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R. Côté

Publications and source records attributed to R. Côté.

33 records · Page 2Linked to original sources

Zeeman coupling and screening corrections to skyrmion excitations in graphene

At half filling of the fourfold degenerate Landau levels |n| \geq 1 in graphene, the ground states are spin polarized quantum Hall states that support spin skyrmion excitations for |n| =1,2,3. Working in the Hartree-Fock approximation, we compute the excitation energy of an unbound spin skyrmion-antiskyrmion excitation as a function of the Zeeman coupling strength for these Landau levels. We find for both the bare and screened Coulomb interactions that the spin skyrmion-antiskyrmion excitation energy is lower than the excitation energy of an unbound spin 1/2 electron-hole pair in a finite range of Zeeman coupling in Landau levels |n| =1,2,3. This range decreases rapidly for increasing Landau level index and is extremely small for |n| =3. For valley skyrmions which should be present at 1/4 and 3/4 fillings of the Landau levels |n| =1,2,3, we show that screening corrections are more important in the latter case. It follows that an unbound valley skyrmion-antiskyrmion excitation has lower energy at 3/4 filling than at 1/4. We compare our results with recent experiments on spin and valley skyrmion excitations in graphene.

cond-mat.mes-hall↗

Quantum Hall ferromagnetic phases in the Landau level N=0 of a graphene bilayer

In a Bernal-stacked graphene bilayer, an electronic state in Landau level $% N=0$ is described by its guiding-center index $X$ (in the Landau gauge) and by its valley, spin, and orbital indices $ξ=\pm K,σ=\pm 1,$ and $% n=0,1.$ When Coulomb interaction is taken into account, the chiral two-dimensional electron gas (C2DEG) in this system can support a variety of quantum Hall ferromagnetic (QHF)\ ground states where the spins and/or valley pseudospins and/or orbital pseudospins collectively align in space. In this work, we give a comprehensive account of the phase diagram of the C2DEG at integer filling factors $ν\in [-3,3] $ in Landau level N=0 when an electrical potential difference $Δ_{B}$ between the two layers is varied. We consider states with or without layer, spin, or orbital coherence. For each phase, we discuss the behavior of the transport gap as a function of $Δ_{B},$ the spectrum of collective excitations and the optical absorption due to orbital pseudospin-wave modes. We also study the effect of an external in-plane electric field on a coherent state that has both valley and spin coherence and show that it is possible, in such a state, to control the spin polarization by varying the strength of the external in-plane electric field.

cond-mat.mes-hall↗

Phase diagram of insulating crystal and quantum Hall states in ABC-stacked trilayer graphene

In the presence of a perpendicular magnetic field, ABC-stacked trilayer graphene's chiral band structure supports a 12-fold degenerate N=0 Landau level (LL). Along with the valley and spin degrees of freedom, the zeroth LL contains additional quantum numbers associated with the LL orbital index $% n=0,1,2$. Remote inter-layer hopping terms and external potential difference $Δ_{B}$ between the layers lead to LL splitting by introducing a gap $% Δ_{LL}$ between the degenerate zero-energy triplet LL orbitals. Assuming that the spin and valley degrees of freedom are frozen, we study the phase diagram of this system resulting from competition of the single particle LL splitting and Coulomb interactions within the Hartree-Fock approximation at integer filling factors. Above a critical value $Δ_{LL}^{c}$ of the external potential difference i,e, for $|Δ_{LL}| >Δ_{LL}^{c}$, the ground state is a uniform quantum Hall state where the electrons occupy the lowest unoccupied LL orbital index. For $|Δ_{LL}| <Δ_{LL}^{c}$ (which corresponds to large positive or negative values of $Δ_{B}$) the uniform QH state is unstable to the formation of a crystal state at integer filling factors. This phase transition should be characterized by a Hall plateau transition as a function of $Δ_{LL}$ at a fixed filling factor. We also study the properties of this crystal state and discuss its experimental detection.

cond-mat.mes-hall↗

Influence of a Feshbach resonance on the photoassociation of LiCs

We analyse the formation of ultracold 7Li133Cs molecules in the rovibrational ground state through photoassociation into the B1Pi state, which has recently been reported [J. Deiglmayr et al., Phys. Rev. Lett. 101, 133004 (2008)]. Absolute rate constants for photoassociation at large detunings from the atomic asymptote are determined and are found to be surprisingly large. The photoassociation process is modeled using a full coupled-channel calculation for the continuum state, taking all relevant hyperfine states into account. The enhancement of the photoassociation rate is found to be caused by an `echo' of the triplet component in the singlet component of the scattering wave function at the inner turning point of the lowest triplet a3Sigma+ potential. This perturbation can be ascribed to the existence of a broad Feshbach resonance at low scattering energies. Our results elucidate the important role of couplings in the scattering wave function for the formation of deeply bound ground state molecules via photoassociation.

