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R. Dubey

Publications and source records attributed to R. Dubey.

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Observation of Thermal Deuteron-Deuteron Fusion in Ion Tracks

A direct observation of the deuteron-deuteron (DD) fusion reaction at thermal meV energies, although theoretically possible, is not succeeded up to now. The electron screening effect that reduces the repulsive Coulomb barrier between reacting nuclei in metallic environments by several hundreds of eV and is additionally increased by crystal lattice defects in the hosting material, leads to strongly enhanced cross sections which means that this effect might be studied in laboratories. Here we present results of the 2H(d,p)3H reaction measurements performed on a ZrD2 target down to the lowest deuteron energy in the center mass system of 675 eV, using an ultra-high vacuum accelerator system, recently upgraded to achieve high beam currents at very low energies. The experimental thick target yield, decreasing over seven orders of magnitude for lowering beam energies, could be well described by the electron screening energy of 340 eV, which is much higher than the value of about 100 eV for a defect free material. At the energies below 2.5 keV, a constant plateau yield value could be observed. As indicated by significantly increased energies of emitted protons, this effect can be associated with the thermal DD fusion. A theoretical model explains the experimental observations by creation of ion tracks induced in the target by projectiles, and a high phonon density which locally increases temperature above the melting point. The nuclear reaction rate taking into account recently observed DD threshold resonance agrees very well with the experimental data.

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Experimental signatures of a new channel of the DD reaction at very-low energy

The discovery of a new, strong reaction channel of the deuteron-deuteron fusion at very low energies might have major consequences for the construction of a future clean and efficient energy source. Following the first theoretical and experimental indications for the existence of the deuteron-deuteron threshold resonance in the $^4$He nucleus and its dominant decay by the internal $e^+e^-$ pair creation, we present here an extensive experimental study confirming emission of high-energy electrons and positrons. A simultaneous use of Si charged particle detectors of different thicknesses and large volume NaI(Tl) and HPGe detectors has allowed for the first time to determine the branching ratio between emitted protons, neutrons and $e^+e^-$ pairs for deuteron energies down to 5 keV. The high-energy positrons could be unambiguously detected by their bremsstrahlung spectra and annihilation radiation, supported by the Monte Carlo Geant4 simulations. The theoretical calculations, based on a destructive interference between the threshold resonance and the known broad resonance in $^4$He, agree very well with experimentally observed increase of branching ratios for lowering projectile energies. The partial width of the threshold resonance for the $e^+e^-$ pair creation should be at least 10 times larger than that of the proton channel.

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High-energy electron measurements with thin Si detectors

A technique for measuring high-energy electrons using Si detectors of various thicknesses that are much smaller than the range of the examined electrons is presented. The advantages of the method are discussed on the basis of electron-positron pair creation recently studied in deuteron-deuteron fusion reactions at very low energies. Careful Geant 4 Monte Carlo simulations enabled the identification of the main spectral contributions of emitted electrons and positrons resulting from the energy loss mechanisms and scattering processes within the target, detector and their holders. Significant changes in the intensity of the detected electrons, depending on the detector thickness and the thicknesses of absorption foils placed in the front of the detector could be observed. The corresponding correction factors have been calculated and can be used for different applications in basic and applied research.

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First observation of electron emission from the DD threshold resonance

Electron emission in the deuteron-deuteron reaction supporting existence of the single-particle threshold resonance in 4 He has been observed for the first time. The measured electron energy spectrum and the electron-proton branching ratio agree very well with the assumed electron-positron pair creation decay of the 0+ resonance state to the ground state and the detailed Monte Carlo simulations of the experimental energy spectrum.

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$^{138}{\rm Ba}(d,\alpha)$ study of states in $^{136}{\rm Cs}$: Implications for new physics searches with xenon detectors

We used the $^{138}$Ba$(d,\alpha)$ reaction to carry out an in-depth study of states in $^{136}$Cs, up to around 2.5~MeV. In this work, we place emphasis on hitherto unobserved states below the first $1^+$ level, which are important in the context of solar neutrino and fermionic dark matter (FDM) detection in large-scale xenon experiments. We identify for the first time candidate metastable states in $^{136}$Cs, which would allow a real-time detection of solar neutrino and FDM events in xenon detectors, with high background suppression. Our results are also compared with shell-model calculations performed with three Hamiltonians that were previously used to evaluate the nuclear matrix element (NME) for $^{136}$Xe neutrinoless double beta decay. We find that one of these Hamiltonians, which also systematically underestimates the NME compared to the others, dramatically fails to describe the observed low-energy $^{136}$Cs spectrum, while the other two show reasonably good agreement.

