arXiv subjects

R. A. Baggott

Publications and source records attributed to R. A. Baggott.

4 recordsLinked to original sources

arXiv2024

Extended X-ray absorption spectroscopy using an ultrashort pulse laboratory-scale laser-plasma accelerator

Laser-driven compact particle accelerators can provide ultrashort pulses of broadband X-rays, well suited for undertaking X-ray absorption spectroscopy measurements on a femtosecond timescale. Here the Extended X-ray Absorption Fine Structure (EXAFS) features of the K-edge of a copper sample have been observed over a 250 eV window in a single shot using a laser wakefield accelerator, providing information on both the electronic and ionic structure simultaneously. This unique capability will allow the investigation of ultrafast processes, and in particular, probing high-energy-density matter and physics far-from-equilibrium where the sample refresh rate is slow and shot number is limited. For example, states that replicate the tremendous pressures and temperatures of planetary bodies or the conditions inside nuclear fusion reactions. Using high-power lasers to pump these samples also has the advantage of being inherently synchronised to the laser-driven X-ray probe. A perspective on the additional strengths of a laboratory-based ultrafast X-ray absorption source is presented.

physics.plasm-ph↗

arXiv2021

Temperature Equilibration Due to Charge State Fluctuations in Dense Plasmas

The charge states of ions in dense plasmas fluctuate due to collisional ionization and recombination. Here we show how, by modifying the ion interaction potential, these fluctuations can mediate energy exchange between the plasma electrons and ions. Moreover, we develop a theory for this novel electron-ion energy transfer mechanism. Calculations using a random walk approach for the fluctuations suggest that the energy exchange rate from charge state fluctuations could be comparable to direct electron-ion collisions. This mechanism is, however, predicted to exhibit a complex dependence on the temperature and ionization state of the plasma, which could contribute to our understanding of significant variation in experimental measurements of equilibration times.

physics.plasm-ph↗

arXiv2020

Calculating Opacity in Hot, Dense Matter using Second-Order Electron-Photon and Two-Photon Transitions to Approximate Line Broadening

Calculations of the opacity of hot, dense matter require models for plasma line broadening. However, the most general theories are too complex to calculate directly and some approximation is inevitably required. The most widely-used approaches focus on the line centre, where a Lorentzian shape is obtained. Here, we demonstrate that in the opposite limit, far from the line centre, the opacity can be expressed in terms of second-order transitions, such as electron-photon and two-photon processes. We suggest that this insight could form the basis for a new approach to improve calculations of opacity in hot, dense matter. Preliminary calculations suggest that this approach could yield increased opacity away from absorption lines.

physics.plasm-ph↗

arXiv2019

Single-shot multi-keV X-ray absorption spectroscopy using an ultrashort laser wakefield accelerator source

Single-shot absorption measurements have been performed using the multi-keV X-rays generated by a laser wakefield accelerator. A 200 TW laser was used to drive a laser wakefield accelerator in a mode which produced broadband electron beams with a maximum energy above 1 GeV and a broad divergence of $\approx15$ miliradians FWHM. Betatron oscillations of these electrons generated $1.2\pm0.2\times10^6$ photons/eV in the 5 keV region, with a signal-to-noise ratio of approximately 300:1. This was sufficient to allow high-resolution XANES measurements at the K-edge of a titanium sample in a single shot. We demonstrate that this source is capable of single-shot, simultaneous measurements of both the electron and ion distributions in matter heated to eV temperatures by comparison with DFT simulations. The unique combination of a high-flux, large bandwidth, few femtosecond duration X-ray pulse synchronised to a high-power laser will enable key advances in the study of ultra-fast energetic processes such as electron-ion equilibration.

physics.plasm-ph↗