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Qiwen Zhan

Publications and source records attributed to Qiwen Zhan.

At least 19 recordsLinked to original sources

Phase amplification microscopy with femtometer-level accuracy

We demonstrate a major breakthrough in laser interferometry and microscopy achieving femtometer-level measurement accuracy and beyond, termed Phase Amplification microscopy (Φ-Amp). By exploiting the native silicide substrate as a phase cavity, our phase-gain theory predicts that weak sub-atomic phase signals can be magnified over 1000-fold, thus bypassing the shot-noise limit. We experimentally achieved a 158.2-fold phase gain for graphene in ambient air, corresponding ~ 730 femtometer accuracy. To fully unleash the potential of Φ-Amp for atomic fabrication and quantum measurement, we quantified interlayer spacing differences between AB-stacked and 30-degree-twisted bilayer graphene to be ~ 0.77 Angstroms and further detected atomic impurities and defects on large atomic structures. As the first wide-field metrology tool, we envision Φ-Amp may accelerate the scaling up of atomic quantum devices.

physics.optics

Material-Anisotropy-Driven Topological Optical Lattices on Thin-Film Lithium Niobate

Integrated structured-light sources usually obtain high-dimensional orbital angular momentum (OAM) states by encoding each channel into separate gratings, waveguides or metasurfaces, which ties modal capacity to structural complexity. Here we show that intrinsic material anisotropy can instead act as a built-in angular-momentum coupler. In an X-cut thin-film lithium niobate (TFLN) microring vortex emitter, the in-plane optical axis causes a circulating whispering-gallery mode to sample a periodically varying effective index, producing continuous azimuthal phase modulation. This modulation converts each resonance from a nominal single-charge emitter into a coherent topological sideband lattice with charges l=l_p+2n and Bessel-weighted amplitudes. Broadband measurements resolve a representative principal-charge series from l_p=-13 to +13, while additional devices with 100 and 200 GHz free spectral ranges (FSRs) show scalable resonance addressability. The emitted lattices are reproduced by a forward-calculated Fourier--Bessel model, supported by OAM projection measurements, and exhibit focusing into annular perfect-vortex fields and self-healing after obstruction. Waveguide-induced circular polarization further adds a vectorial spin--orbit channel. These results turn TFLN anisotropy from a material constraint into a compact mechanism for resonance-addressed high-dimensional structured-light generation.

physics.optics

Coherence toroidal vortices and statistic-veiled correlation topologies

Toroidal vortices in fluid and gas dynamics underpin a broad spectrum of scientific and technological fields, from elementary particle physics to condensed matter systems, and have recently garnered significant attention in optics because of their inherent topological stability. Here we report the experimental observation of toroidal vortices in stochastic optical wavefields with partial coherence, termed coherence toroidal vortices, which eliminates deterministic topological signatures in conventional optical degrees of freedom while unveiling statistically hidden correlation topologies. These underlying topologies-including both fundamental and higher-order hopfionic textures-emerge exclusively in second-order field correlations and are accessible only through statistical measurements. We further examine the impact of chaotic channels on the stability of these statistically veiled correlation topologies, demonstrating that their topological invariants remain robust under realistic environmental perturbations. These findings are experimentally validated and offer novel insights into the potential of toroidal light vortices serving as controllable channels for directional energy and information transfer within complex media.

physics.optics

Temporal Focusing Enables Distortion-Resistant high-intensity Spatiotemporal Optical Vortices

Spatiotemporal optical vortices (STOVs) carry transverse orbital angular momentum and offer new degrees of freedom for light-matter interactions. Yet conventional focusing of STOVs introduces spatiotemporal astigmatism: the beam diffracts while the pulse duration stays constant, causing the vortex to deform away from focus. Here we overcome this limitation by introducing spectral phase modulation into a temporal focusing configuration, where angular dispersion forces the pulse to compress only at the geometric focus so that the spatial and temporal dimensions focus and defocus together. Our approach generates stable STOVs with self-similar, distortion-free evolution over an extended focal region. Besides, the orbital angular momentum vector can be continuously steered from purely longitudinal to strongly tilted orientations by adjusting the spatial dispersion, objective focal length, or input beam size. More importantly, our method offers full compatibility with high NA focusing geometry, allowing high-intensity and high-resolution applications. We validate these properties through femtosecond laser ablation under high-NA conditions and interferometric spatiotemporal field reconstruction under low-NA conditions.

