arXiv subjects

R. J. Charity

Publications and source records attributed to R. J. Charity.

At least 19 recordsLinked to original sources

arXiv2026

Differential cross sections for ${{^{12}\mathrm{C}(n,α_{0})}}$, ${{^{16}\mathrm{O}(n,α_{0})}}$ and ${{^{16}\mathrm{O}(n,α_{1,2,3})}}$ between ${E_n}$ = 7.2 and 10 MeV with an active-target Time Projection Chamber

Data for the ${{^{12}\mathrm{C}(n,α_{0})}}$, ${{^{16}\mathrm{O}(n,α_{0})}}$ and ${{^{16}\mathrm{O}(n,α_{1,2,3})}}$ differential cross sections are important for several different areas of nuclear physics such as understanding neutron transmutation in nuclear reactors. The TexAT Time Projection Chamber was used to measure the differential and angle-integrated cross sections in active-target mode. The chamber was filled with CO$_2$ gas and used a quasi-monoenergetic neutron beam from the $d(d,n)$ reaction at Edwards Accelerator Lab at Ohio University. A comparison between our current and previous results at overlapping energies and angles which showed good agreement in angular dependence and absolute cross section. A broader angular coverage than previous results demonstrated that the integrated cross section for the \po16 reaction deviates from ENDFVIII.0 evaluations. This first instance of neutron-induced measurements with an active-target Time Projection Chamber demonstrates the use of this method for high-quality differential cross section data across a broad angular range, generating good statistics with a relatively low-intensity beam.

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arXiv2026

Comparing invariant-mass spectroscopy of 8B with ab initio predictions

Levels in 8B have been investigated experimentally using the invariant-mass technique and compared to ab initio calculations. Data sets obtained using E/A=69-MeV 9C and 13O beams on a Be target have been further analyzed to extend the level scheme of 8B for Ex<10 MeV. New levels were observed in the 2p+6Li, p+3He+alpha, and the p+7Be+gamma exit channels. Momentum correlations between the decay fragments were also investigated in order to deduce the decay pathways and whether the decays are prompt or sequential. This nucleus and its mirror were also investigated in the ab initio symmetry-adapted no-core shell model. Correspondence between the newly observed and predicted levels were made based on the level energy and the decay modes. For positive parity levels with J<=3, all predicted levels can be connected to an experimental counter part (as least tentatively) for Ex<8.4 MeV.

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arXiv2025

Triplet of kindred prompt-2p emitters in mass-8 proton-rich nuclei

A triplet of kindred prompt-2p emitters in A=8 nuclei has been demonstrated. Two of these are the ground state of 8C and its isobaric analog state in 8B, both of which are analogs of the halo or thick-skinned nucleus 8He. The third member is the recently found fourth 1+ state in 8B. This new 8B state at E*=8.4 MeV was observed to decay to the ground state of 6Li by 2p emission. Momentum correlations between the decay products indicate that it is not a sequential 2p decay through a 7Be intermediate state, but indicative of prompt 2p emission with correlations similar to those of the other members of the triplet. Ab initio calculations with the symmetry-adapted nocore shell model indicate that these three states have very similar spatial wavefunctions, but with nucleons coupling to different spins, isospins, and isospin projections. The triplet of 2p emitters all have oblate shapes and by stripping two protons equatorially, decay to states which have prolate shapes.

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arXiv2025

Deviations from the Isobaric Multiplet Mass Equation due to threshold states

Recent studies have completed the A=16 isospin quintets for states with spin/parity Jπ =0+ and 2+. The dependence of their masses as a function of isospin projection shows evidence for deviations from quadratic behavior indicating isospin violation beyond the expectation from two- body forces. The deviation is most pronounced for the 2+ states. Predictions from the Shell Model Embedded in the Continuum (SMEC) allow us to explain that this isospin violation is associated with a modification of the nuclear structure due to the open-quantum-system nature of the proton- rich members of the quintet. In particular, the 0+ and 2+ states in 16Ne and the 2+ state in 16F are threshold resonances located just above a proton-decay threshold where s-wave coupling to the continuum is expected. The measured deviations of these threshold states from the quadratic behavior of the remaining members of the multiplets makes it possible to obtain information on the magnitude and the energy dependence of the continuum-coupling energy correction. Continuum coupling is also indicated for the ground state of 8C, but this time through p-wave coupling.

