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R. B. Muniz

Publications and source records attributed to R. B. Muniz.

36 records · Page 2Linked to original sources
arXiv2012

Dynamic RKKY interaction in graphene

The growing interest in carbon-based spintronics has stimulated a number of recent theoretical studies on the RKKY interaction in graphene, based on which the energetically favourable alignment between magnetic moments embedded in this material can be calculated. The general consensus is that the strength of the RKKY interaction in graphene decays as 1/D3 or faster, where D is the separation between magnetic moments. Such an unusually fast decay for a 2-dimensional system suggests that the RKKY interaction may be too short ranged to be experimentally observed in graphene. Here we show in a mathematically transparent form that a far more long ranged interaction arises when the magnetic moments are taken out of their equilibrium positions and set in motion. We not only show that this dynamic version of the RKKY interaction in graphene decays far more slowly but also propose how it can be observed with currently available experimental methods.

cond-mat.mes-hall↗
arXiv2011

Spin Currents in Metallic Nanostructures; Explicit Calculations

In ultrathin ferromagnets deposited on metallic substrates, excitation of precessional motion of the spins produces a spin current in the substrate that transports angular momentum out of the film. This phenomenon is referred to as spin pumping, and is a source of damping of the spin motion. Spin pumping enters importantly in the description of spin dynamics in other nanoscale and subnanoscale systems as well. In this paper, we present an approach based on the Kubo formalism that allows the explicit calculation of this spin current and its spatial variation. We use the formalism to explore features of the spin current generated by spin motions in a simple model system.

cond-mat.mes-hall↗
arXiv2011

Graphene as a non-magnetic spin-current lens

In spintronics, the ability to transport magnetic information often depends on the existence of a spin current traveling between two different magnetic objects acting as source and probe. A large fraction of this information never reaches the probe and is lost because the spin current tends to travel omni-directionally. We propose that a curved boundary between a gated and a non-gated region within graphene acts as an ideal lens for spin currents despite being entirely of non-magnetic nature. We show as a proof of concept that such lenses can be utilized to redirect the spin current that travels away from a source onto a focus region where a magnetic probe is located, saving a considerable fraction of the magnetic information that would be otherwise lost.

cond-mat.mes-hall↗
arXiv2010

Dynamical magnetic excitations of nanostructures from first-principles

Within time-dependent density functional theory, combined with the Korringa-Kohn-Rostoker Green functions, we devise a real space method to investigate spin dynamics. Our scheme enables one to deduce the Coulomb potential which assures a proper Goldstone mode is present. We illustrate with application to 3$d$ adatoms and dimers on Cu(100).

cond-mat.mtrl-sci↗
arXiv2010

Theory of Local Dynamical Magnetic Susceptibilities from the Korringa-Kohn-Rostoker Green Function Method

Within the framework of time-dependent density functional theory combined with the Korringa-Kohn-Rostoker Green function formalism, we present a real space methodology to investigate dynamical magnetic excitations from first-principles. We set forth a scheme which enables one to deduce the correct effective Coulomb potential needed to preserve the spin-invariance signature in the dynamical susceptibilities, i.e. the Goldstone mode. We use our approach to explore the spin dynamics of 3d adatoms and different dimers deposited on a Cu(001) with emphasis on their decay to particle-hole pairs.

cond-mat.mes-hall↗
arXiv2010

Spin Orbit Coupling and Spin Waves in Ultrathin Ferromagnets: The Spin Wave Rashba Effect

We present theoretical studies of the influence of spin orbit coupling on the spin wave excitations of the Fe monolayer and bilayer on the W(110) surface. The Dzyaloshinskii-Moriya interaction is active in such films, by virtue of the absence of reflection symmetry in the plane of the film. When the magnetization is in plane, this leads to a linear term in the spin wave dispersion relation for propagation across the magnetization. The dispersion relation thus assumes a form similar to that of an energy band of an electron trapped on a semiconductor surfaces with Rashba coupling active. We also show SPEELS response functions that illustrate the role of spin orbit coupling in such measurements. In addition to the modifications of the dispersion relations for spin waves, the presence of spin orbit coupling in the W substrate leads to a substantial increase in the linewidth of the spin wave modes. The formalism we have developed applies to a wide range of systems, and the particular system explored in the numerical calculations provides us with an illustration of phenomena which will be present in other ultrathin ferromagnet/substrate combinations.

