arXiv subjects

R. Dunlop

Publications and source records attributed to R. Dunlop.

At least 19 recordsLinked to original sources

arXiv2023

Decay Spectroscopy of $^{160}$Eu: Quasiparticle Configurations of Excited States and Structure of $K^π$=$4^+$ Band-heads in $^{160}$Gd

\noindent \textbf{Background:} Detailed spectroscopy of neutron-rich, heavy, deformed nuclei is of broad interest for nuclear astrophysics and nuclear structure. Nuclei in the r-process path and following freeze-out region impact the resulting r-process abundance distribution, and the structure of nuclei midshell in both proton and neutron number helps to understand the evolution of subshell gaps and large deformation in these nuclei. \noindent \textbf{Purpose:} To improve the understanding of the nuclear structure of $^{160}$Gd, specifically the $K^π$=$4^+$ bands, as well as study the $β$-decay of $^{160}$Eu into $^{160}$Gd. \noindent \textbf{Methods:} High-statistics decay spectroscopy of $^{160}$Gd resulting from the $β$-decay of $^{160}$Eu was collected using the GRIFFIN spectrometer at the TRIUMF-ISAC facility. \noindent \textbf{Results:} Two new excited states and ten new transitions were observed in $^{160}$Gd. The $β$-decaying half-lives of the low- and high-spin isomer in $^{160}$Eu were determined, and the low-spin state's half-life was measured to be $t_{1/2}=26.0(8)$~s, $\sim$16\% shorter than previous measurements. Lifetimes of the two $K^π$=$4^+$ band-heads in $^{160}$Gd were measured for the first time, as well as $γ$-$γ$ angular correlations and mixing ratios of intense transitions out of those band-heads. \noindent \textbf{Conclusions:} Lifetimes and mixing ratios suggest that the hexadecapole phonon model of the $K^π$=$4^+$ band-heads in $^{160}$Gd is preferred over a simple two-state strong mixing scenario, although further theoretical calculations are needed to fully understand these states. Additionally, the 1999.0 keV state in $^{160}$Gd heavily populated in $β$-decay is shown to have positive parity, which raises questions regarding the structure of the high-spin $β$-decaying state in $^{160}$Eu.

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arXiv2022

High-precision half-life determination of $^{14}$O via direct $β$ counting

The half-life of the superallowed Fermi $β^+$ emitter $^{14}$O was determined to high precision via a direct $β$ counting experiment performed at the Isotope Separator and Accelerator (ISAC) facility at TRIUMF. The result, $T_{1/2}$($^{14}$O) = 70619.2(76) ms, is consistent with, but is more precise than, the world average obtained from 11 previous measurements. Combining the $^{14}$O half-life deduced in the present work with the previous most precise measurements of this quantity leads to a reduction in the overall uncertainty, by nearly a factor of 2. The new world average is $T_{1/2}$($^{14}$O) = 70619.6(63) ms with a reduced $χ^2$ value of 0.87 obtained from 8 degrees of freedom.

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arXiv2021

$^{145}$Ba and $^{145, 146}$La structure from lifetime measurements

The occurrence of octupole shapes in even-mass neutron-rich Ba isotopes has been well established. However, the situation with the odd-mass Ba and odd or odd-odd La nuclei around them is far from settled. In order to shed light on these less-studied isotopes, a fast-timing experiment was performed using GRIFFIN at TRIUMF-ISAC. A wealth of excited-state lifetimes in the 100~ps to few ns range have been measured in $^{144, 145, 146}$Ba and $^{145,146}$La populated in the $β^-$ and $β^--n$ decay of $^{145,146}$Cs. The results do not allow to draw firm conclusions on the possible octupole deformation of these nuclei but suggest different spin and parity assignments than previous works. This work highlights the need for more detailed study of the odd and odd-odd isotopes in this region to properly understand their structure.

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arXiv2021

Spectroscopic studies of neutron-rich $^{129}$In and its $β$-decay daughter, $^{129}$Sn, using the GRIFFIN spectrometer

The $β$-decay of neutron-rich $^{129}$In into $^{129}$Sn was studied using the GRIFFIN spectrometer at the ISAC facility at TRIUMF. The study observed the half-lives of the ground state and each of the $β$-decaying isomers. The level scheme of $^{129}$Sn has been expanded with thirty-one new $γ$-ray transitions and nine new excited levels, leading to a re-evaluation of the $β$-branching ratios and level spin assignments. The observation of the $β$-decay of the (29/2$^{+}$) 1911-keV isomeric state in $^{129}$In is reported for the first time, with a branching ratio of 2.0(5)$\%$.