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arXiv2024

In-beam $γ$-ray spectroscopy towards the proton dripline: The curious case of $^{32}$Ar

High-resolution in-beam $γ$-ray spectroscopy was used to study excited states of the neutron-deficient nucleus $^{32}$Ar populated in fast-beam induced four- and six-nucleon removal reactions from $^{36,38}$Ca. One new $γ$-ray transition and indications for an additional two were found, allowing for a glimpse at the level scheme beyond the known $2^+_1$ state. The nature of the new $1900(4)$-keV transition is discussed in the context of the known energy spectrum of the mirror nucleus $^{32}$Si and shell-model calculations using the FSU and SDPF-M cross-shell effective interactions. Its resulting parent state at $3767(5)$ keV, more than $1.3$ MeV above the proton separation energy, is tentatively assigned to have mixed sd-shell and $2p$-$2h$ character. It might either be the mirror of the $J^π=2^+_2$ state of $^{32}$Si at $4230.8(8)$ keV, but with a decay branch favoring a transition to the $2^+_1$ over the ground state, or the mirror of the $4983.9(11)$-keV state with quantum numbers $0^+$. The resulting mirror-energy differences of $-473(5)$ and $-1218(5)$ keV are both sizable when compared to systematics; in the latter case it would, in fact, be among the largest reported to date in the entire nuclear chart or suggest the potential existence of an additional, hitherto unidentified, low-lying $0^+$ state of $^{32}$Si.

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arXiv2024

In-beam $γ$-ray spectroscopy of negative-parity states of $^{37}$K populated in dissipative reactions

In-beam $γ$-ray spectroscopy was used to study excited states of the neutron-deficient nucleus $^{37}$K populated in fast-beam inelastic-scattering and proton-removal reactions at high-momentum loss. New $γ$-ray transitions and $γγ$ coincidence relationships were established using the $γ$-ray tracking array GRETINA. The extension of the level scheme up to the first $(13/2^-)$ state highlights the potential of this recently demonstrated population pathway for studies of isospin symmetry involving mirror-energy differences. The nature of the newly identified states is discussed in comparison to shell-model calculations with the FSU cross-shell effective interaction. The calculated occupation numbers of individual orbitals are shown to offer a consistent explanation of the measured mirror-energy differences between $^{37}$K and $^{37}$Ar.

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arXiv2024

Probing proton cross-shell excitations through the two-neutron removal from 38Ca

Bound states of the neutron-deficient, near-dripline nucleus $^{36}$Ca were populated in two-neutron removal from the ground state of $^{38}$Ca, a direct reaction sensitive to the single-particle configurations and couplings of the removed neutrons in the projectile wave function. Final-state exclusive cross sections for the formation of $^{36}$Ca and the corresponding longitudinal momentum distributions, both determined through the combination of particle and $γ$-ray spectroscopy, are compared to predictions combining eikonal reaction theory and shell-model two-nucleon amplitudes from the USDB, USDC, and ZBM2 effective interactions. The final-state cross-section ratio $σ(2^+_1)/σ(0^+)$ shows particular sensitivity and is approximately reproduced only with the two-nucleon amplitudes from the ZBM2 effective interaction that includes proton cross-shell excitations into the $pf$ shell. Characterizing the proton $pf$-shell occupancy locally and schematically, an increase of the $sd$-$pf$ shell gap by $250$ keV yields an improved description of this cross-section ratio and simultaneously enables a reproduction of the $B(E2;0^+_1\to2^+_1)$ excitation strength of $^{36}$Ca. This highlights an important aspect if a new shell-model effective interaction for the region was to be developed on the quest to model the neutron-deficient Ca isotopes and surrounding nuclei whose structure is impacted by proton cross-shell excitations.

