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R. F. Berger

Publications and source records attributed to R. F. Berger.

3 recordsLinked to original sources

Spin Order by Quantum Frustration in Triangular Lattice Mott Insulator NaCrO2 : A Neutron Scattering Study

We report high resolution neutron scattering measurements on the triangular lattice Mott insulator Na$_x$CrO$_2$ ($x$=1) which has recently been shown to exhibit an unusually broad fluctuating crossover regime extending far below the onset of spin freezing ($T_c\sim$41K). Our results show that below some crossover temperature ($T\sim0.75T_c$) a small incommensuration develops which helps resolve the spin frustration and drives three-dimensional magnetic order supporting coherent spin wave modes. This incommensuration assisted dimensional crossover suggests that inter-layer frustration is responsible for stabilizing the rare 2D correlated phase above 0.75$T_c$. In contrast to the host compound of 2D cobaltate superconductor such as Na$_x$CoO$_2$ ($ξ_c>50$Å), no magnetic long-range order is observed down to 1.5K ($ξ_c<16$Å).

cond-mat.str-el

Magnetic Structure and Properties of the S = 5/2 Triangular Antiferromagnet $α$-NaFeO$_2$

The magnetic properties of $α$-NaFeO$_2$ are studied by neutron diffraction and magnetization measurements. An ordered phase with spins aligned along the b$_hex$ axis exists at low temperatures (T < 4 K). At intermediate temperatures (4 K < T < 11 K), the system passes through an incommensurate ordered phase before transforming into a short range ordered state at higher temperatures that persists up to at least 50 K. Although the short range ordering does not persist to room temperature according to neutron diffraction, the magnetic susceptibility does not follow Curie-Weiss behavior, even up to 320 K. This rich magnetic behavior can be understood qualitatively as a competition between different magnetic exchange interactions that are similar in magnitude. The delicate balance between these interactions makes $α$-NaFeO$_2$ a candidate for more detailed theoretical work to understand magnetic behavior in frustrated magnetic systems.

cond-mat.str-el

Unconventional Dynamics in Triangular Heisenberg Antiferromagnet NaCrO2

We report magnetization, specific heat, muon spin rotation and Na NMR measurements on the S=3/2 rhombohedrally stacked Heisenberg antiferromagnet NaCrO2. This compound appears to be an ideal candidate for the study of triangular Heisenberg antiferromagnets with very weak interlayer coupling. While specific heat and magnetization measurements indicate the occurrence of a transition in the range 40-46 K, both muon spin rotation and NMR reveal a fluctuating regime extending well below T_c, with a peak of relaxation rate 1/T1 around 30 K. This novel finding is discussed within the context of excitations in the triangular Heisenberg antiferromagnets.

cond-mat.str-el