arXiv subjects

R. J. Chen

Publications and source records attributed to R. J. Chen.

31 records · Page 2Linked to original sources

arXiv2019

New Test of Modulated Electron Capture Decay of Hydrogen-Like $^{142}$Pm Ions: Precision Measurement of Purely Exponential Decay

An experiment addressing electron capture (EC) decay of hydrogen-like $^{142}$Pm$^{60+}$ ions has been conducted at the experimental storage ring (ESR) at GSI. The decay appears to be purely exponential and no modulations were observed. Decay times for about 9000 individual EC decays have been measured by applying the single-ion decay spectroscopy method. Both visually and automatically analysed data can be described by a single exponential decay with decay constants of 0.0126(7) s$^{-1}$ for automatic analysis and 0.0141(7) s$^{-1}$ for manual analysis. If a modulation superimposed on the exponential decay curve is assumed, the best fit gives a modulation amplitude of merely 0.019(15), which is compatible with zero and by 4.9 standard deviations smaller than in the original observation which had an amplitude of 0.23(4).

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arXiv2019

Masses of ground and isomeric states of $^{101}$In and configuration-dependent shell evolution in odd-$A$ indium isotopes

We report first precision mass measurements of the $1/2^-$ isomeric and $9/2^+$ ground states of $^{101}$In. The determined isomeric excitation energy continues a smooth trend of odd-$A$ indium isotopes up to the immediate vicinity of $N=50$ magic number. This trend can be confirmed by dedicated shell model calculations only if the neutron configuration mixing is considered. We find that the single particle energies are different for different states of the same isotope. The presented configuration-dependent shell evolution, type II shell evolution, in odd-$A$ nuclei is discussed for the first time. Our results will facilitate future studies of single-particle neutron states.

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arXiv2019

Masses of neutron-rich $^{\operatorname{52-54}}$Sc and $^{54,56}$Ti nuclides: The $N=32$ subshell closure in scandium

Isochronous mass spectrometry has been applied in the storage ring CSRe to measure the masses of the neutron-rich $^{\operatorname{52-54}}$Sc and $^{54,56}$Ti nuclei. The new mass excess values $ME$($^{52}$Sc) $=$ $-40525(65)$ keV, $ME$($^{53}$Sc) $=$ $-38910(80)$ keV, and $ME$($^{54}$Sc) $=$ $-34485(360)$ keV, deviate from the Atomic Mass Evaluation 2012 by 2.3$σ$, 2.8$σ$, and 1.7$σ$, respectively. These large deviations significantly change the systematics of the two-neutron separation energies of scandium isotopes. The empirical shell gap extracted from our new experimental results shows a significant subshell closure at $N = 32$ in scandium, with a similar magnitude as in calcium. Moreover, we present $ab$ $initio$ calculations using the valence-space in-medium similarity renormalization group based on two- and three-nucleon interactions from chiral effective field theory. The theoretical results confirm the existence of a substantial $N = 32$ shell gap in Sc and Ca with a decreasing trend towards lighter isotones, thus providing a consistent picture of the evolution of the $N = 32$ magic number from the $pf$ into the $sd$ shell.

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arXiv2019

Improving the resolving power of Isochronous Mass Spectrometry by employing an in-ring mechanical slit

Isochronous Mass Spectrometry (IMS) in heavy-ion storage rings is an excellent experimental method for precision mass measurements of exotic nuclei. In the IMS, the storage ring is tuned in a special isochronous ion-optical mode. Thus, the mass-over-charge ratios of the stored ions are directly reflected by their respective revolution times in first order. However, the inevitable momentum spread of secondary ions increases the peak widths in the measured spectra and consequently limits the achieved mass precision. In order to achieve a higher mass resolving power, the ring aperture was reduced to 60 mm by applying a mechanical slit system at the dispersive straight section. The momentum acceptance was reduced as well as better isochronous conditions were achieved. The results showed a significant improvement of the mass resolving power reaching $5.2 \times 10^{5}$, though at the cost of about 40\% ion loss.

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arXiv2018

Experimental Investigation of the Transition Energy $γ_t$ in the Isochronous Mode of the HIRFL-CSRe

The Isochronous Mass Spectrometry (IMS) based on storage rings is a powerful technique for mass measurement of short-lived exotic nuclei. The transition energy $γ_t$ of the storage ring is a vital parameter of the IMS technique. It is difficult to measure the $γ_t$ and its relation to momentum spread or circulating length, especially to monitor the variation of $γ_t$ during experiments. An experimental investigation on the $γ_t$ has been performed for the IMS experiment at the Cooler Storage Ring of the Heavy Ion Research Facility in Lanzhou (HIRFL-CSRe). With the velocity measured by two time-of-flight (TOF) detectors, the $γ_t$ as a function of orbital length can be determined. The influences of higher order magnetic field components on the $γ_t$ function were inferred for isochronous correction. This paper introduces and investigates the influence of dipole magnetic fields, quadrupole magnetic fields and sextupole magnetic fields on the $γ_t$ function. With the quadrupole magnets and sextupole magnets corrections, a mass resolution of 171332 (FWHM) and $σ(T)/T=1.34\times10^{-6}$ were reached, which shall be compared with 31319 (FWHM) and $σ(T)/T=7.35\times10^{-6}$ obtained without correction.