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arXiv2023

Strong evidence for 9N and the limits of existence of atomic nuclei

The boundaries of the Chart of Nuclides contain exotic isotopes that possess extreme proton-toneutron asymmetries. Here we report on strong evidence of 9N, one of the most exotic proton-rich isotopes where more than one half of its constitute nucleons are unbound. With seven protons and two neutrons, this extremely proton-rich system would represent the first-known example of a ground-state five-proton emitter. The invariant-mass spectrum of its decay products can be fit with two peaks whose energies are consistent with the theoretical predictions of an open-quantum-system approach, however we cannot rule out the possibility that only a single resonance-like peak is present in the spectrum.

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arXiv2022

Dissipative reactions with intermediate-energy beams -- a novel approach to populate complex-structure states in rare isotopes

A novel pathway for the formation of multi-particle-multi-hole (np-mh) excited states in rare isotopes is reported from highly energy- and momentum-dissipative inelastic-scattering events measured in reactions of an intermediate-energy beam of 38Ca on a Be target. The negative-parity,complex-structure final states in 38Ca were observed following the in-beam gamma-ray spectroscopy of events in the 9Be(38Ca,38Ca+gamma)X reaction in which the scattered projectile lost longitudinal momentum of order p = 700 MeV/c. The characteristics of the observed final states are discussed and found to be consistent with the formation of excited states involving the rearrangement of multiple nucleons in a single, highly-energetic projectile-target collision. Unlike the far-less dissipative, surface-grazing reactions usually exploited for the in-beam gamma-ray spectroscopy of rare isotopes, these more energetic collisions appear to offer a practical pathway to nuclear-structure studies of more complex multi-particle configurations in rare isotopes - final states conventionally thought to be out of reach with high-luminosity fast-beam-induced reactions.

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arXiv2022

Exploiting dissipative reactions to perform in-beam $γ$-ray spectroscopy of the neutron-deficient isotopes \nuc{38,39}{Ca}

The neutron-deficient Ca isotopes continue to attract attention due to their importance for testing isospin symmetry and their relevance in capture reactions of interest for nova nucleosynthesis and the shape of light curves in Type I X-ray bursts. To date, spectroscopic information on 38,39 Ca is largely limited to data on lower-spin excited states. Here, we report in-beam γ-ray spectroscopy of complementary higher-spin, complex-structure states in 39 Ca populated in fast-beam-induced, momentum-dissipative processes leading to neutron pickup onto excited configurations of the projectile, 9 Be(38 Ca , 39 Ca + γ)X. Such a dissipative reaction was recently characterized for the case of inelastic scattering of 38 Ca off 9 Be, 9 Be(38 Ca, 38 Ca + γ)X. Additional data and discussion on the nuclear structure of 38 Ca is also presented. An explanation for the more-complex-structure states, populated with small cross sections in one-nucleon knockout reactions, and observed in the tails of their longitudinal momentum distributions, is also offered.

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arXiv2021

Nucleon-nucleon correlations in the extreme oxygen isotopes

There has been an upsurge of interest in two-nucleon decays thanks to the studies of nucleon-nucleon correlations. In our previous work, based on a novel time-dependent three-body approach, we demonstrated that the energy and angular correlations of the emitted nucleons can shed light on the structure of nucleonic pairs formed inside the nucleus. In this work, we apply the new framework to study the decay dynamics and properties of some extreme proton-rich and neutron-rich oxygen isotopes, including two-proton ($2p$) decays of $^{11,12}$O and two-neutron ($2n$) decay of $^{26}$O. Here we show that the low-$\ell$ components of $^{11,12}$O wave functions, which are affected by continuum and configuration-interaction effects, strongly impact decay dynamics and asymptotic correlations. In the calculated wave functions of $^{11,12}$O, diproton and cigarlike structures merge together during the tunneling process and the resulting energy- and angular correlations are very consistent with the experimental data. The asymptotic correlations of the $2n$ decay of $^{26}$O dramatically change as the two-neutron decay energy approaches the zero-energy threshold. The small reported value of $Q_{2n}$ suggests that the $2n$ decay of this nucleus can be understood in terms of the universal phase-space limit.

