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R. L. Stamps

Publications and source records attributed to R. L. Stamps.

At least 19 recordsLinked to original sources

Scale-dependent universality class crossover in magnetic skyrmion polymers

Dipolar magnetic skyrmions can assemble into chains with alternating helicity that act as one-dimensional polymers, yet their statistical mechanics violates the universal harmonic scaling observed in actin, DNA, and microtubules. From first principles, we compute the inter-skyrmion pair potential and find a bi-exponential form of competing interactions with two characteristic decay lengths that encode the distinct microscopic mechanisms of repulsion and attraction. Multiscale simulations reveal a power-law temperature dependence with exponent $1$ in the worm-chain limit of a single bond, and exponent $1/2$ in the three-bond limit. We find that the power-law behavior is remarkably independent of magnetic field strength, and the crossover is due to competing radial interactions responsible for the bonds, resulting in a quartic transverse confinement. We show that the precise form of the competing interactions (e.g., Morse or double-Yukawa) does not affect the temperature dependence.

cond-mat.soft

Path sampling for lifetimes of metastable magnetic skyrmions and direct comparison with Kramers' method

We perform a direct comparison between Kramers' method in many dimensions -- i.e., Langer's theory -- adapted to magnetic spin systems, and a path sampling method in the form of forward flux sampling, as a means to compute collapse rates of metastable magnetic skyrmions. We show that a good agreement is obtained between the two methods. We report variations of the attempt frequency associated with skyrmion collapse by three to four orders of magnitude when varying the applied magnetic field by 5$\%$ of the exchange strength, which confirms the existence of a strong entropic contribution to the lifetime of skyrmions. This demonstrates that in complex systems, the knowledge of the rate prefactor, in addition to the internal energy barrier, is essential in order to properly estimate a lifetime.

cond-mat.mes-hall

Thermal stability of metastable magnetic skyrmions: Entropic narrowing and significance of internal eigenmodes

We compute annihilation rates of metastable magnetic skyrmions using a form of Langer's theory in the intermediate-to-high damping (IHD) regime. For a Néel skyrmion, a Bloch skyrmion, and an antiskyrmion, we look at two possible paths to annihilation: collapse and escape through a boundary. We also study the effects of a curved vs. a flat boundary, a second skyrmion and a non-magnetic defect. We find that the skyrmion's internal modes play a dominant role in the thermally activated transitions compared to the spin-wave excitations and that the relative contribution of internal modes depends on the nature of the transition process. Our calculations for a small skyrmion stabilized at zero-field show that collapse on a defect is the most probable path. In the absence of a defect, the annihilation is largely dominated by escape mechanisms, even though in this case the activation energy is higher than that of collapse processes. Escape through a flat boundary is found more probable than through a curved boundary. The potential source of stability of metastable skyrmions is therefore found not to lie in high activation energies, nor in the dynamics at the transition state, but comes from entropic narrowing in the saddle point region which leads to lowered attempt frequencies. This narrowing effect is found to be primarily associated with the skyrmion's internal modes.

cond-mat.mes-hall

Paths to annihilation of first and second-order (anti)skyrmions via (anti)meron nucleation on the frustrated square lattice

We study annihilation mechanisms of small first- and second-order skyrmions and antiskyrmions on the frustrated $J_1-J_2-J_3$ square lattice with broken inversion symmetry (DMI). We find that annihilation happens via the injection of the opposite topological charge in the form of meron or antimeron nucleation. Overall, the exchange frustration generates a complex energy landscape with not only many (meta)stable and unstable local energy solutions, but also many possible paths connecting them. Whenever possible, we compute the activation energy and attempt frequency for the annihilation of isolated topological defects. In particular, we compare the average lifetime of the antiskyrmion calculated with transition state theory with direct Langevin simulations, where an excellent agreement is obtained.

