arXiv subjects

R. Lica

Publications and source records attributed to R. Lica.

16 recordsLinked to original sources

arXiv2026

Exploring $\alpha$- and $\beta$-decay-induced quenching of the $^{229}$Th nuclear-clock isomer in solid-state hosts

The radiative decay dynamics of an ensemble of $^{229\mathrm{m}}$Th nuclei embedded in CaF$_2$ and MgF$_2$ is investigated. The isomer is populated through $\beta$ decay of $^{229}$Ac following ion implantation, and its radiative decay is detected using vacuum-ultraviolet spectroscopy and measured as a function of time. This allows to identify and quantify the quenching of the radiative-decay signal induced by $\alpha$ or $\beta$ radiation. The quenching probability density is determined in different CaF$_2$ crystals and in a MgF$_2$ crystal, revealing differences up to two orders of magnitude between the investigated samples and a strong dependence on the host material and defect densities. The results support a microscopic mechanism mediated by charge carriers in which electronic excitations created by the decay radiation are captured near Th defects, thereby favoring non-radiative decay channels.

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arXiv2025

Modern approach to muonic x-ray spectroscopy demonstrated through the measurement of stable Cl radii

Recent advances in muonic x-ray experiments have reinvigorated efforts in measurements of absolute nuclear charge radii. Here, a modern approach is presented, and demonstrated through determination of the charge radii of the two stable chlorine nuclides $^{35}$Cl and $^{37}$Cl. Knowledge of these radii has implications for fundamental studies in nuclear and atomic physics. For this purpose, a state-of-the-art experiment was performed at the $\pi$E1 beamline in the Paul Scherrer Institute (Switzerland), using a large-scale HPGe detector array in order to extract precise energies of the muonic $^{35}$Cl and $^{37}$Cl $np1s$ transitions. The nuclear charge radius extraction relies on modern calculations for QED effects and nuclear polarization with rigorous uncertainty quantification, including effects that were not accounted for in older studies. Additionally, we established a new method for applying the nuclear shape correction directly from energy density functionals, which are amenable to isotopes for which no high-quality electron scattering experiments are available. The resulting charge radii are $3.3335(23) fm$ for $^{35}$Cl and $3.3445(23) fm$ for $^{37}$Cl, thus improving the uncertainty of the available electron scattering values by a factor of seven. The correlation of several observables was evaluated between the different isotopes in order to produce a more precise value of the differential mean square charge radius $\delta \langle r^2 \rangle^{37, 35}=+0.0771(66) fm^{2}$. In this case, improvement of the uncertainty by more than one order of magnitude was achieved compared to the literature value. This precision is sufficient to use this differential as input for isotope shift factor determination.

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arXiv2025

Nuclear level density of ${}^{128}$Te from $(\mathrm{p},\mathrm{p}'\gamma)$ scattering and complementary photonuclear data

We have extracted the nuclear level density of ${}^{128}$Te from a $(\mathrm{p},\mathrm{p} '\gamma)$ scattering experiment using the large-volume \labr\ and \cebr\ detectors from ELI-NP at the 9~MV Tandem facilities at IFIN-HH. The decay data were normalised using photonuclear data, resulting in nuclear level densities without intrinsic model dependencies from the constant temperature or Fermi gas models. The deduced nuclear level density follows in between the expectations from these two models, but we observe a clear divergence from a microscopic model based on the Skyrme force.

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arXiv2024

Isolated one-phonon mixed-symmetry 2+ state of the radioactive neutron-rich nuclide 132Te

The $M1$ transition strengths between excited $2^+$ states of the neutron-rich, radioactive nuclide $^{132}$Te have been studied through direct lifetime measurements using the Doppler-shift attenuation method in a two-neutron transfer reaction on a $^{130}$Te target. An unambiguous identification of the lowest-lying mixed-symmetry $2^+$ state has been achieved on the basis of the large $B(M1;2^+_2\rightarrow2^+_1$)=0.18(2) $\mu_\mathrm{N}^2$ transition strength, in agreement with shell-model calculations. Results are compared to the shell model, and the analysis of both, data and calculations, unambiguously identifies the second-excited $2^+$ state of $^{132}$Te as the one-quadrupole phonon mixed-symmetry state of this isotope. A lowering of the energy and $B(M1;2^+_\mathrm{ms}\rightarrow 2^+_1)$ strength within the $N$=80 isotones toward the $Z$=50 shell closure is observed, which goes alongside with the lowering of the $E2$ collectivity approaching the magic proton shell.

