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R. J. Birgeneau

Publications and source records attributed to R. J. Birgeneau.

At least 127 records · Page 7Linked to original sources

Energy Spectrum of Spin Fluctuations in Superconducting La2-xSrxCuO4 (0.10 < x < 0.25)

The energy spectrum of incommensurate spin fluctuations in superconducting Sr-doped La2CuO4 has been studied by inelastic neutron scattering experiments. An energy gap in the spin excitation spectrum is observed in the superconducting state of optimally doped (x=0.15) and slightly overdoped (x=0.18) samples. At temperatures well below Tc, the incommensurate peaks diminish rapidly in intensity with decreasing energy below ~8meV and merge into the background below ~3.5meV for x=0.15 and ~4.5meV for x=0.18. For both samples, the energy spectrum of the q-integrated spin susceptibility, x"(w), exhibits an enhancement around 7meV, which is caused by a broadening in the momentum width of the incommensurate peaks. The gap-like structure in the energy spectrum and the enhancement of x"(w) survive at Tc. On the other hand, for both underdoped (x=0.10) and heavily overdoped (x=0.25) samples there is neither a clear energy gap nor an enhancement of x"(w) below Tc.

cond-mat.supr-con↗

Incommensurate Geometry of the Elastic Magnetic Peaks in Superconducting La1.88Sr0.12CuO4

We report magnetic neutron scattering measurements of incommensurate magnetic order in a superconducting single crystal of La1.88Sr0.12CuO4. We find that the incommensurate wavevectors which describe the static magnetism do not lie along high-symmetry directions of the underlying CuO2 lattice. The positions of the elastic magnetic peaks are consistent with those found in excess-oxygen doped La2CuO4+y. This behavior differs from the precise magnetic order found in the low temperature tetragonal La1.6-xNd0.4SrxCuO4 material for which stripes of spin and charge have been observed. These observations have clear implications for any stripe model proposed to describe the static magnetism in orthorhombic La2CuO4-based superconductors.

cond-mat.supr-con↗

Direct Observation of a One Dimensional Static Spin Modulation in Insulating La1.95Sr0.05CuO4

We report the results of an extensive elastic neutron scattering study of the incommensurate (IC) static spin correlations in La1.95Sr0.05CuO4 which is an insulating spin glass at low temperatures. The present neutron scattering experiments on the same x=0.05 crystal employ a narrower instrumental Q-resolution and thereby have revealed that the crystal has only two orthorhombic twins at low temperatures with relative populations of 2:1. We find that, in a single twin, only two satellites are observed at (1, +/-0.064, L)(ortho) and (0, 1+/-0.064, L)(ortho), that is, the modulation vector is only along the orthorhombic b*-axis. This demonstrates unambiguously that La1.95Sr0.05CuO4 has a one-dimensional static diagonal spin modulation at low temperatures, consistent with certain stripe models. We have also reexamined the x=0.04 crystal that previously was reported to show a single commensurate peak. By mounting the sample in the (H, K, 0) zone, we have discovered that the x=0.04 sample in fact has the same IC structure as the $x=0.05$ sample. The incommensurability parameter d for x=0.04 and 0.05, where d is the distance from (1/2, 1/2) in tetragonal reciprocal lattice units, follows the linear relation d=x. These results demonstrate that the insulator to superconductor transition in the under doped regime (0.05 </= x </= 0.06) in La2-xSrxCuO4 is coincident with a transition from diagonal to collinear static stripes at low temperatures thereby evincing the intimate coupling between the one dimensional spin density modulation and the superconductivity.

cond-mat.supr-con↗

Freezing of anisotropic spin clusters in La1.98Sr0.02CuO4

A spin-glass compound, La$_{1.98}$Sr$_{0.02}$CuO$_4$, shows quasi-three-dimensional magnetic ordering below $\sim$40 K. A remarkable feature is that the magnetic correlation length along the orthorhombic $a\rm_{ortho}$ axis is much longer than that along the $b\rm_{ortho}$ axis, suggesting that the spin structure is closely related to the diagonal stripe structure. The spin-glass state can be expressed as a random freezing of quasi-three-dimensional spin clusters with anisotropic spin correlations ($ξ'_a\sim160$ Å, $ξ'_b\sim25$ Å, and $ξ'_c\sim4.7$ Åat 1.6 K). The new magnetic state is important as an intermediate phase between the three-dimensional antiferromagnetic ordered phase in La$_2$CuO$_4$ and the incommensurate phase in La$_{1.95}$Sr$_{0.05}$CuO$_4$ in which the positions of the incommensurate peaks are rotated by 45$^\circ$ in reciprocal space about ($π$,$π$) from those observed in the superconducting La$_2$CuO$_4$ compounds.

