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R. J. Casperson

Publications and source records attributed to R. J. Casperson.

14 recordsLinked to original sources
arXiv2026

ENDF/B-VIII.1: Updated Nuclear Reaction Data Library for Science and Applications

The ENDF/B-VIII.1 library is the newest recommended evaluated nuclear data file by the Cross Section Evaluation Working Group (CSEWG) for use in nuclear science and technology applications, and incorporates advances made in the six years since the release of ENDF/B-VIII.0. Among key advances made are that the $^{239}$Pu file was reevaluated by a joint international effort and that updated $^{16,18}$O, $^{19}$F, $^{28-30}$Si, $^{50-54}$Cr, $^{55}$Mn, $^{54,56,57}$Fe, $^{63,65}$Cu, $^{139}$La, $^{233,235,238}$U, and $^{240,241}$Pu neutron nuclear data from the IAEA coordinated INDEN collaboration were adopted. Over 60 neutron dosimetry cross sections were adopted from the IAEA's IRDFF-II library. In addition, the new library includes significant changes for $^3$He, $^6$Li,$^9$Be, $^{51}$V, $^{88}$Sr, $^{103}$Rh, $^{140,142}$Ce, Dy, $^{181}$Ta, Pt, $^{206-208}$Pb, and $^{234,236}$U neutron data, and new nuclear data for the photonuclear, charged-particle and atomic sublibraries. Numerous thermal neutron scattering kernels were reevaluated or provided for the very first time. On the covariance side, work was undertaken to introduce better uncertainty quantification standards and testing for nuclear data covariances. The significant effort to reevaluate important nuclides has reduced bias in the simulations of many integral experiments with particular progress noted for fluorine, copper, and stainless steel containing benchmarks. Data issues hindered the successful deployment of the previous ENDF/B-VIII.0 for commercial nuclear power applications in high burnup situations. These issues were addressed by improving the $^{238}$U and $^{239,240,241}$Pu evaluated data in the resonance region. The new library performance as a function of burnup is similar to the reference ENDF/B-VII.1 library. The ENDF/B-VIII.1 data are available in ENDF-6 and GNDS format at https://doi.org/10.11578/endf/2571019.

physics.app-ph↗
arXiv2021

Measurement of material isotopics and atom number ratio with alpha-particle spectroscopy for the NIFFTE fission Time Projection Chamber actinide target

We present the results of a measurement of isotopic concentrations and atomic number ratio of a double-sided actinide target with alpha-spectroscopy and mass spectrometry. The double-sided actinide target, with primarily Pu-239 on one side and U-235 on the other, was used in the fission Time Projection Chamber (fissionTPC) for a measurement of the neutron-induced fission cross-section ratio between the two isotopes. The measured atomic number ratio is intended to provide an absolute normalization of the measured fission cross-section ratio. The Pu-239/U-235 atom number ratio was measured with a combination of mass spectrometry and alpha-spectroscopy with a planar silicon detector with uncertainties of less than 1%.

nucl-ex↗
arXiv2021

Measurement of the $^{239}$Pu(n,f)/$^{235}$U(n,f) Cross-Section Ratio with the NIFFTE fission Time Projection Chamber

The $^{239}$Pu(n,f)/$^{235}$U(n,f) cross-section ratio has been measured with the fission Time Projection Chamber (fissionTPC) from 100 keV to 100 MeV. The fissionTPC provides three-dimensional reconstruction of fission-fragment ionization profiles, allowing for a precise quantification of measurement uncertainties. The measurement was performed at the Los Alamos Neutron Science Center which provides a pulsed white source of neutrons. The data are recommended to be used as a cross-section ratio shape. A discussion of the status of the absolute normalization and comparisons to ENDF evaluations and previous measurements is included.

nucl-ex↗
arXiv2020

Neutron Induced Fission Fragment Angular Distributions, Anisotropy, and Linear Momentum Transfer Measured with the NIFFTE Fission Time Projection Chamber