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arXiv2024

Beta delayed neutron emission of $N=84$ $^{132}$Cd

Using the time-of-flight technique, we measured the beta-delayed neutron emission of $^{132}$Cd. From our large-scale shell model (LSSM) calculation using the N$^3$LO interaction [Z.Y. Xu et al., Phys. Rev. Lett. 131, 022501 (2023)], we suggest the decay is dominated by the transformation of a neutron in the $g_{7/2}$ orbital, deep below the Fermi surface, into a proton in the $g_{9/2}$ orbital. We compare the beta-decay half-lives and neutron branching ratios of nuclei with $Z<50$ and $N\geq82$ obtained with our LSSM with those of leading "global" models such as Finite-Range Droplet Model (FRDM). Our calculations match known half-lives and neutron branching ratios well and suggest that current leading models overestimate the yet-to-be-measured half-lives. Our model, backed by the $^{132}$Cd decay data presented here, offers robust predictive power for nuclei of astrophysical interest such as $r$-process waiting points.

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arXiv2024

Statistical properties and photon strength functions of the ${}^{112,114}$Sn isotopes below the neutron separation threshold

Here, we report on the measurements of the $\gamma$-ray strength functions and nuclear level densities of ${}^{112,114}$Sn performed for the first time at the 9~MV Tandem accelerator facilities at IFIN-HH using the Oslo method. We extract thermodynamic properties and gross and fine properties of the pygmy dipole resonance for systematic comparison in the chain of Sn isotopes. The results are compared with microscopic models implemented in the TALYS reaction code and the fully microscopic quasiparticle-phonon model for the underlying nuclear structure of the dipole strength in ${}^{112,114}$Sn. The quasiparticle-phonon model results show the importance of complex configurations to the low-energy dipole response in the pygmy dipole resonance energy region. The experimental data are further included in the cross-section and reaction rate calculations for the $(\mathrm{n},\gamma)$ reaction of the $p$-process nuclei ${}^{112,114}$Sn showing a significant increase in reaction rates at high temperatures compared to existing nuclear databases.

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arXiv2024

Radiative Decay of the $^{229m}$Th Nuclear Clock Isomer in Different Host Materials

A comparative vacuum ultraviolet spectroscopy study conducted at ISOLDE-CERN of the radiative decay of the $^{229m}$Th nuclear clock isomer embedded in different host materials is reported. The ratio of the number of radiative decay photons and the number of $^{229m}$Th embedded are determined for single crystalline CaF$_2$, MgF$_2$, LiSrAlF$_6$, AlN, and amorphous SiO$_2$. For the latter two materials, no radiative decay signal was observed and an upper limit of the ratio is reported. The radiative decay wavelength was determined in LiSrAlF$_6$ and CaF$_2$, reducing its uncertainty by a factor of 2.5 relative to our previous measurement. This value is in agreement with the recently reported improved values from laser excitation.

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arXiv2023

Simultaneous $γ$-ray and electron spectroscopy of $^{182,184,186}$Hg isotopes

Background: The mercury isotopes around $N=104$ are a well-known example of nuclei exhibiting shape coexistence. Mixing of configurations can be studied by measuring the monopole strength $ρ^2(E0)$, however, currently the experimental information is scarce and lacks precision, especially for the $I^π\rightarrow I^π$ ($I \neq 0$) transitions. Purpose: The goals of this study were to increase the precision of the known branching ratios and internal conversion coefficients, to increase the amount of available information regarding excited states in $^{182,184,186}$Hg and to interpret the results in the framework of shape coexistence using different models. Method: The low-energy structures in $^{182,184,186}$Hg were populated in the $β$ decay of $^{182,184,186}$Tl, produced at ISOLDE and purified by laser ionization and mass separation. The $γ$-ray and internal conversion electron events were detected by five germanium clover detectors and a segmented silicon detector, respectively, and correlated in time to build decay schemes. Results: In total, 193, 178 and 156 transitions, including 144, 140 and 108 observed for the first time in a $β$-decay experiment, were assigned to $^{182,184,186}$Hg, respectively. Internal conversion coefficients were determined for 23 transitions, out of which 12 had an $E0$ component. Extracted branching ratios allowed the sign of the interference term in $^{182}$Hg as well as $ρ^2(E0;0^+_2\rightarrow 0^+_1)$ and $B(E2;0^+_2\rightarrow 2^+_1)$ in $^{184}$Hg to be determined. By means of electron-electron coincidences, the $0^+_3$ state was identified in $^{184}$Hg. The experimental results were qualitatively reproduced by five theoretical approaches, the IBM with configuration mixing with two different parametrizations, the General Bohr Hamiltonian, the BMF model and the SCCM model. However, a quantitative description is lacking.

