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Rémi Goerlich

Publications and source records attributed to Rémi Goerlich.

18 recordsLinked to original sources

Piston-Like Information Engine II: Boundary-Controlled Optimum in Active Matter

Information engines convert information into extractable work through measurements and feedback. We realize an engine that employs information to compress a gas of self-propelled bristle bots. Its work per measurement, $\bar{W}$, is controlled by the size of the detection region $Δx$ and the probability $p_1$ that this region is vacant. In thermal systems, $\bar{W}$ follows the universal form $-p_1 \ln p_1$, whereas the active engine shows a qualitatively modified relation. As particle density increases, the maximum of $\bar{W}(Δx)$ switches between two distinct operating regimes. Notably, this transition is also found in the solutions that maximize power output for finite-time cycles with dynamics affected by dry friction. We attribute this nonequilibrium feature to the accumulation of active particles near the boundaries.

cond-mat.stat-mech

Stochastic Resetting: A Non-Equilibrium Framework for Prediction, Inference and Design

Stochastic resetting has evolved from a simple model of diffusive search acceleration into a general framework for predicting, inferring, and controlling stochastic dynamics far from equilibrium. Its defining features, i.e., the creation of non-equilibrium steady states and the acceleration of first-passage kinetics, are increasingly relevant across physical chemistry, from biological restart mechanisms to molecular simulations and colloidal experiments. We review the renewal theory underlying stochastic resetting and show how it enables prediction of reset dynamics from properties of the underlying process, while also allowing the latter to be inferred from the resetting-accelerated dynamics. We then discuss applications to state preparation, enhanced sampling, kinetic inference, and training and sampling of machine learning models. Finally, we review recent advances in adaptive resetting, environmental feedback, many-body dynamics, and thermodynamic costs of resetting. These developments establish new opportunities for controlling stochastic dynamics with resetting across theory, simulations, and experiments.

physics.chem-ph

A particle-resolved rheological study of chirality transfer and odd transport

Chirality, or the breaking of mirror symmetry, appears across all scales in nature, from molecular conformations to the dynamics of bacterial collectives. Environments composed of such symmetry-breaking constituents can give rise to emergent physical phenomena, particularly in the transport and response of embedded tracers. Yet it remains unclear how chiral environments influence such tracers and through which microscopic mechanisms anomalous responses emerge. Here, we present a particle-resolved study of these systems, demonstrating chirality transfer and odd transport of an object embedded in a chiral active bath. In a rheological experiment, a symmetric passive tracer is driven through collisions with the particles of a non-equilibrium chiral bath. Combining table-top experiments, many-body simulations, and a reduced coarse-grained theory, we demonstrate that local collisions transfer chiral active dynamics to the tracer, which displays circular trajectories. We show that the same mechanism gives rise to a systematic transverse drift under a constant pulling force. Crucially, we identify nonlinear friction as an essential factor that rectifies these transferred chiral active fluctuations into a macroscopic odd response. Our results reveal a microscopic mechanism for odd transport in chiral active matter and provide general insights into transverse transport in driven non-equilibrium systems.

cond-mat.stat-mech

Probing the limits of effective temperature consistency in actively driven systems

We investigate the thermodynamic properties of a single inertial probe driven into a nonequilibrium steady-state by random collisions with self-propelled active walkers. The probe and walkers are confined within a gravitational harmonic potential. We evaluate the robustness of the effective temperature concept in this active system by comparing values of distinct, independently motivated definitions: a generalized fluctuation-dissipation relation, a kinetic temperature, and a work fluctuation relation. Our experiments reveal that, under specific conditions, these independent measurements yield a remarkably consistent effective temperature over a wide range of system configurations. Furthermore, we also identify regimes where this consistency breaks down, which delineates the fundamental limits of extending equilibrium-like thermodynamic concepts to athermal, actively driven systems.

cond-mat.stat-mech

Fluctuation-response relation for a nonequilibrium system with resolved Markovian embedding

