arXiv subjects

R. Krücken

Publications and source records attributed to R. Krücken.

At least 19 recordsLinked to original sources

arXiv2026

EXO-200 Public Data Release for AI/ML Applications

We present a public release of a subset of calibration data from the EXO-200 experiment, a liquid xenon time projection chamber designed to search for neutrinoless double-beta decay in $^{136}$Xe. The released dataset consists of approximately one million events collected during $^{228}$Th calibration campaigns performed near the end of Phase-II operations between February 26 and March 2, 2018. For each event, the dataset includes raw detector waveforms from the U-wire, V-wire, and avalanche photodiode (APD) readout channels together with reconstructed event quantities including charge energy, light energy, rotated energy, and charge-cluster information. The dataset is distributed in HDF5 format and is intended to support data preservation, educational activities, and the development of modern machine-learning techniques for rare-event physics. This paper describes the detector, dataset contents, file structure, and public access mechanism.

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arXiv2025

Search for Double Beta Decays of $^{134}$Xe with EXO-200 Phase II

EXO-200 was a leading double beta decay experiment consisting of a single-phase, enriched liquid xenon time projection chamber filled with an admixture of 80.672% $^{136}$Xe and 19.098% $^{134}$Xe. The detector operated at WIPP between 2010 and 2018 and was designed to search for double beta decay of $^{136}$Xe. Data was acquired in two phases separated by a period of detector upgrades. We report on the search for $0νββ$ and $2νββ$ decay of $^{134}$Xe with Phase II EXO-200 data, with median 90% C.L. exclusion sensitivity $T_{1/2}^{0ν} \geq 3.7\times 10^{23}$ yr and $T_{1/2}^{2ν} \geq 2.6 \times 10^{21}$ yr, respectively. No statistically significant signal is observed for either decay mode. We set a world-leading lower limit on the half-life of the neutrinoless decay mode of $^{134}$Xe of $T_{1/2}^{0ν} \geq 8.7\times10^{23}$ (90% C.L.) and the second strongest constraint on the two-neutrino decay of $T_{1/2}^{2ν} \geq 2.9\times10^{21}$ (90% C.L.), a 3-fold improvement over the EXO-200 Phase I measurement. New constraints are also set for the $2νββ$ and $0νββ$ decays of $^{134}$Xe to the lowest excited state of $^{134}$Ba.

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arXiv2024

Towards the Discovery of New Elements: Production of Livermorium (Z=116) with 50Ti

The $^{244}$Pu($^{50}$Ti,$xn$)$^{294-x}$Lv reaction was investigated at Lawrence Berkeley National Laboratory's 88-Inch Cyclotron facility. The experiment was aimed at the production of a superheavy element with $Z\ge 114$ by irradiating an actinide target with a beam heavier than $^{48}$Ca. Produced Lv ions were separated from the unwanted beam and nuclear reaction products using the Berkeley Gas-filled Separator and implanted into a newly commissioned focal plane detector system. Two decay chains were observed and assigned to the decay of $^{290}$Lv. The production cross section was measured to be $σ_{\rm prod}=0.44(^{+58}_{-28})$~pb at a center-of-target center-of-mass energy of 220(3)~MeV. This represents the first published measurement of the production of a superheavy element near the `Island-of-Stability', with a beam of $^{50}$Ti and is an essential precursor in the pursuit of searching for new elements beyond $Z=118$.

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arXiv2023

Search for Two-neutrino Double-Beta Decay of $^{136}\rm Xe$ to the $0^+_1$ excited state of $^{136}\rm Ba$ with the Complete EXO-200 Dataset

A new search for two-neutrino double-beta ($2νββ$) decay of $^{136}\rm Xe$ to the $0^+_1$ excited state of $^{136}\rm Ba$ is performed with the full EXO-200 dataset. A deep learning-based convolutional neural network is used to discriminate signal from background events. Signal detection efficiency is increased relative to previous searches by EXO-200 by more than a factor of two. With the addition of the Phase II dataset taken with an upgraded detector, the median 90$\%$ confidence level half-life sensitivity of $2νββ$ decay to the $0^+_1$ state of $^{136}\rm Ba$ is $2.9 \times 10^{24}~\rm yr$ using a total $^{136}\rm Xe$ exposure of $234.1~\rm kg~yr$. No statistically significant evidence for $2νββ$ decay to the $0^+_1$ state is observed, leading to a lower limit of $T^{2ν}_{1/2}(0^+ \rightarrow 0^+_1) > 1.4\times10^{24}~\rm yr$ at 90$\%$ confidence level, improved by 70$\%$ relative to the current world's best constraint.