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arXiv2021

Using spin alignment of inelastically-excited fast beams to make spin assignments: the spectroscopy of 13O as a test case

Excited states in 13O were investigated using inelastic scattering of an E/A=69.5-MeV 13O beam off of a 9Be target. The excited states were identified in the invariant-mass spectra of the decay products. Both single proton and sequential two-proton decays of the excited states were examined. For a number of the excited states, the protons were emitted with strong anisotropy where emissions transverse to the beam axis are favored. The measured proton-decay angular distributions were compared to predictions from distorted-wave born-approximation (DWBA) calculations of the spin alignment which was shown to be largely independent of the excitation mechanism. The deduced $^{13}$O level scheme is compared to ab initio no-core shell model with continuum (NCSMC) predictions. The lowest-energy excited states decay isotropically consistent with predictions of strong proton 1s1/2 structure. Above these states in the level scheme, we observed a number of higher-spin states not predicted within the model. Possibly these are associated with rotational bands built on deformed cluster configurations predicted by antisymmetrized molecular dynamics (AMD) calculations. The spin alignment mechanism is shown to be useful for making spin assignments and may have widespread use.

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arXiv2020

Isotopically resolved neutron total cross sections at intermediate energies

The neutron total cross sections $σ_{tot}$ of $^{16,18}$O, $^{58,64}$Ni, $^{103}$Rh, and $^{112,124}$Sn have been measured at the Los Alamos Neutron Science Center (LANSCE) from low to intermediate energies (3 $\leq E_{lab} \leq$ 450 MeV) by leveraging waveform-digitizer technology. The $σ_{tot}$ relative differences between isotopes are presented, revealing additional information about the isovector components needed for an accurate optical-model description away from stability. Digitizer-enabled $σ_{tot}$-measurement techniques are discussed and a series of uncertainty-quantified dispersive optical model (DOM) analyses using these new data is presented, validating the use of the DOM for modeling light systems ($^{16,18}$O) and systems with open neutron shells ($^{58,64}$Ni and $^{112,124}$Sn). The valence-nucleon spectroscopic factors extracted for each isotope reaffirm the usefulness of high-energy proton reaction cross sections for characterizing depletion from the mean-field expectation.

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arXiv2020

Systematic Matter and Binding-Energy Distributions from a Dispersive Optical Model Analysis

We present the first systematic nonlocal dispersive optical model analysis using both bound-state and scattering data of $^{16,18}$O, $^{40,48}$Ca, $^{58,64}$Ni, $^{112,124}$Sn, and $^{208}$Pb. In all systems, roughly half the total nuclear binding energy is associated with the most-bound 10% of the total nucleon density. The extracted neutron skins reveal the interplay of asymmetry, Coulomb, and shell effects on the skin thickness. Our results indicate that simultaneous optical model fits of inelastic scattering and structural data on isotopic pairs are effective for constraining asymmetry-dependent nuclear structural quantities otherwise difficult to observe experimentally.

