arXiv subjects

R. C. Budhani

Publications and source records attributed to R. C. Budhani.

At least 55 records · Page 3Linked to original sources

arXiv2009

Magnetotransport in polycrystalline La$_{2/3}$Sr$_{1/3}$MnO$_{3}$ thin films of controlled granularity

Polycrystalline La$_{2/3}$Sr$_{1/3}$MnO$_{3}$ (LSMO) thin films were synthesized by pulsed laser ablation on single crystal (100) yttria-stabilized zirconia (YSZ) substrates to investigate the mechanism of magneto-transport in a granular manganite. Different degrees of granularity is achieved by using the deposition temperature (T$_{D}$) of 700 and 800 $^{0}$C. Although no significant change in magnetic order temperature (T$_C$) and saturation magnetization is seen for these two types of films, the temperature and magnetic field dependence of their resistivity ($ρ$(T, H)) is strikingly dissimilar. While the $ρ$(T,H) of the 800 $^{0}$C film is comparable to that of epitaxial samples, the lower growth temperature leads to a material which undergoes insulator-to-metal transition at a temperature (T$_{P}$ $\approx$ 170 K) much lower than T$_C$. At T $\ll$ T$_P$, the resistivity is characterized by a minimum followed by ln $\emph{T}$ divergence at still lower temperatures. The high negative magnetoresistance ($\approx$ 20$%$) and ln $\emph{T}$ dependence below the minimum are explained on the basis of Kondo-type scattering from blocked Mn-spins in the intergranular material. Further, a striking feature of the T$_D$ = 700 $^{0}$C film is its two orders of magnitude larger anisotropic magnetoresistance (AMR) as compared to the AMR of epitaxial films. We attribute it to unquenching of the orbital angular momentum of 3d electrons of Mn ions in the intergranular region where crystal field is poorly defined.

cond-mat.str-el↗

arXiv2009

Tailoring exchange bias in half-metallic La$_{2/3}$Sr$_{1/3}$MnO$_{3}$ thin films for spin-valve applications

We have utilized the antiferromagnetic nature and structural/chemical compatibility of La$_{0.45}$Sr$_{0.55}$MnO$_{3}$ with highly spin polarized La$_{0.67}$Sr$_{0.33}$MnO$_{3}$ to prepare epitaxial exchange bias couples. A robust exchange bias (EB) shift of magnetization hysteresis with associated interfacial exchange energy J $\approx$ 0.13 erg/cm$^2$ at 10 K along with enhanced coercivity are reported. The EB effect was engineered to bring coercivity contrast between La$_{0.67}$Sr$_{0.33}$MnO$_{3}$ and cobalt films in La$_{0.45}$Sr$_{0.55}$MnO$_{3}$/La$_{0.67}$Sr$_{0.33}$MnO$_{3}$/SrTiO$_{3}$/Co magnetic tunnel junctions.

cond-mat.str-el↗

arXiv2008

Polaronic Pseudogap in the Metallic Phase of La$_{0.625}$Ca$_{0.375}$MnO$_3$ Thin Films

The electronic density of states (DOS) of La$_{0.625}$Ca$_{0.375}$MnO$_3$(LCMO) strain free epitaxial thin films with an insulator-metal transition temperature (T$_{IM}$) of 250 K was probed using variable temperature scanning tunneling microscopy and spectroscopy. We find a depression in the DOS with a finite zero bias conductance (ZBC) signifying a pseudogap (PG) in 78-310 K temperature range. With cooling, the ZBC is found to increase indicating an increased DOS near E$_F$. We interpret PG as a signature of Jahn-Teller polarons while ZBC change, in agreement with the bulk insulator-metal transition, optical Drude peak, and photoemission experiments indicates the presence of free carriers at the Fermi energy in the metallic phase. The free carriers are discussed in terms of correlated polaronic states.

cond-mat.str-el↗

arXiv2008

Magnetization depinning transition, anisotropic magnetoresistance and inplane anisotropy in two polytypes of La$_{2 / 3}$Sr$_{1 / 3}$MnO$_{3}$ epitaxial films