Fluctuation-response relations must be modified to describe nonequilibrium systems with non-Markovian dynamics. Here, we experimentally demonstrate that such relation is quantitatively recovered when the appropriate Markovian embedding of the dynamics is explicitly resolved. Using a colloidal particle optically trapped in a harmonic potential and driven out of equilibrium by a controlled colored noise, we study the response to a perturbation of the stiffness of the confining potential. While the reduced dynamics violates equilibrium fluctuation-response relations, we show that the dynamical response to the stiffness perturbation is fully determined by steady-state correlations involving the exact conjugate observable in the Markovian embedding.

cond-mat.stat-mech

Consistent thermodynamics reconstructed from transitions between nonequilibrium steady-states

Constructing a thermodynamic framework for nonequilibrium systems remains a major challenge, as quantities such as temperature and free energy often become ambiguous when inferred solely from steady-state properties. Here we take a transformation-based approach and experimentally examine transitions between nonequilibrium steady states (NESS). Using an optically trapped microparticle driven by a tunable correlated stochastic force, we generate active-like steady states with controllable noise statistics. By abruptly changing the trap stiffness, we measure the stochastic work, heat, and entropy produced during NESS-to-NESS transformations. We identify a state-dependent effective temperature that restores the second law for these transitions, enabling the definition of a generalized work that incorporates the consequence of the nonequilibrium fluctuations. With this quantity, we derive and experimentally verify a Crooks-like fluctuation relation linking work distributions to a nonequilibrium free-energy difference defined through the effective temperature. Finally, we establish a fluctuation-response relation for the positional variance following stiffness changes. We demonstrate that this relation is key to distinguishing systems that can be described by a unique effective temperature (i.e., those under equilibrium or white-noise conditions) from those under colored-noise, where an equilibrium-like response cannot be restored. These results delineate the applicability and limits of effective-temperature thermodynamics in driven systems.

cond-mat.stat-mech

Piston-Like Information Engine I: Universal Features in Equilibrium

The ability to measure the stochastic degrees of freedom of a thermal system enables the extraction of energy from an equilibrium heat bath. This is the underlying principle of Maxwell's demon and subsequent information engines. Here, we experimentally realize a microscopic information engine configured as a compressible piston containing a thermalized colloidal suspension. The particle positions are recorded to identify when a predefined region near the wall is empty, allowing the piston to compress the colloidal suspension without applying work on the system. We find that the stored compression energy is universally set by the probability of a positive measurement outcome, which in turn is controlled by parameters such as density and compression step size. We further demonstrate that mechanical work can be extracted during the decompression of the piston, thereby closing the engine's operating cycle.

cond-mat.stat-mech

Time-energy tradeoff in stochastic resetting using optimal control

Stochastic resetting is a driving mechanism that is known to minimize the first passage time to reach a target, at the cost of energy expenditure. The choice of the physical implementation of each resetting event determines the tradeoff between the acceleration of the search process and its energetic cost. Here, we present an optimal transport protocol that balances the duration and the energetic cost of each resetting event. This protocol drives a harmonically trapped Brownian particle between two equilibrium states within a finite time and with minimal energetic cost. An explicit comparison with other types of finite-time protocols further shows its specific thermodynamic properties. Its cost is both a lower bound on the cost of unoptimized shortcut protocols and an upper bound on the cost of optimal protocols which do not ensure final equilibrium. When applying the optimal transport protocol to implement stochastic resetting, a single lower time-energy bound is reached: this protocol allows to reach the best tradeoff between energetic cost and search time.