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arXiv2020

In-beam $γ$-ray spectroscopy at the proton dripline: $^{40}$Sc

We report on the first in-beam $γ$-ray spectroscopy of the proton-dripline nucleus $^{40}$Sc using two-nucleon pickup onto an intermediate-energy rare-isotope beam of $^{38}$Ca. The $^{9}$Be($^{38}$Ca,$^{40}$Sc$+γ$)X reaction at 60.9 MeV/nucleon mid-target energy selectively populates states in $^{40}$Sc for which the transferred proton and neutron couple to high orbital angular momentum. In turn, due to angular-momentum selection rules in proton emission and the nuclear structure and energetics of $^{39}$Ca, such states in $^{40}$Sc then exhibit $γ$-decay branches although they are well above the proton separation energy. This work uniquely complements results from particle spectroscopy following charge-exchange reactions on $^{40}$Ca as well as $^{40}$Ti EC/$β^+$ decay which both display very different selectivities. The population and $γ$-ray decay of the previously known first $(5^-)$ state at 892 keV and the observation of a new level at 2744 keV are discussed in comparison to the mirror nucleus and shell-model calculations. On the experimental side, this work shows that high-resolution in-beam $γ$-ray spectroscopy is possible with new generation Ge arrays for reactions induced by rare-isotope beams on the level of a few $μ$b of cross section.

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arXiv2020

A dispersive optical model analysis of $^{208}$Pb generating a neutron-skin prediction beyond the mean field

A nonlocal dispersive-optical-model analysis has been carried out for neutrons and protons in $^{208}$Pb. Elastic-scattering angular distributions, total and reaction cross sections, single-particle energies, the neutron and proton numbers, the charge distribution, and the binding energy have been fitted to extract the neutron and proton self-energies both above and below the Fermi energy. From the single-particle propagator derived from these self-energies, we have determined the charge and matter distributions in $^{208}$Pb. The predicted spectroscopic factors are consistent with results from the $(e,e'p)$ reaction and inelastic-electron-scattering data to very high spin states. Sensible results for the high-momentum content of neutrons and protons are obtained with protons appearing more correlated, in agreement with experiment and \textit{ab initio} calculations of asymmetric matter. A neutron skin of $0.25\pm0.05$ fm is deduced. An analysis of several nuclei leads to the conclusion that finite-size effects play a non-negligible role in the formation of the neutron skin in finite nuclei.

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arXiv2020

Particle decays of levels in $^{11,12}$N and $^{12}$O investigated with the invariant-mass method

Particle-decaying states of the light nuclei $^{11,12}$N and $^{12}$O were studied using the invariant-mass method. The decay energies and intrinsic widths of a number of states were measured, and the momentum correlations of three-body decaying states were considered. A second 2$p$-decaying 2$^+$ state of $^{12}$O was observed for the first time, and a higher energy $^{12}$O state was observed in the 4$p$+2$α$ decay channel. This 4$p$+2$α$ channel also contains contributions from fission-like decay paths, including $^6$Be$_{g.s.}$+$^{6}$Be$_{g.s.}$. Analogs to these states in $^{12}$O were found in $^{12}$N in the 2$p$+$^{10}$B and 2$p$+$α$+$^6$Li channels. The momentum correlations for the prompt 2$p$ decay of $^{12}$O$_{g.s.}$ were found to be nearly identical to those of $^{16}$Ne$_{g.s.}$, and the correlations for the new 2$^+$ state were found to be consistent with sequential decay through excited states in $^{11}$N. The momentum correlations for the 2$^+_1$ state in $^{12}$O provide a new value for the $^{11}$N ground-state energy. The states in $^{12}$N/$^{12}$O that belong to the $A$=12 isobaric sextet do not deviate from the quadratic isobaric multiplet mass equation (IMME) form.

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arXiv2019

Invariant-mass spectroscopy of $^{14}$O excited states

Excited states in $^{14}$O have been investigated both experimentally and theoretically. Experimentally, these states were produced via neutron-knockout reactions with a fast $^{15}$O beam and the invariant-mass technique was employed to isolate the 1$p$ and 2$p$ decay channels and determine their branching ratios. The spectrum of excited states was also calculated with the Shell Model Embedded in the Continuum that treats bound and scattering states in a unified model. By comparing energies, widths and decay branching patterns, spin and parity assignments for all experimentally observed levels below 8 MeV are made. This includes the location of the second 2$^{+}$ state that we find is in near degeneracy with the third 0$^{+}$ state. An interesting case of sequential 2$p$ decay through a pair of degenerate $^{13}$N excited states with opposite parities was found where the interference between the two sequential decay pathways produces an unusual relative-angle distribution between the emitted protons.

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