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arXiv2020

High-Precision Branching Ratio Measurement and Spin Assignment Implications for $^{62}$Ga Superallowed $β$ Decay

A high-precision branching ratio measurement for the superallowed Fermi $β^{+}$ emitter $^{62}$Ga was performed with the Gamma-Ray Infrastructure for Fundamental Investigations of Nuclei (GRIFFIN) spectrometer at the Isotope Separator and Accelerator (ISAC) radioactive ion beam facility at TRIUMF. The high efficiency of the GRIFFIN spectrometer allowed 63 $γ$-ray transitions, with intensities down to $\approx$1 part per million (ppm) per $^{62}$Ga $β^{+}$ decay, to be placed in the level scheme of the daughter nucleus $^{62}$Zn, establishing the superallowed $β$ branching ratio for $^{62}$Ga decay to be 99.8577$^{+0.0023}_{-0.0029}\%$, a factor of 4 more precise than the previous world average. For several cascades, $γ-γ$ angular correlation measurements were performed to assign spins and/or determine the mixing ratios of transitions. In particular, the spin of the 2.342 MeV excited state in the daughter nucleus $^{62}$Zn was definitively assigned as $J = 0$. This assignment resolves a discrepancy between previous measurements and has important implications for the isospin symmetry breaking correction, $δ_{C1}$, in $^{62}$Ga superallowed Fermi $β$ decay.

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arXiv2020

Spectroscopic study of $^{47}$Ca from the $β^-$ decay of $^{47}$K

The $β^-$ decay of $^{47}$K to $^{47}$Ca is an appropriate mechanism for benchmarking interactions spanning the $sd$ and $pf$ shells, but current knowledge of the $β^-$-decay scheme is limited. We have performed a high-resolution, high-efficiency study of the $β^-$-decay of $^{47}$K with the GRIFFIN spectrometer at TRIUMF-ISAC. The study revealed 48 new transitions, a more precise value for the $^{47}$K half-life (17.38(3)~s), and new spin and parity assignments for eight excited states. Levels placed for the first time here raise the highest state observed in $β^-$ decay to within 568(3) keV of the $Q$-value and confirm the previously measured large $β^-$-decay branching ratios to the low-lying states. Previously unobserved $β^-$-feeding to 3/2$^+$ states between 4.5 and 6.1~MeV excitation energy was identified with a total $β^-$-feeding intensity of 1.29(2)\%. The sum of the $B(GT)$ values for these states indicates that the $1s_{1/2}$ proton hole strength near this excitation energy is comparable to the previously known $1s_{1/2}$ proton and neutron hole strengths near 2.6 MeV.

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arXiv2020

Decay Spectroscopy of $^{129}$Cd

Excited states of $^{129}$In populated following the $β$-decay of $^{129}$Cd were experimentally studied with the GRIFFIN spectrometer at the ISAC facility of TRIUMF, Canada. A 480-MeV proton beam was impinged on a uranium carbide target and $^{129}$Cd was extracted using the Ion Guide Laser Ion Source (IG-LIS). $β$- and $γ$-rays following the decay of $^{129}$Cd were detected with the GRIFFIN spectrometer comprising the plastic scintillator SCEPTAR and 16 high-purity germanium (HPGe) clover-type detectors. %, along with the $β$-particles were detected with SCEPTAR. From the $β$-$γ$-$γ$ coincidence analysis, 32 new transitions and 7 new excited states were established, expanding the previously known level scheme of $^{129}$In. The $\log ft$ values deduced from the $β$-feeding intensities suggest that some of the high-lying states were populated by the $ν0 g_{7/2} \rightarrow π0 g_{9/2}$ allowed Gamow-Teller (GT) transition, which indicates that the allowed GT transition is more dominant in the $^{129}$Cd decay than previously reported. Observation of fragmented Gamow-Teller strengths is consistent with theoretical calculations.

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arXiv2020

$β$ Decay of $^{132}$In and Spectroscopy of $^{132}$Sn and $^{131}$Sb with the GRIFFIN Spectrometer

Spectroscopy of doubly magic $^{132}_{50}$Sn$_{82}$ has been performed with the GRIFFIN spectrometer at TRIUMF-ISAC following the $β$ decay of $^{132}_{49}$In$_{83}$. The analysis has allowed for the placement of a total of 70 transitions and 29 excited states in $^{132}$Sn. Detailed spectroscopy has also been performed on $^{131}$Sb, resulting from the $β$ decay of $^{131}$Sn, produced from the $β$-delayed neutron decay of $^{132}$In. Measurement of $γ$-rays in both $^{131}$Sn and $^{131}$Sb has led to the determination of the $β$-delayed neutron emission probability, $P_{n}$, from $^{132}$In. This is the first time the $P_{n}$ has been measured for this nucleus using $γ$ spectroscopy, and the new value of 12.3(4)% is consistent with the most recent $β-n$ counting experiment. Additionally, $γ$-$γ$ angular correlations have been performed in $^{132}$Sn, supporting the spin assignments of several excited states. Novel ab initio calculations are presented which describe several of the excited states, and these are compared to the experimental spectrum.

