arXiv subjects

R. Caballero-Folch

Publications and source records attributed to R. Caballero-Folch.

At least 19 recordsLinked to original sources

arXiv2026

First observation of the fine structure of the Pygmy Dipole Resonance in a nucleus away from stability via the $β^-$ decay of $^{92}$Rb to $^{92}$Sr

A comprehensive $γ$-ray spectroscopy study of excited states in $^{92}$Sr populated via $β^-$ decay of $^{92}$Rb ($J^π=0^-$, $Q_β=8095(6)$~keV) was performed with the GRIFFIN spectrometer at the Isotope Separator and Accelerator (ISAC) radioactive ion beam facility at TRIUMF. The high $γ$-ray efficiency of the GRIFFIN spectrometer combined with the intense rubidium beams produced allowed for 864 $γ$-ray transitions to be placed in the level scheme with 190 excited levels populated, most of them identified for the first time. The excitation energies of low-spin states in $^{92}$Sr are well reproduced by large-scale Shell Model calculations up to 5~MeV. The $β$-feeding intensities are in very good agreement with results from a recent study employing Modular Total Absorption Spectroscopy, indicating a significant suppression of the Pandemonium effect. The experimental picture reveals the energy level dependence of log~$ft$ values in unprecedented detail. These log~$ft$ values are well reproduced by Multiple-Commutator Model calculations that identify the features in the excited levels' wavefunctions that enable the population of high-lying levels with a low effective Q-value that belong to the Pygmy Dipole Resonance.

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arXiv2025

Investigation of the Excited States of $^{114}\mathrm{Sn}$ Using the GRIFFIN Spectrometer at TRIUMF

The semi-magic $^{110-122}\mathrm{Sn}$ isotopes display signs of shape coexistence in their excited $0^+$ states, which, in contrast to the spherical $0^+$ ground states, are deformed. This paper investigates the nuclear structure of $^{114}\mathrm{Sn}$ using the competing $β^+$ decay and electron capture of a radioactive beam of $^{114}\mathrm{Sb}$ produced at the TRIUMF-ISAC facility using the GRIFFIN spectrometer. This study will allow for an in-depth understanding of the excited $0^+$ states in $^{114}\mathrm{Sn}$, by focusing on their decay patterns. In the present experiment, transitions at 856.2-keV and 1405.0-keV, which were observed in an earlier $β^+$ decay study but not placed in the $^{114}\mathrm{Sn}$ level scheme, have been assigned to the level scheme in connection to the $0^+_3$ level at 2156.0-keV. Properly assigning these transitions refines the level scheme and enhances our understanding of the nuclear structure in $^{114}\mathrm{Sn}$.

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arXiv2024

First Exploration of Monopole-Driven Shell Evolution above the N = 126 shell closure: new Millisecond Isomers in 213Tl and 215Tl

Isomer spectroscopy of heavy neutron-rich nuclei beyond the N=126 closed shell has been performed for the first time at the Radioactive Isotope Beam Factory of the RIKEN Nishina Center. New millisecond isomers have been identified at low excitation energies, 985.3(19) keV in 213Tl and 874(5) keV in 215Tl. The measured half-lives of 1.34(5) ms in 213Tl and 3.0(3) ms in 215Tl suggest spins and parities 11/2- with the single proton-hole configuration h11/2 as leading component. They are populated via E1 transitions by the decay of higher-lying isomeric states with proposed spin and parity 17/2+, interpreted as arising from a single s1/2 proton hole coupled to the 8+ seniority isomer in the (A+1)Pb cores. The lowering of the 11/2- states is ascribed to an increase of the h11/2 proton effective single-particle energy as the second g9/2 orbital is filled by neutrons, owing to a significant reduction of the proton-neutron monopole interaction between the h11/2 and g9/2 orbitals. The new ms-isomers provide the first experimental observation of shell evolution in the almost unexplored N>126 nuclear region below doubly-magic 208Pb.