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arXiv2023

An integrated online radioassay data storage and analytics tool for nEXO

Large-scale low-background detectors are increasingly used in rare-event searches as experimental collaborations push for enhanced sensitivity. However, building such detectors, in practice, creates an abundance of radioassay data especially during the conceptual phase of an experiment when hundreds of materials are screened for radiopurity. A tool is needed to manage and make use of the radioassay screening data to quantitatively assess detector design options. We have developed a Materials Database Application for the nEXO experiment to serve this purpose. This paper describes this database, explains how it functions, and discusses how it streamlines the design of the experiment.

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arXiv2023

Generative Adversarial Networks for Scintillation Signal Simulation in EXO-200

Generative Adversarial Networks trained on samples of simulated or actual events have been proposed as a way of generating large simulated datasets at a reduced computational cost. In this work, a novel approach to perform the simulation of photodetector signals from the time projection chamber of the EXO-200 experiment is demonstrated. The method is based on a Wasserstein Generative Adversarial Network - a deep learning technique allowing for implicit non-parametric estimation of the population distribution for a given set of objects. Our network is trained on real calibration data using raw scintillation waveforms as input. We find that it is able to produce high-quality simulated waveforms an order of magnitude faster than the traditional simulation approach and, importantly, generalize from the training sample and discern salient high-level features of the data. In particular, the network correctly deduces position dependency of scintillation light response in the detector and correctly recognizes dead photodetector channels. The network output is then integrated into the EXO-200 analysis framework to show that the standard EXO-200 reconstruction routine processes the simulated waveforms to produce energy distributions comparable to that of real waveforms. Finally, the remaining discrepancies and potential ways to improve the approach further are highlighted.

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arXiv2023

Fundamental Symmetries, Neutrons, and Neutrinos (FSNN): Whitepaper for the 2023 NSAC Long Range Plan

This whitepaper presents the research priorities decided on by attendees of the 2022 Town Meeting for Fundamental Symmetries, Neutrons and Neutrinos, which took place December 13-15, 2022 in Chapel Hill, NC, as part of the Nuclear Science Advisory Committee (NSAC) 2023 Long Range Planning process. A total of 275 scientists registered for the meeting. The whitepaper makes a number of explicit recommendations and justifies them in detail.

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arXiv2023

Search for MeV Electron Recoils from Dark Matter in EXO-200

We present a search for electron-recoil signatures from the charged-current absorption of fermionic dark matter using the EXO-200 detector. We report an average electron recoil background rate of $6.8 \times 10^{-4}\, \mathrm{cts}\,\mathrm{kg}^{-1}\mathrm{yr}^{-1}\mathrm{keV}^{-1}$ above $4\,\mathrm{MeV}$ and find no statistically significant excess over our background projection. Using a total ${}^{136}\mathrm{Xe}$ exposure of $234.1\,\mathrm{kg}\,\mathrm{yr}$ we exclude new parameter space for the charged-current absorption cross-section for dark matter masses between $m_χ= 2.6\,\mathrm{MeV} - 11.6\,\mathrm{MeV}$ with a minimum of $6\times 10^{-51}\,\mathrm{cm}^2$ at $8.3\,\mathrm{MeV}$ at the $90\%$ confidence level.

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arXiv2022

Performance of novel VUV-sensitive Silicon Photo-Multipliers for nEXO

Liquid xenon time projection chambers are promising detectors to search for neutrinoless double beta decay (0$νββ$), due to their response uniformity, monolithic sensitive volume, scalability to large target masses, and suitability for extremely low background operations. The nEXO collaboration has designed a tonne-scale time projection chamber that aims to search for 0$νββ$ of \ce{^{136}Xe} with projected half-life sensitivity of $1.35\times 10^{28}$~yr. To reach this sensitivity, the design goal for nEXO is $\leq$1\% energy resolution at the decay $Q$-value ($2458.07\pm 0.31$~keV). Reaching this resolution requires the efficient collection of both the ionization and scintillation produced in the detector. The nEXO design employs Silicon Photo-Multipliers (SiPMs) to detect the vacuum ultra-violet, 175 nm scintillation light of liquid xenon. This paper reports on the characterization of the newest vacuum ultra-violet sensitive Fondazione Bruno Kessler VUVHD3 SiPMs specifically designed for nEXO, as well as new measurements on new test samples of previously characterised Hamamatsu VUV4 Multi Pixel Photon Counters (MPPCs). Various SiPM and MPPC parameters, such as dark noise, gain, direct crosstalk, correlated avalanches and photon detection efficiency were measured as a function of the applied over voltage and wavelength at liquid xenon temperature (163~K). The results from this study are used to provide updated estimates of the achievable energy resolution at the decay $Q$-value for the nEXO design.