cond-mat.str-el↗

The first-order phase transition between dimerized-antiferromagnetic and uniform-antiferromagnetic phases in Cu_(1-x)M_xGeO_3

We have performed detailed magnetic susceptibility measurements as well as synchrotron x-ray diffraction studies to determine the temperature vs concentration ($T$ - $x$) phase diagram of Cu${}_{1-x}$Mg${}_x$GeO${}_3$. We observe clear double peaks in the magnetic susceptibility implying two antiferromagnetic (AF) transition temperatures in samples with Mg concentrations in the range 0.0237 $\le x \le$ 0.0271. We also observe a drastic change in the inverse correlation length in this concentration range by x-ray diffraction. The drastic change of the AF transition temperature as well as the disappearance of the spin-Peierls (SP) phase have been clarified; these results are consistent with a first-order phase transition between dimerized AF (D-AF) and uniform AF (U-AF) phases as reported by T. Masuda {\it et al.} \lbrack Phys. Rev. Lett. {\bf 80}, 4566 (1998)\rbrack. The $T$ - $x$ phase diagram of Cu${}_{1-x}$Zn${}_x$GeO${}_3$ is similar to that of Cu${}_{1-x}$Mg${}_x$GeO${}_3$, which suggests that the present phase transition is universal for Cu${}_{1-x}M_{x}$GeO${}_3$.

cond-mat.str-el↗

Reentrant Spin-Peierls Transition in Mg-Doped CuGeO_3

We report a synchrotron x-ray scattering study of the diluted spin-Peierls (SP) material Cu_{1-x}Mg_xGeO_3. In a recent paper we have shown that the SP dimerization attains long-range order only for x < x_c = 0.022(0.001). Here we report that the SP transition is reentrant in the vicinity of the critical concentration x_c. This is manifested by broadening of the SP dimerization superlattice peaks below the reentrance temperature, T_r, which may mean either the complete loss of the long-range SP order or the development of a short-range ordered component within the long-range ordered SP state. Marked hysteresis and very large relaxation times are found in the samples with Mg concentrations in the vicinity of x_c. The reentrant transition is likely related to the competing Neel transition which occurs at a temperature similar to T_r. We argue that impurity-induced competing interchain interactions play an essential role in these phenomena.

cond-mat.str-el↗

Structural Critical Scattering Study of Mg-Doped CuGeO3

We report a synchrotron x-ray scattering study of the diluted spin-Peierls (SP) material Cu_(1-x)Mg_xGeO_3. We find that for x>0 the temperature T_m at which the spin gap is established is significantly higher than the temperature T_s at which the SP dimerization attains long-range order. The latter is observed only for x x_c the SP correlation length quickly decreases with increasing x. We argue that impurity-induced competing interactions play a central role in these phenomena.

cond-mat.str-el↗

Neutron Scattering Study of Spin Density Wave Order in the Superconducting State of Excess-Oxygen-Doped La2CuO4+y

We report neutron scattering measurements of spin density wave order within the superconducting state of a single crystal of predominately stage-4 La2CuO4+y with a Tc(onset) of 42 K. The low temperature elastic magnetic scattering is incommensurate with the lattice and is characterized by long-range order in the copper-oxide plane with the spin direction identical to that in the insulator. Between neighboring planes, the spins exhibit short-range correlations with a stacking arrangement reminiscent of that in the undoped antiferromagnetic insulator. The elastic magnetic peak intensity appears at the same temperature within the errors as the superconductivity, suggesting that the two phenomena are strongly correlated. These observations directly reveal the persistent influence of the antiferromagnetic order as the doping level increases from the insulator to the superconductor. In addition, our results confirm that spin density wave order for incommensurabilities near 1/8 is a robust feature of the La2CuO4-based superconductors.

cond-mat.supr-con↗

Spin-Peierls Transition in CuGeO_3: Critical, Tricritical, or Mean Field?