cond-mat.mes-hall

Level Attraction Due to Dissipative Magnon-Photon Coupling

We report dissipative magnon-photon coupling caused by cavity Lenz effect, where the magnons in a magnet induce a rf current in the cavity, leading to a cavity back action that impedes the magnetization dynamics. This effect is revealed in our experiment as level attraction with a coalescence of hybridized magnon-photon modes, which is distinctly different from level repulsion with mode anticrossing caused by coherent magnon-photon coupling. We develop a method to control the in- terpolation of coherent and dissipative magnon-photon coupling, and observe a matching condition where the two effects cancel. Our work sheds light on the so-far hidden side of magnon-photon coupling, opening a new avenue for controlling and utilizing light-matter interactions.

cond-mat.mes-hall

Internal structure of hexagonal skyrmion lattices in cubic helimagnets

We have utilised a high spatial resolution imaging method, Differential Phase Contrast (DPC) performed in a scanning transmission electron microscope (STEM), for precise measurement of the magnetic induction distribution in skyrmion states in noncentrosymmetric magnetically ordered materials. Applied to investigate the internal structure of hexagonal skyrmion lattice cells, stabilised by an out-plane applied magnetic field in an FeGe nanowedge specimen, mapping of the in-plane component of magnetic induction has yielded "average" skyrmion profiles and observation of internal six-fold symmetry. With increasing field strength, the diameter of "average" skyrmion cores was observed to decrease accompanied by a non-linear variation of the lattice periodicity. Variations in structure for individual skyrmions were studied utilising an advanced DPC detection scheme with a variety of symmetry lowering distortions being observed. Our observations are consistent with a theoretical phenomenological model, which has predicted the structure of hexagonal skyrmion lattice cells and also that twisting states near to the material surfaces provide a basis for energetic stabilisation of the skyrmion lattice over the conical phase. There was good agreement with experiment for predictions of bulk skyrmion structure and their response (core-size & lattice periodicity variation) to an applied field.

cond-mat.mes-hall

Vogel-Fulcher-Tammann Freezing of a Thermally Fluctuating Artificial Spin Ice Probed by X-ray Photon Correlation Spectroscopy

We report on the crossover from the thermal to athermal regime of an artificial spin ice formed from a square array of magnetic islands whose lateral size, 30~nm~$\times$~70~nm, is small enough that they are superparamagnetic at room temperature. We used resonant magnetic soft x-ray photon correlation spectroscopy (XPCS) as a method to observe the time-time correlations of the fluctuating magnetic configurations of spin ice during cooling, which are found to slow abruptly as a freezing temperature $T_0 = 178 \pm 5$~K is approached. This slowing is well-described by a Vogel-Fulcher-Tammann law, implying that the frozen state is glassy, with the freezing temperature being commensurate with the strength of magnetostatic interaction energies in the array. The activation temperature, $T_\mathrm{A} = 40 \pm 10$~K, is much less than that expected from a Stoner-Wohlfarth coherent rotation model. Zero-field-cooled/field-cooled magnetometry reveals a freeing up of fluctuations of states within islands above this temperature, caused by variation in the local anisotropy axes at the oxidised edges. This Vogel-Fulcher-Tammann behavior implies that the system enters a glassy state on freezing, which is unexpected for a system with a well-defined ground state.

cond-mat.dis-nn

Chiral surface twists and skyrmion stability in nanolayers of cubic helimagnets

Lorentz transmission electron microscopy (LTEM) investigations of modulated states in a FeGe wedge and detailed calculations demonstrate that chiral twists arising near the surfaces of noncentrosymmetric ferromagnets (Meynell et al. Phys. Rev. B, 90, 014406 (2014)) provide a stabilization mechanism for skyrmion lattices and helicoids in cubic helimagnet nanolayers. The calculated magnetic phase diagram for free standing cubic helimagnet nanolayers shows that magnetization processes in these compounds fundamentally differ from those in bulk cubic helimagnets and are characterized by the first-order transitions between modulated phases and the formation of specific multidomain states. The paper reports LTEM observations of multidomain patterns in FeGe free-standing nanolayers.