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Re-investigation of the interplay of fission modes and non-equilibrium fission processes in heavy actinide nuclei 249Bk and 257Md

Measurements of mass and angular distributions of fission fragments from actinide nuclei 249Bk and 257Md, produced in fusion reactions 11B and 19F + 238238U, are presented. Experimentally observed mass ratio distributions indicate 'multi-chance fission' through the interplay of fission modes in the fission process, and they agree well with predictions from calculations using the GEF ('GEneral description of Fission observables') model code. Furthermore, to test the signatures of events from non-compound nuclear processes in the fission of 249Bk and 257Md nuclei, Monte Carlo statistical decay model calculations using GEMINI++ were performed for the measured mass distribution at all energies. For comparison purposes, the fission fragment mass distributions of neighboring heavy actinide nuclei, previously measured in the fission of 250Cf and 254Fm nuclei produced by 12C and 16O projectiles on a 238U target, are also presented. The measured angular anisotropy data for the 19F + 238U reaction differ from the results of the Transition State Model at energies below the fusion barrier. As a result of the present study, we suggest considering the interplay between K relaxation time, dynamic dissipation, and their influence on shell correction to understand the evolution of fission dynamics in heavy-ion-induced actinide nuclei

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Search for stabilizing effects of $\bm{Z=82}$ shell closure against fission

Presence of closed proton and/or neutron shells causes deviation from macroscopic properties of nuclei which are understood in terms of the liquid drop model. It is important to investigate experimentally the stabilizing effects of shell closure, if any, against fission. This work aims to investigate probable effects of proton shell ($Z = 82$) closure in the compound nucleus, in enhancing survival probability of the evaporation residues formed in heavy ion-induced fusion-fission reactions. Evaporation residue cross sections have been measured for the reactions $^{19}$F+$^{180}$Hf, $^{19}$F+$^{181}$Ta and $^{19}$F+$^{182}$W from $\simeq9\%$ below to $\simeq42\%$ above the Coulomb barrier, leading to formation of compound nuclei with same number of neutrons ($N = 118$) but different number of protons across $Z = 82$. Measured excitation functions have been compared with statistical model calculation, in which reduced dissipation coefficient is the only adjustable parameter. Evaporation residue cross section, normalized by capture cross section, is found to decrease gradually with increasing fissility of the compound nucleus. Measured evaporation residue cross sections require inclusion of nuclear viscosity in the model calculations. Reduced dissipation coefficient in the range of 1\textendash3 $\times$ $10^{21}$ s$^{-1}$ reproduces the data quite well. No abrupt enhancement of evaporation residue cross sections has been observed in the reaction forming compound nucleus with $Z = 82$. Thus, this work does not find enhanced stabilizing effects of $Z = 82$ shell closure against fission in the compound nucleus. One may attempt to measure cross sections of individual exit channels for further confirmation of our observation.

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Effect of direct reaction channels on deep sub-barrier fusion in asymmetric systems

A steeper fall of fusion excitation function, compared to the predictions of coupled-channels models, at energies below the lowest barrier between the reaction partners, is termed as deep sub-barrier fusion hindrance. This phenomenon has been observed in many symmetric and nearly-symmetric systems. Different physical origins of the hindrance have been proposed. This work aims to study the probable effects of direct reactions on deep sub-barrier fusion cross sections. Fusion (evaporation residue) cross sections have been measured for the system $^{19}$F+$^{181}$Ta, from above the barrier down to the energies where fusion hindrance is expected to come into play. Coupled-channels calculation with standard Woods-Saxon potential gives a fair description of the fusion excitation function down to energies $\simeq 14\%$ below the barrier for the present system. This is in contrast with the observation of increasing fusion hindrance in asymmetric reactions induced by increasingly heavier projectiles, \textit{viz.} $^{6,7}$Li, $^{11}$B, $^{12}$C and $^{16}$O. The asymmetric reactions, which have not shown any signature of fusion hindrance within the measured energy range, are found to be induced by projectiles with lower $α$ break-up threshold, compared to the reactions which have shown signatures of fusion hindrance. In addition, most of the $Q$-values for light particles pick-up channels are negative for the reactions which have exhibited strong signatures of fusion hindrance, \textit{viz.} $^{12}$C+$^{198}$Pt and $^{16}$O+$^{204,208}$Pb. Thus, break-up of projectile and particle transfer channels with positive $Q$-values seem to compensate for the hindrance in fusion deep below the barrier. Inclusion of break-up and transfer channels within the framework of coupled-channels calculation would be of interest.

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Fission fragment mass distributions in reactions populating 200Pb

The fission fragment mass distributions have been measured in the reactions 16O + 184W and 19F+ 181Ta populating the same compound nucleus 200Pb? at similar excitation energies. It is found that the widths of the mass distribution increases monotonically with excitation energy, indicating the absence of quasi-fission for both reactions. This is contrary to two recent claims of the presence of quasi-fission in the above mentioned reactions.

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Interplay of fission modes in mass distribution of light actinide nuclei 225,227Pa

Fission-fragment mass distributions were measured for 225,227Pa nuclei formed in fusion reactions of 19F + 206, 208Pb around fusion barrier energies. Mass-angle correlations do not indicate any quasi-fission like events in this bombarding energy range. Mass distributions were fitted by Gaussian distribution and mass variance extracted. At below-barrier energies, the mass variance was found to increase with decrease in energy for both nuclei. Results from present work were compared with existing data for induced fission of 224, 226Th and 228U around barrier energies. Enhancement in mass variance of 225, 227Pa nuclei at below-barrier energies shows evidence for presence of asymmetric fission events mixed with symmetric fission events. This is in agreement with the results of mass distributions of nearby nuclei 224, 226Th and 228U where two-mode fission process was observed. Two-mode feature of fission arises due to the shell effects changing the landscape of the potential energy surfaces at low excitation energies. The excitation-energy dependence of the mass variance gives strong evidence for survival of microscopic shell effects in fission of light actinide nuclei 225, 227Pa with initial excitation energy ~30 - 50 MeV.

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