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arXiv2022

NEXO: Neutrinoless double beta decay search beyond $10^{28}$ year half-life sensitivity

The nEXO neutrinoless double beta decay experiment is designed to use a time projection chamber and 5000 kg of isotopically enriched liquid xenon to search for the decay in $^{136}$Xe. Progress in the detector design, paired with higher fidelity in its simulation and an advanced data analysis, based on the one used for the final results of EXO-200, produce a sensitivity prediction that exceeds the half-life of $10^{28}$ years. Specifically, improvements have been made in the understanding of production of scintillation photons and charge as well as of their transport and reconstruction in the detector. The more detailed knowledge of the detector construction has been paired with more assays for trace radioactivity in different materials. In particular, the use of custom electroformed copper is now incorporated in the design, leading to a substantial reduction in backgrounds from the intrinsic radioactivity of detector materials. Furthermore, a number of assumptions from previous sensitivity projections have gained further support from interim work validating the nEXO experiment concept. Together these improvements and updates suggest that the nEXO experiment will reach a half-life sensitivity of $1.35\times 10^{28}$ yr at 90% confidence level in 10 years of data taking, covering the parameter space associated with the inverted neutrino mass ordering, along with a significant portion of the parameter space for the normal ordering scenario, for almost all nuclear matrix elements. The effects of backgrounds deviating from the nominal values used for the projections are also illustrated, concluding that the nEXO design is robust against a number of imperfections of the model.

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arXiv2022

Development of a $^{127}$Xe calibration source for nEXO

We study a possible calibration technique for the nEXO experiment using a $^{127}$Xe electron capture source. nEXO is a next-generation search for neutrinoless double beta decay ($0νββ$) that will use a 5-tonne, monolithic liquid xenon time projection chamber (TPC). The xenon, used both as source and detection medium, will be enriched to 90% in $^{136}$Xe. To optimize the event reconstruction and energy resolution, calibrations are needed to map the position- and time-dependent detector response. The 36.3 day half-life of $^{127}$Xe and its small $Q$-value compared to that of $^{136}$Xe $0νββ$ would allow a small activity to be maintained continuously in the detector during normal operations without introducing additional backgrounds, thereby enabling in-situ calibration and monitoring of the detector response. In this work we describe a process for producing the source and preliminary experimental tests. We then use simulations to project the precision with which such a source could calibrate spatial corrections to the light and charge response of the nEXO TPC.

physics.ins-det↗

arXiv2021

The EXO-200 detector, part II: Auxiliary Systems

The EXO-200 experiment searched for neutrinoless double-beta decay of $^{136}$Xe with a single-phase liquid xenon detector. It used an active mass of 110 kg of 80.6%-enriched liquid xenon in an ultra-low background time projection chamber with ionization and scintillation detection and readout. This paper describes the design and performance of the various support systems necessary for detector operation, including cryogenics, xenon handling, and controls. Novel features of the system were driven by the need to protect the thin-walled detector chamber containing the liquid xenon, to achieve high chemical purity of the Xe, and to maintain thermal uniformity across the detector.

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arXiv2021

Proton inelastic scattering reveals deformation in $^8$He

A measurement of proton inelastic scattering of $^8$He at $8.25A$~MeV at TRIUMF shows a resonance at 3.54(6)~MeV with a width of 0.89(11)~MeV. The energy of the state is in good agreement with coupled cluster and no-core shell model with continuum calculations, with the latter successfully describing the measured resonance width as well. Its differential cross section analyzed with phenomenological collective excitation form factor and microscopic coupled reaction channels framework consistently reveals a large deformation parameter $β_2$ = 0.40(3), consistent with no-core shell model predictions of a large neutron deformation. This deformed double-closed shell at the neutron drip-line opens a new paradigm.

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arXiv2021

First direct measurement of $^{59}$Cu(p,$α$)$^{56}$Ni: A step towards constraining the Ni-Cu cycle in the Cosmos

Reactions on the proton-rich nuclides drive the nucleosynthesis in Core-Collapse Supernovae (CCSNe) and in X-ray bursts (XRBs). CCSNe eject the nucleosynthesis products to the interstellar medium and hence are a potential inventory of p-nuclei, whereas in XRBs nucleosynthesis powers the light curves. In both astrophysical sites the Ni-Cu cycle, which features a competition between $^{59}$Cu(p,$α$)$^{56}$Ni and $^{59}$Cu(p,$γ$)$^{60}$Zn, could potentially halt the production of heavier elements. Here, we report the first direct measurement of $^{59}$Cu(p,$α$)$^{56}$Ni using a re-accelerated $^{59}$Cu beam and cryogenic solid hydrogen target. Our results show that the reaction proceeds predominantly to the ground state of $^{56}$Ni and the experimental rate has been found to be lower than Hauser-Feshbach-based statistical predictions. New results hint that the $νp$-process could operate at higher temperatures than previously inferred and therefore remains a viable site for synthesizing the heavier elements.

