arXiv subjects

R. D. H. Hinlopen

Publications and source records attributed to R. D. H. Hinlopen.

7 recordsLinked to original sources

arXiv2026

$H$-linear magnetoresistance in NbSe$_2$ due to impeded cyclotron motion

Linear magnetoresistance (LMR) is a widespread phenomenon observed in a host of quantum materials ranging from semiconductor nanostructures to quantum critical and strange metals. While multiple scenarios to explain LMR have been proposed, a complete understanding of the phenomenon remains elusive. Indeed, it is highly likely that the origin of LMR depends on the specific electronic state. Here, we report a study of the impact of disorder on the form of the magnetoresistance of the prototypical charge-density-wave (CDW) compound 2$H$-NbSe$_2$. The magnetoresistance is shown to exhibit strong qualitative and quantitative agreement with Boltzmann transport analysis incorporating impeded cyclotron motion (ICM). We identify the source of ICM in 2$H$-NbSe$_2$ as strong scattering sinks where the CDW order connects the high temperature Fermi cylinders. Such unusual "hotspots" provide an explanation for the observed LMR as well as for the long-unexplained absence of quantum oscillations inside the charge ordered state in 2$H$-NbSe$_2$. These findings provide strong evidence that ICM generates LMR in certain correlated metals.

cond-mat.str-el↗

arXiv2026

Programmable superconducting diode from nematic domain control in FeSe

The superconducting diode effect (SDE) allows polarity-dependent critical currents when time-reversal and current-inverting spatial symmetries are broken. Superconducting diodes show promise for applications, but inversion asymmetry is usually encoded in sample geometry or non-centrosymmetric crystals, rendering them static circuit elements. Here we demonstrate a programmable superconducting diode whose functionality is encoded in correlated electronic domains. We use the nematic superconductor FeSe as a platform and report a large intrinsic SDE with efficiencies up to $η\sim 75\%$ due to vortices interacting with nematic twin boundaries. The domain wall configuration thus encodes the SDE of the device. Through intense microsecond current pulses to quench the nematic order at rates exceeding $10^7$ K/s, we modify the domain pattern and control the polarity and strength of the SDE. These results establish a new paradigm in which superconducting circuit elements can be programmed through patterns imprinted into correlated electronic states.

cond-mat.supr-con↗

arXiv2025

Evidence for spin-fluctuation-mediated superconductivity in electron-doped cuprates

In conventional, phonon-mediated superconductors, the transition temperature $T_c$ and normal-state scattering rate $1/τ$ - deduced from the linear-in-temperature resistivity $ρ(T)$ - are linked through the electron-phonon coupling strength $λ_{\rm ph}$. In cuprate high-$T_c$ superconductors, no equivalent $λ$ has yet been identified, despite the fact that at high doping, $α$ - the low-$T$ $T$-linear coefficient of $ρ(T)$ - also scales with $T_c$. Here, we use dc resistivity and high-field magnetoresistance to extract $τ^{-1}$ in electron-doped La$_{2-x}$Ce$_x$CuO$_4$ (LCCO) as a function of $x$ from optimal doping to beyond the superconducting dome. A highly anisotropic inelastic component to $τ^{-1}$ is revealed whose magnitude diminishes markedly across the doping series. Using known Fermi surface parameters and subsequent modelling of the Hall coefficient, we demonstrate that the form of $τ^{-1}$ in LCCO is consistent with scattering off commensurate antiferromagnetic spin fluctuations of variable strength $λ_{\rm sf}$. The clear correlation between $α$, $λ_{\rm sf}$ and $T_c$ then identifies low-energy spin-fluctuations as the primary pairing glue in electron-doped cuprates. The contrasting magnetotransport behaviour in hole-doped cuprates suggests that the higher $T_c$ in the latter cannot be attributed solely to an increase in $λ_{\rm sf}$. Indeed, the success in modelling LCCO serves to reinforces the notion that resolving the origin of high-temperature superconductivity in hole-doped cuprates may require more than a simple extension of BCS theory.

cond-mat.supr-con↗

arXiv2023

Lifshitz transition enabling superconducting dome around the quantum critical point in TiSe$_2$

Superconductivity often emerges as a dome around a quantum critical point (QCP) where long-range order is suppressed to zero temperature. So far, this has been mostly studied in magnetically ordered materials. By contrast, the interplay between charge order and superconductivity at a QCP is not fully understood. Here, we present resistance measurements proving that a dome of superconductivity surrounds the charge-density-wave (CDW) QCP in pristine samples of 1$T$-TiSe$_2$ tuned with hydrostatic pressure. Furthermore, we use quantum oscillation measurements to show that the superconductivity sets in at a Lifshitz transition in the electronic band structure. We use density functional theory to identify the Fermi pockets enabling superconductivity: large electron and hole pockets connected by the CDW wave vector $\vec{Q}$ which emerge upon partial suppression of the zero-pressure CDW gap. Hence, we conclude that superconductivity is of interband type enabled by the presence of hole and electron bands connected by the CDW $\vec{Q}$ vector. Earlier calculations show that interband interactions are repulsive, which suggests that unconventional s$_{\pm}$ superconductivity is realised in TiSe$_2$ - similar to the iron pnictides. These results highlight the importance of Lifshitz transitions in realising unconventional superconductivity and help understand its interaction with CDW order in numerous materials.