The isothermal magnetoresistance [R($θ$)] of [001] and [110] epitaxial films of La$_{2 / 3}$Sr$_{1 / 3}$MnO$_{3}$ measured as a function of the angle $θ$ between current ($\vec{I}$) and magnetic field ($\vec{H}$), both in the plane of the film, is measured at several temperatures between 10 and 300K. The magnetic easy axis of these polytypes is intimately related to the orientation of Mn - O - Mn bonds with respect to the crystallographic axis on the plane of the substrate and energy equivalence of some of these axes. The magnetization vector ($\vec{M}$) of the [001] and [110] type films is pinned along the [110] and [001] directions respectively at low fields. A magnetization orientation phase transition (MRPT) which manifests itself as a discontinuity and hysteresis in $R(ψ)$ where $ψ$ is the angle between $\vec{H}$ and the easy axis for the $\vec{H}$ below a critical value $\vec{H}^*$ has been established. The boundary of the pinned and depinned phase on the H-T plane has been established. The highly robust pinning of magnetization seen in [110] films is related to their uniquely defined easy axis. The isothermal resistance R$_\bot$ and R$_\|$ for $\vec{I} \bot \vec{H}$ and $\vec{I} \| \vec{H}$, respectively for both polytypes follows the inequality R$_\bot >$ R$_\|$ for all ranges of fields ($0 \leq H \leq 3500Oe$) and temperatures (10K - 300K). A full fledged analysis of the rotational magnetoresistance is carried out in the framework of Döring theory for MR in single crystal samples. Strong deviations from the predicted angular dependence are seen in the irreversible regime of magnetization.

cond-mat.mtrl-sci↗

arXiv2008

Diverging Giant Magnetoresistance in the Limit of Infinitely Conducting Spacer

The relevance of pair-breaking by exchange and dipolar fields, and by injected spins in a low carrier density cuprate Y$_{1-x}$Pr$_x$Ba$_2$Cu$_3$O$_7$ sandwiched between two ferromagnetic La$_{2 / 3}$Sr$_{1 / 3}$MnO$_{3}$ layers is examined. At low external field ($H_{ext}$), the system shows a giant magnetoresistance(MR), which diverges deep in the superconducting state. We establish a distinct dipolar contribution to MR near the switching field(H$_c$) of the magnetic layers. At H$_{ext} \gg$ H$_c$, a large positive MR, resulting primarily from the motion of Josephson vortices and pair breaking by the in-plane field, is seen.

cond-mat.supr-con↗

arXiv2008

Lattice-mismatch-induced granularity in CoPt-NbN and NbN-CoPt superconductor-ferromagnet heterostructures: Effect of strain

The effect of strain due to lattice mismatch and of ferromagnetic (FM) exchange field on superconductivity (SC) in NbN-CoPt bilayers is investigated. Two different bilayer systems with reversed deposition sequence are grown on MgO (001) single crystals. While robust superconductivity with high critical temperature (T_c ~ 15.3 K) and narrow transition width DelT_c ~ 0.4 K) is seen in two types of CoPt-NbN/MgO heterostructures where the magnetic anisotropy of CoPt is in-plane in one case and out-of-plane in the other, the NbN-CoPt/MgO system shows markedly suppressed SC response. The reduced SC order parameter of this system, which manifests itself in Tc, temperature dependence of critical current density J_c (T), and angular (Phi) variation of flux-flow resistivity Rho_f is shown to be a signature of the structure of NbN film and not a result of the exchange field of CoPt. The Rho_f (H,T,Phi) data further suggest that the domain walls in the CoPt film are of the Neel type and hence do not cause any flux in the superconducting layer. A small, but distinct increase in the low-field critical current of the CoPt-NbN couple is seen when the magnetic layer has perpendicular anisotropy.

cond-mat.supr-con↗

arXiv2008

Correlations between morphology, crystal structure and magnetization of epitaxial cobalt-platinum films grown with pulsed laser ablation

