arXiv subjects

R. Cote

Publications and source records attributed to R. Cote.

At least 19 recordsLinked to original sources

arXiv2021

Kinetics and Nucleation Dynamics in Ion-Seeded Atomic Clusters

The time-dependent kinetics of formation and evolution of nano-size atomic clusters is investigated and illustrated with the nucleation dynamics of ion-seed Ar$_n$H$^+$ particles. The rates of growth and degradation of Ar-atomic shells around the seed ion are inferred from Molecular Dynamics (MD) simulations. Simulations of cluster formation have been performed with accurate quantum-mechanical binary interaction potentials. Both the nonequilibrium and equilibrium growth of Ar$_n$H$^+$ are investigated at different temperature and densities of the atomic gas and seed ions. Formation of Ar$_{n\leq 40}$ shells is the main mechanism which regulates the kinetics of nano-cluster growth and the diffusive fluctuations of the cluster size distribution. The time-evolution of the cluster intrinsic energy and cluster size distributions are analyzed at the non-thermal, quasi-equilibrium, and thermal equilibrium stages of Ar$_n$H$^+$ formation. We've determined the self-consistent model parameters for the temporal fluctuations of the cluster size and found coefficients of the diffusive growth mechanism describing the equilibrium distribution of nano-clusters. Nucleation of haze and nano-dust particles in astrophysical and atmospheric ionized gases are discussed.

physics.atm-clus↗

arXiv2012

Quantum Hall to charge-density-wave phase transitions in ABC-trilayer graphene

ABC-stacked trilayer graphene's chiral band structure results in three ($n=0,1,2$) Landau level orbitals with zero kinetic energy. This unique feature has important consequences on the interaction driven states of the 12-fold degenerate (including spin and valley) N=0 Landau level. In particular, at many filling factors $ν_{T} =\pm5,\pm4,\pm2,\pm1$ a quantum phase transition from a quantum Hall liquid state to a triangular charge density wave occurs as a function of the single-particle induced LL orbital splitting $Δ_{LL}$. This phase transition should be characterized by a re-entrant integer quantum Hall effect with the Hall conductivity corresponding to the {\it adjacent} interaction driven integer quantum Hall plateau.

cond-mat.mes-hall↗

arXiv2011

Bilayer graphene as an helical quantum Hall ferromagnet

The two-dimensional electron gas in a bilayer graphene in the Bernal stacking supports a variety of uniform broken-symmetry ground states in Landau level N=0 at integer filling factors $ν\in [-3,4].$ When an electric potential difference (or bias) is applied between the layers at filling factors $ν=-1,3$, the ground state evolves from an interlayer coherent state at small bias to a state with orbital coherence at higher bias where \textit{electric} dipoles associated with the orbital pseudospins order spontaneously in the plane of the layers. In this paper, we show that by further increasing the bias at these two filling factors, the two-dimensional electron gas goes first through a Skyrmion crystal state and then into an helical state where the pseudospins rotate in space. The pseudospin textures in both the Skyrmion and helical states are due to the presence of a Dzyaloshinskii-Moriya interaction in the effective pseudospin Hamiltonian when orbital coherence is present in the ground state. We study in detail the electronic structure of the helical and Skyrmion crystal states as well as their collective excitations and then compute their electromagnetic absorption.

cond-mat.mes-hall↗

arXiv2010

Orbital and interlayer Skyrmions crystals in bilayer graphene

A graphene bilayer in a transverse magnetic field has a set of Landau levels with energies $E=\pm \sqrt{N(N+1)}\hslash ω_{c}^{\ast}$ where $ω_{c}^{\ast}$ is the effective cyclotron frequency and $% N=0,1,2,...$ All Landau levels but N=0 are four times degenerate counting spin and valley degrees of freedom. The Landau level N=0 has an extra degeneracy due to the fact that orbitals $n=0$ and $n=1$ both have zero kinetic energies. At integer filling factors, Coulomb interactions produce a set of broken-symmetry states with partial or full alignement in space of the valley and orbital pseudospins. These quantum Hall pseudo-ferromagnetic states support topological charged excitations in the form of orbital and valley Skyrmions. Away from integer fillings, these topological excitations can condense to form a rich variety of Skyrme crystals with interesting properties. We study in this paper different crystal phases that occur when an electric field is applied between the layers. We show that orbital Skyrmions, in analogy with spin Skyrmions, have a texture of electrical dipoles that can be controlled by an in-plane electric field. Moreover, the modulation of electronic density in the crystalline phases are experimentally accessible through a measurement of their local density of states

