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R. Cuerno

Publications and source records attributed to R. Cuerno.

At least 19 recordsLinked to original sources

Discrete Lattice Models for Interface Growth on a Complete Graph

We investigate the behavior of discrete interface growth models belonging to the Edwards--Wilkinson (EW) and Kardar--Parisi--Zhang (KPZ) universality classes, when defined on a complete graph, a topology commonly used to probe the infinite-dimensional limit of statistical mechanical systems. Our aim is to assess to what extent discrete lattice models reproduce the behavior of their corresponding continuum equations in this highly connected setting. After assessing the trivial behavior shown by some well known cases (like random deposition with surface relaxation or the etching model), we focus on two paradigmatic models associated with the KPZ universality class, the Restricted Solid-on-Solid (RSOS) and Ballistic Deposition (BD) models, and assess non-trivial behavior through several observables including the roughness, height fluctuations, power spectra, and two-time autocorrelation functions. Still, despite similarities with continuum equations, important differences arise in the fluctuations and long-time dynamics. In both discrete models the rescaled height fluctuations display a pronounced left tail, indicating the presence of lagging nodes. While the RSOS model exhibits a saturation roughness that decreases with system size, similarly to the EW and KPZ equations, the BD model exhibits a saturation roughness that increases with system size and an additional ultrafast growth regime, placing it outside the KPZ universality class on a complete graph.

cond-mat.stat-mech

On the upper critical dimension of the KPZ universality class: KPZ and related equations on a fully connected graph

We investigate the infinite-dimensional limit of nonequilibrium surface growth by numerically integrating stochastic growth equations on a fully connected graph. In particular, we study the Edwards-Wilkinson (EW), Kardar-Parisi-Zhang (KPZ), and tensionless KPZ (TKPZ) equations. Using a network discretization adapted to the all-to-all interaction topology, we analyze the global roughness, height-fluctuation statistics, time power spectra, and two-time correlations. For the EW equation, we obtain an exact expression for the roughness that matches the numerical simulations and shows that the interface becomes flat as the number of nodes in the graph, $N$, tends to infinity. We also compute analytically the time power spectrum, show that height fluctuations are Gaussian, and derive an explicit expression for the two-time height autocorrelation function, indicating that the aging behavior is trivial. For the KPZ equation, finite-size and strong-coupling effects can cause deviations from EW behavior at moderate system sizes $N$, often accompanied by numerical instabilities; however, these differences disappear as $N$ increases. In the large-$N$ limit, KPZ dynamics converges to EW behavior, as the four observables analyzed exhibit identical scaling properties. Overall, our results indicate that on a fully connected graph the KPZ nonlinearity is irrelevant as $N\to\infty$, leading to EW-like dynamics with asymptotically flat interfaces. These findings are interpreted in the context of the upper critical dimension of the KPZ universality class.

cond-mat.stat-mech

Numerical Integration of the KPZ and Related Equations on Networks: The Case of the Cayley Tree

The numerical integration of stochastic growth equations on non-Euclidean networks presents unique challenges due to the nonlinearities that occur in many relevant models and of the structural constraints of the networks. In this work, we integrate the KPZ, Edwards-Wilkinson, and tensionless KPZ equations on Cayley trees using different numerical schemes and compare their behavior with previous results obtained for discrete growth models. By assessing the stability and accuracy of these methods, we explore how network topology influences interface growth and how boundary effects shape the observed scaling properties. Our results show good agreement with previous studies on discrete models, reinforcing key scaling behaviors while highlighting some differences. These findings contribute to a better understanding of surface growth on networked substrates and provide a computational framework for studying nonlinear stochastic processes beyond Euclidean lattices.

cond-mat.stat-mech

Microscopic fluctuations in the spreading fronts of circular wetting liquid droplets

We study numerically the kinetic roughening properties of the precursor fronts of nonvolatile liquid droplets spreading on solid substrates, for the case of circular droplets, more frequently addressed in experiments. To this end, we perform kinetic Monte Carlo (kMC) simulations of a lattice gas model whose kinetic roughening behavior has been recently assessed in a band geometry [J.\ M.\ Marcos {\em et al.}, Phys.\ Rev.\ E {\bf 105}, 054801 (2022)]. We compare the scaling behaviors of the spreading fronts obtained for the two geometries, in view of the occurrence of, for example, different universality subclasses for different growth geometries for the related important Kardar-Parisi-Zhang (KPZ) universality class. For circular droplets we obtain that the average front position increases (sub-)diffusively as $R\sim t^{\delta}$, where $\delta \lesssim 1/2$ shows a stronger dependence on the conditions considered for temperature and substrate wettability than in band geometry. In spite of this, front fluctuations for circular droplets behave qualitatively similar to those seen for band geometries, with kinetic roughening exponent values which similarly depend on temperature $T$ but become $T$-independent for sufficiently high $T$. Circular droplets also display intrinsic anomalous scaling with different values of the roughness exponent at short and large length scales, and fluctuations statistics which are close to the Tracy-Widom probability distribution function that applies in the corresponding KPZ universality subclass, now the one expected for interfaces with an overall circular symmetry.

