arXiv subjects

R. D. Zhong

Publications and source records attributed to R. D. Zhong.

At least 37 records · Page 2Linked to original sources

arXiv2017

Static Charge Density Wave Order in the Superconducting State of La2-xBaxCuO4

Charge density wave (CDW) correlations feature prominently in the phase diagram of the cuprates, motivating competing theories of whether fluctuating CDW correlations aid superconductivity or whether static CDW order coexists with superconductivity in inhomogeneous or spatially modulated states. Here we report Cu $L$-edge resonant x-ray photon correlation spectroscopy (XPCS) measurements of CDW correlations in superconducting La$_{2-x}$Ba$_x$CuO$_4$ $x=0.11$. Static CDW order is shown to exist in the superconducting state at low temperatures and to persist up to at least 85\% of the CDW transition temperature. We discuss the implications of our observations for how \emph{nominally} competing order parameters can coexist in the cuprates.

cond-mat.supr-con↗

arXiv2017

Vertical temperature-boundary of the pseudogap under the superconducting dome of the Bi2Sr2CaCu2O8+d phase-diagram

Combining electronic Raman scattering experiments with cellular dynamical mean field theory, we present evidence of the pseudogap in the superconducting state of various hole-doped cuprates. In Bi2Sr2CaCu2O8+d we track the superconducting pseudogap hallmark, a peak-dip feature, as a function of temperature T and doping p, well beyond the optimal one. We show that, at all temperatures under the superconducting dome, the pseudogap disappears at the doping pc, between 0.222 and 0.226, where also the normal-state pseudogap collapses at a Lifshitz transition. This demonstrates that the superconducting pseudogap boundary forms a vertical line in the T-p phase diagram.

cond-mat.supr-con↗

arXiv2017

Spectroscopic evidence for bulk-band inversion and three-dimensional massive Dirac fermions in ZrTe5

Three-dimensional topological insulators (3D TIs) represent novel states of quantum matters in which surface states are protected by time-reversal symmetry and an inversion occurs between bulk conduction- and valence-bands. However, the bulk-band inversion which is intimately tied to the topologically nontrivial nature of 3D TIs has rarely been investigated by experiments. Besides, 3D massive Dirac fermions with nearly near band dispersions were seldom observed in TIs. Recently, a van der Waals crystal, ZrTe5, was theoretically predicted to be a TI. Here, we report an infrared transmission study of a high-mobility (~33,000 cm$^2$/(Vs)) multilayer ZrTe5 flake at magnetic fields ($B$) up to 35 T. Our observation of a linear relationship between the zero-magnetic-field optical absorption and the photon energy, a bandgap of ~10 meV and a $\sqrt{B}$ dependence of the Landau level (LL) transition energies at low magnetic fields demonstrates 3D massive Dirac fermions with nearly linear band dispersions in this system. More importantly, the reemergence of the intra-LL transitions at magnetic fields higher than 17 T reveals the energy cross between the two zeroth LLs, which reflects the inversion between the bulk conduction- and valence-bands. Our results not only provide spectroscopic evidence for the TI state in ZrTe5 but also open up a new avenue for fundamental studies of Dirac fermions in van der Waals materials.

cond-mat.mes-hall↗

arXiv2016

Superconductivity with two-fold symmetry in topological superconductor SrxBi2Se3

Topological superconductivity is the quantum condensate of paired electrons with an odd parity of the pairing function. One of the candidates is the triplet pairing superconductor derived from topological insulator Bi2Se3 by chemical doping. Theoretically it was predicted that a two-fold superconducting order parameter may exist in this kind of bulk topological superconductor. Earlier experiments by nuclear magnetic resonance and angle-resolved magnetocaloric measurements seem to support this picture. By using a Corbino-shape like electrode configuration, we measure the c-axis resistivity without the influence of the vortex motion and find clear evidence of two-fold superconductivity in the recently discovered topological superconductor SrxBi2Se3. The Laue diffraction measurements on these samples show that the maximum gap direction is either parallel or perpendicular to the main crystallographic axis.

cond-mat.supr-con↗

arXiv2016

Phonon anomalies in some iron-telluride materials

The detailed temperature dependence of the infrared-active mode in Fe$_{1.03}$Te ($T_N\simeq 68$ K) and Fe$_{1.13}$Te ($T_N\simeq 56$ K) has been examined, and the position, width, strength, and asymmetry parameter determined using an asymmetric Fano profile superimposed on an electronic background. In both materials the frequency of the mode increases as the temperature is reduced; however, there is also a slight asymmetry in the line shape, indicating that the mode is coupled to either spin or charge excitations. Below $T_N$ there is an anomalous decrease in frequency and the mode shows little temperature dependence, at the same time becoming more symmetric, suggesting a reduction in spin- or electron-phonon coupling. The frequency of the infrared-active mode and the magnitude of the shift below $T_N$ are predicted reasonably well by first-principles calculations; however, the predicted splitting of the mode is not observed. In superconducting FeTe$_{0.55}$Se$_{0.45}$ ($T_c\simeq 14$ K) the infrared-active $E_u$ mode displays asymmetric line shape at all temperatures, which is most pronounced between 100 - 200 K, indicating the presence of either spin- or electron-phonon coupling, which may be a necessary prerequisite for superconductivity in this class of materials.