cond-mat.stat-mech

Harnessing non-equilibrium forces to optimize work extraction

While optimal control theory offers effective strategies for minimizing energetic costs in noisy microscopic systems over finite durations, a significant opportunity lies in exploiting the temporal structure of non-equilibrium forces. We demonstrate this by presenting exact analytical forms for the optimal protocol and the corresponding work for any driving force and protocol duration. We also derive a general quasistatic bound on the work, relying only on the coarse-grained, time-integrated characteristics of the applied forces. Notably, we show that the optimal protocols often automatically act as information engines that harness information about non-equilibrium forces and an initial state measurement to extract work. These findings chart new directions for designing adaptive, energy-efficient strategies in noisy, time-dependent environments, as illustrated through our examples of periodic driving forces and active matter systems. By exploiting the temporal structure of non-equilibrium forces, this largely unexplored approach holds promise for substantial performance gains in microscopic devices operating at the nano- and microscale.

cond-mat.stat-mech

Experimental Realizations of Information Engines: Beyond Proof of Concept

Gathering information about a system enables greater control over it. This principle lies at the core of information engines, which use measurement-based feedback to rectify thermal noise and convert information into work. Originating from Maxwell's and Szilárd's thought experiments, the thermodynamics of information engines has steadily advanced, with recent experimental realizations both confirming established results and pushing the field forward. Coupled with technological advances and developments in nonequilibrium thermodynamics, novel implementations of information engines continue to challenge theoretical understanding. In this perspective, we discuss recent progress and highlight new opportunities, such as applying information engines to active, many-body, and inertial systems, and leveraging tools like optimal control to design their driving protocols.

cond-mat.stat-mech

Taming a Maxwell's demon for experimental stochastic resetting

A diffusive process that is reset to its origin at random times, so-called stochastic resetting (SR), is an ubiquitous expedient in many natural systems . Yet, beyond its ability to improve the efficiency of target searching, SR is a true non-equilibrium thermodynamic process that brings forward new and challenging questions . Here, we show how the recent developments of experimental information thermodynamics renew the way to address SR and can lead, beyond a new understanding, to better control on the non-equilibrium nature of SR. This thermodynamically controlled SR is experimentally implemented within a time-dependent optical trapping potential. We show in particular that SR converts heat into work from a single bath continuously and without feedback. This implements a Maxwell's demon that constantly erases information. In our experiments, the erasure takes the form of a protocol that allows to evaluate the true energetic cost of SR. We show that using an appropriate measure of the available information, this cost can be reduced to a reversible minimum while being bounded by the Landauer limit. We finally reveal that the individual trajectories generated by the demon all break ergodicity and thus demonstrate the non-ergodic nature of the demon's modus operandi. Our results offer new approaches to processes, such as SR, where the informational framework provides key experimental tools for their non-equilibrium thermodynamic control.

cond-mat.stat-mech

Shortcuts to adiabaticity in harmonic traps: a quantum-classical analog

We present a new technique for efficiently transitioning a quantum system from an initial to a final stationary state in less time than is required by an adiabatic (quasi-static) process. Our approach makes use of Nelson's stochastic quantization, which represents the quantum system as a classical Brownian process. Thanks to this mathematical analogy, known protocols for classical overdamped systems can be translated into quantum protocols. In particular, one can use classical methods to find optimal quantum protocols that minimize both the time duration and some other cost function to be freely specified. We have applied this method to the time-dependent harmonic oscillator and tested it on two different cost functions: (i) the cumulative energy of the system over time and (ii) the dynamical phase of the wavefunction. In the latter case, it is possible to construct protocols that are "adiabatically optimal", i.e., they minimize their distance from an adiabatic process for a given duration.

quant-ph

Resetting as a swift equilibration protocol in an anharmonic potential

We present and characterize a method to accelerate the relaxation of a Brownian object between two distinct equilibrium states. Instead of relying on a deterministic time-dependent control parameter, we use stochastic resetting to guide and accelerate the transient evolution. The protocol is investigated numerically, and its thermodynamic cost is evaluated with the tools of stochastic thermodynamics. Remarkably, we show that stochastic resetting significantly accelerates the relaxation to the final state. This stochastic protocol exhibits energetic and temporal characteristics that align with the scales observed in previously investigated deterministic protocols. Moreover, it expands the spectrum of stationary states that can be manipulated, incorporating new potential profiles achievable through experimentally viable protocols.