cond-mat.mes-hall↗
arXiv2010

Graphene-based spin-pumping transistor

We demonstrate with a fully quantum-mechanical approach that graphene can function as gate-controllable transistors for pumped spin currents, i.e., a stream of angular momentum induced by the precession of adjacent magnetizations, which exists in the absence of net charge currents. Furthermore, we propose as a proof of concept how these spin currents can be modulated by an electrostatic gate. Because our proposal involves nano-sized systems that function with very high speeds and in the absence of any applied bias, it is potentially useful for the development of transistors capable of combining large processing speeds, enhanced integration and extremely low power consumption.

cond-mat.mes-hall↗
arXiv2010

Carbon nanotube: a low-loss spin-current waveguide

We demonstrate with a quantum-mechanical approach that carbon nanotubes are excellent spin-current waveguides and are able to carry information stored in a precessing magnetic moment for long distances with very little dispersion and with tunable degrees of attenuation. Pulsed magnetic excitations are predicted to travel with the nanotube Fermi velocity and are able to induce similar excitations in remote locations. Such an efficient way of transporting magnetic information suggests that nanotubes are promising candidates for memory devices with fast magnetization switchings.

cond-mat.mes-hall↗
arXiv2009

Emergence of local magnetic moments in doped graphene-related materials

Motivated by recent studies reporting the formation of localized magnetic moments in doped graphene, we investigate the energetic cost for spin polarizing isolated impurities embedded in this material. When a well-known criterion for the formation of local magnetic moments in metals is applied to graphene we are able to predict the existence of magnetic moments in cases that are in clear contrast to previously reported Density Functional Theory (DFT) results. When generalized to periodically repeated impurities, a geometry so commonly used in most DFT-calculations, this criterion shows that the energy balance involved in such calculations contains unavoidable contributions from the long-ranged pairwise magnetic interactions between all impurities. This proves the fundamental inadequacy of the DFT-assumption of independent unit cells in the case of magnetically doped low-dimensional graphene-based materials. We show that this can be circumvented if more than one impurity per unit cell is considered, in which case the DFT results agree perfectly well with the criterion-based predictions for the onset of localized magnetic moments in graphene. Furthermore, the existence of such a criterion determining whether or not a magnetic moment is likely to arise within graphene will be instrumental for predicting the ideal materials for future carbon-based spintronic applications.

cond-mat.mtrl-sci↗
arXiv2008

Indirect exchange coupling between localized magnetic moments in carbon nanotubes: a dynamic approach

Magnetic moments dilutely dispersed in a metallic host tend to be coupled through the conduction electrons of the metal. This indirect exchange coupling, known to occur for a variety of magnetic materials embedded in several different metallic structures, is of rather long range, especially for low-dimensional structures like carbon nanotubes. Motivated by recent claims that the indirect coupling between magnetic moments in precessional motion has a much longer range than its static counterpart, here we consider how magnetic atoms adsorbed to the walls of a metallic nanotube respond to a time-dependent perturbation that induces their magnetic moments to precess. By calculating the frequency-dependent spin susceptibility we are able to identify resonant peaks whose respective widths provide information about the dynamic aspect of the indirect exchange coupling. We show that by departing from a purely static representation to another in which the moments are allowed to precess, we change from what is already considered a long range interaction to another whose range is far superior. In other words, localized magnetic moments embedded in a metallic structure can feel each other's presence more easily when they are set in precessional motion. We argue that such an effect can have useful applications leading to large-scale spintronics devices.

cond-mat.str-el↗
arXiv2006

Spin Waves in Ultrathin Ferromagnets: Intermediate Wave Vectors

Our earlier papers explore the nature of large wave vector spin waves in ultrathin ferromagnets, and also the properties and damping of spin waves of zero wave vector, at the center of the two dimensional Brillouin zone, with application to FMR studies. The present paper explores the behavior of spin waves in such films at intermediate wave vectors, which connect the two regimes. For the case of Fe films on Au(100), we study the wave vector dependence of the linewidth of the lowest frequency mode, to find that it contains a term which varies as the fourth power of the wave vector. It is argued that this behavior is expected quite generally. We also explore the nature of the eigenvectors of the two lowest lying modes of the film, as a function of wave vector. Interestingly, as wave vector increases, the lowest mode localizes onto the interface between the film and the substrate, while the second mode evolves into a surface spin wave, localized on the outer layer. We infer similar behavior for a Co film on Cu(100), though this evolution occurs at rather larger wave vectors where, as we have shown previously, the modes are heavily damped with the consequence that identification of distinct eigenmodes is problematical.