The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) collaboration has performed measurements with a fission time projection chamber (fissionTPC) to study the fission process by reconstructing full three-dimensional tracks of fission fragments and other ionizing radiation. The amount of linear momentum imparted to the fissioning nucleus by the incident neutron can be inferred by measuring the opening angle between the fission fragments. Using this measured linear momentum, fission fragment angular distributions can be converted to the center-of-mass frame for anisotropy measurements. Angular anisotropy is an important experimental observable for understanding the quantum mechanical state of the fissioning nucleus and vital to determining detection efficiency for cross section measurements. Neutron linear momentum transfer to fissioning $^{235}$U, $^{238}$U, and $^{239}$Pu and fission fragment angular anisotropy of $^{235}$U and $^{238}$U as a function of neutron energies in the range 130 keV--250 MeV are presented.

nucl-ex↗
arXiv2019

Determining the average prompt-fission-neutron multiplicity for $^{239}$Pu($n$,$f$) via a $^{240}$Pu($α$,$α^{\prime}f$) surrogate reaction

The average prompt-fission-neutron multiplicity $\barν$ is of significance in the areas of nuclear theory, nuclear nonproliferation, and nuclear energy. In this work, the surrogate-reaction method has been used for the first time to indirectly determine $\barν$ for $^{239}$Pu($n$,$f$) via $^{240}$Pu($α$,$α^{\prime}f$) reactions. A $^{240}$Pu target was bombarded with a beam of 53.9-MeV $α$ particles. Scattered $α$ particles, fission products, and neutrons were measured with the NeutronSTARS detector array. Values of $\barν$ were obtained for a continuous range of equivalent incident neutron energies between 0.25--26.25~MeV, and the results agree well with direct neutron measurements.

nucl-ex↗
arXiv2019

Fission Fragment Angular Anisotropy in Neutron-Induced Fission of $^{235}$U Measured with a Time Projection Chamber

Fission fragment angular distributions can provide an important constraint on fission theory, improving predictive fission codes, and are a prerequisite for a precise ratio cross section measurement. Available anisotropy data is sparse, especially at neutron energies above 5 MeV. For the first time, a three-dimensional tracking detector is employed to study fragment emission angles and provide a direct measurement of angular anisotropy. The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) collaboration has deployed the fission time projection chamber (fissionTPC) to measure nuclear data with unprecedented precision. The fission fragment anisotropy of $^{235}$U has been measured over a wide range of incident neutron energies from 180 keV to 200 MeV; a careful study of the systematic uncertainties complement the data.

nucl-ex↗
arXiv2019

1H(n,el) as a Cross Section Reference in a White Source Neutron Beam With the fissionTPC

We provide a quantitative description of a method to measure neutron-induced fission cross sections in ratio to elastic hydrogen scattering in a white-source neutron beam with the fission Time Projection Chamber. This detector has measured precision fission cross section ratios using actinide references such as $^{235}$U(n,f) and $^{238}$U(n,f). However, by employing a more precise reference such as the H(n,el) cross section there is the potential to further reduce the evaluation uncertainties of the measured cross sections. In principle the fissionTPC could provide a unique measurement by simultaneously measuring both fission fragments and proton recoils over a large solid angle. We investigate one method with a hydrogenous gas target and with the neutron energy determined by the proton recoil kinematics. This method enables the measurement to be performed in a white-source neutron beam and with the current configuration of the fissionTPC. We show that while such a measurement is feasible in the energy range of 0.5 MeV to $\sim$10 MeV, uncertainties on the proton detection efficiency and the neutron energy resolution do not allow us to preform a fission ratio measurement to the desired precision. Utilizing either a direct measurement of the neutron time-of-flight for the recoil proton or a mono-energetic neutron source or some combination of both would provide a path to a sub-percent precision measurement.

nucl-ex↗
arXiv2018

Towards Neutron Capture on Exotic Nuclei: Demonstrating $(d,pγ)$ as a Surrogate Reaction for $(n,γ)$

The neutron-capture reaction plays a critical role in the synthesis of the elements in stars and is important for societal applications including nuclear power generation and stockpile-stewardship science. However, it is difficult - if not impossible - to directly measure neutron capture cross sections for the exotic, short-lived nuclei that participate in these processes. In this Letter we demonstrate a new technique which can be used to indirectly determine neutron-capture cross sections for exotic systems. This technique makes use of the $(d,p)$ transfer reaction, which has long been used as a tool to study the structure of nuclei. Recent advances in reaction theory, together with data collected using this reaction, enable the determination of neutron-capture cross sections for short-lived nuclei. A benchmark study of the $^{95}$Mo$(d,p)$ reaction is presented, which illustrates the approach and provides guidance for future applications of the method with short-lived isotopes produced at rare isotope accelerators.