physics.optics

Nonlinear Nanophotonic Chip-space Interfaces: On-chip Generation of Structured, Topological and Spatiotemporal Lights Via Nonlinear Čerenkov Radiation

Miniaturized and reconfigurable interfaces between confined optical modes within integrated photonic chips and structured light propagating in free space would serve as a cornerstone for fundamental optical science and modern photonic technology. In this work, we exploit the anisotropic nonlinear susceptibility tensors associated with thin-film lithium niobate to construct nanophotonic chip-space interfaces capable of flexibly generating and multi-dimensionally engineering structured light via injections of photons to on-chip waveguides. By harnessing the nonlinear Čerenkov radiation in integrated nonlinear microring resonators, we successfully tailor the spatial profile, polarization state, emission wavelength, topological charge and temporal wave packet of structured optical vortices, exhibiting reconfigurabilities and tuning ranges far beyond the state-of-the-art. To further showcase the capabilities of our platform, we use a single pump to generate tunable optical skyrmions via the spin-orbit coupling and multi-state integrated vortex microcombs in the visible range via synergistic $χ^{(2)}$ and $χ^{(3)}$ nonlinear optical processes. Our work bridges the research fields of structured light and integrated nonlinear optics, providing unprecedented opportunities for spatiotemporal light generation and on-chip multidimensional nonlinear optics.

physics.optics

Robustness Optimization for Compact Free-electron Laser Driven by Laser Wakefield Accelerators

Despite the successful demonstration of compact free electron lasers (FELs) driven by laser wakefield accelerators (LWFAs), the inherent shot-to-shot fluctuations in LWFAs, including both laser and plasma instabilities, remain a primary obstacle to realizing LWFA-driven FELs with robust operation. Here, we present a conceptual design for LWFA-driven FELs with sufficient tolerance against shot-to-shot fluctuations using the Covariance Matrix Adaptation Evolution Strategy (CMA-ES). Start-to-end simulations demonstrated that this systematic optimization resulted in a significant improvement in the robustness of FELs. With the optimized configurations, the radiation energy can be maintained above 1 microjoule at a wavelength of approximately 25 nm, even when accounting for twice the root-mean-square (RMS) ranges of these instabilities. This proposed scheme represents a substantial advancement in the development of compact LWFA-driven FEL systems, enabling robust operation and paving the way for the realization of reliable and widely accessible sources.

physics.plasm-ph

Twisting harmonics: Transfer of orbital angular momentum in solid-state high-harmonic generation

Although solid-state platforms underpin modern electronics, little is known about how intense ultrashort light pulses carrying orbital angular momentum (OAM) interact with solids. This gap persists even though, for more conventional light-matter interactions, the complex underlying electron dynamics can often be confined to a single Brillouin zone and described well within the dipole approximation. Previous studies were restricted to nonlinear, perturbative regimes, largely because the generation of intense ultrashort vortex pulses, particularly in the mid-infrared spectral regime, has remained a long-standing challenge. Consequently, the role of structured light in driving nonlinear, non-perturbative processes in solids, and the associated transfer of angular momentum during these interactions, has not been systematically explored. Here, we investigate solid-state high-harmonic generation (HHG) driven by intense ultrashort structured light using a versatile experimental approach applicable to different materials and geometries. We demonstrate that the OAM of the driving field is coherently transferred to the emitted harmonics. In particular, we show that the OAM is conserved independently of the crystal symmetry, the range of electronic interactions, and the presence of strong spin-orbit coupling. These results establish OAM-resolved HHG as a robust framework for characterizing and controlling angular momentum transfer in solid-state HHG and open new avenues for structured-light-driven quantum technologies and topological materials investigations.