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arXiv2020

Collective 2p-2h intruder states in $^{118}$Sn studied via $β$-decay of $^{118}$In using GRIFFIN

The low-lying structure of semi-magic $^{118}$Sn has been investigated through the $β$-decay of $^{118}$In ($T_{1/2}=4.45$ min) to study shape coexistence via the reduced transition probabilities of states in the 2p-2h proton intruder band. This high-statistics study was carried out at TRIUMF-ISAC with the GRIFFIN spectrometer. In total, 99 transitions have been placed in the level scheme with 43 being newly observed. Three low-lying $γ$-ray transitions with energies near 285 keV have been resolved from which the 2$^+_{\mathrm{intr.}} \rightarrow 0^+_{\mathrm{intr.}}$ 284.52-keV transition was determined to have half of the previous branching fraction leading to a $B(E2;2^+_2\rightarrow 0^+_2)$ of 21(4) W.u. compared to 39(7) W.u. from the previous measurement. Calculations using $sd$ IBM-2 with mixing have also been made to compare the experimental $B(E2)$ values to the theoretical values and to make comparisons to the $^{114,116}$Sn isotopes previously studied using the same theoretical model.

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arXiv2020

Branching ratio of the super-allowed beta decay of 10C

In an experiment performed at the ISOLDE facility of CERN, the super-allowed beta-decay branching ratio of 10C was determined with a high-precision single-crystal germanium detector. In order to evaluate the contribution of the pile-up of two 511 keV gamma quanta to one of the gamma-ray peaks of interest at 1021.7 keV, data were not only taken with 10C, but also with a 19Ne beam. The final result for the super-allowed decay branch is 1.4638(50)%, in agreement with the average from literature.

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arXiv2019

Detailed spectroscopy of $^{46}$Ca: A study of the $β^-$ decay of $^{46}$K

We report on high-statistics data from the $β^-$ decay of the $^{46}$K $J^π$ = 2$^-$ ground state taken with the GRIFFIN spectrometer located at the TRIUMF-ISAC facility. In total, 199 $γ$ rays and 42 excited states were placed in the level scheme, and from the observed $β$ feeding and angular correlations of pairs of cascading $γ$ rays, it was possible to assign spins and parities to excited states and determine mixing ratios for selected $γ$ rays. The level structure of $^{46}$Ca is compared to theoretical predictions from a microscopic valence-space Hamiltonian derived from two- (NN) and three-nucleon (3N) forces. These calculations are in reasonable agreement with the experimental data and indicate that the protons in this region are not as inert as would be expected for semi-magic nuclei.

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arXiv2019

Precise branching ratio measurements in $^{19}$Ne beta decay and fundamental tests of the weak interaction

We used the 8$π$ $γ$-ray spectrometer at the TRIUMF-ISAC radiocative ion beam facility to obtain high-precision branching ratios for $^{19}$Ne $β^+$ decay to excited states in $^{19}$F. Together with other previous work, our measurements determine the superallowed $1/2^+ \to 1/2^+$ beta branch to the ground state in $^{19}$F to be 99.9878(7)\%, which is three times more precise than known previously. The implications of these measurements for testing a variety of weak interaction symmetries are discussed briefly.

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arXiv2019

$β$ and $β$-delayed neutron decay of the $N=82$ nucleus $^{131}_{~49}$In$_{82}$

The half-lives of three $β$ decaying states of $^{131}_{~49}$In$_{82}$ have been measured with the GRIFFIN $γ$-ray spectrometer at the TRIUMF-ISAC facility to be $T_{1/2}(1/2^-)=328(15)$~ms, $T_{1/2}(9/2^+)=265(8)$~ms, and $T_{1/2}(21/2^+)=323(55)$~ms, respectively. The first observation of $γ$-rays following the $βn$ decay of $^{131}$In into $^{130}$Sn is reported. The $β$-delayed neutron emission probability is determined to be $P_{1n} = 12(7)\%$ for the $21/2^+$ state and $2.3(3)\%$ from the combined $1/2^-$ and $9/2^+$ states of $^{131}_{~49}$In$_{82}$ observed in this experiment. A significant expansion of the decay scheme of $^{131}$In, including 17 new excited states and 34 new $γ$-ray transitions in $^{131}_{~50}$Sn$_{81}$ is also reported. This leads to large changes in the deduced $β$ branching ratios to some of the low-lying states of $^{131}$Sn compared to previous work with implications for the strength of the first-forbidden $β$ transitions in the vicinity of doubly-magic $^{132}_{~50}$Sn$_{82}$.

