arXiv subjects

Quirin Buchinger

Publications and source records attributed to Quirin Buchinger.

18 recordsLinked to original sources

arXiv2026

A diode nanocavity for fast, efficient and tunable emission of highly entangled photon pairs and Fourier-transform-limited single photons

Deterministic sources of entangled photon pairs and indistinguishable photons are expected to play a key role in photonic quantum technologies. Semiconductor quantum dots are promising candidates due to their on-demand emission and compatibility with nanophotonic structures. However, current implementations face trade-offs between extraction efficiency, Purcell enhancement, as well as charge noise that causes blinking and degrades indistinguishability. Here we demonstrate a tunable nano-optoelectronic device based on a quantum dot embedded in a p-i-n diode circular-Bragg-grating-resonator and featuring extraction efficiencies up to 0.55(6) and Purcell-factor of $\sim$8. The device generates wavelength-tunable entangled photon pairs with suppressed blinking and raw (corrected) concurrence > 0.89 (0.91) over a range of 1.6 nm. The very same source also emits single, nearly Fourier-limited and highly indistinguishable photons with raw (corrected) $\mathcal{V}_{\text{HOM}}$ = 0.951(4) (0.988(6)). These results demonstrate a viable platform for semiconductor quantum photonics.

quant-ph↗

arXiv2026

Purcell enhanced and blinking free single photons from InAs/GaAs quantum dots in deterministically placed circular Bragg gratings

The development of efficient, deterministic, and tunable single-photon sources is a cornerstone for the realization of long-distance quantum communication, quantum repeaters, and photonic quantum computing technologies. In this study, we demonstrate a bright, charge-tunable single-photon source in the 900 nm wavelength range based on InAs quantum dots (QDs) embedded in a p-i-n doped GaAs membrane, which shows blinking free emission. We use a modified circular Bragg grating (CBG) as a micro-resonator. By adding fourfold symmetric bridges in a labyrinth-like geometry, we provide a conductive pathway to the central disk, thereby enabling electrical contact to the QD while maintaining high Purcell enhancement and photon extraction efficiency (PEE). For the negative trion (X-), we demonstrate a lifetime of $44.3 \pm 0.2$ ps - corresponding to a Purcell factor of $18.0 \pm 0.7$ and a PEE of $68.1% \pm 3.1$ %. Furthermore, the device is blinking-free with very low multi-photon contribution, evidenced by a second-order autocorrelation value $g(2)(0) < 0.017 \pm 0.015$. By applying a vertical diode bias, we demonstrate precise charge-state control, resolving distinct emission plateaus ranging from the single negatively charged trion ($X^-$) to triply negatively charged excitons ($X^{3-}$). These results showcase a robust architecture that simultaneously provides high efficiency, high repetition rates, and deterministic charge control, fulfilling key requirements for the next generation of quantum network hardware.

cond-mat.mes-hall↗

arXiv2026

Molecular beam epitaxy of wafer-scale O-band InAs/InGaAs quantum dots on GaAs for quantum photonics

We report a scalable molecular beam epitaxy strategy to achieve a low density of O-band electrically tunable InAs/InGaAs quantum dots (QDs) on GaAs(001) substrates. Our approach is based on a gradient deposition of InAs in the sub-ML regime and subsequent capping with an InGaA strain-reducing layer to redshift the emission wavelength. For different growth conditions, we investigate the optical properties of the dots using photoluminescence mapping and correlate with structural properties determined by scanning transmission electron microscopy. Using a surface roughness modulation technique and synchronizing InAs sub-monolayer deposition cycles with substrate rotation, we control the dot density and position low-density regions (< 1 QD per um^2) on the substrate. Hyperspectral imaging is used to map the spatial and spectral characteristics of many individual dots in the low-density region, confirming that our approach is universally applicable to conventional MBE growth on (001) surfaces. Finally, we tune the QD emission wavelength within the O-band using electric fields and demonstrate single-photon emission with g(2)(0) = 0.020(14).