physics.optics

Sculpting ultrafast mid-infrared light for solid-state high harmonic generation

The ability to sculpt light in space, time, and polarization has revolutionized studies of light-matter interaction and enabled breakthroughs in optical communication, imaging, and ultrafast science. Among the many degrees of freedom of light, orbital angular momentum (OAM) further expands these capabilities by unlocking new regimes of control in information encoding, particle trapping and manipulation, and symmetry-driven selection rules. However, exploiting OAM to drive nonlinear, non-perturbative effects in solids remains challenging, especially in the mid-infrared (MIR) spectral regime-a key region for accessing these effects in ambient air, where spatial light modulators do not operate. Here, we circumvent this limitation by generating femtosecond, few-cycle MIR Bessel-Gauss vortex (BGV) and perfect optical vortices (POVs), using a robust, static spatial-shaping strategy. By utilizing these beams to drive nonlinear optical processes such as second-harmonic generation (SHG) and high-harmonic generation (HHG) in various solid-state materials, we show that the resulting harmonic beams faithfully inherit the structural characteristics of the drivers: the constant-intensity ring of the POVs is preserved across harmonic orders, while the BGV harmonic beams retain their intrinsic topological charge-dependent intensity profiles. Furthermore, by verifying the linear OAM up-scaling law, we confirm the conservation of OAM during SHG and HHG in solids. These results establish strong-field HHG in solids as a robust platform for synthesizing ultrafast structured harmonic light with controllable, high-value OAM.

physics.optics

Polygonal Spatiotemporal Optical Vortices Wavepackets with Prescribed Vortex Structure

Optical vortices carrying orbital angular momentum offer additional degrees of freedom. According to the orientation of orbital angular momentum, optical vortices can be classified into spatial optical vortex beam carrying longitudinalorbital angular momentum and spatiotemporal optical vortices carrying transverse orbital angular momentum. As an emerging subset of optical vortices, polygonal optical vortices provide a unique platform for a wide range of frontier applications by introducing a new degree of freedom in the form of a customizable intensity structure. In the spatial domain, polygonal spatial optical vortex beam carrying longitudinal orbital angular momentum have already demonstrated great potential in optical manipulation and two-photon lithography. However, polygonal spatiotemporal optical vortex wavepackets contain multiple sub spatiotemporal optical vortices carrying transverse orbital angular momentum remains unrealized to date. In this work, we theoretically propose and experimentally demonstrate polygonal spatiotemporal optical vortices wavepackets embedded with prescribed vortex structures. Within the structure, a prescribed number of sub spatiotemporal optical vortices carrying transverse orbital angular momentum is set along a designed polygonal spatiotemporal trajectory. Using the spatiotemporal holographic shaping approach, we generate polygonal perfect spatiotemporal optical vortex wavepacket and use the combination of multiple polygonal perfect spatiotemporal optical vortex wavepacket to form polygonal spatiotemporal optical vortex wavepacket with the prescribed vortex structure. A full control over multiple key properties of the polygonal spatiotemporal optical vortex wavepackets such as the geometry, number of phase singularities, and spatiotemporal distribution of sub spatiotemporal optical vortices is also achieved.

physics.optics

Spatiotemporally Localized Optical Links and Knots

Optical links and knots have attracted growing attention owing to their exotic topologic features and promising applications in next-generation information transfer and storage. However, current protocols for optical topology realization rely on paraxial propagation of spatial modes, which inherently limits their three-dimensional topological structures to longitudinal space-filling. In this work we propose and experimentally demonstrate a scheme for creating optical knots and links that are localized in space within a transverse plane of a paraxial field, as well as in time. These spatiotemporal topological structures arise from polychromatic wave fields with tightly coupled spatial and temporal degrees of freedom that can be realized in the form of superpositions of toroidal light vortices of opposite topological charges. The (2+1)-dimensional nature of a toroidal light vortex imparts spatiotemporally localized wave fields with nontrivial topological textures, encompassing both individual and nested links or knots configurations. Moreover, the resulting topological textures are localized on an ultrashort timescale propagate at the group velocity of the wave packets and exhibit remarkable topological robustness during propagation as optical carriers. The nascent connection between spatiotemporally localized fields and topology offers exciting prospects for advancing space-time photonic topologies and exploring their potential applications in high-capacity informatics and communications.

