arXiv subjects

R. Movshovich

Publications and source records attributed to R. Movshovich.

At least 19 recordsLinked to original sources

arXiv2026

Zero-Field Long Range Order at $T \sim 40$ mK in the Proximate Quantum Spin Ice Ce$_2$Sn$_2$O$_7$ and Phase Diagram for Magnetic Fields Along [1,1,0]

The Ce$^{3+}$ pseudospin-1/2 degrees of freedom in the pyrochlore magnets Ce$_2$X$_2$O$_7$, with $X$ = Zr, Hf, or Sn, possess dipole-octupole character. The XYZ nearest-neighbor model Hamiltonians which have successfully described their properties make them attractive candidates for quantum spin ice ground states. We report new heat capacity measurements to very low temperatures on a high-quality single crystal of Ce$_2$Sn$_2$O$_7$ grown by hydrothermal techniques. Our zero-field measurements uncover a clear first order transition to long-ranged order at $T \sim 0.04$ K, well below the downturn in the broader Schottky-like anomaly that is a common feature in the zero-field heat capacity for cerium pyrochlores. This observation settles the debate as to whether Ce$_2$Sn$_2$O$_7$ possesses a QSI ground state in zero field - it does not. However, we also find compelling evidence suggesting that spin ice physics is nearby, and remains relevant to Ce$_2$Sn$_2$O$_7$. Application of a magnetic field along the $[1,1,0]$ direction leads to an evolution of this peak to a weak anomaly at higher temperature more characteristic of a continuous, mean field transition. At higher fields along $[1,1,0]$, the Schottky-like anomaly bifurcates similar to expectations for independent polarized $α$ and orthogonal $β$ chains in classical spin ice. These new experimental results demonstrate richness to the phase diagram for Ce-based pyrochlores.

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arXiv2026

Field-Induced Selective Spin Gap Closure and Quantum Criticality in BaNd$_2$ZnS$_5$

We report thermodynamic evidence for field-induced mode-selective quantum criticality in the layered rare-earth magnet BaNd2ZnS5 (BNZS). Below the Neel temperature TN = 2.9 K, spin-orbit-entangled Nd3+ moments form two symmetry-inequivalent low-energy spin-excitation modes arising from Kramers doublet physics under a magnetic field, with distinct gaps Delta_L and Delta_H. For magnetic fields applied along the [110] direction, the lower-energy gap Delta_L softens continuously and collapses at a critical field Hc ~ 2 T, while the higher-energy gap Delta_H remains gapped, leaving the system in an intermediate partially critical phase. Despite the partial nature of the criticality, thermodynamic measurements reveal a continuous quantum phase transition. The ac susceptibility shows universal scaling behavior, with chi_ac(T, H) collapsing onto a single scaling function and following chi_ac ~ T^-0.2 at criticality. A finite residual Sommerfeld coefficient gamma_0 further indicates the emergence of gapless excitations confined to a single symmetry sector near the quantum critical point. In contrast to conventional quantum criticality based on global softening of low-energy excitations, BNZS exhibits a selective breakdown of Kramers-doublet excitations due to its strong anisotropic interactions. Our results establish BNZS as a spin-orbit-coupled rare-earth magnet where quantum criticality is not global but mode-selective, with anisotropic interactions enabling independent criticality in distinct excitation sectors.