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arXiv2018

Application of isochronous mass spectrometry for the study of angular momentum population in projectile fragmentation reactions

Isochronous mass spectrometry was applied to measure isomeric yield ratios of fragmentation reaction products. This approach is complementary to conventional gamma-ray spectroscopy in particular for measuring yield ratios for long-lived isomeric states. Isomeric yield ratios for the high-spin I = 19/2 states in the mirror nuclei 53Fe and 53Co are measured to study angular momentum population following the projectile fragmentation of 78Kr at energies of 480A MeV on a beryllium target. The 19/2 state isomeric ratios of 53Fe produced from different projectiles in the literature have also been extracted as a function of mass number difference between projectile and fragment (mass loss). The results are compared to ABRABLA07 model calculations. The isomeric ratios of 53Fe produced using different projectiles suggest that the theory underestimates not only the previously reported dependence on the spin but also the dependence on the mass loss.

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arXiv2018

A method to measure the transition energy $γ_{t}$ of the isochronously tuned storage ring

The Isochronous Mass Spectrometry (IMS) is a powerful technique developed in heavy-ion storage rings for measuring masses of very short-lived exotic nuclei. The IMS is based on the isochronous setting of the ring. One of the main parameters of this setting is the transition energy $γ_{t}$. %The transition energy $γ_{t}$ plays an important role in the isochronous mass spectrometry (IMS). It has been a challenge to determine the $γ_{t}$ and especially to monitor the variation of $γ_{t}$ during experiments. In this paper we introduce a method to measure the $γ_{t}$ online during IMS experiments by using the acquired experimental data. Furthermore, since the storage ring has (in our context) a relatively large momentum acceptance, the variation of the $γ_{t}$ across the ring acceptance is a source of systematic uncertainty of measured masses. With the installation of two time-of-flight (TOF) detectors, the velocity of each stored ion and its revolution time are simultaneously available for the analysis. These quantities enabled us to determine the $γ_{t}$ as a function of orbital length in the ring. The presented method is especially important for future IMS experiments planned at the new-generation storage ring facilities FAIR in Germany and HIAF in China.

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arXiv2018

Isochronous mass measurements of $T_z=-1$ $fp$-shell nuclei from projectile fragmentation of $^{58}$Ni

Atomic masses of seven $T_z=-1$, $fp$-shell nuclei from $^{44}$V to $^{56}$Cu and two low-lying isomers, $^{44m}$V ($J^π=6^+$) and $^{52m}$Co ($J^π=2^+$), have been measured with relative precisions of $1-4\times 10^{-7}$ with Isochronous Mass Spectrometry (IMS) at CSRe. The masses of $^{56}$Cu, $^{52g,52m}$Co, and $^{44m}$V were measured for the first time in this experiment. The Mass Excesses ($ME^{\prime}$s) of $^{44}$V, $^{48}$Mn, $^{50}$Fe, and $^{54}$Ni are determined with an order of magnitude improved precision compared to the literature values. $^{52g,52m}$Co and $^{56}$Cu are found to be $370$~keV and $400$~keV more bound, respectively, while $^{44g,44m}$V are $\sim 300$~keV less bound than the extrapolations in the Atomic-Mass Evaluation 2012 (AME$^{\prime}$12). The masses of the four $T_z=-1/2$ nuclei $^{45}$V, $^{47}$Cr, $^{49}$Mn, and $^{51}$Fe are re-determined to be in agreement, within the experimental errors, with the recent JYFLTRAP measurements or with the previous IMS measurements in CSRe. Details of the measurements and data analysis are described, and the impact of the new $ME$ values on different aspects in nuclear structure are investigated and discussed.