physics.optics

Annular Channel Eigenmodes: A Physical-Layer Approach to Suppressing OAM Modal Crosstalk

Modal crosstalk is a fundamental limitation for orbital angular momentum (OAM)-based spatial-division multiplexing. Here, we introduce Annular Channel Eigenmodes (ACEs) - rigorously derived as the optimal band-limited solution for maximizing energy concentration within distinct annular channels. This approach reformulates the design as a Hermitian eigenvalue problem, efficiently yielding optimal beams that are physically isolated in space. Numerical simulations demonstrate that under identical conditions, conventional Gaussian-enveloped perfect optical vortices (POVs) exhibit an average modal crosstalk of -16 dB, whereas ACEs suppress crosstalk to nearly -30 dB. Moreover, the crosstalk suppression of ACEs continues to improve exponentially with increasing channel width, while that of POVs saturates at a fundamental limit. We experimentally generated ACEs and confirmed a 36% enhancement in energy confinement relative to POVs. ACEs thus provide a physically robust basis for high-fidelity, high-density OAM communications.

physics.optics

Spatiotemporal Topological Combs for Robust High-Dimensional Information Transmission

Sculpting light across its independent degrees of freedom-from orbital angular momentum to the discrete wavelengths of optical frequency combs-has unlocked vast communication bandwidth by enabling massively parallel information channels. However, the Shannon-Hartley theorem sets a hard limit by tying channel capacity to the trade-off between SNR and rate, a central challenge in communication. Inspired by lock-in amplification in electronics, we encode data on THz optical burst carriers so the signal resides beyond the conventional noise band, yielding exceptional robustness. By leveraging a programmable all-degree-of-freedom (All-DoF) modulator, we generate a spatiotemporal topological comb (ST-Comb) that structures light into a vast, highentropy state space for high-dimensional information encoding. Crucially, we find that the associated topological winding number is preserved under diverse perturbations, ensuring stable information encoding and retrieval. This paradigm illustrates how structured light can simultaneously expand channel dimensionality and maintain robustness, charting a pathway to chip-scale, reconfigurable photonic platforms for the PHz era, while also opening previously inaccessible regimes of light-matter interaction.

physics.optics

A reconfigurable arbitrary retarder array as complex structured matter

Tuneable retarder arrays, such as spatially patterned liquid crystal devices, have given rise to impressive photonic functionality, fuelling diverse applications ranging from microscopy and holography to encryption and communications. Presently these solutions are limited by the controllable degrees of freedom of structured matter, hindering applications that demand photonic systems with high flexibility and reconfigurable topologies. Here we demonstrate a compound modulator that implements a synthetic tuneable arbitrary retarder array as virtual pixels derived by cascading low functionality tuneable devices, realising full dynamic control of its arbitrary elliptical axis geometry, retardance value, and induced phase. Our approach offers unprecedented functionality that is user-defined and possesses high flexibility, allowing our modulator to act as a new beam generator, analyser, and corrector, opening an exciting path to tuneable topologies of light and matter.

physics.optics

Spatiotemporal coupled Airy-Airy wavepacket and its propagation dynamics

Airy beams, celebrated for their self-acceleration, diffraction-free propagation, and self-healing properties, have garnered significant interest in optics and photonics, with applications spanning ultrafast optics, laser processing, nonlinear optics, and optical communications. Recent research primarily aims at independent control of Airy beams in both spatial and spatiotemporal domains. In a pioneering approach, we have successfully generated and controlled a spatiotemporal coupled (STc) Airy-Airy wavepacket, achieving its rotation while preserving vertical distribution in the spatiotemporal domain. Furthermore, we have investigated the self-acceleration and self-healing properties of the STc Airy-Airy wavepacket in this domain, noting that its dynamically adjustable rotation and spatiotemporal coupling capability provide a novel strategy for managing ultrafast lasers, with potential advancements in optical micromanipulation and time-domain coding communication.