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arXiv2026

Pseudo Point Nodal Superconducting Gap in Spin-Triplet UTe$_2$

The unconventional superconductor UTe$_2$ represents a rare example of spin-triplet pairing with potentially topologically protected quantum states. However, conflicting reports on its gap structure, particularly regarding point nodes, have hindered understanding of the order parameter symmetry and topological properties. Here we report high-resolution thermal conductivity measurements on high-quality UTe$_2$ single crystals down to ~50 mK that resolve the gap anisotropy through bulk directional transport. The $b$-axis thermal conductivity $κ_b/T$ exhibits negligible residual conductivity as $T \to 0$, and its temperature dependence is consistent with a small superconducting energy gap along the $b$-axis. Under magnetic fields, the residual $κ_b/T$ shows only weak field-induced enhancement. Remarkably, a threshold field emerges at low fields for $H \parallel a$, characterized by a kink that signals a change in quasiparticle transport normal to the field. Below the threshold, $κ_b/T$ remains isotropic for all field orientations, whereas strong anisotropy between transport along and normal to the field develops above it. These signatures strongly suggest that UTe$_2$ exhibits a fully gapped state with a pseudo point-nodal structure, where gap minima approach but never reach zero. We estimate the minimal gap $Δ_{min}/Δ_0 \sim 0.1$ along the $b$-axis, where $Δ_0$ is the characteristic superconducting gap. This unusual gap structure provides crucial insights into the pairing mechanism and topology of this spin-triplet superconductor and excludes non-unitary mixing of pairing symmetries.

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arXiv2025

Two-Peak Heat Capacity Accounts for $R\ln(2)$ Entropy and Ground State Access in the Dipole-Octupole Pyrochlore Ce$_2$Hf$_2$O$_7$

Magnetic heat capacity measurements of a high-quality single crystal of the dipole-octupole pyrochlore Ce$_2$Hf$_2$O$_7$ down to a temperature of $T = 0.02$ K are reported. These show a two-peaked structure, with a Schottky-like peak at $T_1 \sim 0.065$ K, similar to what is observed in its sister Ce-pyrochlores Ce$_2$Zr$_2$O$_7$ and Ce$_2$Sn$_2$O$_7$. However, a second sharper peak is observed at $T_2 \sim 0.025$ K, signifying the entrance to the ground state. The ground state appears to have gapped excitations, as even the most abrupt extrapolation to $C_P=0$ at $T = 0$ K fully accounts for the $R\ln(2)$ entropy associated with the pseudospin-1/2 doublet for Ce$^{3+}$ in this environment. The ground state could be conventionally ordered, although theory predicts a much larger anomaly in $C_P$ at much higher temperatures than the measured $T_2$ for expectations from an all-in all-out ground state of the XYZ Hamiltonian for Ce$_2$Hf$_2$O$_7$. The sharp low-temperature peak could also signify a cross-over from a classical spin liquid to a quantum spin liquid (QSL). For both scenarios, comparison of the measured $C_P$ with NLC calculations suggests that weak interactions beyond the nearest-neighbor XYZ Hamiltonian become relevant below $T \sim 0.25$ K. The diffuse magnetic neutron scattering observed from Ce$_2$Hf$_2$O$_7$ at low temperatures between $T_2$ and $T_1$ resembles that observed from Ce$_2$Zr$_2$O$_7$, which is well established as a $π$-flux quantum spin ice (QSI). Together with the peak in the heat capacity at $T_2$, this diffuse scattering from Ce$_2$Hf$_2$O$_7$ is suggestive of a classical spin liquid regime above $T_2$ that is distinct from the zero-entropy quantum ground state below $T_2$.

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arXiv2025

Quantum oscillation and topology change of the uncondensed Landau Fermi surface in superconducting CeCoIn5

Metals typically have multiple Fermi surface sheets, and when they enter the superconducting state, some electrons on these sheets may remain uncondensed, or their superconducting pairs can be rapidly destroyed by a magnetic field. Detecting uncondensed electrons within the superconducting state provides key information about the underlying electronic structure; however, this task remains a significant experimental challenge. Here we demonstrate quantum oscillations from the uncondensed electrons in the heavy-fermion superconductor CeCoIn5, observed through thermal conductivity measurements with a magnetic field rotating within the tetragonal a-b plane. We detect a fine structure in thermal conductivity, characterized by multiple small resonances (oscillations) in a rotating magnetic field. Remarkably, the phase of these resonances shifted by as much as π for a field above 9.7 T where spin-density wave (SDW) order emerges and coexists with superconductivity. This phase shift is naturally explained by a change in the Berry phase of the uncondensed Fermi surface, driven by the Fermi surface reconstruction associated with the onset of SDW order. Our work unambiguously shows the existence of uncondensed electrons in the superconducting state of CeCoIn5, thus resolving a longstanding debate on this issue.