cond-mat.mes-hall↗

arXiv2010

CrRb: a molecule with large magnetic and electric dipole moments

We report calculations of Born-Oppenheimer potential energy curves of the chromium-rubidium heteronuclear molecule 52Cr-87Rb, and the long-range dispersion coefficient for the interaction between ground state Cr and Rb atoms. Our calculated van der Waals coefficient (C6=1770 a.u.) has an expected error of 3%. The ground state 6Sigma+ molecule at its equilibrium separation has a permanent electric dipole moment of de (Re=3.34 A) = 2.90 D. We investigate the hyperfine and dipolar collisions between trapped Cr and Rb atoms, finding elastic to inelastic cross section ratio of 100-1000.

physics.atom-ph↗

arXiv2008

Two-photon photoassociative spectroscopy of ultracold 88-Sr

We present results from two-photon photoassociative spectroscopy of the least-bound vibrational level of the X$^1Σ_g^+$ state of the $^{88}$Sr$_2$ dimer. Measurement of the binding energy allows us to determine the s-wave scattering length, $a_{88}=-1.4(6) a_0$. For the intermediate state, we use a bound level on the metastable $^1S_0$-$^3P_1$ potential, which provides large Franck-Condon transition factors and narrow one-photon photoassociative lines that are advantageous for observing quantum-optical effects such as Autler-Townes resonance splittings.

physics.atom-ph↗

arXiv2008

Intra-Landau level Cyclotron Resonance in Bilayer Graphene

Interaction driven integer quantum Hall effects are anticipated in graphene bilayers because of the near-degeneracy of the eight Landau levels which appear near the neutral system Fermi level. We predict that an intra-Landau-level cyclotron resonance signal will appear at some odd-integer filling factors, accompanied by collective modes which are nearly gapless and have approximate $k^{3/2}$ dispersion. We speculate on the possibility of unususal localization physics associated with these modes.

cond-mat.mes-hall↗

arXiv2008

Skyrme and Wigner crystals in graphene

At low-energy, the band structure of graphene can be approximated by two degenerate valleys $(K,K^{\prime})$ about which the electronic spectra of the valence and conduction bands have linear dispersion relations. An electronic state in this band spectrum is a linear superposition of states from the $A$ and $B$ sublattices of the honeycomb lattice of graphene. In a quantizing magnetic field, the band spectrum is split into Landau levels with level N=0 having zero weight on the $B(A)$ sublattice for the $% K(K^{\prime})$ valley. Treating the valley index as a pseudospin and assuming the real spins to be fully polarized, we compute the energy of Wigner and Skyrme crystals in the Hartree-Fock approximation. We show that Skyrme crystals have lower energy than Wigner crystals \textit{i.e.} crystals with no pseudospin texture in some range of filling factor $ν$ around integer fillings. The collective mode spectrum of the valley-skyrmion crystal has three linearly-dispersing Goldstone modes in addition to the usual phonon mode while a Wigner crystal has only one extra Goldstone mode with a quadratic dispersion. We comment on how these modes should be affected by disorder and how, in principle, a microwave absorption experiment could distinguish between Wigner and Skyrme crystals.

cond-mat.mes-hall↗

arXiv2008

Dynamical matrix of two-dimensional electron crystals

In a quantizing magnetic field, the two-dimensional electron (2DEG) gas has a rich phase diagram with broken translational symmetry phases such as Wigner, bubble, and stripe crystals. In this paper, we derive a method to get the dynamical matrix of these crystals from a calculation of the density response function performed in the Generalized Random Phase Approximation (GRPA). We discuss the validity of our method by comparing the dynamical matrix calculated from the GRPA with that obtained from standard elasticity theory with the elastic coefficients obtained from a calculation of the deformation energy of the crystal.