The spin-Peierls phase transition in CuGeO_3 has been extensively studied utilizing a variety of experimental techniques. Interpretations of the phase transition behavior vary from tricritical to mean field to Ising critical to XY critical. We show that the behavior in the vicinity of the phase transition of each of the order parameter, the magnetic energy gap and the heat capacity can be quantitatively fitted with few adjustable parameters with a mean field model incorporating a tricritical to mean field critical crossover in the transition region.

cond-mat.str-el↗

Observation of New Incommensurate Magnetic Correlations at the Lower Critical Concentration for Superconductivity (x=0.05) in La(2-x)Sr(x)CuO4

Neutron-scattering experiments have been performed on lightly-doped La(2-x)Sr(x)CuO4 single crystals in both the insulating (x=0.03,0.04,0.05) and superconducting (x=0.06) regions. Elastic magnetic peaks are observed at low temperatures in all samples with the maximum peak linewidth occuring at the critical concentration x_c=0.05. New incommensurate peaks are observed only at x=0.05, the positions of which are rotated by 45 degrees in reciprocal space about (pi,pi) from those observed for x>=0.06 in the superconducting phase.

cond-mat.supr-con↗

Neutron Scattering Study of Elastic Magnetic Signals in Superconducting La1.94Sr0.06Cu4

Recent neutron-scattering experiments on La(2-x)Sr(x)CuO4 single crystals by Wakimoto et al. have revealed that elastic magnetic peaks appear at low temperatures in both insulating (x=0.02-0.05) and superconducting (x=0.06) samples. We have carried out further investigations particularly on the elastic incommensurate peaks for x=0.06, and found that the integrated intensity drastically changes across the low temperature insulator- superconductor boundary; the intensity of x=0.06 is 4 times smaller than that of x=0.05, while the intensity in the insulating region stays constant.

cond-mat.supr-con↗

Instantaneous Spin Correlations in La2CuO4

We have carried out a neutron scattering study of the instantaneous spin-spin correlations in La2CuO4 (T_N = 325 K) over the temperature range 337 K to 824 K. Incident neutron energies varying from 14.7 meV to 115 meV have been employed in order to guarantee that the energy integration is carried out properly. The results so-obtained for the spin correlation length as a function of temperature when expressed in reduced units agree quantitatively both with previous results for the two dimensional (2D) tetragonal material Sr2CuO2Cl2 and with quantum Monte Carlo results for the nearest neighbor square lattice S=1/2 Heisenberg model. All of the experimental and numerical results for the correlation length are well described without any adjustable parameters by the behavior predicted for the quantum non-linear sigma model in the low temperature renormalized classical regime. The amplitude, on the other hand, deviates subtly from the predicted low temperature behavior. These results are discussed in the context of recent theory for the 2D quantum Heisenberg model.

cond-mat.str-el↗

Quantum Monte Carlo Study of Weakly Coupled Spin Ladders

We report a quantum Monte Carlo study of the thermodynamic properties of arrays of spin ladders with various widths ($n$), coupled via a weak inter-ladder exchange coupling $αJ$, where $J$ is the intra-ladder coupling both along and between the chains. This coupled ladder system serves as a simplified model for the magnetism of presumed ordered spin and charge stripes in the two-dimensional CuO$_2$ planes of hole-doped copper oxides. Our results for $n=3$ with weak inter-ladder coupling $α=0.05$, estimated from the $t-t'-t''-J$ model, show good agreement with the ordering temperature of the recently observed spin density wave condensation in La$_2$CuO$_{4+y}$. We show that there exists a quantum critical point at $α_c \simeq 0.07$ for $n=4$, and determine the phase diagram. Our data at this quantum critical point agree quantitatively with the universal scaling predicted by the quantum nonlinear $σ$ model. We also report results on random mixtures of $n=2$ and $n=3$ ladders, which correspond to the doping region near but above 1/8. Our study on the magnetic static structure factor reveals a saturation of the incommensurability of the spin correlations around 1/8, while the incommensurability of the charge stripes grows linearly with hole concentration. The implications of this result for the interpretation of neutron scattering experiments on the dynamic spin fluctuations in La$_{2-x}$Sr$_x$CuO$_4$ are discussed.