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arXiv2023

Decay Spectroscopy of $^{160}$Eu: Quasiparticle Configurations of Excited States and Structure of $K^π$=$4^+$ Band-heads in $^{160}$Gd

\noindent \textbf{Background:} Detailed spectroscopy of neutron-rich, heavy, deformed nuclei is of broad interest for nuclear astrophysics and nuclear structure. Nuclei in the r-process path and following freeze-out region impact the resulting r-process abundance distribution, and the structure of nuclei midshell in both proton and neutron number helps to understand the evolution of subshell gaps and large deformation in these nuclei. \noindent \textbf{Purpose:} To improve the understanding of the nuclear structure of $^{160}$Gd, specifically the $K^π$=$4^+$ bands, as well as study the $β$-decay of $^{160}$Eu into $^{160}$Gd. \noindent \textbf{Methods:} High-statistics decay spectroscopy of $^{160}$Gd resulting from the $β$-decay of $^{160}$Eu was collected using the GRIFFIN spectrometer at the TRIUMF-ISAC facility. \noindent \textbf{Results:} Two new excited states and ten new transitions were observed in $^{160}$Gd. The $β$-decaying half-lives of the low- and high-spin isomer in $^{160}$Eu were determined, and the low-spin state's half-life was measured to be $t_{1/2}=26.0(8)$~s, $\sim$16\% shorter than previous measurements. Lifetimes of the two $K^π$=$4^+$ band-heads in $^{160}$Gd were measured for the first time, as well as $γ$-$γ$ angular correlations and mixing ratios of intense transitions out of those band-heads. \noindent \textbf{Conclusions:} Lifetimes and mixing ratios suggest that the hexadecapole phonon model of the $K^π$=$4^+$ band-heads in $^{160}$Gd is preferred over a simple two-state strong mixing scenario, although further theoretical calculations are needed to fully understand these states. Additionally, the 1999.0 keV state in $^{160}$Gd heavily populated in $β$-decay is shown to have positive parity, which raises questions regarding the structure of the high-spin $β$-decaying state in $^{160}$Eu.

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arXiv2022

First application of Markov Chain Monte Carlo-based Bayesian data analysis to the Doppler-Shift Attenuation Method

Motivated primarily by the large uncertainties in the thermonuclear rate of the $^{30}$P$(p,γ)^{31}$S reaction that limit our understanding of classical novae, we carried out lifetime measurements of $^{31}$S excited states using the Doppler Shift Lifetimes (DSL) facility at the TRIUMF Isotope Separator and Accelerator (ISAC-II) facility. The $^{31}$S excited states were populated by the $^{3}$He$(^{32}$S$,α)^{31}$S reaction. The deexcitation $γ$ rays were detected by a clover-type high-purity germanium detector in coincidence with the $α$ particles detected by a silicon detector telescope. We have applied modern Markov chain Monte Carlo-based Bayesian methods to perform lineshape analyses of Doppler-shift attenuation method $γ$-ray data for the first time. We have determined the lifetimes of the two lowest-lying $^{31}$S excited states. First experimental upper limits on the lifetimes of four higher-lying states have been obtained. The experimental results were compared to shell-model calculations using five universal $sd$-shell Hamiltonians. Evidence for $γ$ rays originating from the astrophysically important $J^π=3/2^+$, 260-keV $^{30}$P$(p,γ)^{31}$S resonance has also been observed, although strong constraints on the lifetime will require better statistics.

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arXiv2022

Single neutron transfer on 23Ne and its relevance forthepathway ofnucleosynthesis in astrophysical X-ray bursts

We present new experimental measurements of resonance strengths in the astrophysical 23Al(p, γ)24Si reaction, constraining the pathway of nucleosynthesis beyond 22Mg in X-ray burster scenarios. Specifically, we have performed the first measurement of the (d, p) reaction using a radioactive beam of 23Ne to explore levels in 24Ne, the mirror analog of 24Si. Four strong single-particle states were observed and corresponding neutron spectroscopic factors were extracted with a precision of {\sim}20{\%}. Using these spectroscopic factors, together with mirror state identifications, we have reduced uncertainties in the strength of the key {\ell} = 0 resonance at Er= 157 keV, in the astrophysical 23Al(p, γ) reaction, by a factor of 4. Our results show that the 22Mg(p, γ)23Al(p, γ) pathway dominates over the competing 22Mg(α, p) reaction in all but the most energetic X-ray burster events (T>0.85GK), significantly affecting energy production and the preservation of hydrogen fuel.