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arXiv2024

Magnetic field-temperature phase diagram of spin-1/2 triangular lattice antiferromagnet KYbSe$_2$

A quantum spin liquid (QSL) is a state of matter characterized by fractionalized quasiparticle excitations, quantum entanglement, and a lack of long-range magnetic order. However, QSLs have evaded definitive experimental observation. Several Yb$^{3+}$-based triangular lattice antiferromagnets with effective $S$ = $\frac{1}{2}$ have been suggested to stabilize the QSL state as the ground state. Here, we build a comprehensive magnetic temperature phase diagram of a high-quality single crystalline KYbSe$_2$ via heat capacity and magnetocaloric effect down to 30 mK with magnetic field applied along the $a$-axis. At zero magnetic field, we observe the magnetic long-range order at $T_N$ = 0.29 K entering 120 degrees ordered state in heat capacity, consistent with neutron scattering studies. Analysis of the low-temperature ($T$) specific heat ($C$) at zero magnetic field indicates linear $T$-dependence of $C/T$ and a broad hump of $C/T$ in the proximate QSL region above $T_N$. By applying magnetic field, we observe the up-up-down phase with 1/3 magnetization plateau and oblique phases, in addition to two new phases. These observations strongly indicate that while KYbSe$_2$ closely exhibits characteristics resembling an ideal triangular lattice, deviations may exist, such as the effect of the next-nearest-neighbor exchange interaction, calling for careful consideration for spin Hamiltonian modeling. Further investigations into tuning parameters, such as chemical pressure, could potentially induce an intriguing QSL phase in the material.

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arXiv2023

Non-linear magnons and exchange Hamiltonians of delafossite proximate quantum spin liquids

Quantum spin liquids (QSL) are theoretical states of matter with long-range entanglement and exotic quasiparticles. However, they generally elude quantitative theory, rendering their underlying phases mysterious and hampering efforts to identify experimental QSL states. Here we study triangular lattice resonating valence bond QSL candidate materials KYbSe$_2$ and NaYbSe$_2$. We measure the magnon modes in their 1/3 plateau phase, where quantitative theory is tractable, using inelastic neutron scattering and fit them using nonlinear spin wave theory. We also fit the KYbSe$_2$ heat capacity using high temperature series expansion. Both KYbSe$_2$ fits yield the same magnetic Hamiltonian to within uncertainty, confirming previous estimates and showing the Heisenberg $J_2/J_1$ to be an accurate model for these materials. Most importantly, comparing KYbSe$_2$ and NaYbSe$_2$ shows that smaller $A$-site Na$^+$ ion has a larger $J_2/J_1$ ratio. However, hydrostatic pressure applied to KYbSe$_2$ increases the ordering temperature (a result consistent with density functional theory calculations), indicating that pressure decreases $J_2/J_1$. These results show how periodic table and hydrostatic pressure can tune the $A$YbSe$_2$ materials in a controlled way.