The effects of growth rate (G_r), deposition temperature (T_d), film thickness (t_F), and substrate induced strain (epsilon) on morphological, crystallographic and magnetic characteristics of equiatomic CoPt epitaxial films synthesized with PLD are investigated. The (001) substrates of MgO, STO and LAO provide different degree of epitaxial strain for growth of the disordered face centered cubic (fcc) and ordered face centered tetragonal (L1_0) phases of CoPt. The films deposited at T_d~600 ^0C on all three substrates are fcc with in-plane magnetization and a narrow hysteresis loop of width~200 Oe. The L1_0 phase, stabilized only at T_d~700 ^0C becomes predominantly c-axis oriented as T_d is increased to 800 ^0C. While the crystallographic structure of the films depends solely on the T_d, their microstructure and magnetization characteristics are decided by the growth rate. At the higher G_r (~1A/sec) the L1_0 films have a maze-like structure which converts to a continuous film as the t_F is increased from 20 to 50 nm. The H_c of these films increases as the L1_0 phase fraction grows with T_d and its orientation becomes out of the film plane. The evolution of microstructure with T_d is remarkably different at lower growth rate (~0.4A /sec). Here the structure changes from a self-similar fractal pattern to an assembly of nano-dots as the T_d is raised from 700 to 800 ^0C, and is understood in terms of the imbalance between strain and interfacial energies. MFM of such films reveals no distinct domain walls within the nano-islands while a clear contrast is seen between the islands of reversed magnetization. The simple picture of coherent rotation of moment appears incompatible with the time dependence of the remanent magnetization in these films.

cond-mat.mtrl-sci↗

arXiv2008

Inhomogeneous vortex-state-driven enhancement of superconductivity in nanoengineered ferromagnet-superconductor heterostructures

Thin film heterostructures provide a powerful means to study the antagonism between superconductivity (SC) and ferromagnetism (FM). One interesting issue in FM-SC hybrids which defies the notion of antagonistic orders is the observation of magnetic field induced superconductivity (FIS). Here we show that in systems where the FM domains/islands produce spatial inhomogeneities of the SC order parameter, the FIS can derive significant contribution from different mobilities of the magnetic flux identified by two distinct critical states in the inhomogeneous superconductor. Our experiments on nanoengineered bilayers of ferromagnetic CoPt and superconducting NbN where CoPt/NbN islands are separated by a granular NbN, lend support to this alternative explanation of FIS in certain class of FM-SC hybrids.

cond-mat.supr-con↗

arXiv2007

Tunneling Study of the Charge-Ordering Gap on the Surface of La$_{0.350}$Pr$_{0.275}$Ca$_{0.375}$MnO$_3$ Thin Films

Variable temperature scanning tunneling microscopy/spectroscopy studies on (110) oriented epitaxial thin films of La$_{0.350}$Pr$_{0.275}$Ca$_{0.375}$MnO$_3$ are reported in the temperature range of 77 to 340 K. The films, grown on lattice matched NdGaO$_3$ substrates, show a hysteretic metal-insulator transition in resistivity at 170 K. The topographic STM images show step-terrace morphology while the conductance images display a nearly homogeneous surface. The normalized conductance spectra at low temperatures (T$<$150 K) show an energy gap of 0.5 eV while for T$\geq$180 K a gap of 0.16 eV is found from the activated behavior of the zero bias conductance. The presence of energy gap and the absence of phase separation on the surface over more than 2 $μ$m$\times$2 $μ$m area contradicts the metallic behavior seen in resistivity measurements at low temperatures. We discuss the measured energy gap in terms of the stabilization of the insulating CO phase at the film surface.

cond-mat.str-el↗

arXiv2007

Complementarity of perturbations driving insulator-to-metal transition in a charge ordered manganite

Modulation of charge carrier dynamics and hence electrical conductivity of solids by photoexcitation has been a rich field of research with numerous applications. Similarly, electric and magnetic field assisted enhancement of conductivity are of fundamental importance and technological use. Hole doped manganites of the type (A$_{1-x}$B$_{x})$MnO$_{3}$, where A and B are rare and alkaline earth metals respectively have the distinction of showing all three effects. Here we establish the complementarity of the electric, magnetic and photon fields in driving an insulator-metal transition in epitaxial thin films of La$_{0.175}$Pr$_{0.45}$Ca$_{0.375}$MnO$_{3}$ whose electrical ground state is insulating. Both pulsed and CW lasers cause a giant photon flux dependent enhancement of conductivity. It is further observed that electric and magnetic fields trigger the persistent enhancement of conductivity whose magnitude can be accentuated by application of these fields in parallel.