cond-mat.mtrl-sci↗

arXiv2026

Cascaded Metasurface Interferometer for Multipath Interference with Classical and Quantum Light

Beamsplitters represent fundamental components in both classical and quantum optical systems, enabling the distribution of light, as well as the generation of interference, superposition and entanglement. However, optical networks constructed from conventional bulk 2x2-beamsplitters encounter inherent scalability issues, as the number of required beamsplitters scales quadratically with the number of optical modes for a fully connected network. Metasurfaces offer a promising route to overcome these constraints. By manipulating light at the wavelength scale compact optical components with advanced functionalities can be constructed, which address several modes simultaneously. In this work, we design and experimentally utilize a metasurface as a multiport beamsplitter. Furthermore, we realize a multimode interferometer composed of two cascaded metasurfaces. We characterize the individual and cascaded metasurfaces using classical light, showing controllable splitting ratios through tunable phase relations. We then expand the approach to quantum light, employing single photons to demonstrate second- and third-order photon correlations, as well as single photon interference across multiple spatial paths. These results establish metasurface-based multiport beamsplitters as a scalable and reconfigurable platform bridging classical and quantum photonics.

physics.optics↗

arXiv2025

A Spin-Photon Interface in the Telecom C-Band with Long Hole Spin Dephasing Time

Matter qubits that maintain coherence over extended timescales are essential for many pursued applications in quantum communication and quantum computing. Significant progress has already been made on extending coherence times of spins in semiconductor quantum dots while interfacing them with photons in the near-infrared wavelength range. However, similar results for quantum dots emitting at the telecom range, crucial for many applications, have so far lagged behind. Here, we report on InAs/InAlGaAs quantum dots integrated in a deterministically placed circular Bragg grating emitting at $1.55\,\mu\mathrm{m}$. We quantify the g-factors of electrons and holes from polarization-resolved measurements of a positive trion in an in-plane magnetic field and study the dynamics of the ground-state hole spin qubit. We then herald the hole spin in a pulsed two-photon correlation measurement and determine its inhomogeneous dephasing time to $T_{2}^{*}=(15.9 \pm 1.7)$ ns.

quant-ph↗

arXiv2025

High-Performance Labyrinth Circular Bragg Grating Design for Charge and Stark-Tunable Quantum Light Sources Spanning Visible to Telecom Wavelengths

Semiconductor quantum dots embedded in circular Bragg gratings (CBGs) are among the most efficient integrated single-photon sources. However, the fully etched rings of conventional CBGs restrict the implementation of charge and Stark tuning via electrical contacts. To overcome this limitation, a labyrinth CBG geometry with four bridges has been proposed, yet the added bridges significantly degraded optical performance. In this work, we numerically demonstrate that a periodic labyrinth CBG design preserves both high coupling efficiency and strong Purcell enhancement while enabling electrical integration if optimized after introducing the bridges. We show three optimized designs at emission wavelengths of 780 nm, 930 nm, and 1550 nm, because these wavelengths are among the most relevant for quantum dots and show the general applicability of our approach. At all three wavelengths collection efficiencies exceeding 90% into a numerical aperture of 0.7 and Purcell factors greater than 25 are achieved. Furthermore, we propose a device layout incorporating a barrier layer that separates p- and n-doped semiconductor regions, which is incorporated to prevent tunneling of one of the charge carriers for selective charging. Also this design can be reoptimized to retain the performance of a device without tunnel barrier. These results establish labyrinth CBGs as a platform for electrically tunable quantum dot single-photon sources with high efficiency and scalability.

quant-ph↗

arXiv2025

Enhanced spectral range of strain-induced tuning of quantum dots in circular Bragg grating cavities