cond-mat.str-el↗

arXiv2016

Collapse of the Normal State Pseudogap at a Lifshitz Transition in Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ Cuprate Superconductor

We report a fine tuned doping study of strongly overdoped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ single crystals using electronic Raman scattering. Combined with theoretical calculations, we show that the doping, at which the normal state pseudogap closes, coincides with a Lifshitz quantum phase transition where the active hole-like Fermi surface becomes electron-like. This conclusion suggests that the microscopic cause of the pseudogap is sensitive to the Fermi surface topology. Furthermore, we find that the superconducting transition temperature is unaffected by this transition, demonstrating that their origins are different on the overdoped side.

cond-mat.supr-con↗

arXiv2016

Energy dissipation in the time domain governed by bosons in a correlated material

In complex materials various interactions play important roles in determining the material properties. Angle Resolved Photoelectron Spectroscopy (ARPES) has been used to study these processes by resolving the complex single particle self energy $Σ(E)$ and quantifying how quantum interactions modify bare electronic states. However, ambiguities in the measurement of the real part of the self energy and an intrinsic inability to disentangle various contributions to the imaginary part of the self energy often leave the implications of such measurements open to debate. Here we employ a combined theoretical and experimental treatment of femtosecond time-resolved ARPES (tr-ARPES) and show how measuring the population dynamics using tr-ARPES can be used to separate electron-boson interactions from electron-electron interactions. We demonstrate the analysis of a well-defined electron-boson interaction in the unoccupied spectrum of the cuprate Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$ characterized by an excited population decay time constant $τ_{QP}$ that maps directly to a discrete component of the equilibrium self energy not readily isolated by static ARPES experiments.

cond-mat.str-el↗

arXiv2015

Fully gapped superconductivity in In-doped topological crystalline insulator Pb$_{0.5}$Sn$_{0.5}$Te

Superconductors derived from topological insulators and topological crystalline insulators by doping have long been considered to be candidates as topological superconductors. Pb$_{0.5}$Sn$_{0.5}$Te is a topological crystalline insulator with mirror symmetry protected surface states on (001), (011) and (111) oriented surfaces. The superconductor (Pb$_{0.5}$Sn$_{0.5}$)$_{0.7}$In$_{0.3}$Te is induced by In doping in Pb$_{0.5}$Sn$_{0.5}$Te, and is thought to be a topological superconductor. Here we report the first scanning tunneling spectroscopy measurement of the superconducting state as well as the superconducting energy gap in (Pb$_{0.5}$Sn$_{0.5}$)$_{0.7}$In$_{0.3}$Te on a (001)-oriented surface. The spectrum can be well fitted by an anisotropic $s$-wave gap function of $Δ=0.72+0.18\cos4θ$ meV using Dynes model. The results show that the quasi-particle density of states seem to be fully gapped without any in-gap states, in contradiction with the expectation of a topological superconductor.

cond-mat.supr-con↗

arXiv2015

Dependence of superconductivity in CuxBi2Se3 on quenching conditions

Topological superconductivity, implying gapless protected surface states, has recently been proposed to exist in the compound CuxBi2Se3. Unfortunately, low diamagnetic shielding fractions and considerable inhomogeneity have been reported in this compound. In an attempt to understand and improve on the finite superconducting volume fractions, we have investigated the effects of various growth and post-annealing conditions. With a melt-growth (MG) method, diamagnetic shielding fractions of up to 56% in Cu0.3Bi2Se3 have been obtained, the highest value reported for this method. We investigate the efficacy of various quenching and annealing conditions, finding that quenching from temperatures above 560C is essential for superconductivity, whereas quenching from lower temperatures or not quenching at all is detrimental. A modified floating zone (FZ) method yielded large single crystals but little superconductivity. Even after annealing and quenching, FZ-grown samples had much less chance of being superconducting than MG-grown samples. From the low shielding fractions in FZ-grown samples and the quenching dependence, we suggest that a metastable secondary phase having a small volume fraction in most of the samples may be responsible for the superconductivity.