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arXiv2022

Improved measurement of the $0_2^+\rightarrow0_1^+$ E0 transition strength for $^{72}$Se using the SPICE spectrometer

The selenium isotopes lie at the heart of a tumultuous region of the nuclear chart where shape coexistence effects grapple with neutron-proton pairing correlations, triaxiality, and the impending proton dripline. In this work a study of $^{72}$Se by internal conversion electron and $γ$-ray spectroscopy was undertaken with the SPICE and TIGRESS arrays. New measurements of the branching ratio and lifetime of the $0_2^+$ state were performed yielding a determination of $ρ^2(E0;0_2^+{\rightarrow}0_1^+)=29(3)$ milliunits. two state mixing calculations were performed that highlighted the importance of interpretation of such $E0$ strength values in the context of shape-coexistence.

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arXiv2022

High-precision half-life determination of $^{14}$O via direct $β$ counting

The half-life of the superallowed Fermi $β^+$ emitter $^{14}$O was determined to high precision via a direct $β$ counting experiment performed at the Isotope Separator and Accelerator (ISAC) facility at TRIUMF. The result, $T_{1/2}$($^{14}$O) = 70619.2(76) ms, is consistent with, but is more precise than, the world average obtained from 11 previous measurements. Combining the $^{14}$O half-life deduced in the present work with the previous most precise measurements of this quantity leads to a reduction in the overall uncertainty, by nearly a factor of 2. The new world average is $T_{1/2}$($^{14}$O) = 70619.6(63) ms with a reduced $χ^2$ value of 0.87 obtained from 8 degrees of freedom.

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arXiv2022

Coulomb excitation of the $\left|T_z\right|=\frac{1}{2}$, $A=23$ mirror pair

Background: Electric-quadrupole ($E2$) strengths relate to the underlying quadrupole deformation of a nucleus and present a challenge for many nuclear theories. Mirror nuclei in the vicinity of the line of $N=Z$ represent a convenient laboratory for testing deficiencies in such models, making use of the isospin-symmetry of the systems. Purpose: Uncertainties associated with literature $E2$ strengths in \textsuperscript{23}Mg are some of the largest in $T_z=\left|\frac{1}{2}\right|$ nuclei in the $sd$-shell. The purpose of the present work is to improve the precision with which these values are known, to enable better comparison with theoretical models. Methods: Coulomb-excitation measurements of $^{23}$Mg and $^{23}$Na were performed at the TRIUMF-ISAC facility using the TIGRESS spectrometer. They were used to determine the $E2$ matrix elements of mixed $E2$/$M1$ transitions. Results: Reduced $E2$ transition strengths, $B(E2)$, were extracted for \textsuperscript{23}Mg and \textsuperscript{23}Na. Their precision was improved by factors of approximately six for both isotopes, while agreeing within uncertainties with previous measurements. Conclusions: A comparison was made with both shell-model and {\it ab initio} valence-space in-medium similarity renormalization group calculations. Valence-space in-medium similarity-renormalization-group calculations were found to underpredict the absolute $E2$ strength - in agreement with previous studies.