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arXiv2020

Decay studies of the long-lived states in $^{186}$Tl

Decay spectroscopy of the long-lived states in $^{186}$Tl has been performed at the ISOLDE Decay Station at ISOLDE, CERN. The $α$ decay from the low-spin $(2^-)$ state in $^{186}$Tl was observed for the first time and a half-life of $3.4^{+0.5}_{-0.4}$ s was determined. Based on the $α$-decay energy, the relative positions of the long-lived states were fixed, with the $(2^-)$ state as the ground state, the $7^{(+)}$ state at 77(56)~keV and the $10^{(-)}$ state at 451(56) keV. The level scheme of the internal decay of the $^{186}$Tl($10^{(-)}$) state ($T_{1/2} = 3.40(9)$ s), which was known to decay solely through emission of 374 keV $γ$-ray transition, was extended and a lower-limit for the $β$-decay branching $b_β> 5.9(3)\%$ was determined. The extracted retardation factors for the $γ$ decay of the $10^{(-)}$ state were compared to the available data in neighboring odd-odd thallium isotopes indicating the importance of the $πd_{3/2}$ shell in the isomeric decay and significant structure differences between $^{184}$Tl and $^{186}$Tl.

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arXiv2020

Shape Coexistence at Zero Spin in 64Ni Driven by the Monopole Tensor Interaction

The low-spin structure of the semimagic 64Ni nucleus has been considerably expanded: combining four experiments, several 0+ and 2+ excited states were identified below 4.5 MeV, and their properties established. The Monte Carlo shell model accounts for the results and unveils an unexpectedly complex landscape of coexisting shapes: a prolate 0+ excitation is located at a surprisingly high energy (3463 keV), with a collective 2+ state 286 keV above it, the first such observation in Ni isotopes. The evolution in excitation energy of the prolate minimum across the neutron N = 40 subshell gap highlights the impact of the monopole interaction and its variation in strength with N.

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arXiv2020

Detailed spectroscopy of doubly magic $^{132}$Sn

The structure of the doubly magic $^{132}_{50}$Sn$_{82}$ has been investigated at the ISOLDE facility at CERN, populated both by the $β^-$decay of $^{132}$In and $β^-$-delayed neutron emission of $^{133}$In. The level scheme of $^{132}$Sn is greatly expanded with the addition of 68 $γ$-transitions and 17 levels observed for the first time in the $β$ decay. The information on the excited structure is completed by new $γ$-transitions and states populated in the $β$-n decay of $^{133}$In. Improved delayed neutron emission probabilities are obtained both for $^{132}$In and $^{133}$In. Level lifetimes are measured via the Advanced Time-Delayed $βγγ$(t) fast-timing method. An interpretation of the level structure is given based on the experimental findings and the particle-hole configurations arising from core excitations both from the \textit{N} = 82 and \textit{Z} = 50 shells, leading to positive and negative parity particle-hole multiplets. The experimental information provides new data to challenge the theoretical description of $^{132}$Sn.

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arXiv2019

High-resolution study of excited states in 158Gd with (p,t) reactions

The excitation spectra in the deformed nucleus 158Gd have been studied with high energy resolution by means of the (p,t) reaction using the Q3D spectrograph facility at the Munich Tandem accelerator. The angular distributions of tritons were measured for more than 200 excited states seen in the triton spectra up to 4.3 MeV. A number of 36 excited 0+ states (five tentative), have been assigned by comparison of experimental angular distributions with the calculated ones using the CHUCK code. Assignments for levels with higher spins are the following: 95 for 2+ states, 64 for 4+ states, 14 for 6+ states and about 20 for negative parity states. Sequences of states which can be treated as rotational bands are selected. The analysis of the moments of inertia defined for these bands is carried out. This high number of excited states in a deformed nucleus, close to a complete level scheme, constitutes a very good ground to check models of nuclear structure. The large ensembles of states with the same spin-parity offer unique opportunities for statistical analysis. Such an analysis for the 0+, 2+ and 4+ states sequences, for all K-values and for well-determined projections K of the angular momentum is performed. The obtained data may indicate on a K symmetry breaking. Experimental data are compared with interacting boson model (IBM) calculations using the spdf version of the model. The energies of the low-lying levels, the transition probabilities in the first bands and the distribution in transfer intensity of the 0+ states are calculated and compared with experiment.