cond-mat.supr-con↗

arXiv2014

Observation of the chiral magnetic effect in ZrTe5

The chiral magnetic effect is the generation of electric current induced by chirality imbalance in the presence of magnetic field. It is a macroscopic manifestation of the quantum anomaly in relativistic field theory of chiral fermions (massless spin $1/2$ particles with a definite projection of spin on momentum) -- a dramatic phenomenon arising from a collective motion of particles and antiparticles in the Dirac sea. The recent discovery of Dirac semimetals with chiral quasi-particles opens a fascinating possibility to study this phenomenon in condensed matter experiments. Here we report on the first observation of chiral magnetic effect through the measurement of magneto-transport in zirconium pentatelluride, ZrTe_5. Our angle-resolved photoemission spectroscopy experiments show that this material's electronic structure is consistent with a 3D Dirac semimetal. We observe a large negative magnetoresistance when magnetic field is parallel with the current. The measured quadratic field dependence of the magnetoconductance is a clear indication of the chiral magnetic effect. The observed phenomenon stems from the effective transmutation of Dirac semimetal into a Weyl semimetal induced by the parallel electric and magnetic fields that represent a topologically nontrivial gauge field background.

cond-mat.str-el↗

arXiv2014

Imaging Dirac-Mass Disorder from Magnetic Dopant-Atoms in the Ferromagnetic Topological Insulator Cr$_x$(Bi$_{0.1}$Sb$_{0.9}$)$_{2-x}$Te$_3$

To achieve and utilize the most exotic electronic phenomena predicted for the surface states of 3D topological insulators (TI),it is necessary to open a "Dirac-mass gap" in their spectrum by breaking time-reversal symmetry. Use of magnetic dopant atoms to generate a ferromagnetic state is the most widely used approach. But it is unknown how the spatial arrangements of the magnetic dopant atoms influence the Dirac-mass gap at the atomic scale or, conversely, whether the ferromagnetic interactions between dopant atoms are influenced by the topological surface states. Here we image the locations of the magnetic (Cr) dopant atoms in the ferromagnetic TI Cr$_{0.08}$(Bi$_{0.1}$Sb$_{0.9}$)$_{1.92}$Te$_3$. Simultaneous visualization of the Dirac-mass gap $Δ(r)$ reveals its intense disorder, which we demonstrate directly is related to fluctuations in $n(r)$, the Cr atom areal density in the termination layer. We find the relationship of surface-state Fermi wavevectors to the anisotropic structure of $Δ(r)$ consistent with predictions for surface ferromagnetism mediated by those states. Moreover, despite the intense Dirac-mass disorder, the anticipated relationship $Δ(r)\propto n(r)$ is confirmed throughout, and exhibits an electron-dopant interaction energy $J^*$=145$meV\cdot nm^2$. These observations reveal how magnetic dopant atoms actually generate the TI mass gap locally and that, to achieve the novel physics expected of time-reversal-symmetry breaking TI materials, control of the resulting Dirac-mass gap disorder will be essential.

cond-mat.mtrl-sci↗

arXiv2014

Spectral weight transfer in strongly correlated Fe$_{1.03}$Te

The temperature dependence of the in-plane optical conductivity has been determined for Fe$_{1.03}$Te above and below the magnetic and structural transition at $T_N\simeq 68$ K. The electron and hole pockets are treated as two separate electronic subsystems; a strong, broad Drude response that is largely temperature independent, and a much weaker, narrow Drude response with a strong temperature dependence. Spectral weight is transferred from high to low frequency below $T_N$, resulting in the dramatic increase of both the low-frequency conductivity and the related plasma frequency. The change in the plasma frequency is due to an increase in the carrier concentration resulting from the closing of the pseudogap on the electron pocket, as well as the likely decrease of the effective mass in the antiferromagnetic state.

cond-mat.str-el↗

arXiv2014

Aharonov-Bohm Oscillations in a Quasi-Ballistic 3D Topological Insulator Nanowire

In three-dimensional topological insulators (3D TI) nanowires, transport occurs via gapless surface states where the spin is fixed perpendicular to the momentum[1-6]. Carriers encircling the surface thus acquire a πBerry phase, which is predicted to open up a gap in the lowest-energy 1D surface subband. Inserting a magnetic flux (Φ) of h/2e through the nanowire should cancel the Berry phase and restore the gapless 1D mode[7-8]. However, this signature has been missing in transport experiments reported to date[9-11]. Here, we report measurements of mechanically-exfoliated 3D TI nanowires which exhibit Aharonov-Bohm oscillations consistent with topological surface transport. The use of low-doped, quasi-ballistic devices allows us to observe a minimum conductance at Φ = 0 and a maximum conductance reaching e^2/h at Φ = h/2e near the lowest subband (i.e. the Dirac point), as well as the carrier density dependence of the transport.