Tunable sources of entangled and single photons are essential for implementing entanglement-based quantum information protocols, as quantum teleportation and entanglement swapping depend on photon indistinguishability. Tunable devices are fabricated from indium arsenide (InAs) quantum dots (QDs) embedded in gallium arsenide (GaAs) nanomembranes placed on monolithic piezoelectric substrates. Circular Bragg grating (CBG) resonators enhance emission brightness and exploit the Purcell effect; however, the inclusion of CBGs reduces strain-mediated tunability compared to planar nanomembranes. A simple and effective solution is introduced: filling the CBG trenches with a stiff dielectric (aluminum oxide) via atomic layer deposition (ALD) restores up to 95% of the tunability of planar structures. Finite element analysis (FEA) confirms that the tunability loss originates from bending in the device layers due to strain relief in the CBG geometry. Lowering the stiffness of intermediate layers between the QDs and the piezoelectric actuator, such as in bonding or reflector layers, further increases strain losses in uncoated CBGs. Coated devices maintain 98-99% strain-tuning efficiency across all simulated underlayer stiffnesses. The results demonstrate that advantageous optical cavity properties can be effectively combined with piezoelectric strain tuning, enabling scalable, bright, and tunable quantum light sources.

cond-mat.mtrl-sci↗

arXiv2025

Deterministic Quantum Dot Cavity Placement Using Hyperspectral Imaging with High Spatial Accuracy and Precision

Single emitters in solid state are great sources of single and entangled photons. To boost their extraction efficiency and tailor their emission properties, they are often incorporated in photonic nanostructures. However, achieving accurate and reproducible placement inside the cavity is challenging but necessary to ensure the highest mode overlap and optimal device performance. For many cavity types -- such as photonic crystal cavities or circular Bragg grating cavities -- even small displacements lead to a significantly reduced emitter-cavity coupling. For circular Bragg grating cavities, this yields a significant reduction in Purcell effect, a slight reduction in efficiency and it introduces polarization on the emitted photons. Here we show a method to achieve high accuracy and precision for deterministically placed cavities on the example of circular Bragg gratings on randomly distributed semiconductor quantum dots. We introduce periodic alignment markers for improved marker detection accuracy and investigate overall imaging accuracy achieving $(9.1 \pm 2.5) nm$ through image correction. Since circular Bragg grating cavities exhibit a strong polarization response when the emitter is displaced, they are ideal devices to probe the cavity placement accuracy far below the diffraction limit. From the measured device polarizations, we derive a total spatial process accuracy of $(33.5 \pm 9.9) nm$ based on the raw data, and an accuracy of $(15 \pm 11) nm$ after correcting for the system response, resulting in a device yield of $68 \%$ for well-placed cavities.

cond-mat.mes-hall↗

arXiv2025

Ability of entanglement and purity to help to detect systematic experimental errors

Measurements are central in all quantitative sciences, and a fundamental challenge is to make observations without systematic measurement errors. This holds in particular for quantum information processing, where other error sources, such as noise and decoherence, are unavoidable. Consequently, methods for detecting systematic errors have been developed, but the required quantum state properties are yet unexplored. We theoretically develop a direct and efficient method to detect systematic errors in quantum experiments and demonstrate it experimentally using quantum state tomography of photon pairs emitted from a semiconductor quantum dot. Our method can be scaled to multi-qubit systems, and we find that entanglement and quantum states with high purity can help identify systematic errors.

quant-ph↗

arXiv2024

Quantum teleportation with dissimilar quantum dots over a hybrid quantum network

Photonic quantum information processing in metropolitan quantum networks lays the foundation for cloud quantum computing [1, 2], secure communication [3, 4], and the realization of a global quantum internet [5, 6]. This paradigm shift requires on-demand and high-rate generation of flying qubits and their quantum state teleportation over long distances [7]. Despite the last decade has witnessed an impressive progress in the performances of deterministic photon sources [8-11], the exploitation of distinct quantum emitters to implement all-photonic quantum teleportation among distant parties has remained elusive. Here, we overcome this challenge by using dissimilar quantum dots whose electronic and optical properties are engineered by light-matter interaction [12], multi-axial strain [13] and magnetic fields [14] so as to make them suitable for the teleportation of polarization qubits. This is demonstrated in a hybrid quantum network harnessing both fiber connections and 270 m free-space optical link connecting two buildings of the University campus in the center of Rome. The protocol exploits GPS-assisted synchronization, ultra-fast single photon detectors as well as stabilization systems that compensate for atmospheric turbulence. The achieved teleportation state fidelity reaches up to 82+-1%, above the classical limit by more than 10 standard deviations. Our field demonstration of all-photonic quantum teleportation opens a new route to implement solid-state based quantum relays and builds the foundation for practical quantum networks.