cond-mat.supr-con↗

arXiv2022

Compartmentalizing the cuprate strange metal

It has long been recognized that the key to unlocking the mystery of cuprate high-Tc superconductivity lies in understanding the anomalous normal state from which pairs form and condense. While many of its defining properties have been identified, they are often considered either at a singular doping level or as an isolated phenomenon as a function of doping. As a result, their relation to each other and to the pseudogap (PG), strange metal (SM) and non-superconducting (non-SC) regimes that define the cuprate phase diagram has yet to be elucidated. Here, we report a high-field in-plane MR study on several cuprate families spanning all 3 regimes that reveal a complex yet nonetheless systematic evolution of the form of the MR, with each regime possessing its own distinct scaling behavior. In the PG regime, the MR exhibits pure H/T^2 scaling at low fields and H-linearity at the highest field strengths. While the H-linearity persists inside the SM regime, the scaling changes abruptly to H/T. The size of the H-linear slope, meanwhile, is found to be correlated with both the T-linear resistivity coefficient and Tc, strengthening the characterization of the SM regime as a quantum critical phase. We interpret the omnipresence of H-linear MR across both regimes as a signature of highly anisotropic, possibly discontinuous features on the Fermi surface. Finally, within the non-SC, Fermi-liquid regime, we observe a recovery of conventional Kohler scaling. This comprehensive study establishes the distinct nature of the magnetotransport within each regime and identifies power-law scaling of the normal state MR as a defining feature of SC hole-doped cuprates. The incompatibility of such power-law scaling with any known variant of Boltzmann transport theory motivates the quest for an altogether new theoretical framework, one in which the MR is entirely decoupled from elastic impurity scattering.

cond-mat.supr-con↗

arXiv2022

$B^2$ to $B$-linear magnetoresistance due to impeded orbital motion

Strange metals exhibit a variety of anomalous magnetotransport properties, the most striking of which is a resistivity that increases linearly with magnetic field $B$ over a broad temperature and field range. The ubiquity of this behavior across a spectrum of correlated metals - both single- and multi-band, with either dominant spin and/or charge fluctuations, of varying levels of disorder or inhomogeneity and in proximity to a quantum critical point or phase - obligates the search for a fundamental underlying principle that is independent of the specifics of any material. Strongly anisotropic (momentum-dependent) scattering can generate $B$-linear magnetoresistance but only at intermediate field strengths. At high enough fields, the magnetoresistance must eventually saturate. Here, we consider the ultimate limit of such anisotropy, a region or regions on the Fermi surface that impede all orbital (cyclotron) motion through them, but whose imposition can be modelled nonetheless through a modified Boltzmann theoretical treatment. Application of the proposed theorem suggests that the realization of quadratic-to-linear magnetoresistance requires the presence of a bounded sector on the Fermi surface possibly separating two distinct types of carriers. While this bounded sector may have different origins or manifestations, we expect its existence to account for the anomalous magnetotransport found in a wide range of correlated materials.

cond-mat.str-el↗

arXiv2017

Quasi-two-dimensional Fermi surfaces with localized $f$ electrons in the layered heavy-fermion compound CePt$_2$In$_7$

We report measurements of the de Haas-van Alphen effect in the layered heavy-fermion compound CePt$_2$In$_7$ in high magnetic fields up to 35 T. Above an angle-dependent threshold field, we observed several de Haas-van Alphen frequencies originating from almost ideally two-dimensional Fermi surfaces. The frequencies are similar to those previously observed to develop only above a much higher field of 45 T, where a clear anomaly was detected and proposed to originate from a change in the electronic structure [M. M. Altarawneh et al., Phys. Rev. B 83, 081103 (2011)]. Our experimental results are compared with band structure calculations performed for both CePt$_2$In$_7$ and LaPt$_2$In$_7$, and the comparison suggests localized $f$ electrons in CePt$_2$In$_7$. This conclusion is further supported by comparing experimentally observed Fermi surfaces in CePt$_2$In$_7$ and PrPt$_2$In$_7$, which are found to be almost identical. The measured effective masses in CePt$_2$In$_7$ are only moderately enhanced above the bare electron mass $m_0$, from 2$m_0$ to 6$m_0$.

cond-mat.str-el↗