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arXiv2018

The GRIFFIN Facility for Decay-Spectroscopy Studies at TRIUMF-ISAC

Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei, GRIFFIN, is a new high-efficiency $γ$-ray spectrometer designed for use in decay spectroscopy experiments with low-energy radioactive ion beams provided by TRIUMF's Isotope Separator and Accelerator (ISAC-I) facility. GRIFFIN is composed of sixteen Compton-suppressed large-volume clover-type high-purity germanium (HPGe) $γ$-ray detectors combined with a suite of ancillary detection systems and coupled to a custom digital data acquisition system. The infrastructure and detectors of the spectrometer as well as the performance characteristics and the analysis techniques applied to the experimental data are described.

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arXiv2018

Half-Lives of Neutron Rich $^{130}$Cd and $^{131}$In

The half-lives of isotopes around the $N=82$ shell closure are an important ingredient in astrophysical simulations and strongly influence the magnitude of the second $r$-process abundance peak in the $A\sim130$ region. The most neutron-rich $N=82$ nuclei are not accessible to the current generation of radioactive beam facilities and $r$-process simulations must therefore rely on calculations of the half-lives of the isotopes involved. Half-life measurements of the experimentally accessible nuclei in this region are important in order to benchmark these calculations. The half-life of $^{130}$Cd is particularly important as it is used to tune the Gamow-Teller quenching in shell-model calculations for the $β$ decay of other nuclei in this region. In this work, the GRIFFIN $γ$-ray spectrometer at the TRIUMF-ISAC facility was used to measure the half-life of $^{130}_{~48}$Cd$_{82}$ to be $T_{1/2}= 126(4)$ ms. In addition, the half-lives of the three $β$ decaying states of $^{131}_{~49}$In$_{82}$ were measured to be $T_{1/2}(1/2^-)=328(15)$ ms, $T_{1/2}(9/2^+)=265(8)$ ms, and $T_{1/2}(21/2^+)=323(50)$ ms, respectively, providing an important benchmark for half-life calculations in this region.

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arXiv2018

High-resolution (p,t) reaction measurements as spectroscopic tests of {\it ab-initio} theory in the mid $pf$-shell

Detailed spectroscopic measurements of excited states in $^{50}$Cr and $^{62}$Zn were performed using 24~MeV (p,t) transfer reactions on $^{52}$Cr and $^{64}$Zn, respectively. In total, forty-five states in $^{50}$Cr and sixty-seven states in $^{62}$Zn were observed up to excitation energies of 5.5~MeV, including several previously unobserved states. These experimental results are compared to {\it ab-initio} shell-model calculations using chiral effective field theory ($χ$-EFT) with the valence-space in-medium similarity renormalization group (VS-IMSRG) method. This comparison demonstrates good agreement in the level orderings with these new theoretical methods, albeit with a slight over binding in the calculations. This work is part of a continued push to benchmark {\it ab-initio} theoretical techniques to nuclear structure data in $0^+\rightarrow0^+$ superallowed Fermi $β$ decay systems.

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arXiv2018

In-beam internal conversion electron spectroscopy with the SPICE detector

The SPectrometer for Internal Conversion Electrons (SPICE) has been commissioned for use in conjunction with the TIGRESS $γ$-ray spectrometer at TRIUMF's ISAC-II facility. SPICE features a permanent rare-earth magnetic lens to collect and direct internal conversion electrons emitted from nuclear reactions to a thick, highly segmented, lithium-drifted silicon detector. This arrangement, combined with TIGRESS, enables in-beam $γ$-ray and internal conversion electron spectroscopy to be performed with stable and radioactive ion beams. Technical aspects of the device, capabilities, and initial performance are presented.

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arXiv2017

Characteristics of GRIFFIN high-purity germanium clover detectors

The Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei, GRIFFIN, is a new experimental facility for radioactive decay studies at the TRIUMF-ISAC laboratory. The performance of the 16 high-purity germanium (HPGe) clover detectors that will make up the GRIFFIN spectrometer is reported. The energy resolution, efficiency, timing resolution, crosstalk and preamplifier properties of each crystal were measured using a combination of analogue and digital data acquisition techniques. The absolute efficiency and add-back factors are determined for the energy range of 80 - 3450 keV. The detectors show excellent performance with an average over all 64 crystals of a FWHM energy resolution of 1.89(6) keV and relative efficiency with respect to a 3"x3" NaI detector of 41(1)% at 1.3 MeV.

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