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Quanchao Du

Publications and source records attributed to Quanchao Du.

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Odd-Parity Chiral Magnons in Collinear Antiferromagnetic Multiferroics

Odd-parity magnetism represents an intriguing frontier in unconventional magnets; however, its realization has traditionally relied on noncollinear magnetic orders accompanied by broken spin conservation, which inevitably causes spin relaxation and dissipative transport of spin-encoded information. Here, we uncover a distinct route toward spin-conserving odd-parity magnon splitting enabled by antichiral Haldane-like flux (AHF) in collinear antiferromagnetic multiferroics. Symmetry analysis reveals that such AHF driven by intra-sublattice Dzyaloshinskii-Moriya interactions (DMI) gives rise to symmetry-dependent odd-parity magnon splittings, ranging from $p$-wave and $f$-wave to nodeless forms. Moreover, the coupling between ferroelectric modes and DMI provides an electric-field knob for manipulating chiral band splitting and magnon transport. Combining density functional theory (DFT) calculations, we identify a series of promising candidate materials in both 2D and bulk antiferromagnetic multiferroics. Our work provides new insights into the realization of odd-parity chiral magnons in collinear antiferromagnets and magnetoelectric coupling mechanisms in multiferroics.

cond-mat.mtrl-sci

Ferroelectric Switchable Topological Magnon Hall Effect in Type-I Multiferroics

Electric control of magnetism at room temperature is crucial for developing next-generation, low-power spintronic devices. However, the intrinsic incompatibility between ferroelectricity and magnetism in crystal symmetry, along with the absence of strong magnetoelectric coupling mechanisms, continues to pose major challenges. In this work, we propose a general theoretical framework for magnon manipulation based on ferroelectric polarization switching in two-dimensional multiferroics. Taking monolayer multiferroics $\mbox{Ti}_{2}\mbox{F}_{3}$ as an example, our calculations demonstrate that ferroelectric switching can significantly modulate spin exchanges, thereby enabling nonvolatile and reversible electric control of the magnons. More importantly, the ferroelectric polarization reversal leads to a sign change in the Berry curvature, ensuring effective control over the valley Hall and nonlinear Hall response of magnons. This study provides a new way for realizing low-power and electrically controllable magnonic devices.

cond-mat.mtrl-sci

Nonreciprocal magnons in layered antiferromagnets VPX3(X =S,Se,Te)

Nonreciprocal magnons, characterized by propagation with differing energies along the k and -k directions, are crucial for modern spintronics applications. However, their realization in van der Waals layered antiferromagnets remains elusive. In this letter, we report robust nonreciprocal magnon behavior in layered honeycomb antiferromagnets VPX3(X =S,Se,Te). Our results demonstrate that, in addition to their intrinsic Dzyaloshinskii-Moriya interaction (DMI), the nonreciprocity of magnons is strongly influenced by the layer number, interlayer coupling, and magnon-magnon interactions. More importantly, in such layered antiferromagnets, the magnon nonreciprocity exhibits an asymmetric periodic dependence on the Neel vector, offering a novel route for experimentally probing antiferromagnetic order parameters in the 2D limit.

cond-mat.mtrl-sci

Topological switching in bilayer magnons via electrical control

Topological magnons, quantized spin waves featuring nontrivial boundary modes, present a promising route toward lossless information processing. Realizing practical devices typically requires magnons excited in a controlled manner to enable precise manipulation of their topological phases and transport behaviors. However, their inherent charge neutrality and a high frequency nature pose a significant challenge for nonvolatile control, especially via electric means. Herein, we propose a general strategy for electrical control of topological magnons in bilayer ferromagnetic insulators. With strong spin-layer coupling, an applied vertical electric field induces an interlayer potential imbalance that modifies intralayer Heisenberg exchanges between adjacent layers. This electric-field-driven modulation competes with the bilayer's intrinsic Dzyaloshinskii-Moriya interaction, enabling the accurate tuning of the band topology and nonreciprocal dynamics of magnons. More importantly, such an electric control mechanism exhibits strong coupling with external magnetic fields, unveiling new perspectives on magnetoelectric coupling in charge-neutral quasiparticles

cond-mat.mes-hall

Nonvolatile Magnonics in Bilayer Magnetic Insulators

Nonvolatile control of spin order or spin excitations offers a promising avenue for advancing spintronics; however, practical implementation remains challenging. In this letter, we propose a general framework to realize electrical control of magnons in 2D magnetic insulators. We demonstrate that in bilayer ferromagnetic insulators with strong spin-layer coupling, electric field Ez can effectively manipulate the spin exchange interactions between the layers, enabling nonvolatile control of the corresponding magnons. Notably, in this bilayer, Ez can induce nonzero Berry curvature and orbital moments of magnons, the chirality of which are coupled to the direction of Ez. This coupling facilitates Ez manipulate the corresponding magnon valley and orbital Hall currents. Furthermore, such bilayers can be easily engineered, as demonstrated by our density-functional-theory calculations on Janus bilayer Cr-based ferromagnets. Our work provides an important step toward realizing nonvolatile magnonics and paves a promising way for future magnetoelectric coupling devices.

cond-mat.mtrl-sci