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arXiv2018

The Masses of the $T_z=-3/2$ Nuclei $^{27}$P and $^{29}$S

Isochronous mass spectrometry has been applied in the storage ring CSRe to measure the masses of the $T_z=-3/2$ nuclei $^{27}$P and $^{29}$S. The new mass excess value $ME$($^{29}$S) $=-3094(13)$~keV is 66(52)~keV larger than the result of the previous $^{32}$S($^3$He,$^{6}$He)$^{29}$S reaction measurement in 1973 and a factor of 3.8 more precise. The new result for $^{29}$S, together with those of the $T=3/2$ isobaric analog states (IAS) in $^{29}$P, $^{29}$Si, and $^{29}$Al, fit well into the quadratic form of the Isobaric Multiplet Mass Equation IMME. The mass excess of $^{27}$P has been remeasured to be $ME(^{27}$P$)=-685(42)$ keV. By analyzing the linear and quadratic coefficients of the IMME in the $T_z=-3/2$ $sd$-shell nuclei, it was found that the ratio of the Coulomb radius parameters is $R\approx0.96$ and is nearly the same for all $T=3/2$ isospin multiplets. Such a nearly constant $R$-value, apparently valid for the entire light mass region with $A>9$, can be used to set stringent constraints on the isovector and isotensor components of the isospin non-conserving forces in theoretical calculations.

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arXiv2018

Mass Measurements of Neutron-Deficient Y, Zr, and Nb Isotopes and Their Impact on $rp$ and $νp$ Nucleosynthesis Processes

Using isochronous mass spectrometry at the experimental storage ring CSRe in Lanzhou, the masses of $^{82}$Zr and $^{84}$Nb were measured for the first time with an uncertainty of $\sim 10$ keV, and the masses of $^{79}$Y, $^{81}$Zr, and $^{83}$Nb were re-determined with a higher precision. %The latter differ significantly from their literature values. The latter are significantly less bound than their literature values. Our new and accurate masses remove the irregularities of the mass surface in this region of the nuclear chart. Our results do not support the predicted island of pronounced low $α$ separation energies for neutron-deficient Mo and Tc isotopes, making the formation of Zr-Nb cycle in the $rp$-process unlikely. The new proton separation energy of $^{83}$Nb was determined to be 490(400)~keV smaller than that in the Atomic Mass Evaluation 2012. This partly removes the overproduction of the $p$-nucleus $^{84}$Sr relative to the neutron-deficient molybdenum isotopes in the previous $νp$-process simulations.

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arXiv2016

Identification of the Lowest $T=2$, $J^{π=}0^+$ Isobaric Analog State in $^{52}$Co and Its Impact on the Understanding of $β$-Decay Properties of $^{52}$Ni

Masses of $^{52g,52m}$Co were measured for the first time with an accuracy of $\sim 10$ keV, an unprecedented precision reached for short-lived nuclei in the isochronous mass spectrometry. Combining our results with the previous $β$-$γ$ measurements of $^{52}$Ni, the $T=2$, $J^π=0^+$ isobaric analog state (IAS) in $^{52}$Co was newly assigned, questioning the conventional identification of IASs from the $β$-delayed proton emissions. Using our energy of the IAS in $^{52}$Co, the masses of the $T=2$ multiplet fit well into the Isobaric Multiplet Mass Equation. We find that the IAS in $^{52}$Co decays predominantly via $γ$ transitions while the proton emission is negligibly small. According to our large-scale shell model calculations, this phenomenon has been interpreted to be due to very low isospin mixing in the IAS.

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arXiv2016

An improvement of isochronous mass spectrometry: Velocity measurements using two time-of-flight detectors

Isochronous mass spectrometry (IMS) in storage rings is a powerful tool for mass measurements of exotic nuclei with very short half-lives down to several tens of microseconds, using a multicomponent secondary beam separated in-flight without cooling. However, the inevitable momentum spread of secondary ions limits the precision of nuclear masses determined by using IMS. Therefore, the momentum measurement in addition to the revolution period of stored ions is crucial to reduce the influence of the momentum spread on the standard deviation of the revolution period, which would lead to a much improved mass resolving power of IMS. One of the proposals to upgrade IMS is that the velocity of secondary ions could be directly measured by using two time-of-flight (double TOF) detectors installed in a straight section of a storage ring. In this paper, we outline the principle of IMS with double TOF detectors and the method to correct the momentum spread of stored ions.

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arXiv2014

Accurate correction of magnetic field instabilities for high-resolution isochronous mass measurements in storage rings

Isochronous mass spectrometry (IMS) in storage rings is a successful technique for accurate mass measurements of short-lived nuclides with relative precision of about $10^{-5}-10^{-7}$. Instabilities of the magnetic fields in storage rings are one of the major contributions limiting the achievable mass resolving power, which is directly related to the precision of the obtained mass values. A new data analysis method is proposed allowing one to minimise the effect of such instabilities. The masses of the previously measured at the CSRe $^{41}$Ti, $^{43}$V, $^{47}$Mn, $^{49}$Fe, $^{53}$Ni and $^{55}$Cu nuclides were re-determined with this method. An improvement of the mass precision by a factor of $\sim 1.7$ has been achieved for $^{41}$Ti and $^{43}$V. The method can be applied to any isochronous mass experiment irrespective of the accelerator facility. Furthermore, the method can be used as an on-line tool for checking the isochronous conditions of the storage ring.

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