cond-mat.stat-mech

Universal interface fluctuations in the contact process

We study the interface representation of the contact process (CP) at its directed-percolation critical point, where the scaling properties of the interface can be related to those of the original particle model. Interestingly, such a behavior happens to be intrinsically anomalous and more complex than that described by the standard Family-Vicsek dynamic scaling Ansatz of surface kinetic roughening. We expand on a previous numerical study by Dickman and Mu\~noz [Phys. Rev. E 62, 7632 (2000)] to fully characterize the kinetic roughening universality class for interface dimensions $d=1, 2$, and 3. Beyond obtaining scaling exponent values, we characterize the interface fluctuations via their probability density function (PDF) and covariance, seen to display universal properties which are qualitatively similar to those recently assessed for the Kardar-Parisi-Zhang (KPZ) and other important universality classes of kinetic roughening. Quantitatively, while for $d=1$ the interface covariance seems to be well described by the KPZ, Airy$_1$ covariance, no such agreement occurs in terms of the fluctuation PDF nor the scaling exponents.

cond-mat.stat-mech

Large-scale kinetic roughening behavior of coffee-ring fronts

We have studied the kinetic roughening behavior of the fronts of coffee-ring aggregates via extensive numerical simulations of the off-lattice model considered for this context in [C.\ S.\ Dias {\it et al.}, Soft Matter {\bf 14}, 1903 (2018)]. This model describes ballistic aggregation of patchy colloids and depends on a parameter $r_\mathrm{AB}$ which controls the affinity of the two patches, A and B. Suitable boundary conditions allow us to elucidate a discontinuous pinning-depinning transition at $r_\mathrm{AB}=0$, with the front displaying intrinsic anomalous scaling, but with unusual exponent values $α\simeq 1.2$, $α_{\rm loc} \simeq 0.5$, $β\simeq 1$, and $z\simeq 1.2$. For $0 0.01$ and the system suffers a strong crossover dominated by the $r_\mathrm{AB}=0$ behavior for $r_\mathrm{AB}\le 0.01$. A detailed analysis of correlation functions shows that the aggregate fronts are always in the moving phase for $0<r_\mathrm{AB}\le 1$ and that their kinetic roughening behavior is intrinsically anomalous for $r_\mathrm{AB}\le 0.01$.

cond-mat.soft

Anomalous dynamic scaling of Ising interfaces

Until very recently, the asymptotic occurrence of intrinsic anomalous scaling has been expected to require concomitant effects for kinetically rough interfaces, like quenched disorder or morphological instabilities. However, counterexamples have been recently reported for simpler situations dominated by time-dependent noise, as in the discrete growth system associated with an Ising model proposed by H.\ Dashti-Naserabadi {\em et al.}\ [Phys.\ Rev.\ E {\bf 100}, 060101(R) (2019)], who assessed the equilibrium behavior of the model. Here we revisit this system to characterize its time-dependent behavior in two and three dimensions (one-and two-dimensional interfaces, respectively). While the 3D case seems dominated by a fast evolution beyond critical dynamics, in the 2D case numerical simulations of an associated time-dependent Ginzburg-Landau equation retrieve the same static (roughness) exponents and the same intrinsic anomalous scaling Ansatz as in the equilibrium case, throughout the full time evolution. However, the dynamic exponent is seen to cross over between two different values, none of which enables identification with previously known universality classes of kinetic roughening. Simulations for larger system sizes moreover suggest breakdown of scaling behavior at the largest scales, suggesting that the previously reported scaling behavior may be effective and restricted to relatively small systems.

cond-mat.stat-mech

Spreading fronts of wetting liquid droplets: microscopic simulations and universal fluctuations