physics.atom-ph↗

Orbital order in bilayer graphene at filling factor $ν=-1 $

In a graphene bilayer with Bernal stacking both $n=0$ and $n=1$ orbital Landau levels have zero kinetic energy. An electronic state in the N=0 Landau level consequently has three quantum numbers in addition to its guiding center label: its spin, its valley index $K$ or $K^{\prime}$, and an orbital quantum number $n=0,1.$ The two-dimensional electron gas (2DEG) in the bilayer supports a wide variety of broken-symmetry states in which the pseudospins associated these three quantum numbers order in a manner that is dependent on both filling factor $ν$ and the electric potential difference between the layers. In this paper, we study the case of $ν=-1$ in an external field strong enough to freeze electronic spins. We show that an electric potential difference between layers drives a series of transitions, starting from interlayer-coherent states (ICS) at small potentials and leading to orbitally coherent states (OCS) that are polarized in a single layer. Orbital pseudospins carry electric dipoles with orientations that are ordered in the OCS and have Dzyaloshinskii-Moriya interactions that can lead to spiral instabilities. We show that the microwave absorption spectra of ICSs, OCSs, and the mixed states that occur at intermediate potentials are sharply distinct.

cond-mat.mes-hall↗

Observation of Electric Quadrupole Transitions to Rydberg nd States of Ultracold Rubidium Atoms

We report the observation of dipole-forbidden, but quadrupole-allowed, one-photon transitions to high Rydberg states in Rb. Using pulsed UV excitation of ultracold atoms in a magneto-optical trap, we excite $5s \to nd$ transitions over a range of principal quantum numbers $n=27-59$. Compared to dipole-allowed (E1) transitions from $5s \to np$, these E2 transitions are weaker by a factor of approximately 2000. We also report measurements of the anomalous $np_{3/2} : np_{1/2}$ fine-structure transition strength ratio for $n=28-75$. Both results are in agreement with theoretical predictions.

physics.atom-ph↗

Many-body dynamics of Rydberg excitation using the $Ω$-expansion

We investigate the excitation dynamics of Rydberg atoms in ultracold atomic samples by expanding the excitation probability and the correlation function between excited atoms in powers of the isolated atom Rabi frequency $Ω$. In the Heisenberg picture, we give recurrence relations to calculate any order of the expansions, which ere expected to be well-behaved for arbitrarily strong interactions. For homogeneous large samples, we give the explicit form of the expansions, up to $Ω^4$, averaged over all possible random spatial distributions of atoms, for the most important cases of excitation pulses and interactions.

quant-ph↗

Long-range potentials and $(n-1)d+ns$ molecular resonances in an ultracold rydberg gas

We have calculated long-range molecular potentials of the $0_g^{+}$, $0_u^{-}$ and $1_u$ symmetries between highly-excited rubidium atoms. Strong $np+np$ potentials characterized by these symmetries are important in describing interaction-induced phenomena in the excitation spectra of high $np$ Rydberg states. Long-range molecular resonances are such phenomena and they were first reported in S.M. Farooqi {\it et al.}, Phys. Rev. Lett. {\bf 91} 183002. One class of these resonances occurs at energies corresponding to excited atom pairs $(n-1)d+ns$. Such resonances are attributed to $\ell$-mixing due to Rydberg-Rydberg interactions so that otherwise forbidden molecular transitions become allowed. We calculate molecular potentials in Hund's case (c), use them to find the resonance lineshape and compare to experimental results.

physics.atom-ph↗

Many-body Rabi oscillations of Rydberg excitation in small mesoscopic samples

We investigate the collective aspects of Rydberg excitation in ultracold mesoscopic systems. Strong interactions between Rydberg atoms influence the excitation process and impose correlations between excited atoms. The manifestations of the collective behavior of Rydberg excitation are the many-body Rabi oscillations, spatial correlations between atoms as well as the fluctuations of the number of excited atoms. We study these phenomena in detail by numerically solving the many-body Schrëdinger equation.

quant-ph↗

Fluctuations and topological transitions of quantum Hall stripes: nematics as anisotropic hexatics

We study fluctuations and topological melting transitions of quantum Hall stripes near half-filling of intermediate Landau levels. Taking the stripe state to be an anisotropic Wigner crystal (AWC) allows us to identify the quantum Hall nematic state conjectured in previous studies of the 2D electron gas as an {\em anisotropic hexatic}. The transition temperature from the AWC to the quantum Hall nematic state is explicitly calculated, and a tentative phase diagram for the 2D electron gas near half-filling is suggested.

