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Qun Zhu

Publications and source records attributed to Qun Zhu.

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Distinct Surface and Bulk Superconductivity in the Kagome Superconductor SrSn$_3$

Surface and bulk superconductivity may possess fundamentally different superconducting properties in quantum materials with nontrivial electronic structures, yet their superimposed spectroscopic signatures often prevent direct experimental access to each superconducting channel. Here we reveal, in epitaxial films of the kagome superconductor SrSn$_3$, distinct surface and bulk superconducting channels with markedly different superconducting gaps, upper critical fields, and vortex-core electronic states by tuning the tunneling junction resistance in scanning tunneling spectroscopy. The surface superconductivity is characterized by a thickness-independent superconducting gap and an enhanced upper critical field, whereas the bulk superconducting channel exhibits a larger superconducting gap that decreases with reducing film thickness and a much lower upper critical field. Within magnetic vortex cores, robust non-split zero-bias conductance peaks are observed exclusively in the surface superconducting channel, while pronounced zero-bias suppression is consistently associated with the bulk superconducting channel. These findings demonstrate that the vortex-core electronic structure depends sensitively on the underlying superconducting channel, providing new insight into vortex-bound states in topological quantum materials.

cond-mat.supr-con

Tip-Tuned Renormalization-Group Spectroscopy Unmasks a False-positive Topological Superconducting Vortex

Clean, nonsplit vortex zero-bias peaks (ZBPs) can be misinterpreted as Majorana zero modes (MZMs), making static scanning tunneling microscopy intrinsically ambiguous. Here we use the STM tip coupling to drive a local boundary-renormalization-group (boundary RG) flow, turning dynamical Coulomb blockade into a falsification test for Majorana-like ZBPs. Experimentally, in a $\mathrm{SrSn}_3$ thin film, normal-state spectra establish an Ohmic dissipative environment, and a common boundary-RG/thermodynamic-Bethe-ansatz analysis of the superconducting-gap and vortex-center spectra yields consistent dissipation strengths within the $r < 1/2$ Majorana-filter regime. Lowering the tip nevertheless drives a clean, non-split vortex-center ZBP into a zero-bias dip, opposite to the protected flow of an isolated MZM, unmasking the peak as a Majorana false positive produced by a conventional vortex-core state. The same flow selectively suppresses the strongly tip-coupled channel, resolving the two-gap superconductivity. Dissipative STM thus tests dynamical protection rather than spectral appearance.

cond-mat.mes-hall

Antiferromagnetic Quantum Criticality in Infinite-Layer Cuprates Sr1-xNdxCuO2

The interplay between quantum criticality and Fermi surface reconstruction is central to elucidating the phase diagram of high-temperature cuprate superconductors. While studies on electron-doped T'-structure cuprates suggest an antiferromagnetic origin of this reconstruction, quantitative consensus has been hindered by apical oxygen instabilities and uncontrolled oxygen vacancies. Here, we overcome these limitations by utilizing ozone-assisted molecular beam epitaxy to synthesize high-quality, oxygen-stoichiometric thin films of infinite-layer cuprate Sr1-xNdxCuO2 across its entire superconducting dome. Hall transport measurements reveal a sharp carrier-type transition signaling a Fermi surface reconstruction at a critical doping xc ~ 0.155. We show that a spin-density-wave tight-binding model quantitatively reproduces the transport evolution, supporting an antiferromagnetic origin of this quantum phase transition. Furthermore, upon suppressing superconductivity with magnetic fields, the normal-state resistivity exhibits a pristine strange metal behavior that persists down to 2 K in the vicinity of xc. Our findings establish an intrinsic, universal antiferromagnetic quantum criticality in electron-doped cuprates, positioning the structurally simplest infinite-layer cuprates as a clean benchmark platform for theories of unconventional superconductivity.

cond-mat.supr-con

Enhancement of superconductivity in electron-hole coexisting Sr$_{1-x}$Eu$_{x}$CuO$_{2+y}$ films

We report transport measurements of infinite-layer cuprate Sr$_{1-x}$Eu$_{x}$CuO$_{2+y}$ films with controlled electron (by trivalent europium) and hole (by interstitial apical oxygen) carriers grown on SrTiO$_3$(001) with molecular beam epitaxy. An unusual enhancement of superconductivity upon moderate electron-hole coexistence in the films is found, which spans over the whole superconducting phase diagram and becomes more prominent in the underdoped regime. The superconductivity exhibits a two-dimensional nature with a thickness of approximately 5.2 nm, irrespective of the varying carriers, confirmed by angle-resolved magnetoresistance measurements and the Berzzinsky-Kosterlitz-Thouless transition. Nevertheless, the electron-hole coexistence enlarges the thermal activation energy of vortex motion that deviates obviously from the usual logarithmic evolution with the magnetic field. Our results offer a promising perspective to understand and enhance the high-temperature superconductivity in cuprates.

cond-mat.supr-con

Anomalous superconducting proximity effect of planar Pb-RhPb2 heterojunctions in the clean limit

Interest in superconducting proximity effect has been revived by the exploitation of Andreev states and by the possible emergence of Majorana bound states at the interface. Spectroscopy of these states has been so far restricted to just a handful of superconductor-metal systems in the diffusion regime, whereas reports in otherwise clean superconductor-superconductor heterojunctions are scarce. Here, we realize molecular beam epitaxy growth of atomically sharp planar heterojunctions between Pb and a topological superconductor candidate RhPb2 that allows us to spectroscopically image the proximity effect in the clean limit. The measured energy spectra of RhPb2 vary with the spatial separation from proximal Pb, and exhibit unusual modifications in the pairing gap structure and size that extend over a distance far beyond the coherence length. This anomalously long-range proximity (LRP) effect breaks the rotational symmetry of Cooper pair potential in real space and largely deforms the Abrikosov vortex cores. Our work opens promising avenues for fundamental studies of the Andreev physics and extraordinary states in clean superconducting heterojunctions.

cond-mat.supr-con