cond-mat.mes-hall↗

arXiv2014

Bulk Signatures of Pressure-Induced Band Inversion and Topological Phase Transitions in Pb$_{1-x}$Sn$_x$Se

The characteristics of topological insulators are manifested in both their surface and bulk properties, but the latter remain to be explored. Here we report bulk signatures of pressure-induced band inversion and topological phase transitions in Pb$_{1-x}$Sn$_x$Se ($x=$0.00, 0.15, and 0.23). The results of infrared measurements as a function of pressure indicate the closing and the reopening of the band gap as well as a maximum in the free carrier spectral weight. The enhanced density of states near the band gap in the topological phase give rise to a steep interband absorption edge. The change of density of states also yields a maximum in the pressure dependence of the Fermi level. Thus our conclusive results provide a consistent picture of pressure-induced topological phase transitions and highlight the bulk origin of the novel properties in topological insulators.

cond-mat.mtrl-sci↗

arXiv2014

Superconductivity induced by In substitution into the topological crystalline insulator Pb(0.5)Sn(0.5)Te

Indium substitution turns the topological crystalline insulator (TCI) Pb$_{0.5}$Sn$_{0.5}$Te into a possible topological superconductor. To investigate the effect of the indium concentration on the crystal structure and superconducting properties of (Pb$_{0.5}$Sn$_{0.5}$)$_{1-x}$In$_{x}$Te, we have grown high-quality single crystals using a modified floating-zone method, and have performed systematic studies for indium content in the range $0\leq x\leq 0.35$. We find that the single crystals retain the rock salt structure up to the solubility limit of indium ($x\sim0.30$). Experimental dependences of the superconducting transition temperature ($T_c$) and the upper critical magnetic field ($H_{c2}$) on the indium content $x$ have been measured. The maximum $T_c$ is determined to be 4.7 K at $x=0.30$, with $μ_0H_{c2}(T=0)\approx 5$ T.

cond-mat.supr-con↗

arXiv2014

Power Law Like Correlation between Condensation Energy and Superconducting Transition Temperatures in Iron Pnictide/Chalcogenide Superconductors: Beyond the BCS Understanding

Superconducting condensation energy $U_0^{int}$ has been determined by integrating the electronic entropy in various iron pnictide/chalcogenide superconducting systems. It is found that $U_0^{int}\propto T_c^n$ with $n$ = 3 to 4, which is in sharp contrast to the simple BCS prediction $U_0^{BCS}=1/2N_FΔ_s^2$ with $N_F$ the quasiparticle density of states at the Fermi energy, $Δ_s$ the superconducting gap. A similar correlation holds if we compute the condensation energy through $U_0^{cal}=3γ_n^{eff}Δ_s^2/4π^2k_B^2$ with $γ_n^{eff}$ the effective normal state electronic specific heat coefficient. This indicates a general relationship $γ_n^{eff} \propto T_c^m$ with $m$ = 1 to 2, which is not predicted by the BCS scheme. A picture based on quantum criticality is proposed to explain this phenomenon.

cond-mat.supr-con↗

arXiv2013

A spectroscopic fingerprint of electron correlation in high temperature superconductors

The so-called "strange metal phase" [1] of high temperature (high Tc) superconductors remains at the heart of the high Tc mystery. Better experimental data and insightful theoretical work would improve our understanding of this enigmatic phase. In particular, the recent advance in angle resolved photoelectron spectroscopy (ARPES) [2, 3], incorporating low photon energies (about 7 eV), has given a much more refined view of the many body interaction in these materials. Here, we report a new ARPES feature of Bi2Sr2CaCu2O8+d that we demonstrate to have the key ability to distinguish between different classes of theories of the normal state. This feature---the anomaly in the nodal many body density of states (nMBDOS)---is clearly observed in the low energy ARPES data, but also observed in more conventional high energy ARPES data, when a sufficient temperature range is covered. We show that key characteristics of this anomaly are explained by a strong electron correlation model; the electron-hole asymmetry and the momentum dependent self energy emerge as key required ingredients.

cond-mat.supr-con↗

arXiv2013

Optimizing the superconducting transition temperature and upper critical field of Sn(1-x)In(x)Te

Sn(1-x)In(x)Te is a possible candidate for topological superconductivity. Previous work has shown that substitution of In for Sn in the topological crystalline insulator SnTe results in superconductivity, with the transition temperature, Tc, growing with In concentration. We have performed a systematic investigation of Sn(1-x)In(x)Te for a broad range of x, synthesizing single crystals (by a modified floating zone method) as well as polycrystalline samples. The samples have been characterized by x-ray diffraction, resistivity, and magnetization. For the single crystals, the maximum Tc is obtained at x=0.45 with a value of of 4.5 K, as determined by the onset of diamagnetism.

cond-mat.supr-con↗