cond-mat.mes-hall

Study of strong photon-magnon coupling in a YIG-film split-ring resonant system

By using the stripline Microwave Vector Network Analyzer Ferromagnetic Resonance and Pulsed Inductive Microwave Magnetometry spectroscopy techniques, we study a strong coupling regime of magnons to microwave photons in the planar geometry of a lithographically formed split-ring resonator (SRR) loaded by a single-crystal epitaxial yttrium-iron garnet (YIG) film. Strong anti-crossing of the photon modes of SRR and of the magnon modes of the YIG film is observed in the applied-magnetic-field resolved measurements. The coupling strength extracted from the experimental data reaches 9 percent at 3 GHz. Theoretically, we propose an equivalent circuit model of an SRR loaded by a magnetic film. This model follows from the results of our numerical simulations of the microwave field structure of the SRR and of the magnetization dynamics in the YIG film driven by the microwave currents in the SRR. The equivalent circuit model is in good agreement with the experiment. It provides a simple physical explanation of the process of mode anti-crossing. Our findings are important for future applications in microwave quantum photonic devices as well as in magnetically tunable metamaterials exploiting the strong coupling of magnons to microwave photons.

cond-mat.mtrl-sci

Standing spin-wave mode structure and linewidth in partially disordered perpendicularly magnetized sub-micron Permalloy disc arrays

Standing spin wave mode frequencies and linewidths in partially disordered perpendicular magnetized arrays of sub-micron Permalloy discs are measured using broadband ferromagnetic resonance and compared to analytical results from a single, isolated disc. The measured mode structure qualitatively reproduces the structure expected from the theory. Fitted demagnetizing parameters decrease with increasing array disorder. The frequency difference between the first and second radial modes is found to be higher in the measured array systems than predicted by theory for an isolated disc. The relative frequencies between successive spin wave modes are unaffected by reduction of the long-range ordering of discs in the array. An increase in standing spin wave resonance linewidth at low applied magnetic fields is observed and grows more severe with increased array disorder.

cond-mat.mes-hall

Emergence of skyrmion lattices and bimerons in diluted chiral magnetic thin films

Skyrmions are topologically protected field configurations with particle-like properties that play important roles in various fields of science. Recently, skyrmions have been directly observed in chiral magnets. Here, we investigate the effects of nonmagnetic impurities (structural point-like defects) on the different initial states (random or helical states) and on the formation of the skyrmion crystal in a discrete lattice. By using first-principle calculations and Monte Carlo techniques, we have shown that even a small percentage of spin vacancies present in the chiral magnetic thin film affects considerably the skyrmion order. The main effects of impurities are somewhat similar to thermal effects. The presence of these spin vacancies also induces the formation of compact merons (bimerons) in both the helical and skyrmion states. We have also investigated the effects of adjacent impurities producing only one hole (with an almost circular shape) intentionally inserted into the plate (forming a non-simply connected manifold) on the skyrmion crystal.

cond-mat.str-el

Spatially periodic domain wall pinning potentials: Asymmetric pinning and dipolar biasing

Domain wall propagation has been measured in continuous, weakly disordered, quasi-two-dimensional, Ising-like magnetic layers that are subject to spatially periodic domain wall pinning potentials. The potentials are generated non-destructively using the stray magnetic field of ordered arrays of magnetically hard [Co/Pt]$_m$ nanoplatelets which are patterned above and are physically separated from the continuous magnetic layer. The effect of the periodic pinning potentials on thermally activated domain wall creep dynamics is shown to be equivalent, at first approximation, to that of a uniform, effective retardation field, $H_{ret}$, which acts against the applied field, $H$. We show that $H_{ret}$ depends not only on the array geometry but also on the relative orientation of $H$ and the magnetization of the nanoplatelets. A result of the latter dependence is that wall-mediated hysteresis loops obtained for a set nanoplatelet magnetization exhibit many properties that are normally associated with ferromagnet/antiferromagnet exchange bias systems. These include a switchable bias, coercivity enhancement and domain wall roughness that is dependent on the applied field polarity.

cond-mat.mes-hall

Disorder strength and field-driven ground state domain formation in artificial spin ice: experiment, simulation and theory