nucl-ex↗
arXiv2018

Measurement of the normalized $^{238}$U(n,f)/$^{235}$U(n,f) cross section ratio from threshold to 30 MeV with the fission Time Projection Chamber

The normalized $^{238}$U(n,f)/$^{235}$U(n,f) cross section ratio has been measured using the NIFFTE fission Time Projection Chamber from the reaction threshold to $30$~MeV. The fissionTPC is a two-volume MICROMEGAS time projection chamber that allows for full three-dimensional reconstruction of fission-fragment ionization profiles from neutron-induced fission. The measurement was performed at the Los Alamos Neutron Science Center, where the neutron energy is determined from neutron time-of-flight. The $^{238}$U(n,f)/$^{235}$U(n,f) ratio reported here is the first cross section measurement made with the fissionTPC, and will provide new experimental data for evaluation of the $^{238}$U(n,f) cross section, an important standard used in neutron-flux measurements. Use of a development target in this work prevented the determination of an absolute normalization, to be addressed in future measurements. Instead, the measured cross section ratio has been normalized to ENDF/B-VIII.$β$5 at 14.5 MeV.

nucl-ex↗
arXiv2016

First observation of low-energy γ-ray enhancement in the rare-earth region

The γ-ray strength function and level density in the quasi-continuum of 151,153Sm have been measured using BGO shielded Ge clover detectors of the STARLiTeR system. The Compton shields allow for an extraction of the γ strength down to unprecedentedly low γ energies of about 500 keV. For the first time an enhanced low- energy γ-ray strength has been observed in the rare-earth region. In addition, for the first time both the upbend and the well known scissors resonance have been observed simultaneously for the same nucleus. Hauser-Feshbach calculations show that this strength enhancement at low γ energies could have an impact of 2-3 orders of magnitude on the (n,γ) reaction rates for the r-process nucleosynthesis.

nucl-ex↗
arXiv2009

Spectroscopy of Neutron-Rich 168,170Dy: Yrast Band Evolution Close to the NpNn Valence Maximum

The yrast sequence of the neutron-rich dysprosium isotope 168Dy has been studied using multi-nucleon transfer reactions following collisions between a 460-MeV 82Se beam and a 170Er target. The reaction products were identified using the PRISMA magnetic spectrometer and the gamma rays detected using the CLARA HPGe-detector array. The 2+ and 4+ members of the previously measured ground state rotational band of 168Dy have been confirmed and the yrast band extended up to 10+. A tentative candidate for the 4+ to 2+ transition in 170Dy was also identified. The data on these nuclei and on the lighter even-even dysprosium isotopes are interpreted in terms of Total Routhian Surface calculations and the evolution of collectivity in the vicinity of the proton-neutron valence product maximum is discussed.

nucl-ex↗
arXiv2009

Regularities and symmetries of subsets of collective 0+ states

The energies of subsets of excited 0+ states in geometric collective models are investigated and found to exhibit intriguing regularities. In models with an infinite square well potential, it is found that a single formula, dependent on only the number of dimensions, describes a subset of 0+ states. The same behavior of a subset of 0+ states is seen in the large boson number limit of the Interacting Boson Approximation (IBA) model near the critical point of a first order phase transition, in contrast to the fact that these 0+ state energies exhibit a harmonic behavior in all three limiting symmetries of the IBA. Finally, the observed regularities in 0+ energies are analyzed in terms of the underlying group theoretical framework of the different models.

nucl-th↗
arXiv2008

Simple, empirical order parameter for a first order quantum phase transition in atomic nuclei

A simple, empirical signature of a first order phase transition in atomic nuclei is presented, the ratio of the energy of the 6+ level of the ground state band to the energy of the first excited 0+ state. This ratio provides an effective order parameter which is not only easy to measure, but also distinguishes between first and second order phase transitions and takes on a special value in the critical region. Data in the Nd-Dy region show these characteristics. In addition, a repeating degeneracy between alternate yrast states and successive excited 0+ states is found to correspond closely to the line of a first order phase transition in the framework of the Interacting Boson Approximation (IBA) model in the large N limit, pointing to a possible underlying symmetry in the critical region.

nucl-th↗