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R. D. Dawson

Publications and source records attributed to R. D. Dawson.

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Fast Microwave-free State Preparation and Measurement of Superconducting Qubits

Fast, high-fidelity, scalable state preparation and measurement is critical to the realization of a quantum computing system. The state-of-the-art methods for preparation and readout of superconducting qubits require finely tuned microwave signals and ~100 ns of measurement time, which are major obstacles to the scalability and performance of superconducting quantum computers. Here, we have demonstrated novel, microwave-free methods for both preparation and readout of superconducting qubits with >99% fidelity in only 10 ns for either operation while maintaining qubit coherence. This technology is compatible with scalable superconducting digital control systems, and using quantum flux parametrons for amplification, we demonstrated full quantum-to-digital conversion in only 15 ns, which is an order of magnitude faster than state-of-the-art microwave-based techniques.

quant-ph

Photoinduced phase switching at a Mott insulator-to-metal transition

Achieving fundamental understanding of insulator-to-metal transitions (IMTs) in strongly correlated systems and their persistent and reversible control via nonequilibrium drive are prime targets of current condensed matter research. Photoinduced switching between competing orders in correlated insulators requires a free-energy landscape with nearly degenerate ground states, which is commonly reached through doping, strain, or static electric field. The associated spatial inhomogeneity leads to a photoinduced phase transition that remains confined near the illuminated region. Here we report optical spectroscopy experiments at the first-order IMT in the 4d-electron compound Ca$_3$(Ru$_{0.99}$Ti$_{0.01}$)$_2$O$_7$ and show that specific Ru d-d interband transitions excited by light with a threshold fluence corresponding to the planar density of Ru atoms can trigger reversible, avalanche-like coherent propagation of phase interfaces across the full extent of a macroscopic sample, in the absence of assisting external stimuli. Based on detailed comparison of spectroscopic data to density functional calculations, we attribute the extraordinary photo-sensitivity of the IMT to an exceptionally shallow free-energy landscape generated by the confluence of electron-electron and electron-lattice interactions. Our findings suggest Ca$_3$(Ru$_{0.99}$Ti$_{0.01}$)$_2$O$_7$ as an ideal model system for building and testing a theory of Mott transition dynamics in the presence of strong electron-lattice coupling and may pave the way towards nanoscale devices with quantum-level photosensitivity.

cond-mat.str-el

Approaching two-dimensional superconductivity in ultrathin DyBa$_2$Cu$_3$O$_{7-δ}$

The temperature dependence of the superfluid density $ρ_s(T)$ has been measured for a series of ultrathin MBE-grown DyBa$_2$Cu$_3$O$_{7-δ}$ superconducting (SC) films by sub-mm wave interferometry combined with time-domain THz spectroscopy and IR ellipsometry. We find that all films 10 u.c. and thicker show the same universal temperature dependence of $ρ_s(T)$, which follows the critical behavior characteristic of single crystal YBa$_2$Cu$_3$O$_{7-δ}$ as $T$ approaches $T_c$. In 7 u.c. thick films, $ρ_s(T)$ declines steeply upon approaching $T_c$, as expected for the Berezinskii-Kosterlitz-Thouless vortex unbinding transition. Our analysis provides evidence for a sharply defined 4 u.c. non-SC interfacial layer, leaving a quasi-2D SC layer on top. We propose that the SC state in this interfacial layer is suppressed by competing (possibly charge) order.

cond-mat.supr-con

Infrared phonon spectra of quasi-one-dimensional Ta$_2$NiSe$_5$ and Ta$_2$NiS$_5$

Using a combination of infrared ellipsometry, time-domain terahertz spectroscopy, and far-infrared reflectometry we have obtained the $ac$-plane complex dielectric function of monoclinic ($C2/c$) Ta$_2$NiSe$_5$ and orthorhombic ($Cmcm$) Ta$_2$NiS$_5$ single crystals. The identified dipole-active phonon modes polarized along $a$ and $c$ axes are in good agreement with density functional theory calculations. With increasing temperature the $a$-axis phonon modes of Ta$_2$NiSe$_5$ become poorly discernible, as they are superimposed on the electronic background which gradually fills the energy gap near the monoclinic-to-orthorhombic phase transition temperature $T_c$ = 326 K. In Ta$_2$NiS$_5$, which does not exhibit such a structural transition and remains orthorhombic down to low temperatures, the $a$-axis phonon modes are superimposed on a persistent broad electronic mode centered near 16 meV. We attribute this difference to strongly overlapping exciton-phonon complexes in Ta$_2$NiSe$_5$, as opposed to isolated instances of the same in Ta$_2$NiS$_5$, and find this to be in good agreement with an excitonic insulator state below $T_c$ in the former, as compared to the absence of one in the latter.

cond-mat.str-el