cond-mat.mes-hall↗

arXiv2007

Collective modes of CP(3) Skyrmion crystals in quantum Hall ferromagnets

The two-dimensional electron gas in a bilayer quantum Hall system can sustain an interlayer coherence at filling factor nu=1 even in the absence of tunneling between the layers. This system has low-energy charged excitations which may carry textures in real spin or pseudospin. Away from filling factor nu =1 a finite density of these is present in the ground state of the 2DEG and forms a crystal. Depending on the relative size of the various energy scales, such as tunneling (Delta_SAS), Zeeman coupling (Delta_Z) or electrical bias (Delta_b), these textured crystal states can involve spin, pseudospin, or both intertwined. In this article, we present a comprehensive numerical study of the collective excitations of these textured crystals using the GRPA. For the pure spin case, at finite Zeeman coupling the state is a Skyrmion crystal with a gapless phonon mode, and a separate Goldstone mode that arises from a broken U(1) symmetry. At zero Zeeman coupling, we demonstrate that the constituent Skyrmions break up, and the resulting state is a meron crystal with 4 gapless modes. In contrast, a pure pseudospin Skyrme crystal at finite tunneling has only the phonon mode. For Delta_SAS=0, the state evolves into a meron crystal and supports an extra gapless U(1) mode in addition to the phonon. For a CP(3) Skyrmion crystal, we find a U(1) gapless mode in the presence of the symmetry-breaking fields. In addition, a second mode with a very small gap is present in the spectrum.

cond-mat.mes-hall↗

arXiv2006

Superradiance in ultracold Rydberg gases

Experiments in dense, ultracold gases of rubidium Rydberg atoms show a considerable decrease of the radiative excited state lifetimes compared to dilute gases. This accelerated decay is explained by collective and cooperative effects, leading to superradiance. A novel formalism to calculate effective decay times in a dense Rydberg gas shows that for these atoms the decay into nearby levels increases by up to three orders of magnitude. Excellent agreement between theory and experiment follows from this treatment of Rydberg decay behavior.

quant-ph↗

arXiv2006

Pseudospin vortex-antivortex states with interwoven spin textures in double layer quantum Hall systems

Recent experiments on strongly correlated bilayer quantum Hall systems strongly suggest that, contrary to the usual assumption, the electron spin degree of freedom is not completely frozen either in the quantum Hall or in the compressibles states that occur at filling factor $ν=1.$ These experiments imply that the quasiparticles at $ν=1$ could have both spin and pseudospin textures i.e. they could be CP$^{3}$ skyrmions. Using a microscopic unrestricted Hartree-Fock approximation, we compute the energy of several crystal states with spin, pseudospin and mixed spin-pseudospin textures around $ν=1$ as a function of interlayer separation $d$ for different values of tunneling ($Δ_{SAS}$), Zeeman ($Δ_{Z}$), and bias ($Δ_{b}$) energies. We show that in some range of these parameters, crystal states involving a certain amount of spin depolarization have lower energy than the fully spin polarized crystals. We study this depolarization dependence on $d,Δ_{SAS},Δ_{Z}$ and $Δ_{b}$ and discuss how it can lead to the fast NMR relaxation rate observed experimentally.

cond-mat.mes-hall↗

arXiv2006

Schemes for robust quantum computation with polar molecules

We propose to use a new platform - ultracold polar molecules - for quantum computing with switchable interactions. The on/off switch is accomplished by selective excitation of one of the "0" or "1" qubits - long-lived molecular states - to an "excited" molecular state with a considerably different dipole moment. We describe various schemes based on this switching of dipolar interactions where the selective excitation between ground and excited states is accomplished via optical, micro-wave, or electric fields. We also generalize the schemes to take advantage of the dipole blockade mechanism when dipolar interactions are very strong. These schemes can be realized in several recently proposed architectures.

quant-ph↗

arXiv2005

Spectroscopic determination of the s-wave scattering lengths of 86Sr and 88Sr

We report the use of photoassociative spectroscopy to determine the ground state s-wave scattering lengths for the main bosonic isotopes of strontium, 86Sr and 88Sr. Photoassociative transitions are driven with a laser red-detuned by up to 1400 GHz from the 1S0-1P1 atomic resonance at 461 nm. A minimum in the transition amplitude for 86Sr at -494+/-5 GHz allows us to determine the scattering lengths 610a0 < a86 < 2300a0 for 86Sr and a much smaller value of -1a0 < a88 < 13a0 for 88Sr.