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arXiv2021

Reflectivity of VUV-sensitive Silicon Photomultipliers in Liquid Xenon

Silicon photomultipliers are regarded as a very promising technology for next-generation, cutting-edge detectors for low-background experiments in particle physics. This work presents systematic reflectivity studies of Silicon Photomultipliers (SiPM) and other samples in liquid xenon at vacuum ultraviolet (VUV) wavelengths. A dedicated setup at the University of Münster has been used that allows to acquire angle-resolved reflection measurements of various samples immersed in liquid xenon with 0.45° angular resolution. Four samples are investigated in this work: one Hamamatsu VUV4 SiPM, one FBK VUV-HD SiPM, one FBK wafer sample and one Large-Area Avalanche Photodiode (LA-APD) from EXO-200. The reflectivity is determined to be 25-36% at an angle of incidence of 20° for the four samples and increases to up to 65% at 70° for the LA-APD and the FBK samples. The Hamamatsu VUV4 SiPM shows a decline with increasing angle of incidence. The reflectivity results will be incorporated in upcoming light response simulations of the nEXO detector.

physics.ins-det↗

arXiv2021

Event Reconstruction in a Liquid Xenon Time Projection Chamber with an Optically-Open Field Cage

nEXO is a proposed tonne-scale neutrinoless double beta decay ($0νββ$) experiment using liquid ${}^{136}Xe$ (LXe) in a Time Projection Chamber (TPC) to read out ionization and scintillation signals. Between the field cage and the LXe vessel, a layer of LXe ("skin" LXe) is present, where no ionization signal is collected. Only scintillation photons are detected, owing to the lack of optical barrier around the field cage. In this work, we show that the light originating in the skin LXe region can be used to improve background discrimination by 5% over previous published estimates. This improvement comes from two elements. First, a fraction of the $γ$-ray background is removed by identifying light from interactions with an energy deposition in the skin LXe. Second, background from ${}^{222}Rn$ dissolved in the skin LXe can be efficiently rejected by tagging the $α$ decay in the ${}^{214}Bi-{}^{214}Po$ chain in the skin LXe.

physics.ins-det↗

arXiv2020

Single-particle structure in neutron-rich Sr isotopes approaching the N = 60 shape transition

Background: Neutron-rich nuclei around neutron number N = 60 show a dramatic shape transition from spherical ground states to prolate deformation in 98Sr and heavier nuclei. Purpose: The purpose of this study is to investigate the single-particle structure approaching the shape transitional region. Method: The level structures of neutron-rich 93,94,95Sr were studied via the d(94,95,96Sr,t) one-neutron stripping reactions at TRIUMF using a beam energy of 5.5 AMeV. γ-rays emitted from excited states and recoiling charged particles were detected by using the TIGRESS and SHARC arrays, respectively. States were identified by gating on the excitation energy and, if possible, the coincident γ radiation. Results: Triton angular distributions for the reactions populating states in ejectile nuclei 93,94,95Sr were compared with distorted wave Born approximation calculations to assign and revise spin and parity quantum numbers and extract spectroscopic factors. The results were compared with shell model calculations and the reverse (d,p) reactions and good agreement was obtained. Conclusions: The results for the d(94Sr,t)93Sr and d(95Sr,t)94Sr reactions are in good agreement with shell model calculations. A two level mixing analysis for the 0+ states in 94Sr suggest strong mixing of two shapes. For the d(96Sr,t)95Sr reaction the agreement with the shell model is less good. The configuration of the ground state of 96Sr is already more complex than predicted, and therefore indications for the shape transition can already be observed before N = 60.

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arXiv2020

Decay Spectroscopy of $^{129}$Cd

Excited states of $^{129}$In populated following the $β$-decay of $^{129}$Cd were experimentally studied with the GRIFFIN spectrometer at the ISAC facility of TRIUMF, Canada. A 480-MeV proton beam was impinged on a uranium carbide target and $^{129}$Cd was extracted using the Ion Guide Laser Ion Source (IG-LIS). $β$- and $γ$-rays following the decay of $^{129}$Cd were detected with the GRIFFIN spectrometer comprising the plastic scintillator SCEPTAR and 16 high-purity germanium (HPGe) clover-type detectors. %, along with the $β$-particles were detected with SCEPTAR. From the $β$-$γ$-$γ$ coincidence analysis, 32 new transitions and 7 new excited states were established, expanding the previously known level scheme of $^{129}$In. The $\log ft$ values deduced from the $β$-feeding intensities suggest that some of the high-lying states were populated by the $ν0 g_{7/2} \rightarrow π0 g_{9/2}$ allowed Gamow-Teller (GT) transition, which indicates that the allowed GT transition is more dominant in the $^{129}$Cd decay than previously reported. Observation of fragmented Gamow-Teller strengths is consistent with theoretical calculations.

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