We have used kinetic Monte Carlo (kMC) simulations of a lattice gas to study front fluctuations in the spreading of a non-volatile liquid droplet onto a solid substrate. Our results are consistent with a diffusive growth law for the radius of the precursor layer, $R \sim t^δ$, with $δ\approx 1/2$ in all the conditions considered for temperature and substrate wettability, in good agreement with previous studies. The fluctuations of the front exhibit kinetic roughening properties with exponent values which depend on temperature $T$, but become $T$-independent for sufficiently high $T$. Moreover, strong evidences of intrinsic anomalous scaling have been found, characterized by different values of the roughness exponent at short and large length scales. Although such a behavior differs from the scaling properties of the one-dimensional Kardar-Parisi-Zhang (KPZ) universality class, the front covariance and the probability distribution function of front fluctuations found in our kMC simulations do display KPZ behavior, agreeing with simulations of a continuum height equation proposed in this context. However, this equation does not feature intrinsic anomalous scaling, at variance with the discrete model.

cond-mat.stat-mech

The derivative of the Kardar-Parisi-Zhang equation is not in the KPZ universality class

The Kardar-Parisi-Zhang (KPZ) equation is a paradigmatic model of nonequilibrium low-dimensional systems with spatiotemporal scale invariance, recently highlighting universal behavior in fluctuation statistics. Its space derivative, namely the noisy Burgers equation, has played a very important role in its study, predating the formulation of the KPZ equation proper, and being frequently held as an equivalent system. We show that, while differences in the scaling exponents for the two equations are indeed due to a mere space derivative, the fluctuations behave in a remarkably different way: while KPZ displays Tracy-Widom statistics, its derivative displays Gaussian behavior, hence being in a different universality class. We reach this conclusion via direct numerical simulations of the equations, supported by a dynamic renormalization group analysis of field statistics.

cond-mat.stat-mech

Kardar-Parisi-Zhang universality class for the critical dynamics of reaction-diffusion fronts

We have studied front dynamics for the discrete $A+A \leftrightarrow A$ reaction-diffusion system, which in the continuum is described by the (stochastic) Fisher-Kolmogorov-Petrovsky-Piscunov equation. We have revisited this discrete model in two space dimensions by means of extensive numerical simulations and an improved analysis of the time evolution of the interface separating the stable and unstable phases. In particular, we have measured the full set of critical exponents which characterize the spatio-temporal fluctuations of such front for different lattice sizes, focusing mainly in the front width and correlation length. These exponents are in very good agreement with those computed in [E. Moro, Phys. Rev. Lett. 87, 238303 (2001)] and correspond to those of the Kardar-Parisi-Zhang (KPZ) universality class for one-dimensional interfaces. Furthermore, we have studied the one-point statistics and the covariance of rescaled front fluctuations, which had remained thus far unexplored in the literature and allows for a further stringent test of KPZ universality.

cond-mat.stat-mech

Universal behavior of crystalline membranes: crumpling transition and Poisson ratio of the flat phase

We revisit the universal behavior of crystalline membranes at and below the crumpling transition, which pertains to the mechanical properties of important soft and hard matter materials, such as the cytoskeleton of red blood cells or graphene. Specifically, we perform large-scale Monte Carlo simulations of a triangulated two-dimensional phantom network which is freely fluctuating in three-dimensional space. We obtain a continuous crumpling transition characterized by critical exponents which we estimate accurately through the use of finite-size techniques. By controlling the scaling corrections, we additionally compute with high accuracy the asymptotic value of the Poisson ratio in the flat phase, thus characterizing the auxetic properties of this class of systems. We obtain agreement with the value which is universally expected for polymerized membranes with a fixed connectivity.

cond-mat.stat-mech

Ion-beam nanopatterning of silicon surfaces under co-deposition of non-silicide-forming impurities

We report experiments on surface nanopatterning of Si targets which are irradiated with 2 keV Ar + ions impinging at near-glancing incidence, under concurrent co-deposition of Au impurities simultaneously extracted from a gold target by the same ion beam. Previous recent experiments by a number of groups suggest that silicide formation is a prerequisite for pattern formation in the presence of metallic impurities. In spite of the fact that Au is known not to form stable compounds with the Si atoms, ripples nonetheless emerge in our experiments with nanometric wavelengths and small amplitudes, and with an orientation that changes with distance to the Au source. We provide results of sample analysis through Auger electron and energy-dispersive X-ray spectroscopies for their space-resolved chemical composition, and through atomic force, scanning transmission electron, and high-resolution transmission microscopies for their morphological properties. We discuss these findings in the light of current continuum models for this class of systems. The composition of and the dynamics within the near-surface amorphized layer that ensues is expected to play a relevant role to account for the unexpected formation of these surface structures.