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arXiv2020

Decay Spectroscopy of $^{129}$Cd

Excited states of $^{129}$In populated following the $β$-decay of $^{129}$Cd were experimentally studied with the GRIFFIN spectrometer at the ISAC facility of TRIUMF, Canada. A 480-MeV proton beam was impinged on a uranium carbide target and $^{129}$Cd was extracted using the Ion Guide Laser Ion Source (IG-LIS). $β$- and $γ$-rays following the decay of $^{129}$Cd were detected with the GRIFFIN spectrometer comprising the plastic scintillator SCEPTAR and 16 high-purity germanium (HPGe) clover-type detectors. %, along with the $β$-particles were detected with SCEPTAR. From the $β$-$γ$-$γ$ coincidence analysis, 32 new transitions and 7 new excited states were established, expanding the previously known level scheme of $^{129}$In. The $\log ft$ values deduced from the $β$-feeding intensities suggest that some of the high-lying states were populated by the $ν0 g_{7/2} \rightarrow π0 g_{9/2}$ allowed Gamow-Teller (GT) transition, which indicates that the allowed GT transition is more dominant in the $^{129}$Cd decay than previously reported. Observation of fragmented Gamow-Teller strengths is consistent with theoretical calculations.

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arXiv2019

Direct observation of proton emission in 11Be

The elusive $β^-\text{p}^+$ decay was observed in $^{11}$Be by directly measuring the emitted protons and their energy distribution for the first time with the prototype Active Target Time Projection Chamber (pAT-TPC) in an experiment performed at ISAC-TRIUMF. The measured $β^-\text{p}^+$ branching ratio is orders of magnitude larger than any previous theoretical model predicted. This can be explained by the presence of a narrow resonance in $^{11}$B above the proton separation energy.

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arXiv2019

Shape coexistence in the neutron-deficient lead region: A systematic study of lifetimes in the even-even $^{188-200}$Hg with GRIFFIN

Lifetimes of $2^+_1$ and $4^+_1$ states, as well as some negative-parity and non-yrast states, in $^{188-200}$Hg were measured using $γ-γ$ electronic fast timing techniques with the LaBr$_3$(Ce) detector array of the GRIFFIN spectrometer. The excited states were populated in the $ε/β^+$-decay of $J^π=7^+/2^-$ $^{188-200}$Tl produced at the TRIUMF-ISAC facility. The deduced B(E2) values are compared to different interacting boson model predictions. The precision achieved in this work over previous ones allows for a meaningful comparison with the different theoretical models of these transitional Hg isotopes, which confirms the onset of state mixing in $^{190}$Hg.

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arXiv2019

Isospin symmetry in $B(E2)$ values: Coulomb excitation study of ${}^{21}$Mg

The $T_z$~=~$-\frac{3}{2}$ nucleus ${}^{21}$Mg has been studied by Coulomb excitation on ${}^{196}$Pt and ${}^{110}$Pd targets. A 205.6(1)-keV $γ$-ray transition resulting from the Coulomb excitation of the $\frac{5}{2}^+$ ground state to the first excited $\frac{1}{2}^+$ state in ${}^{21}$Mg was observed for the first time. Coulomb excitation cross-section measurements with both targets and a measurement of the half-life of the $\frac{1}{2}^+$ state yield an adopted value of $B(E2;\frac{5}{2}^+\rightarrow\frac{1}{2}^+)$~=~13.3(4)~W.u. A new excited state at 1672(1)~keV with tentative $\frac{9}{2}^+$ assignment was also identified in ${}^{21}$Mg. This work demonstrates large difference of the $B(E2;\frac{5}{2}^+\rightarrow\frac{1}{2}^+)$ values between $T$~=~$\frac{3}{2}$, $A$~=~21 mirror nuclei. The difference is investigated in the shell-model framework employing both isospin conserving and breaking USD interactions and using modern \textsl{ab initio} nuclear structure calculations, which have recently become applicable in the $sd$ shell.

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arXiv2018

The GRIFFIN Facility for Decay-Spectroscopy Studies at TRIUMF-ISAC

Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei, GRIFFIN, is a new high-efficiency $γ$-ray spectrometer designed for use in decay spectroscopy experiments with low-energy radioactive ion beams provided by TRIUMF's Isotope Separator and Accelerator (ISAC-I) facility. GRIFFIN is composed of sixteen Compton-suppressed large-volume clover-type high-purity germanium (HPGe) $γ$-ray detectors combined with a suite of ancillary detection systems and coupled to a custom digital data acquisition system. The infrastructure and detectors of the spectrometer as well as the performance characteristics and the analysis techniques applied to the experimental data are described.