cond-mat.stat-mech

A many-body Szilard engine with giant number fluctuations

Szilárd's information engine is a canonical example in the field of thermodynamics of information. We realize experimentally a macroscopic many-particle Szilárd engine that consists of active particles and use it to lift a mass against gravity. We show that the extractable work per cycle increases when the raised weight is changed more gradually during the process. Interestingly, we find that the ideal extractable work grows with the number of particles due to giant number fluctuations. This is in contrast to the calculated behavior of a similar engine operating on thermal particles.

cond-mat.stat-mech

Optimal time-entropy bounds and speed limits for Brownian thermal shortcuts

By controlling in real-time the variance of the radiation pressure exerted on an optically trapped microsphere, we engineer temperature protocols that shortcut thermal relaxation when transferring the microsphere from one thermal equilibrium state to an other. We identify the entropic footprint of such accelerated transfers and derive optimal temperature protocols that either minimize the production of entropy for a given transfer duration or accelerate as much as possible the transfer for a given entropic cost. Optimizing the trade-off yields time-entropy bounds that put speed limits on thermalization schemes. We further show how optimization expands the possibilities for accelerating Brownian thermalization down to its fundamental limits. Our approach paves the way for the design of optimized, finite-time thermodynamic cycles at the mesoscale. It also offers a platform for investigating fundamental connections between information geometry and finite-time processes.

cond-mat.stat-mech

Harvesting information to control non-equilibrium states of active matter

We propose to use a correlated noise bath to drive an optically trapped Brownian particle that mimics active biological matter. Thanks to the flexibility and precision of our setup, we are able to control the different parameters that drive the stochastic motion of the particle with unprecedented accuracy, thus reaching strongly correlated regimes that are not easily accessible with real active matter. In particular, by using the correlation time (i.e., the "color") of the noise as a control parameter, we can trigger transitions between two non-equilibrium steady states with no expended work, but only a calorific cost. Remarkably, the measured heat production is directly proportional to the spectral entropy of the correlated noise, in a fashion that is reminiscent of Landauer's principle. Our procedure can be viewed as a method for harvesting information from the active fluctuations.

cond-mat.soft

Probing quantum effects with classical stochastic analogs

We propose a method to construct a classical analog of an open quantum system, namely a single quantum particle confined in a potential well and immersed in a thermal bath. The classical analog is made out of a collection of identical wells where classical particles of mass $m$ are trapped. The distribution $n(x,t)$ of the classical positions is used to reconstruct the quantum Bohm potential $V_{\rm Bohm} = -\frac{\hbar^2}{2 m} \frac{Δ\sqrt{n}}{\sqrt{n}}$, which in turn acts on the shape of the potential wells. As a result, the classical particles experience an effective "quantum" force. This protocol is tested with numerical simulations using single- and double-well potentials, evidencing typical quantum effects such as long-lasting correlations and quantum tunneling. For harmonic confinement, the analogy is implemented experimentally using micron-sized dielectric beads optically trapped by a laser beam.

quant-ph

Noise and ergodic properties of Brownian motion in an optical tweezer: looking at the crossover between Wiener and Ornstein-Uhlenbeck processes

We characterize throughout the spectral range of an optical trap the nature of the noise at play and the ergodic properties of the corresponding Brownian motion of an overdamped trapped single microsphere, comparing experimental, analytical and simulated data. We carefully analyze noise and ergodic properties $(i)$ using the Allan variance for characterizing the noise and $(ii)$ exploiting a test of ergodicity tailored for experiments done over finite times. We derive these two observables in the low-frequency Ornstein-Uhlenbeck trapped-diffusion regime and study analytically their evolution towards the high-frequency Wiener free-diffusion regime, in a very good agreement with simulated and experimental results. This leads to reveal noise and ergodic spectral signatures associated with the distinctive features of both regimes.

cond-mat.stat-mech