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arXiv2019

Normal and intruder configurations in $^{34}$Si populated in the $β^-$ decay of $^{34}$Mg and $^{34}$Al

The structure of $^{34}$Si was studied through $γ$ spectroscopy separately in the $β^-$ decays of $^{34}$Mg and $^{34}$Al at the ISOLDE facility of CERN. Different configurations in $^{34}$Si were populated independently from the two recently identified $β$-decaying states in $^{34}$Al having spin-parity assignments $J^π= 4^-$ dominated by the normal configuration $π(d_{5/2})^{-1} \otimes ν(f_{7/2})$ and $J^π= 1^+$ by the intruder configuration $π(d_{5/2})^{-1} \otimes ν(d_{3/2})^{-1}(f_{7/2})^{2}$. The paper reports on spectroscopic properties of $^{34}$Si such as an extended level scheme, spin and parity assignments based on log($ft$) values and $γ$-ray branching ratios, absolute $β$ feeding intensities and neutron emission probabilities. A total of 11 newly identified levels and 26 transitions were added to the previously known level scheme of $^{34}$Si. Large scale shell-model calculations using the {\sc sdpf-u-mix} interaction, able to treat higher order intruder configurations, are compared with the new results and conclusions are drawn concerning the predictive power of {\sc sdpf-u-mix}, the $N=20$ shell gap, the level of mixing between normal and intruder configurations for the 0$_1^+$, 0$_2^+$ and 2$_1^+$ states and the absence of triaxial deformation in $^{34}$Si.

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arXiv2019

Excited states of the odd-odd nucleus 158Eu from the (d,alpha) reaction

Excited states in the 158Eu nucleus have been determined with the 160Gd(d, alpha)158Eu reaction, studied at an incident energy of 18.0 MeV with the Munich tandem and the Q3D spectrograph. More than 50 excited states have been determined up to 1.6 MeV excitation, some of them corresponding to states previously observed in the beta-decay of 158Sm. The number of levels found in this nucleus at low excitation energies follows the systematic trend of the level densities in the other isotopes with mass 152-156.

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arXiv2018

New data on $0^+$ states in $^{158}$Gd

Excited states in the deformed nucleus $^{158}$Gd have been studied in the (p,t) reaction by using the Munich Tandem and Q3D spectrograph. 30 new excited 0$^+$ states (three tentative) have been assigned up to the 4.3 MeV excitation energy. The total number of 34 excited 0$^+$ states (four tentatively assigned) in a deformed nucleus, close to a complete level scheme, offers a new opportunity to test nuclear models and obtain more information on the structure of these special states.

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arXiv2018

First Accurate Normalization of the $β$-delayed $α$ Decay of $^{16}$N and Implications for the $^{12}$C$(α,γ)^{16}$O Astrophysical Reaction Rate

The $^{12}\text{C}(α,γ){}^{16}\text{O}$ reaction plays a central role in astrophysics, but its cross section at energies relevant for astrophysical applications is only poorly constrained by laboratory data. The reduced $α$ width, $γ_{11}$, of the bound $1^-$ level in $^{16}$O is particularly important to determine the cross section. The magnitude of $γ_{11}$ is determined via sub-Coulomb $α$-transfer reactions or the $β$-delayed $α$ decay of $^{16}$N, but the latter approach is presently hampered by the lack of sufficiently precise data on the $β$-decay branching ratios. Here we report improved branching ratios for the bound $1^-$ level [$b_{β,11} = (5.02\pm 0.10)\times 10^{-2}$] and for $β$-delayed $α$ emission [$b_{βα} = (1.59\pm 0.06)\times 10^{-5}$]. Our value for $b_{βα}$ is 33% larger than previously held, leading to a substantial increase in $γ_{11}$. Our revised value for $γ_{11}$ is in good agreement with the value obtained in $α$-transfer studies and the weighted average of the two gives a robust and precise determination of $γ_{11}$, which provides significantly improved constraints on the $^{12}$C$(α,γ)$ cross section in the energy range relevant to hydrostatic He burning.

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