cond-mat.str-el↗

An X-Ray Induced Structural Transition in La_0.875Sr_0.125MnO_3

We report a synchrotron x-ray scattering study of the magnetoresistive manganite La_0.875Sr_0.125MnO_3. At low temperatures, this material undergoes an x-ray induced structural transition at which charge ordering of Mn^3+ and Mn^4+ ions characteristic to the low-temperature state of this compound is destroyed. The transition is persistent but the charge-ordered state can be restored by heating above the charge-ordering transition temperature and subsequently cooling. The charge-ordering diffraction peaks, which are broadened at all temperatures, broaden more upon x-ray irradiation, indicating the finite correlation length of the charge-ordered state. Together with the recent reports on x-ray induced transitions in Pr_(1-x)Ca_xMnO_3, our results demonstrate that the photoinduced structural change is a common property of the charge-ordered perovskite manganites.

cond-mat.str-el↗

Spin correlations in an isotropic spin-5/2 two-dimensional antiferromagnet

We report a neutron scattering study of the spin correlations for the spin 5/2, two-dimensional antiferromagnet Rb_2MnF_4 in an external magnetic field. Choosing fields near the system's bicritical point, we tune the effective anisotropy in the spin interaction to zero, constructing an ideal S=5/2 Heisenberg system. The correlation length and structure factor amplitude are closely described by the semiclassical theory of Cuccoli et al. over a broad temperature range but show no indication of approaching the low-temperature renormalized classical regime of the quantum non-linear sigma model.

cond-mat.str-el↗

Monte Carlo Study of Correlations in Quantum Spin Chains at Non-Zero Temperature

Antiferromagnetic Heisenberg spin chains with various spin values ($S=1/2,1,3/2,2,5/2$) are studied numerically with the quantum Monte Carlo method. Effective spin $S$ chains are realized by ferromagnetically coupling $n=2S$ antiferromagnetic spin chains with $S=1/2$. The temperature dependence of the uniform susceptibility, the staggered susceptibility, and the static structure factor peak intensity are computed down to very low temperatures, $T/J \approx 0.01$. The correlation length at each temperature is deduced from numerical measurements of the instantaneous spin-spin correlation function. At high temperatures, very good agreement with exact results for the classical spin chain is obtained independent of the value of $S$. For $S$=2 chains which have a gap $Δ$, the correlation length and the uniform susceptibility in the temperature range $Δ< T < J$ are well predicted by a semi-classical theory due to Damle and Sachdev.

cond-mat.str-el↗

Spin Correlations in the Two-Dimensional Spin-5/2 Heisenberg Antiferromagnet Rb2MnF4

We report a neutron scattering study of the instantaneous spin correlations in the two-dimensional spin S=5/2 square-lattice Heisenberg antiferromagnet Rb_2MnF_4. The measured correlation lengths are quantitatively described, with no adjustable parameters, by high-temperature series expansion results and by a theory based on the quantum self-consistent harmonic approximation. Conversely, we find that the data, which cover the range from about 1 to 50 lattice constants, are outside of the regime corresponding to renormalized classical behavior of the quantum non-linear sigma model. In addition, we observe a crossover from Heisenberg to Ising critical behavior near the Neel temperature; this crossover is well described by a mean-field model with no adjustable parameters.

cond-mat.str-el↗

Correlations and Néel Order of Randomly Diluted Quantum Spin Ladders

We present a Monte Carlo study of the correlation length $ξ$ of randomly diluted antiferromagnetic Heisenberg ladders, composed of two spin--1/2 chains. For weak and intermediate inter--chain couplings, $J_{\bot}/J \leq 1$, we find an enhancement of correlations that is strongest for a fraction $z^* \approx J_{\bot}/(8J)$ of dilutants. We are able to access the experimentally relevant low--temperature regime, $T/J \approx 1/500$, and find that the recently inferred Néel temperature of $Sr(Cu_{1-z}Zn_z)_2O_3$ corresponds to a curve of constant correlation length $ξ\approx 18$ of the single diluted ladder with $J_{\bot}/J \alt 1/2$. The primary reason for the Néel ordering is argued to be a strong enhancement of two--dimensional correlations due to a Cu--Sr--Cu exchange coupling of $\approx 10 meV$ in the stacking direction of the ladders.

cond-mat.str-el↗