arXiv subjects

R. Giri

Publications and source records attributed to R. Giri.

10 recordsLinked to original sources

arXiv2022

Elastic scattering of 3He+4He with SONIK

Measurements of the elastic scattering cross section of 3He and 4He are important in order to improve constraints on theoretical models of 4He(3He,g)7Be, a key reaction in Big Bang nucleosynthesis and solar neutrino production. The astrophysical S-factor for this reaction is a significant source of uncertainty in the standard solar-model prediction of the 7Be and 8B solar neutrino fluxes. The elastic scattering measurements reported in the literature do not extend to low energies and lack proper uncertainty quantification. A new measurement of the 4He(3He,3He)4He reaction has been made at center-of-mass energies Ec.m. = 0.38-3.13 MeV using the Scattering of Nuclei in Inverse Kinematics (SONIK) scattering chamber: a windowless, extended gas target surrounded by an array of 30 collimated silicon charged particle detectors situated at TRIUMF. This is the first elastic scattering measurement of 3He+4He made below 500 keV and it has greater angular range and better precision than previous measurements. The elastic scattering data were analyzed using both R-matrix and Halo Effective Field Theory (Halo EFT) frameworks, and values of the s-wave scattering length and effective range were extracted. The resulting improvement in knowledge of the s-wave effective-range function at low energies will reduce the overall uncertainty in S34 at solar energies.

nucl-ex↗

arXiv2022

Direct measurement of resonances in $^7$Be($α,γ$)$^{11}$C relevant to $νp$-process nucleosynthesis

We have performed the first direct measurement of two resonances of the $^7$Be($α,γ$)$^{11}$C reaction with unknown strengths using an intense radioactive $^7$Be beam and the DRAGON recoil separator. We report on the first measurement of the 1155 and 1110 keV resonance strengths of $1.73 \pm 0.25(stat.) \pm 0.40(syst.)$ eV and $125 ^{+27}_{-25}(stat.) \pm 15(syst.)$ meV, respectively. The present results have reduced the uncertainty in the $^7$Be($α,γ$)$^{11}$C reaction rate to $\sim$ 9.4-10.7% over T = 1.5-3 GK, which is relevant for nucleosynthesis in the neutrino-driven outflows of core-collapse supernovae ($νp$-process). We find no effect of the new, constrained reaction rate on $νp$-process nucleosynthesis.

nucl-ex↗

arXiv2022

First inverse kinematics measurement of resonances in $^7$Be($α,γ$)$^{11}$C relevant to neutrino-driven wind nucleosynthesis using DRAGON

A possible mechanism to explain the origin of the light $p$-nuclei in the Galaxy is the nucleosynthesis in the proton-rich neutrino-driven wind ejecta of core-collapse supernovae via the $νp$-process. However this production scenario is very sensitive to the underlying supernova dynamics and the nuclear physics input. As far as the nuclear uncertainties are concerned, the breakout from the $pp$-chains via the $^7$Be($α,γ$)$^{11}$C reaction has been identified as an important link which can influence the nuclear flow and therefore the efficiency of the $νp$-process. However its reaction rate is poorly known over the relevant temperature range, T = 1.5-3 GK. We report on the first direct measurement of two resonances of the $^7$Be($α,γ$)$^{11}$C reaction with previously unknown strengths using an intense radioactive $^7$Be beam from the ISAC facility and the DRAGON recoil separator in inverse kinematics. We have decreased the $^7$Be($α,γ$)$^{11}$C reaction rate uncertainty to $\sim$ 9.4-10.7% over the relevant temperature region.

nucl-ex↗

arXiv2022

Proton and neutron exchange as a prelude to fusion at near-barrier energies

Systematic examination of fusion for $^{39,41,45,47}$K + $^{28}$Si and $^{36,44}$Ar + $^{28}$Si provides insight into the impact of neutron and proton exchange on fusion for nuclei at and near the N=20 and N=28 shells. Comparison of the reduced excitation functions reveals a marked difference between the behavior of open-shell and closed-shell systems. While coupled channels calculations provide a good description for the closed-shell nuclei they significantly under-predict the fusion cross-section for open-shell nuclei. The observed trends are examined in the context of a potential energy surface, including shell effects, and multi-nucleon exchange with consideration of Pauli-blocking.