cond-mat.str-el↗

arXiv2007

Spin wave resonances in La_{0.7}Sr_{0.3}MnO_{3} films: measurement of spin wave stiffness and anisotropy field

We studied magnetic field dependent microwave absorption in epitaxial La$_{0.7}$Sr$_{0.3}$MnO$_{3}$ films using an X-band Bruker ESR spectrometer. By analyzing angular and temperature dependence of the ferromagnetic and spin-wave resonances we determine spin-wave stiffness and anisotropy field. The spin-wave stiffness as found from the spectrum of the standing spin-wave resonances in thin films is in fair agreement with the results of inelastic neutron scattering studies on a single crystal of the same composition [Vasiliu-Doloc et al., J. Appl. Phys. \textbf{83}, 7343 (1998)].

cond-mat.str-el↗

arXiv2007

Scaled frequency-dependent transport in the mesoscopically phase-separated colossal magnetoresistive manganite La_{0.625-y}Pr_yCa_{0.375}MnO_3

We address the issue of massive phase separation (PS) in manganite family of doped Mott insulators through ac conductivity measurements on La$_{0.625-y}$Pr$_{y}$Ca$_{0.375}$MnO$_{3}$ (0.375 $\leq$ y $\leq$ 0.275), and establish applicability of the scaling theory of percolation in the critical regime of the PS. Measurements of dc resistivity, magnetization (M(T)) and electron diffraction show incomplete growth of a ferromagnetic (FM) metallic component on cooling the high temperature charge ordered (CO) phase well below Curie temperature. The impedance $\mid$Z(T,f)$\mid$ measured over a frequency (f) range of 10 Hz to 10 MHz in the critical regime follows a universal scaling of the form $\approx$ R(T,0)g(f$ξ^{2+θ}$) with $θ$ $\approx$ 0.86 and the normalized correlation length varying from 1 to 4, suggesting anomalous diffusion of holes in percolating FM clusters.

cond-mat.str-el↗

arXiv2007

Nonresonant microwave absorption in epitaxial La-Sr-Mn-O films and its relation to colossal magnetoresistance

We study magnetic-field-dependent nonresonant microwave absorption and dispersion in thin La$_{0.7}$Sr$_{0.3}$MnO$_{3}$ films and show that it originates from the colossal magnetoresistance. We develop the model for magnetoresistance of a thin ferromagnetic film in oblique magnetic field. The model accounts fairly well for our experimental findings, as well as for results of other researchers. We demonstrate that nonresonant microwave absorption is a powerful technique that allows contactless measurement of magnetic properties of thin films, including magnetoresistance, anisotropy field and coercive field.

cond-mat.str-el↗

arXiv2007

Anomalous exchange coupling in transition-metal-oxide based superlattices with antiferromagnetic spacer layers

A direct correlation is seen between the coercive field (HC) and the magnetic-field-dependent resistivity (MR) in SrMnO3/SrRuO3 superlattices of perpendicular magnetic anisotropy. The magnetoresistance shows a sharp jump at Hc for in-plane current and the out-of-plane magnetic field. Both HC and high-field MR also oscillate with the thickness of the SrMnO3 spacer layers separating the metallic ruthenate. Since the spacer in these superlattices has no mobile carriers to facilitate an oscillatory coupling, we attribute the observed behavior to the spin-polarized quantum tunneling of electrons between the ferromagnetic layers and antiferromagnetically ordered t2g spins of SrMnO3.

cond-mat.str-el↗

arXiv2007

Correlation between incoherent phase fluctuations and disorder in Y$_{1-x}$Pr$_x$Ba$_2$Cu$_3$O$_{7-δ}$ epitaxial films from Nernst effect measurements

