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R K Gopal

Publications and source records attributed to R K Gopal.

3 recordsLinked to original sources

Photon Momentum Enabled Symmetry Breaking and Nonlinear Photocurrents in the Centrosymmetric Dirac Semimetal PdTe

In centrosymmetric Dirac semimetals, second order nonlinear photocurrents are forbidden by the coexistence of time-reversal and inversion symmetries. Here, we demonstrate that finite photon momentum transfer acts as a dynamic symmetry breaking mechanism in PdTe, enabling nonlinear optical responses that are nominally forbidden in the centrosymmetric bulk. Through polarization sensitive measurements, we resolve distinct contributions from the circular photogalvanic effect (CPGE), geometric shift currents, and photon drag mediated processes. We show that the helicity dependent current vanishes at normal incidence and reverses sign with the angle of incidence, reflecting the coupling between photons and spin polarized surface states. Crucially, thickness dependent analysis reveals that the helicity dependent photocurrent component C scales with film thickness, establishing a robust bulk contribution enabled by momentum transfer. This confirms that incident photons provide the directional axis required to probe interband quantum geometry, rather than the response originating solely from surface states or strain. Our results demonstrate that optical excitation can dynamically reduce the effective symmetry of the system, enabling access to quantum geometric tensors and establishing PdTe as a promising platform for exploring nonequilibrium dynamics governed by photon momentum in high symmetry topological materials.

cond-mat.mes-hall

Magnetoconductance evolution across the topological-trivial phase transition in ${In_{x}}({Bi_{0.3}}{Sb_{0.7}})_{2-x}{Te_3}$ thin films

We investigate the evolution of electronic transport across the topological-trivial phase transition in ${\rm In}_{x}({\rm Bi}_{0.3}{\rm Sb}_{0.7})_{2-x}{\rm Te}_3$ thin films by systematically tuning the indium concentration $x$. Increasing $x$ reduces the effective spin-orbit coupling, driving a topological quantum phase transition near $x \approx 7\%$, and at higher disorder a crossover from diffusive to strongly localized transport around $x \approx 15\%$. In the diffusive regime, the magnetoconductance is well described by the Hikami-Larkin-Nagaoka formalism, with the evolution of the WAL prefactor $\alpha$ correlating with the band-inversion transition. Beyond the diffusive limit, transport crosses into variable-range hopping, accompanied by a striking reversal of magnetoconductance from negative to positive. The observed positive low-field magnetoconductance, its pronounced anisotropy, and its temperature evolution point to an orbital origin of the response. These features are naturally captured by incorporating the incoherent hopping mechanism of Raikh \textit{et al.} together with wavefunction shrinkage, rather than by conventional quantum-correction frameworks. Our results provide a unified picture of how topology, spin-orbit coupling, and disorder collectively determine the full field-temperature magnetotransport landscape in this material class, establishing a clear experimental link between the topological phase transition and the onset of incoherent hopping-dominated conduction.

cond-mat.mtrl-sci

Parallel and series conduction model in Topological Insulators

In the past few years there has been a surge in the material science engineering in order to synthesize bulk insulating and surface metallic Topological Insulating (TI) materials. This quest is not only theoretically important but also promising from the novel application perspective. The dependence of temperature on resistance (R-T) of a particular sample reveals a plethora of information about the electronic properties especially in a unique sample like TI where there are two components comprising of an insulating bulk and metallic surface states. Depending on the amount of intrinsic doping during the sample formation, the bulk can either couple or remain decoupled with the surface. The former leads to a metallic R-T profile whereas the latter is captured by an insulating R-T behavior. These two behaviors can be represented by series and parallel resistor models respectively. In this work we study the R-T behavior in the framework of resistor models capturing the essential features of our sample.

cond-mat.str-el