nucl-ex↗

arXiv2020

Beyond the acceptance limit of DRAGON: the case of the $\mathrm{^6Li(α,γ)^{10}B}$ reaction

Radiative capture reactions play a pivotal role for our understanding of the origin of the elements in the cosmos. Recoil separators provide an effective way to study these reactions, in inverse kinematics, and take advantage of the use of radioactive ion beams. However, a limiting factor in the study of radiative capture reactions in inverse kinematics is the momentum spread of the product nuclei, which can result in an angular spread larger than the geometric acceptance of the separator. The DRAGON facility at TRIUMF is a versatile recoil separator, designed to study radiative capture reactions relevant to astrophysics in the $\mathrm{A \sim 10-30}$ region. In this work we present the first attempt to study with DRAGON a reaction, $\mathrm{^6Li(α,γ)^{10}B}$ , for which the recoil angular spread exceeds DRAGON's acceptance. Our result is in good agreement with the literature value, showing that DRAGON can measure resonance strengths of astrophysically important reactions even when not all the recoils enter the separator.

physics.ins-det↗

arXiv2020

Constraining the destruction rate of $^{40}$K in stellar nucleosynthesis through the study of the $^{40}$Ar(p,n)$^{40}$K reaction

40K plays a significant role in the radiogenic heating of earth-like exoplanets, which can affect the development of a habitable environment on their surfaces. The initial amount of 40K in the interior of these planets depends on the composition of the interstellar clouds from which they formed. Within this context, nuclear reactions that regulate the production of 40K during stellar evolution can play a critical role. In this study, we constrain for the first time the astrophysical reaction rate of 40K(n,p)40Ar, which is responsible for the destruction of 40K during stellar nucleosynthesis. We performed differential cross-section measurements on the 40Ar(p,n)40K reaction, for six energies in the center-of-mass between 3.2 and 4.0 MeV and various angles between 0-deg and 135-deg. The experiment took place at the Edwards Accelerator Laboratory at Ohio University using the beam swinger target location and a standard neutron time-of-flight technique. The total and partial cross-sections varied with energy due to the contribution from isobaric analog states and Ericson type fluctuations. The energy-averaged neutron angular distributions were symmetrical relative to 90-deg and consistent with the theoretical predictions of the statistical model. Based on the experimental data, local transmission coefficients were extracted and were used to calculate the astrophysical reaction rates of 40Ar(p,n)40K and 40K(n,p)40Ar reactions. Our results support that the destruction rate of 40K in massive stars via the 40K(n,p)40Ar reaction is larger compared to previous estimates. This result directly affects the predicted stellar yields of 40K from nucleosynthesis, which is a critical input parameter for the galactic chemical evolution models that are currently employed for the study of significant properties of exoplanets.

nucl-ex↗

arXiv2019

$s$-wave scattering lengths for the $^7$Be+p system from an $\textit{R}$-matrix analysis

The astrophysical $S$-factor for the radiative proton capture reaction on $^7$Be ($S_{17}$) at low energies is affected by the $s$-wave scattering lengths. We report the measurement of elastic and inelastic scattering cross sections for the $^7$Be+p system in the center-of-mass energy range 0.474 - 2.740 MeV and center-of-mass angular range of 70$^\circ$- 150$^\circ$. A radioactive $^7$Be beam produced at Oak Ridge National Laboratory's (ORNL) Holifield Radioactive Ion Beam Facility was accelerated and bombarded a thin polypropylene (CH$_{2}$)$_\text n$ target. Scattered ions were detected in the segmented Silicon Detector Array. Using an $\textit{R}$-matrix analysis of ORNL and Louvain-la-Neuve cross section data, the $s$-wave scattering lengths for channel spins 1 and 2 were determined to be 17.34$^{+1.11}_{-1.33}$ and -3.18$^{+0.55}_{-0.50}$ fm, respectively. The uncertainty in the $s$-wave scattering lengths reported in this work is smaller by a factor of 5-8 compared to the previous measurement, which may reduce the overall uncertainty in $S_{17}$ at zero energy. The level structure of $^8$B is discussed based upon the results from this work. Evidence for the existence of 0$^+$ and 2$^+$ levels in $^8$B at 1.9 and 2.21 MeV, respectively, is observed.