cond-mat.mes-hall↗

Anisotropic states of two-dimensional electrons in high magnetic fields

We study the collective states formed by two-dimensional electrons in Landau levels of index $n\ge 2$ near half-filling. By numerically solving the self-consistent Hartree-Fock (HF) equations for a set of oblique two-dimensional lattices, we find that the stripe state is an anisotropic Wigner crystal (AWC), and determine its precise structure for varying values of the filling factor. Calculating the elastic energy, we find that the shear modulus of the AWC is small but finite (nonzero) within the HF approximation. This implies, in particular, that the long-wavelength magnetophonon mode in the stripe state vanishes like $q^{3/2}$ as in an ordinary Wigner crystal, and not like $q^{5/2}$ as was found in previous studies where the energy of shear deformations was neglected.

cond-mat.mes-hall↗

Solitonic Excitations in Linearly Coherent Channels of Bilayer Quantum Hall Stripes

In some range of interlayer distances, the ground state of the two-dimensional electron gas at filling factor nu =4N+1 with N=0,1,2,... is a coherent stripe phase in the Hartree-Fock approximation. This phase has one-dimensional coherent channels that support charged excitations in the form of pseudospin solitons. In this work, we compute the transport gap of the coherent striped phase due to the creation of soliton-antisoliton pairs using a supercell microscopic unrestricted Hartree-Fock approach. We study this gap as a function of interlayer distance and tunneling amplitude. Our calculations confirm that the soliton-antisoliton excitation energy is lower than the corresponding Hartree-Fock electron-hole pair energy. We compare our results with estimates of the transport gap obtained from a field-theoretic model valid in the limit of slowly varying pseudospin textures.

cond-mat.mes-hall↗

Replica study of pinned bubble crystals

In higher Landau levels ($N>1$), the ground state of the two-dimensional electron gas in a strong perpendicular magnetic field evolves from a Wigner crystal for small filling $ν$ of the partially filled Landau level, into a succession of bubble states with increasing number of guiding centers per bubble as $ν$ increases, to a modulated stripe state near $ν=0.5$. In this work, we compute the frequency-dependent longitudinal conductivity $% σ_{xx}(ω) $ of the Wigner and bubble crystal states in the presence of disorder. We apply an elastic theory to the crystal states which is characterized by a shear and a bulk modulus. We obtain both moduli from the microscopic time-dependent Hartree-Fock approximation. We then use the replica and Gaussian variational methods to handle the effects of disorder. Within the semiclassical approximation we get the dynamical conductivity as well as the pinning frequency as functions of the Landau level filling factor and compare our results with recent microwave experiments.

cond-mat.mes-hall↗

Local Blockade of Rydberg Excitation in an Ultracold Gas

In the laser excitation of ultracold atoms to Rydberg states, we observe a dramatic suppression caused by van der Waals interactions. This behavior is interpreted as a local excitation blockade: Rydberg atoms strongly inhibit excitation of their neighbors. We measure suppression, relative to isolated atom excitation, by up to a factor of 6.4. The dependence of this suppression on both laser irradiance and atomic density are in good agreement with a mean-field model. These results are an important step towards using ultracold Rydberg atoms in quantum information processing.

physics.atom-ph↗

Radiative charge transfer lifetime of the excited state of (NaCa)$^+$

New experiments were proposed recently to investigate the regime of cold atomic and molecular ion-atom collision processes in a special hybrid neutral-atom--ion trap under high vacuum conditions. The collisional cooling of laser pre-cooled Ca$^+$ ions by ultracold Na atoms is being studied. Modeling this process requires knowledge of the radiative lifetime of the excited singlet A$^1Σ^+$ state of the (NaCa)$^+$ molecular system. We calculate the rate coefficient for radiative charge transfer using a semiclassical approach. The dipole radial matrix elements between the ground and the excited states, and the potential curves were calculated using Complete Active Space Self-Consistent field and Möller-Plesset second order perturbation theory (CASSCF/MP2) with an extended Gaussian basis, 6-311+G(3df). The semiclassical charge transfer rate coefficient was averaged over a thermal Maxwellian distribution. In addition we also present elastic collision cross sections and the spin-exchange cross section. The rate coefficient for charge transfer was found to be $2.3\times 10^{-16}$ cm$^3$/sec, while those for the elastic and spin-exchange cross sections were found to be several orders of magnitude higher ($1.1\times 10^{-8}$ cm$^3$/sec and $2.3\times 10^{-9}$ cm$^3$/sec, respectively). This confirms our assumption that the milli-Kelvin regime of collisional cooling of calcium ions by sodium atoms is favorable with the respect to low loss of calcium ions due to the charge transfer.

physics.atom-ph↗