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R. Bruce Weisman

Publications and source records attributed to R. Bruce Weisman.

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Single-Walled Carbon Nanotube Sample Purification

Removal of impurities and aggregates from as-grown single walled-carbon nanotube (SWCNT) materials remains an important challenge in nanotube research and applications. We report a simple but effective purification method that uses permanent magnets to remove nanotube aggregates, as well as residual metallic catalyst, from surfactant-coated aqueous SWCNT suspensions. Samples have been characterized by optical absorption, fluorescence and Raman spectroscopies; AFM and near-IR fluorescence microscopies; and TGA. We found that magnetic purification gives samples with reduced absorption backgrounds and high fluorescence efficiencies comparable to those prepared by ultracentrifugation. Nanotubes in magnetically processed HiPco samples are at least 80% individualized. We propose that SWCNT aggregates are preferentially removed because they contain disproportionate amounts of ferromagnetic catalyst particles. As compared to ultracentrifugation, magnetic processing offers major advantages in cost, simplicity, energy consumption, and scalability.

cond-mat.mes-hall

Biexciton, single carrier, and trion generation dynamics in single-walled carbon nanotubes

We present a study of free carrier photo-generation and multi-carrier bound states, such as biexcitons and trions (ionized excitons), in semiconducting single-walled carbon nanotubes. Pump-and-probe measurements performed with fs pulses reveal the effects of strong Coulomb interactions between carriers on their dynamics. Biexciton formation by optical transition from exciton population results in an induced absorption line (binding energy 130 meV). Exciton-exciton annihilation process is shown to evolve at high densities towards an Auger process that can expel carriers from nanotubes. The remaining carriers give rise to an induced absorption due to trion formation (binding energy 190 meV). These features show the dynamics of exciton and free carriers populations.

cond-mat.mes-hall

Structure-Dependent Fluorescence Efficiencies of Individual Single-Walled Carbon Nanotubes

Single-nanotube photometry was used to measure the product of absorption cross-section and fluorescence quantum yield for 12 (n,m) structural species of semiconducting SWNTs in aqueous SDBS suspension. These products ranged from 1.7 to 4.5 x 10(-19) cm2/C atom, generally increasing with optical band gap as described by the energy gap law. The findings suggest fluorescent quantum yields of ~8% for the brightest, (10,2) species and introduce the empirical calibration factors needed to deduce quantitative (n,m) distributions from bulk fluorimetric intensities.

physics.optics

Stepwise Quenching of Exciton Fluorescence in Carbon Nanotubes by Single Molecule Reactions

Single-molecule chemical reactions with individual single-walled carbon nanotubes were observed through near-infrared photoluminescence microscopy. The emission intensity within distinct submicrometer segments of single nanotubes changes in discrete steps after exposure to acid, base, or diazonium reactants. The steps are uncorrelated in space and time, and reflect the quenching of mobile excitons at localized sites of reversible or irreversible chemical attack. Analysis of step amplitudes reveals an exciton diffusional range of about 90 nanometers, independent of nanotube structure. Each exciton visits approximately 104 atomic sites during its lifetime, providing highly efficient sensing of local chemical and physical perturbations.

physics.optics

Absorption spectroscopy of individual single-walled carbon nanotubes

Current methods for producing single-walled carbon nanotubes (SWNTs) lead to heterogeneous samples containing mixtures of metallic and semiconducting species with a variety of lengths and defects. Optical detection at the single nanotube level should thus offer the possibility to examine these heterogeneities provided that both SWNT species are equally well detected. Here, we used photothermal heterodyne detection to record absorption images and spectra of individual SWNTs. Because this photothermal method relies only on light absorption, it readily detects metallic nanotubes as well as the emissive semiconducting species. The first and second optical transitions in individual semicontucting nanotubes have been probed. Comparison between the emission and absorption spectra of the lowest-lying optical transition reveal mainly small Stokes shifts. Side bands in the near-infrared absorption spectra are observed and assigned to exciton-phonon bound states. No such sidebands are detected around the lowest transition of metallic nanotubes.

physics.optics