nucl-ex↗

arXiv2018

Selective measurement of charge dynamics in an ensemble of nitrogen-vacancy centers in nano- and bulk diamonds

Nitrogen-vacancy (NV) centers in diamond have attracted considerable interest in sensing of weak magnetic fields, such as those created by biological systems. Detecting such feeble signals requires near-surface NV centers, to reduce the distance between NVs and sources. Moreover, dense ensembles of NVs are highly desirable to reduce measurement time. However, robust charge state switching is often observed in these systems, resulting in a complex interplay between charge and spin dynamics that can reduce the attainable level of spin polarization, and consequently, sensitivity. Understanding the mechanisms behind charge state switching is, therefore, crucial to developing NV based sensors. Here, we demonstrate a novel method to selectively measure charge dynamics in an ensemble of NVs by quenching the spin polarization using an off-axis magnetic field. Utilizing this technique, we show that, in nanodiamonds, charge state instability increases with increasing NV density. In the case of bulk single crystal diamond, we show that NV centers located near the surface are more stable in the neutral (NV$^{0}$) charge state, while the negatively charged (NV$^{-}$) form is more stable in bulk.

cond-mat.mes-hall↗

arXiv2018

Fast and sensitive detection of hemoglobin and other paramagnetic species using coupled charge and spin dynamics in strongly fluorescent nanodiamonds

Sensing of a few unpaired electron spins, such as metal ions and radicals, is a useful but difficult task in nanoscale physics, biology, and chemistry. Single nitrogen-vacancy (NV) centers in diamond offer high sensitivity and spatial resolution in the optical detection of weak magnetic fields produced by a spin bath, but often require long acquisition times, of the order of seconds. Here we use a novel approach, based on coupled spin and charge dynamics in dense NV ensembles in strongly fluorescent nanodiamonds (NDs) to sense external magnetic dipoles. We apply this approach to various paramagnetic species, including gadolinium complexes, magnetite nanoparticles and hemoglobin in whole blood. Taking advantage of the high NV density, we demonstrate detection of subnanomolar amounts of Gd spins with ultrashort acquisition time approaching 10 ms. Strong luminescence, high sensitivity and short acquisition time make dense NV- ensembles in NDs a powerful tool for biosensing and bioimaging applications.

cond-mat.mes-hall↗

arXiv2017

Coupled charge and spin dynamics in high-density ensembles of nitrogen-vacancy centers in diamond

We studied the spin depolarization of ensembles of nitrogen-vacancy (NV) centers in nitrogen-rich single crystal diamonds. We found a strong dependence of the evolution of the polarized state in the dark on the concentration of NV centers. At low excitation power, we observed a simple exponential decay profile in the low-density regime and a paradoxical inverted exponential profile in the high-density regime. At higher excitation power, we observed complex behavior, with an initial sharp rise in luminescence signal after the preparation pulse followed by a slower exponential decay. Magnetic field and excitation laser power-dependent measurements suggest that the rapid initial increase of the luminescence signal is related to recharging of the nitrogen-vacancy centers (from neutral to negatively charged) in the dark. The slow relaxing component corresponds to the longitudinal spin relaxation of the NV ensemble. The shape of the decay profile reflects the interplay between two mechanisms: the NV charge state conversion in the dark and the longitudinal spin relaxation. These mechanisms, in turn, are influenced by ionization, recharging and polarization dynamics during excitation. Interestingly, we found that charge dynamics are dominant in NV-dense samples even at very feeble excitation power. These observations may be important for the use of ensembles of NV centers in precession magnetometry and sensing applications.

cond-mat.mes-hall↗