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arXiv2023

Anisotropic field-induced changes in the superconducting order parameter of UTe2

UTe2 is a newly discovered unconventional superconductor, where electron Cooper pairs combine into a spin-triplet ground state. Here we report the specific heat C(H,T) of a high-quality single crystal of UTe2 with a single specific heat anomaly at the superconducting transition temperature T_c {\approx} 2 K and a small zero-field residual Sommerfeld coefficient γ_0 = C/T (T=0) = 10 mJ/mol-K^2. We applied magnetic field up to 12 T along the three principal crystallographic axes of UTe2 to probe the nature of the superconducting state. The evolution of the residual Sommerfeld coefficient as a function of magnetic field, γ_0 (H), is highly anisotropic and reveals distinct regions. In magnetic field up to 4 T applied along a, b, and c axes, we find γ_0{\approx}α_i {\square}H, with i=a,b,c, as expected for an unconventional superconductor with nodes (zeros) of the superconducting order parameter on the Fermi surface. A pronounced kink in γ_0(H), however, is observed at roughly 4 T for field applied along both a and b axes, whereas a smooth change from square-root to linear behaviour is observed at 4 T for H//c. These results strongly indicate that a zero-field ground state is stable up to 4 T and undergoes a field-induced evolution above 4 T. {α_c} > {α_a} > {α_b}, indicating that the nodes in the low-field state are predominantly located in the vicinity of the a-b plane. The modification of the order parameter is strongest when field is applied in the a-b plane, which causes nodes to move away from the direction of the applied field. Both d_(B_2u)+id_(B_1u) and d_(B_2u)+id_(A_u) two-component order parameters can account for our observations, with d_(B_2u)+id_(B_1u) a more likely candidate. In either scenario, our measurements indicate that B_2u is the primary superconducting order parameter in UTe2.

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arXiv2023

Quantum Spin Ice Response to a Magnetic Field in the Dipole-Octupole Pyrochlore Ce$_2$Zr$_2$O$_7$

We report new heat capacity measurements on single crystal Ce$_2$Zr$_2$O$_7$ down to $\sim$ 0.1 K in a magnetic field along the $[1,\bar{1}, 0]$ direction. These new measurements show that the broad hump in the zero-field heat capacity moves higher in temperature with increasing field strength and is split into two humps by the $[1,\bar{1}, 0]$ field at $\sim$ 2 T. These separate features are due to the decomposition of the pyrochlore lattice into effectively decoupled chains for fields in this direction: one set of chains ($α$-chains) is polarized by the field while the other ($β$-chains) remains free. Our theoretical modelling suggests that the $β$-chains are close to a critical state, with nearly-gapless excitations. We also report new elastic and inelastic neutron scattering measurements on single crystal Ce$_2$Zr$_2$O$_7$ in $[1, \bar{1}, 0]$ and $[0, 0, 1]$ magnetic fields at temperatures down to 0.03 K. The elastic scattering behaves consistently with the formation of independent chains for a $[1, \bar{1}, 0]$ field, while the $[0, 0, 1]$ field produces a single field-induced magnetic Bragg peak at $(0, 2, 0)$ and equivalent wavevectors, indicating a polarized spin ice for fields above $\sim$ 3 T. For both $[1, \bar{1}, 0]$ and $[0, 0, 1]$ fields, our inelastic neutron scattering results show an approximately-dispersionless continuum of scattering that increases in both energy and intensity with increasing field strength. By modelling the complete set of experimental data using numerical linked cluster and semiclassical molecular dynamics calculations, we demonstrate the dominantly multipolar nature of the exchange interactions in Ce$_2$Zr$_2$O$_7$ and the smallness of the parameter $θ$ which controls the mixing between dipolar and octupolar degrees of freedom. These results support previous estimates of the microscopic exchange parameters.

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arXiv2023

Witnessing quantum criticality and entanglement in the triangular antiferromagnet KYbSe$_2$

The Heisenberg triangular lattice quantum spin liquid and the phase transitions to nearby magnetic orders have received much theoretical attention, but clear experimental manifestations of these states are rare. This work investigates a new spin-half Yb$^{3+}$ delafossite material, KYbSe$_2$, whose inelastic neutron scattering spectra reveal a diffuse continuum with a sharp lower bound. Applying entanglement witnesses to the data reveals significant multipartite entanglement spread between its neighbors, and analysis of its magnetic exchange couplings shows close proximity to the triangular lattice Heisenberg quantum spin liquid. Key features of the data are reproduced by Schwinger-boson theory and tensor network calculations with a significant second-neighbor coupling $J_2$. The strength of the dynamical structure factor at the $K$ point shows a scaling collapse in $\hbarω/k_\mathrm{B}T$ down to 0.3 K, indicating a second-order quantum phase transition. Comparing this to previous theoretical work suggests that the proximate phase at larger $J_2$ is a gapped $\mathbb{Z}_2$ spin liquid, resolving a long-debated issue. We thus show that KYbSe$_2$ is close to a spin liquid phase, which in turn sheds light on the theoretical phase diagram itself.