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arXiv2018

Half-Lives of Neutron Rich $^{130}$Cd and $^{131}$In

The half-lives of isotopes around the $N=82$ shell closure are an important ingredient in astrophysical simulations and strongly influence the magnitude of the second $r$-process abundance peak in the $A\sim130$ region. The most neutron-rich $N=82$ nuclei are not accessible to the current generation of radioactive beam facilities and $r$-process simulations must therefore rely on calculations of the half-lives of the isotopes involved. Half-life measurements of the experimentally accessible nuclei in this region are important in order to benchmark these calculations. The half-life of $^{130}$Cd is particularly important as it is used to tune the Gamow-Teller quenching in shell-model calculations for the $β$ decay of other nuclei in this region. In this work, the GRIFFIN $γ$-ray spectrometer at the TRIUMF-ISAC facility was used to measure the half-life of $^{130}_{~48}$Cd$_{82}$ to be $T_{1/2}= 126(4)$ ms. In addition, the half-lives of the three $β$ decaying states of $^{131}_{~49}$In$_{82}$ were measured to be $T_{1/2}(1/2^-)=328(15)$ ms, $T_{1/2}(9/2^+)=265(8)$ ms, and $T_{1/2}(21/2^+)=323(50)$ ms, respectively, providing an important benchmark for half-life calculations in this region.

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arXiv2018

First determination of $β$-delayed multiple neutron emission beyond A = 100 through direct neutron measurement: The P$_{2n}$ value of $^{136}$Sb

Background: $β$-delayed multiple neutron emission has been observed for some nuclei with A$\leq$100, with $^{100}$Rb being the heaviest $β$2n emitter measured to date. So far, only 25 P$_{2n}$ values have been determined for the $\sim$300 nuclei that may decay in this way. Accordingly, it is of interest to measure P$_{2n}$ values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such measurement for nuclei with A$>$100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition, the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the $r$-process, and safety inputs for nuclear reactors. Purpose: To determine for the first time the two neutron branching ratio, P$_{2n}$ value, for $^{136}$Sb through a direct neutron measurement, and to provide precise P$_{1n}$ values for $^{136}$Sb and $^{136}$Te. Method: Pure beams were provided by the JYFLTRAP at the IGISOL facility of the University of Jyväskylä, Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point, and the BELEN detector, based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the $β$- and neutron- growth-and-decay curves and the $β$-one-neutron and $β$-two-neutron time correlations. Results: The P$_{2n}$ value of $^{136}$Sb was found to be 0.14(3)\% and the measured P$_{1n}$ values for $^{136}$Sb and $^{136}$Te were found to be 32.2(15)\% and 1.47(6)\%, respectively. The measured P$_{2n}$ value is a factor 44 smaller than predicted by the FRDM+QRPA model used for $r$-process calculations.

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arXiv2018

In-beam internal conversion electron spectroscopy with the SPICE detector

The SPectrometer for Internal Conversion Electrons (SPICE) has been commissioned for use in conjunction with the TIGRESS $γ$-ray spectrometer at TRIUMF's ISAC-II facility. SPICE features a permanent rare-earth magnetic lens to collect and direct internal conversion electrons emitted from nuclear reactions to a thick, highly segmented, lithium-drifted silicon detector. This arrangement, combined with TIGRESS, enables in-beam $γ$-ray and internal conversion electron spectroscopy to be performed with stable and radioactive ion beams. Technical aspects of the device, capabilities, and initial performance are presented.

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arXiv2018

Commissioning of the BRIKEN detector for the measurement of very exotic beta-delayed neutron emitters

A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter, a detection system sensitive to the implantation and decay of radioactive ions, and gamma-ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and beta-delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background.

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