cond-mat.mes-hall

Role of Thermal Fluctuations in Nonlinear Thin Film Dewetting

The spontaneous formation of droplets via dewetting of a thin fluid film from a solid substrate allows for materials nanostructuring, under appropriate experimental control. While thermal fluctuations are expected to play a role in this process, their relevance has remained poorly understood, particularly during the nonlinear stages of evolution. Within a stochastic lubrication framework, we show that thermal noise speeds up and substantially influences the formation and evolution of the droplet arrangement. As compared with their deterministic counterparts, for a fixed spatial domain, stochastic systems feature a smaller number of droplets, with a larger variability in sizes and space distribution. Finally, we discuss the influence of stochasticity on droplet coarsening for very long times.

cond-mat.soft

Solid flow drives surface nanopatterning by ion-beam irradiation

Ion Beam Sputtering (IBS) is known to produce surface nanopatterns over macroscopic areas on a wide range of materials. However, in spite of the technological potential of this route to nanostructuring, the physical process by which these surfaces self-organize remains poorly under- stood. We have performed detailed experiments of IBS on Si substrates that validate dynamical and morphological predictions from a hydrodynamic description of the phenomenon. Our results elucidate flow of a nanoscopically thin and highly viscous surface layer, driven by the stress created by the ion-beam, as a description of the system. This type of slow relaxation is akin to flow of macroscopic solids like glaciers or lead pipes, that is driven by defect dynamics.

cond-mat.mtrl-sci

One-dimensional pattern of Au nanodots by ion-beam-sputtering: formation and mechanism

Highly ordered one-dimensional arrays of nanodots, or nanobeads, are fabricated by forming nanoripples and nanodots in sequence, entirely by ion-beamsputtering (IBS) of Au(001). This demonstrates the capability of IBS for the fabrication of sophisticated nanostructures via hierarchical self-assembly. The intricate nanobead pattern ideally serves to identify the governing mechanisms for the pattern formation: Non-linear effects, especially local redeposition and surface-confined transport, are essential both for the formation and the preservation of the pattern order.

cond-mat.mes-hall

Generic equations for pattern formation in evolving interfaces

We present a general formalism which allows us to derive the evolution equations describing one-dimensional (1D) and isotropic 2D interfacelike systems, that is based on symmetries, conservation laws, multiple scale arguments, and exploits the relevance of coarsening dynamics. Our approach becomes especially significant in the presence of surface morphological instabilities and allows us to classify the most relevant nonlinear terms in the continuum description of these systems. The formalism applies to systems ranging from eroded nanostructures to macroscopic pattern formation. In particular, we show the validity of the theory for novel experiments on ion plasma erosion.

cond-mat.other

Influence of Collision Cascade Statistics on Pattern Formation of Ion-Sputtered Surfaces

Theoretical continuum models that describe the formation of patterns on surfaces of targets undergoing ion-beam sputtering, are based on Sigmund's formula, which describes the spatial distribution of the energy deposited by the ion. For small angles of incidence and amorphous or polycrystalline materials, this description seems to be suitable, and leads to the classic BH morphological theory [R.M. Bradley and J.M.E. Harper, J. Vac. Sci. Technol. A 6, 2390 (1988)]. Here we study the sputtering of Cu crystals by means of numerical simulations under the binary-collision approximation. We observe significant deviations from Sigmund's energy distribution. In particular, the distribution that best fits our simulations has a minimum near the position where the ion penetrates the surface, and the decay of energy deposition with distance to ion trajectory is exponential rather than Gaussian. We provide a modified continuum theory which takes these effects into account and explores the implications of the modified energy distribution for the surface morphology. In marked contrast with BH's theory, the dependence of the sputtering yield with the angle of incidence is non-monotonous, with a maximum for non-grazing incidence angles.

cond-mat.mtrl-sci

Roughening of ion-eroded surfaces

Recent experimental studies focusing on the morphological properties of surfaces eroded by ion-bombardment report the observation of self-affine fractal surfaces, while others provide evidence about the development of a periodic ripple structure. To explain these discrepancies we derive a stochastic growth equation that describes the evolution of surfaces eroded by ion bombardment. The coefficients appearing in the equation can be calculated explicitly in terms of the physical parameters characterizing the sputtering process. Exploring the connection between the ion-sputtering problem and the Kardar-Parisi-Zhang and Kuramoto-Sivashinsky equations, we find that morphological transitions may take place when experimental parameters, such as the angle of incidence of the incoming ions or their average penetration depth, are varied. Furthermore, the discussed methods allow us to calculate analytically the ion-induced surface diffusion coefficient, that can be compared with experiments. Finally, we use numerical simulations of a one dimensional sputtering model to investigate certain aspects of the ripple formation and roughening.

cond-mat.stat-mech