cond-mat.other↗
arXiv2005

Ferromagnetic Resonance Linewidths in Ultrathin Structures: Theoretical Studies of Spin Pumping

We present theoretical studies of the spin pumping contribution to the ferromagnetic resonance linewidth for various ultrathin film ferromagnetic structures. We consider the isolated film on a substrate, with Fe on Au(100) and Fe on W(110) as examples. We explore as well the linewidth from this mechanism for the optical and acoustical collective modes of FM/Cu$_{\rm N}$/FM/Cu(100) structures. The calculations employ a realistic electronic structure, with self consistent ground states generated from the empirical tight binding method, with nine bands for each material in the structure. The spin excitations are generated through use of the random phase approximation applied to the system, including the semi infinite substrate on which the structure is grown. We calculate the frequency response of the system directly by examining the spectral density associated with collective modes whose wave vector parallel to the surface is zero. Linewidths with origin in leakage of spin angular momentum from the adsorbed structure to the semi infinite substrate may be extracted from these results. We discuss a number of issues, including the relationship between the interfilm coupling calculated adiabatically for trilayers, and that extracted from the (dynamical) spin wave spectrum. We obtain excellent agreement with experimental data, within the framework of calculations with no adjustable parameters.

cond-mat.other↗
arXiv2003

Localization lengths of ultrathin disordered gold and silver nanowires

The localization lengths of ultrathin disordered Au and Ag nanowires are estimated by calculating the wire conductances as functions of wire lengths. We study Ag and Au monoatomic linear chains, and thicker Ag wires with very small cross sections. For the monoatomic chains we consider two types of disorder: bounded random fluctuations of the interatomic distances, and the presence of random substitutional impurities. The effect of impurity atoms on the nanowire conductance is much stronger. Our results show that electrical transport in ultrathin disordered wires may occur in the strong localization regime, and with relatively small amounts of disorder the localization lengths may be rather small. The localization length dependence on wire thickness is investigated for Ag nanowires with different impurity concentrations.

cond-mat.dis-nn↗
arXiv2000

Spin waves in ultrathin ferromagnetic overlayers

The influence of a non-magnetic metallic substrate on the spin wave excitations in ultrathin ferromagnetic overlayers is investigated for different crystalline orientations. We show that spin wave dumping in these systems occur due to the tunneling of holes from the substrate into the overlayer, and that the spin wave energies may be considerably affected by the exchange coupling mediated by the substrate.

cond-mat↗
arXiv1998

Exponential behavior of the interlayer exchange coupling across non-magnetic metallic superlattices

It is shown that the coupling between magnetic layers separated by non-magnetic metallic superlattices can decay exponentially as a function of the spacer thickness $N$, as opposed to the usual $N^{-2}$ decay. This effect is due to the lack of constructive contributions to the coupling from extended states across the spacer. The exponential behavior is obtained by properly choosing the distinct metals and the superlattice unit cell composition.

cond-mat.mes-hall↗
arXiv1996

Exchange Coupling Between Iron Layers Separated by BCC Copper

The exchange coupling between Fe layers separated by BCC Cu is calculated for Fe/Cu/Fe (001) trilayers. It is shown that the coupling is basically regulated by three extrema of the bulk BCC Cu Fermi surface. The contributions from those extrema are all of the same order of magnitude, but that associated with the ``belly'' at the $Γ$-point dominates. The calculated temperature dependence of the coupling varies considerably with spacer layer thickness. Individually, the amplitudes of these extrema contribution decrease with temperature, each according to a different rate. Such an effect may cause an actual increase of coupling with temperature for some Cu thicknesses.

cond-mat↗
arXiv1994

The Nature and Validity of the RKKY limit of exchange coupling in magnetic trilayers

The effects on the exchange coupling in magnetic trilayers due to the presence of a spin-independent potential well are investigated. It is shown that within the RKKY theory no bias nor extra periods of oscillation associated with the depth of the well are found, contrary to what has been claimed in recent works. The range of validity of the RKKY theory is also discussed.

cond-mat↗