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R. Acevedo-Esteves

Publications and source records attributed to R. Acevedo-Esteves.

4 recordsLinked to original sources

Structural and magnetic properties of TbCuAs$_2$ studied by X-ray and neutron scattering

We investigated antiferromagnetic metal TbCuAs$_2$, which exhibits an anomalous resistivity upturn at low temperatures. This resistivity upturn has been proposed to originate from the material's magnetic ground state; however, the precise nature of the antiferromagnetic ordering in this compound has not been previously established. Here, we present a combined single crystal neutron diffraction, X-ray resonant magnetic scattering, and single crystal X-ray diffraction study of TbCuAs$_2$. These measurements unambiguously determine the Tb magnetic moment direction, the antiferromagnetic arrangement along high symmetry directions, the interplay between structure and magnetism, and their temperature dependence. Our observations are compared with previous studies on sister compounds in the rare-earth copper arsenide family ($R$CuAs$_2$, $R$ = Sm and Gd), which also displays resistivity anomalies. We suggest a common underlying physics governing the structural and magentic properties of rare-earth copper arsenides that exhibit low-temperature resistivity anomalies.

cond-mat.str-el

Low temperature magnetic structure and lattice response in SmCuAs$_2$

We investigated the structural and magnetic properties of single-crystalline SmCuAs$_2$ using high-resolution synchrotron X-ray diffraction and X-ray resonant magnetic scattering (XRMS) at the Sm $L_2$ and $L_3$ edges. Temperature-dependent diffraction measurements confirm that SmCuAs$_2$ maintains its tetragonal symmetry from room temperature down to 8 K, with lattice parameters showing anomalous behavior below the resistivity minimum ($T \approx$ 30 K). Notably, the \textbf{c}-axis lattice parameter exhibits a plateau and subsequent increase near the Néel temperature, indicating magnetoelastic coupling. XRMS measurements reveal a commensurate antiferromagnetic structure with a propagation vector \textbf{\textit{q}} = (0, 0, 0.5). Our measurement shows that the Sm moments are aligned within the \textbf{\textit{ab}} plane and arranged in a $++--$ stacking along the \textbf{\textit{c}}-axis. Comparison with related \textit{RE}CuAs$_2$ compounds (\textit{RE} = Pr, Nd, and Gd) suggests that in-plane moment orientation and associated magnetic frustration play a key role in the emergence of the resistivity minimum. Differences in spin-orbit and magnetoelastic coupling across the series highlight their importance in governing low-temperature transport behavior.

cond-mat.str-el

Emergence of spinons in layered trimer iridate Ba4Ir3O10

Spinons are well-known as the elementary excitations of one-dimensional antiferromagnetic chains, but means to realize spinons in higher dimensions is the subject of intense research. Here, we use resonant x-ray scattering to study the layered trimer iridate Ba4Ir3O10, which shows no magnetic order down to 0.2 K. An emergent one-dimensional spinon continuum is observed that can be well-described by XXZ spin-1/2 chains with magnetic exchange of ~55 meV and a small Ising-like anisotropy. With 2% isovalent Sr doping, magnetic order appears below TN=130 K along with sharper excitations, indicating that the spinons become more confined in (Ba1-xSrx)4Ir3O10. We propose that the frustrated intra-trimer interactions effectively reduce the system into decoupled spin chains, the subtle balance of which can be easily tipped by perturbations such as chemical doping. Our results put Ba4Ir3O10 between the one-dimensional chain and two-dimensional quantum spin liquid scenarios, illustrating a new way to suppress magnetic order and realize fractional spinons.

cond-mat.str-el

Charge density waves in cuprate superconductors beyond the critical doping

The unconventional normal-state properties of the cuprates are often discussed in terms of emergent electronic order that onsets below a putative critical doping of xc = 0.19. Charge-density wave (CDW) correlations represent one such order; however, experimental evidence for such order generally spans a limited range of doping that falls short of the critical value xc, leading to questions regarding its essential relevance. Here, we use x-ray diffraction to demonstrate that CDW correlations in La2-xSrxCuO4 persist up to a doping of at least x = 0.21. The correlations show strong changes through the superconducting transition, but no obvious discontinuity through xc = 0.19, despite changes in Fermi surface topology and electronic transport at this doping. These results demonstrate the interaction between CDWs and superconductivity even in overdoped cuprates and prompt a reconsideration of the role of CDW correlations in the high-temperature cuprate phase diagram.

cond-mat.supr-con