physics.atom-ph↗

arXiv2004

Dynamical Conductivity of Disordered Quantum Hall Stripes

We present a detailed theory for finite-frequency conductivities Re$[σ_{αβ}(ω)]$ of quantum Hall stripes, which form at Landau level $N\geq 2$ close to half filling, in the presence of weak Gaussian disorder. We use an effective elastic theory to describe the low-energy dynamics of the stripes with the dynamical matrix being determined through matching the density-density correlation function obtained in the microscopic time-dependent Hartree-Fock approximation. We then apply replicas and the Gaussian variational method to deal with the disorder. Within this method, a set of saddle point equations for the retarded self energies are obtained, which are solved numerically to get Re$[σ_{αβ}(ω)]$. We find a quantum depinning transition as $Δν$, the fractional part of the filling factor, approaches a critical value $Δν_c$ from below. For $Δν<Δν_c$, the pinned state is realized in a replica symmetry breaking (RSB) solution, and the frequency-dependent conductivities in both the directions perpendicular and parallel to the stripes show resonant peaks. These peaks shift to zero frequency as $Δν\to Δν_c$. For $Δν\geΔν_c$, we find a partial RSB (PRSB) solution in which there is RSB perpendicular to the stripes, but replica symmetry along the stripes, leading to free sliding along the stripe direction. The quantum depinning transition is in the Kosterlitz-Thouless universality class. The result is consistent with a previous renormalization group analysis.

cond-mat.mes-hall↗

arXiv2004

Photoassociative spectroscopy at long range in ultracold strontium

We report photoassociative spectroscopy of $^{88}$Sr$_2$ in a magneto-optical trap operating on the ${^1S_0}\to{^3P_1}$ intercombination line at 689 nm. Photoassociative transitions are driven with a laser red-detuned by 600-2400 MHz from the ${^1S_0}\to{^1P_1}$ atomic resonance at 461 nm. Photoassociation takes place at extremely large internuclear separation, and the photoassociative spectrum is strongly affected by relativistic retardation. A fit of the transition frequencies determines the ${^1P_1}$ atomic lifetime ($τ=5.22 \pm 0.03$ ns) and resolves a discrepancy between experiment and recent theoretical calculations.

physics.atom-ph↗

arXiv2004

Quantum Depinning Transition of Quantum Hall Stripes

We examine the effect of disorder on the electromagnetic response of quantum Hall stripes using an effective elastic theory to describe their low-energy dynamics, and replicas and the Gaussian variational method to handle disorder effects. Within our model we demonstrate the existence of a depinning transition at a critical partial Landau level filling factor $Δν_c$. For $Δν<Δν_c$, the pinned state is realized in a replica symmetry breaking (RSB) solution, and the frequency-dependent conductivities in both perpendicular and parallel to the stripes show resonant peaks. These peaks shift to zero frequency as $Δν\to Δν_c$. For $Δν\geΔν_c$, we find a {\em partial RSB (PRSB)} solution in which there is free sliding only along the stripe direction. The transition is analogous to the Kosterlitz-Thouless phase transition.

cond-mat.mes-hall↗

arXiv2004

Dynamics of electrons in the quantum Hall bubble phases

In Landau levels N > 1, the ground state of the two-dimensional electron gas (2DEG) in a perpendicular magnetic field evolves from a Wigner crystal for small filling of the partially filled Landau level, into a succession of bubble states with increasing number of guiding centers per bubble as the filling increases, to a modulated stripe state near half filling. In this work, we show that these first-order phase transitions between the bubble states lead to measurable discontinuities in several physical quantities such as the density of states and the magnetization of the 2DEG. We discuss in detail the behavior of the collective excitations of the bubble states and show that their spectra have higher-energy modes besides the pinned phonon mode. The frequencies of these modes, at small wavevector k, have a discontinuous evolution as a function of filling factor that should be measurable in, for example, microwave absorption experiments.

cond-mat.mes-hall↗