Quenched disorder affects how non-equilibrium systems respond to driving. In the context of artificial spin ice, an athermal system comprised of geometrically frustrated classical Ising spins with a two-fold degenerate ground state, we give experimental and numerical evidence of how such disorder washes out edge effects, and provide an estimate of disorder strength in the experimental system. We prove analytically that a sequence of applied fields with fixed amplitude is unable to drive the system to its ground state from a saturated state. These results should be relevant for other systems where disorder does not change the nature of the ground state.

cond-mat.mes-hall

Domain dynamics and fluctuations in artificial square ice at finite temperatures

The thermally-driven formation and evolution of vertex domains is studied for square artificial spin ice. A self consistent mean field theory is used to show how domains of ground state ordering form spontaneously, and how these evolve in the presence of disorder. The role of fluctuations is studied, using Monte Carlo simulations and analytical modelling. Domain wall dynamics are shown to be driven by a biasing of random fluctuations towards processes that shrink closed domains, and fluctuations within domains are shown to generate isolated small excitations, which may stabilise as the effective temperature is lowered. Domain dynamics and fluctuations are determined by interaction strengths, which are controlled by inter-element spacing. The role of interaction strength is studied via experiments and Monte Carlo simulations. Our mean field model is applicable to ferroelectric `spin' ice, and we show that features similar to that of magnetic spin ice can be expected, but with different characteristic temperatures and rates.

cond-mat.stat-mech

Interfacial coupling across a modified interface studied with ferromagnetic resonance

Using spin waves we directly probe the interface of an exchange biased Ni$_{80}$Fe$_{20}$/Ir$_{25}$Mn$_{75}$ film which has been modified by the presence of an Au dusting layer. Combining this experimental data with a discretised simulation model, parameters relating to interface exchange coupling and modification of interface magnetisation are determined. Exchange coupling is found to be relatively uniform as gold thickness is increased, and undergoes a sudden drop at 1.5$\textrmÅ$ of gold. Interface magnetisation decreases as a function of the gold dusting thickness. Antiparallel alignment of the ferromagnet and antiferromagnet supress the interface magnetisation compared to when they are in parallel alignment. These findings imply that the interface region has specific magnetisation states which depend on the ferromagnet orientation.

cond-mat.mes-hall

Diversity enabling equilibration: disorder and the ground state in artificial spin ice

We report a novel approach to the question of whether and how the ground state can be achieved in square artificial spin ices where frustration is incomplete. We identify two types of disorder: quenched disorder in the island response to fields and disorder in the sequence of driving fields. Numerical simulations show that quenched disorder can lead to final states with lower energy, and disorder in the driving fields always lowers the final energy attained by the system. We use a network picture to understand these two effects: disorder in island responses creates new dynamical pathways, and disorder in driving fields allows more pathways to be followed.

cond-mat.mes-hall

Disorder regimes and equivalence of disorder types in artificial spin ice

The field-induced dynamics of artificial spin ice are determined in part by interactions between magnetic islands, and the switching characteristics of each island. Disorder in either of these affects the response to applied fields. Numerical simulations are used to show that disorder effects are determined primarily by the strength of disorder relative to inter-island interactions, rather than by the type of disorder. Weak and strong disorder regimes exist and can be defined in a quantitative way.

cond-mat.mes-hall

Model of bound interface dynamics for coupled magnetic domain walls

A domain wall in a ferromagnetic system will move under the action of an external magnetic field. Ultrathin Co layers sandwiched between Pt have been shown to be a suitable experimental realization of a weakly disordered 2D medium in which to study the dynamics of 1D interfaces (magnetic domain walls). The behavior of these systems is encapsulated in the velocity-field response v(H) of the domain walls. In a recent paper [P.J. Metaxas et al., Phys. Rev. Lett. 104, 237206 (2010)] we studied the effect of ferromagnetic coupling between two such ultrathin layers, each exhibiting different v(H) characteristics. The main result was the existence of bound states over finite-width field ranges, wherein walls in the two layers moved together at the same speed. Here, we discuss in detail the theory of domain wall dynamics in coupled systems. In particular, we show that a bound creep state is expected for vanishing H and we give the analytical, parameter free expression for its velocity which agrees well with experimental results.

cond-mat.mtrl-sci