arXiv subjects

R. Kato

Publications and source records attributed to R. Kato.

25 records · Page 2Linked to original sources

arXiv2012

Inter-Band Effects of Magnetic Field on Hall Conductivity in Multi Layered Massless Dirac Fermion System $α$-(BEDT-TTF)$_2$I$_3$

We have discovered two-dimensional zero-gap material with a layered structure in the organic conductor $α$-(BEDT-TTF)$_2$I$_3$ under high hydrostatic pressure. In contrast to graphene, the electron-hole symmetry is not good except at the vicinity of the Dirac points. Thus, temperature dependence of the chemical potential, $μ$, plays an important role in the transport in this system. The experimental formula of $μ$ is revealed. We succeeded in detecting the inter-band effects of a magnetic field on the Hall conductivity when $μ$ passes the Dirac point.

cond-mat.mes-hall↗

arXiv2010

Spin and Valley Splittings in Multilayered Massless Dirac Fermion System

The inter-layer magnetoresistance in a multilayered massless Dirac fermion system, $α$-(BEDT-TTF)$_2$I$_3$, under hydrostatic pressure was investigated. We succeeded in detecting the zero-mode (n=0) Landau level and its spin splitting in the magnetic field normal to the 2D plane. We demonstrated that the effective Coulomb interaction in the magnetic field intensifies the spin splitting of zero-mode Landau carriers. At temperatures below 2K, magnetic fields above several Tesla break the twofold valley degeneracy.

cond-mat.mtrl-sci↗

arXiv2009

Effects of the Zero-Mode Landau Level on Inter-Layer Magnetoresistance in Multilayer Massless Dirac Fermion Systems

We report on the experimental results of interlayer magnetoresistance in multilayer massless Dirac fermion system $α$-(BEDT-TTF)$_2$I$_3$ under hydrostatic pressure and its interpretation. We succeeded in detecting the zero-mode Landau level (n=0 Landau level) that is epected to appear at the contact points of Dirac cones in the magnetic field normal to the two-dimensional plane. The characteristic feature of zero-mode Landau carriers including the Zeeman effect is clearly seen in the interlayer magnetoresistance.

cond-mat.mtrl-sci↗

arXiv2007

Suppression of electronic susceptibility in metal-Mott insulator alternating material, (Me-3,5-DIP)[Ni(dmit)2]2

Frequency shifts and nuclear relaxations of 13C NMR of the metal-insulator alternating material, (Me-3,5-DIP)[Ni(dmit)2]2, are presented. The NMR absorption lines originating from metallic and insulating layers are well resolved, which evidences the coexistence of localized spins (π_loc) and conduction π-electrons. The insulating layer is newly found to undergo antiferromagnetic long range order at about 2.5 K, suggesting emergence of S=1/2 Mott insulator. In the metallic layer, we found significant suppressions of static and dynamical susceptibilities of conduction electrons below 35 K, where antiferromagnetic correlation in the insulating layer evolves. We propose a dynamical effect through strong π-π_loc coupling between the metallic and insulating layers as an origin of the reduction of the density of states.

cond-mat.str-el↗

arXiv2005

Temperature dependent Luttinger surfaces

The Luttinger surface of an organic metal (TTF-TCNQ), possessing charge order and spin-charge separation, is investigated using temperature dependent angle-resolved photoemission spectroscopy. The Luttinger surface topology, obtained from momentum distribution curves, changes from quasi-2D(dimensional) to quasi-1D with temperature. The high temperature quasi-2D surface exhibits 4$k_F$ charge-density-wave (CDW) superstructure in the TCNQ derived holon band, in the absence of 2$k_F$ order. Decreasing temperature results in quasi-1D nested 2$k_F$ CDW order in the TCNQ spinon band and in the TTF surface. The results establish the link in momentum-space between charge order and spin-charge separation in a Luttinger liquid.

cond-mat.str-el↗

arXiv2002

Fermi Surface Study of Quasi-Two-Dimensional Organic Conductors by Magnetooptical Measurements

Magnetooptical measurements of several quasi-two-dimensional (q2D) organic conductors, which have simple Fermi surface structure, have been performed by using a cavity perturbation technique. Despite of the simple Fermi surface structure, magnetooptical resonance results show a dramatic difference for each sample. Cyclotron resonances (CR) were observed for q-(BEDT-TTF)2I3 and (BEDT-TTF)3Br(pBIB), while periodic orbit resonances (POR) were observed for (BEDT-TTF)2Br(DIA) and (BEDT-TTF)3Cl(DFBIB). The selection of the resonance seems to correspond with the skin depth for each sample. The effective mass of POR seems to have a mass enhancement due to the many-body effect, while effective mass of CR is independent of the strength of the electron-electron interaction. The scattering time deduced from each resonance's linewidth will be also presented.

cond-mat.str-el↗

arXiv2002

Observation of High-Order Harmonic Resonances in Magnetooptical Measurements of (BEDT-TTF)2Br(DIA)

Magnetooptical measurements of a quasi-two-dimensional (q2D) organic conductor (BEDT-TTF)2Br(DIA) (DIA=diiodoacetylene) were performed using a cavity perturbation technique with a millimeter vector network analyzer (MVNA). Harmonic resonances were observed periodically as a function of the inverse field up to the 7th order. This is the first observation of higher-order harmonics up to the 7th order in an organic conductor. The observed resonance is assigned as a periodic orbit resonance (POR) which arises from a q2D elliptic Fermi surface (FS). The obtained effective mass (4.7me) is consistent with Shubnikov-de Haas measurements. Temperature dependence of the spectra observed in two different sample configurations will be presented.

cond-mat.str-el↗