Measurements of Nernst effect, resistivity and Hall angle on epitaxial films of Y$_{1-x}$Pr$_x$Ba$_2$Cu$_3$O$_{7-δ}$(Pr-YBCO, 0$\leq x\leq$0.4) are reported over a broad range of temperature and magnetic field. While the Hall and resistivity data suggest a broad pseudogap regime in accordance with earlier results, these first measurements of the Nernst effect on Pr-YBCO show a large signal above the superconducting transition temperature(T$_c$). This effect is attributed to vortex-like excitations in the phase incoherent condensate existing above T$_c$. A correlation between disorder and the width of the phase fluctuation regime has been established for the YBCO family of cuprates, which suggests a T$_c\approx$110K for disorder-free YBa$_2$Cu$_3$O$_{7-δ}$.

cond-mat.supr-con↗

arXiv2007

Reentrant stability of superconducting films

We propose a mechanism responsible for the abrupt vanishing of the dendritic flux instability found in many superconducting films when an increasing magnetic field is applied. The onset of flux avalanches and the subsequent reentrance of stability in NbN films was investigated using magneto-optical imaging, and the threshold fields were measured as functions of critical current density, $j_c$. The results are explained with excellent quantitative agreement by a thermomagnetic model published recently, Phys. Rev. B73, 014512 (2006), showing that the reentrant stability is a direct consequence of a monotonously decreasing $j_c$ versus field.

cond-mat.supr-con↗

arXiv2006

Studies of structural, magnetic, electrical and photoconducting properties of Bi$_{1-x}$Ca$_{x}$MnO$_{3}$ epitaxial thin films

The dynamics of the charge ordered (CO) state under non-equilibrium conditions created by strong dc-electric field (~106 V/cm) and photo-illumination with short (~ 6 ns) laser pulses is investigated in Bi1-xCaxMnO3 (x > 0.5) epitaxial films. A pulsed laser deposition method was used to synthesize films on (100) LaAlO3 (LAO) and (100) SrTiO3 (STO) substrates. The crystallographic structure, temperature dependence of electrical resistivity and magnetization of the samples of different composition prepared under different oxygen partial pressure (pO2) and deposition temperature (TD) are studied. For the x = 0.6 sample grown on LAO, a clear signature of charge ordering at ~275 K is seen in the magnetization and at ~ 260 K in the resistivity data. The same sample grown on STO revealed a complex behavior, which entails charge ordering at ~300 K, a Neel order at ~150 K and finally a weak ferromagnetic phase below 50 K. A strong correlation between charge ordering temperature (TCO) and the c-axis lattice parameter (c) of the type (dTCO/dc ~-350 K/A) imerges from measurements on films deposited under different growth conditions. Since the out of plane lattice parameter (c) increases with in plane compressive strain, this effect directly show a compressive strain induced suppression of the TCO. The current (I)- voltage (V) characteristics of the samples at T < TCO show hysteresis due to a compound effect of Joule heating and collapse of the CO state. Transient changes in conductivity of lifetime ranging from nano to microseconds are seen at T < TCO on illumination with pulsed UV (355 nm) radiation. These observations are explained on the basis of the topological and electronic changes in the charge ordered phase.

cond-mat.str-el↗

arXiv2006

Antiferromagnetic coupling and enhanced magnetization in all-ferromagnetic superlattices

The structural and magnetic properties of a series of superlattices consisting of two ferromagnetic metals La$_{0.7}$Sr$_{0.3}$MnO$_3$ (LSMO) and SrRuO$_3$ (SRO) grown on (001) oriented SrTiO$_3$ are studied. Superlattices with a fixed LSMO layer thickness of 20 unit cells (u.c.) and varying SRO layer thickness show a sudden drop in magnetization on cooling through temperature where both LSMO and SRO layers are ferromagnetic. This behavior suggests an antiferromagnetic coupling between the layers. In addition, the samples having thinner SRO layers (n \TEXTsymbol{<} 6) exhibit enhanced saturation magnetization at 10 K. These observations are attributed to the possible modification in the stereochemistry of the Ru and Mn ions in the interfacial region.

cond-mat.mtrl-sci↗