged as a promising candidate for quantum light sources, as individual QDs are reliable single photon emitters even at room temperature. However, photon bunching, a key signature of collective many-body states, has been so far largely observed at cryogenic temperatures in perovskite materials, limiting their applications under ambient conditions. Here, we report the observation of collective blinking and photon bunching in perovskite QD superlattices at room temperature. Sub-wavelength-sized (100 - 500 nm) CsPbBr3 QD superlattices, fabricated via a self-assembly process, exhibit an unusual two-level blinking behavior similar to that of single QDs, and demonstrate photon bunching with a degree of up to 2.75. Time-resolved photoluminescence (PL) measurements and super-resolution imaging reveal that the superlattices have a significantly longer PL lifetime than individual QDs and that their emission is spatially confined to regions tens of nanometers in size. These observations suggest long-range exciton migration to a localized energy trap within the superlattice. Excitation power dependent degree of bunching and analysis of the bunching dynamics indicate that the photon bunching originates from exciton-biexciton cascade emission, a key mechanism for generating entangled photons. These findings establish perovskite QD superlattices as a promising platform for room-temperature collective optical phenomena and quantum light generation, advancing scalable quantum photonic technologies.

physics.optics

Physics-Informed Neural Networks for the Korteweg-de Vries Equation for Internal Solitary Wave Problem: Forward Simulation and Inverse Parameter Estimation

Physics-informed neural networks (PINNs) have emerged as a transformative framework for addressing operator learning and inverse problems involving the Korteweg-de Vries (KdV) equation for internal solitary waves. By integrating physical constraints with data-driven optimization, PINNs overcome the critical challenges of parameter unmeasurability in the KdV equation for internal solitary waves in two-layer fluid systems. This work addresses two problems: (1) Operator learning constructs a mapping from parameters to solutions, enabling wave evolution predictions from unknown parameters. Comparative studies demonstrate prediction errors as low as $10^{-4}$ when using 1000 training points. (2) Inverse problem solving leverages sparse and potentially noisy observational data with physics-regularized constraints to invert nonlinear coefficients successfully. Compared to conventional approaches, this end-to-end differentiable paradigm unifies operator learning and inverse problem-solving while overcoming mesh discretization errors and high-dimensional parameter space iteration costs. The method shows effectiveness for internal wave problems in stratified fluids, providing both accurate forward modeling and robust parameter inversion capabilities, even under noise.

physics.flu-dyn