quant-ph↗

arXiv2024

Wavevector-resolved polarization entanglement from radiative cascades

The generation of entangled photons from radiative cascades has enabled milestone experiments in quantum information science with several applications in photonic quantum technologies. Significant efforts are being devoted to pushing the performances of near-deterministic entangled-photon sources based on single quantum emitters often embedded in photonic cavities, so to boost the flux of photon pairs. The general postulate is that the emitter generates photons in a nearly maximally entangled state of polarization, ready for application purposes. Here, we demonstrate that this assumption is unjustified. We show that in radiative cascades there exists an interplay between photon polarization and emission wavevector, strongly affecting quantum correlations when emitters are embedded in micro-cavities. We discuss how the polarization entanglement of photon pairs from a biexciton-exciton cascade in quantum dots strongly depends on their propagation wavevector, and it can even vanish for large emission angles. Our experimental results, backed by theoretical modelling, yield a brand-new understanding of cascaded emission for various quantum emitters. In addition, our model provides quantitative guidelines for designing optical microcavities that retain both a high degree of entanglement and collection efficiency, moving the community one step further towards an ideal source of entangled photons for quantum technologies.

quant-ph↗

arXiv2023

Purcell-Enhanced Single-Photon Emission in the Telecom C-Band

Purcell-enhanced quantum dot single-photon emission in the telecom C-band from InAs quantum dots inside circular Bragg grating cavities is shown. The InAs quantum dots are grown by means of molecular beam epitaxy on an InP substrate and are embedded into a quaternary $\mathrm{In}_{0.53}\mathrm{Al}_{0.23}\mathrm{Ga}_{0.24}\mathrm{As}$ membrane structure. In a post-growth flip-chip process with subsequent substrate removal and electron beam-lithography, circular Bragg grating ("bullseye") resonators are defined. Micro-photoluminescence studies of the devices at cryogenic temperatures of T = 5 K reveal individual quantum dot emission lines into a pronounced cavity mode. Time-correlated single-photon counting measurements under above-band gap excitation yield Purcell-enhanced excitonic decay times of $\tau = (180 \pm 3)$ ps corresponding to a Purcell factor of $F_P = (6.7 \pm 0.6)$. Pronounced photon antibunching with a background limited $g^{(2)}(0) = (0.057 \pm 0.004)$ is observed, which demonstrates that the light originated mostly from one single quantum dot.

cond-mat.mes-hall↗

arXiv2023

Post-fabrication tuning of circular Bragg resonators for enhanced emitter-cavity coupling

Solid-state quantum emitters embedded in circular Bragg resonators are attractive due to their ability to emit quantum states of light with high brightness and low multi-photon probability. As for any emitter-microcavity system, fabrication imperfections limit the spatial and spectral overlap of the emitter with the cavity mode, thus limiting their coupling strength. Here, we show that an initial spectral mismatch can be corrected after device fabrication by repeated wet chemical etching steps. We demonstrate ~16 nm wavelength tuning for optical modes in AlGaAs resonators on oxide, leading to a 4-fold Purcell enhancement of the emission of single embedded GaAs quantum dots. Numerical calculations reproduce the observations and suggest that the achievable performance of the resonator is only marginally affected in the explored tuning range. We expect the method to be applicable also to circular Bragg resonators based on other material platforms, thus increasing the device yield of cavity-enhanced solid-state quantum emitters.

quant-ph↗

arXiv2023

Polarized and Un-Polarized Emission from a Single Emitter in a Bullseye Resonator