physics.optics

Propagation Dynamics of Photonic Toroidal Vortices Mediated by Orbital Angular Momenta

The dynamics of vortex rings in fluids have long captivated researchers due to the intriguing complexity of their behavior, despite the apparent simplicity of their structure. In optics, photonic toroidal vortices constitute a novel class of three-dimensional, space-time nonseparable structured light fields that carry transverse orbital angular momentum. However, as solutions to the dispersive form of Maxwell's equations, these wavepackets do not survive upon nondispersive propagation, and their dynamics remain elusive. In this article, the dynamics of photonic toroidal vortices under various dispersion regimes, mediated by both transverse and longitudinal orbital angular momentum, are investigated through simulations and experiments. The results reveal that the motion of a toroidal vortex is strongly affected by the presence of longitudinal orbital angular momentum. The swirling flow destabilizes the toroidal structure under dispersion conditions and induces topological transformations in the vortex line characterized by its annihilation and subsequent reformation in vacuum. Remarkably, the renascent toroidal vortex exhibits robust propagation in vacuum while maintaining its toroidal structure. These findings are supported by experimental validation and highlight the potential of photonic toroidal vortices as controllable channels for directional energy and information transfer.

physics.optics

Full space-time abrupt autofocusing spherical Airy wavepacket

The ability to precisely focus optical beams is crucial for numerous applications, yet conventional Gaussian beams exhibit slow intensity transitions near the focal point, limiting their effectiveness in scenarios requiring sharp focusing. In this work, the spherical Airy wavepacket, a three dimensional light field with an Airy function distribution in the radial direction in the full space time domain, is introduced and experimentally demonstrated. Leveraging the recently developed spatiotemporal hologram technique and an exponential polar coordinate transformation, spherical Airy wavepacket is sculpted to exhibit ultrafast autofocusing with a dramatically reduced depth of focus compared to conventional Gaussian beams and circular Airy beams. Experimental measurements confirm its nonlinear intensity surge and tight spatiotemporal confinement.

physics.optics

Spatiotemporal Airy rings wavepackets

Airy waves, known for their non-diffracting and self-accelerating properties, have been extensively studied in spatial and temporal domains, but their spatiotemporal (ST) counterparts remain largely unexplored. We report the first experimental realization of a spatiotemporal Airy rings wavepacket, which exhibits an Airy function distribution in the radial dimension of the ST domain. The wavepacket demonstrates abrupt autofocusing under the combined effects of diffraction and dispersion, achieving a 110 um spatial and 320 fs temporal focus with a sharp intensity contrast along the propagation direction - ideal for nonlinear microscopy and multiphoton 3D printing. Notably, the wavepacket retains its autofocusing capability even after spatial obstruction, showcasing robust self-healing. Furthermore, by embedding a vortex phase, we create an ST-Airy vortex wavepacket that confines transverse orbital angular momentum (t-OAM) within a compact ST volume, enabling new avenues for studying light-matter interactions with t-OAM. Our findings advance the fundamental understanding of ST Airy waves and highlight their potential for transformative applications in ultrafast optics, structured light, and precision laser processing.

physics.optics

Spatiotemporal Photonic Emulator of Potential-free Schrödinger Equation

Photonic quantum emulator utilizes photons to emulate the quantum physical behavior of a complex quantum system. Recent study in spatiotemporal optics has enriched the toolbox for designing and manipulating complex spatiotemporal optical wavepackets, bringing new opportunities in building such quantum emulators. In this work, we demonstrate a new type of photonic quantum emulator enabled by spatiotemporal localized wavepackets with spherical harmonic symmetry. The spatiotemporal field distribution of these wavepackets has the same distributions of the wavefunction solutions to the potential-free Schrödinger equation with two controllable quantum numbers. A series of such localized wavepackets are experimentally generated with their localized feature verified. These localized wavepackets can propagate invariantly in space-time like particles, forming a new type of photonic quantum emulator that may provide new insight in studying quantum physics and open up new applications in studying light-matter interactions and quantum optics.

physics.optics