We present polarized |S|=0.99$\pm$0.01, and unpolarized |S|=0.03$\pm$0.01 emission from a single emitter embedded in a single, cylindrically symmetric device design. We show that the polarization stems from a position offset of the single emitter with respect to the cavity center, which breaks the cylindrical symmetry, and a position-dependent coupling to the frequency degenerate eigenmodes of the resonator structure. The experimental results are interpreted by using numerical simulations and by experimental mapping of the polarization-resolved far-field emission patterns. Our findings can be generalized to any nanophotonic structure where two orthogonal eigenmodes are not fully spatially overlapping.

physics.optics↗

arXiv2022

A source of entangled photons based on a cavity-enhanced and strain-tuned GaAs quantum dot

A quantum-light source that delivers photons with a high brightness and a high degree of entanglement is fundamental for the development of efficient entanglement-based quantum-key distribution systems. Among all possible candidates, epitaxial quantum dots are currently emerging as one of the brightest sources of highly entangled photons. However, the optimization of both brightness and entanglement currently requires different technologies that are difficult to combine in a scalable manner. In this work, we overcome this challenge by developing a novel device consisting of a quantum dot embedded in a circular Bragg resonator, in turn, integrated onto a micromachined piezoelectric actuator. The resonator engineers the light-matter interaction to empower extraction efficiencies up to 0.69(4). Simultaneously, the actuator manipulates strain fields that tune the quantum dot for the generation of entangled photons with corrected fidelities to a maximally entangled state up to 0.96(1). This hybrid technology has the potential to overcome the limitations of the key rates that plague QD-based entangled sources for entanglement-based quantum key distribution and entanglement-based quantum networks.

quant-ph↗

arXiv2022

Signatures of the Optical Stark Effect on Entangled Photon Pairs from Resonantly-Pumped Quantum Dots

Two-photon resonant excitation of the biexciton-exciton cascade in a quantum dot generates highly polarization-entangled photon pairs in a near-deterministic way. However, the ultimate level of achievable entanglement is still debated. Here, we observe the impact of the laser-induced AC-Stark effect on the quantum dot emission spectra and on entanglement. For increasing pulse-duration/lifetime ratios and pump powers, decreasing values of concurrence are recorded. Nonetheless, additional contributions are still required to fully account for the observed below-unity concurrence.

quant-ph↗

arXiv2022

Experimental Multi-state Quantum Discrimination in the Frequency Domain with Quantum Dot Light

The quest for the realization of effective quantum state discrimination strategies is of great interest for quantum information technology, as well as for fundamental studies. Therefore, it is crucial to develop new and more efficient methods to implement discrimination protocols for quantum states. Among the others, single photon implementations are more advisable, because of their inherent security advantage in quantum communication scenarios. In this work, we present the experimental realization of a protocol employing a time-multiplexing strategy to optimally discriminate among eight non-orthogonal states, encoded in the four-dimensional Hilbert space spanning both the polarization degree of freedom and photon energy. The experiment, built on a custom-designed bulk optics analyser setup and single photons generated by a nearly deterministic solid-state source, represents a benchmarking example of minimum error discrimination with actual quantum states, requiring only linear optics and two photodetectors to be realized. Our work paves the way for more complex applications and delivers a novel approach towards high-dimensional quantum encoding and decoding operations.

quant-ph↗

arXiv2022

Optical properties of circular Bragg gratings with labyrinth geometry to enable electrical contacts

We present an optical study of various device designs for electrically contactable circular Bragg grating cavities in labyrinth geometries. To create an electrical connection between the central disk and the surrounding membrane, which are separated through air gaps, we introduce connections between the adjacent rings. We propose to rotate these connections, creating a labyrinth like structure, to disable waveguiding and keep the mode confinement. To investigate how different arrangement and size of the connections affect the optical properties and to find the optimal design, six different layouts with either 3-fold or 4-fold symmetry and one with 2-fold symmetry are investigated experimentally and by numerical simulations. Reflectivity measurements and simulations show that rotating the connections improves the mode confinement, far-field pattern and Purcell factor compared to layouts with connections arranged in straight lines. We compare results between different layouts for different connection widths and perform polarization resolved measurements to investigate whether the connections create asymmetries in the photonic confinement that would impede the performance of the device.

physics.optics↗