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arXiv2023

Ubiquitous Spin Freezing in the Superconducting State of UTe2

In most superconductors electrons form Cooper pairs in a spin-singlet state mediated by either phonons or by long-range interactions such as spin fluctuations. The superconductor UTe$_2$ is a rare material wherein electrons are believed to form pairs in a unique spin-triplet state with potential topological properties. While spin-triplet pairing may be mediated by ferromagnetic or antiferromagnetic fluctuations, experimentally, the magnetic properties of UTe$_2$ are unclear. By way of muon spin rotation/relaxation ($μ$SR) measurements on independently grown UTe$_2$ single crystals we demonstrate the existence of magnetic clusters that gradually freeze into a disordered spin frozen state at low temperatures. Our findings suggest that inhomogeneous freezing of magnetic clusters is linked to the ubiquitous residual linear term in the temperature dependence of the specific heat ($C$) and the low-temperature upturn in $C/T$ versus $T$. The omnipresent magnetic inhomogeneity has potential implications for experiments aimed at establishing the intrinsic low-temperature properties of UTe$_2$.

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arXiv2022

Reply to "Comment on: 'Case for a U(1)$_π$ Quantum Spin Liquid Ground State in the Dipole-Octupole Pyrochlore $\mathrm{Ce}_2\mathrm{Zr}_2\mathrm{O}_7$' "

In his comment [arXiv:2209.03235], S. W. Lovesey argues that our analysis of neutron scattering experiments performed on Ce$_2$Zr$_2$O$_7$ is invalid. Lovesey argues that we have not properly accounted for the higher-order multipolar contributions to the magnetic scattering and that our use of pseudospin-$1/2$ operators to describe the scattering is inappropriate. In this reply, we show that the multipolar corrections discussed by Lovesey only become significant at scattering wavevectors exceeding those accessed in our experiments. This in no way contradicts or undermines our work, which never claimed a direct observation of scattering from higher-order multipoles. We further show that Lovesey's objections to our use of pseudospins are unfounded, and that the pseudospin operators are able to describe all magnetic scattering processes at the energy scale of our experiments, far below the crystal field gap. Finally, we comment on certain assumptions in Lovesey's calculations of the scattering amplitude which are inconsistent with experiment.

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arXiv2021

The case for a U(1)$_π$ Quantum Spin Liquid Ground State in the Dipole-Octupole Pyrochlore Ce$_2$Zr$_2$O$_7$

The Ce$^{3+}$ pseudospin-$\frac{1}{2}$ degrees of freedom in the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ are known to possess dipole-octupole (DO) character, making it a candidate for novel quantum spin liquid (QSL) ground states at low temperatures. We report new polarized neutron diffraction at low temperatures, as well as heat capacity ($C_p$) measurements on single crystal Ce$_2$Zr$_2$O$_7$. The former bears both similarities and differences from that measured in the canonical dipolar spin ice compound Ho$_2$Ti$_2$O$_7$, while the latter rises sharply at low temperatures, initially plateauing near 0.08 K, before falling off towards a high temperature zero beyond 3 K. Above $\sim$0.5 K, the $C_p$ data set can be fit to the results of a quantum numerical linked cluster (NLC) calculation, carried out to 4$^{\mathrm{th}}$ order, that allows estimates for the terms in the near-neighbour XYZ Hamiltonian expected for such DO pyrochlore systems. Fits of the same theory to the temperature dependence of the magnetic susceptibility and unpolarized neutron scattering complement this analysis. A comparison between the resulting best fit NLC calculation and the polarized neutron diffraction shows both agreement and discrepancies, mostly in the form of zone-boundary diffuse scattering in the non-spin flip channel, which are attributed to interactions beyond near-neighbours. The lack of an observed thermodynamic anomaly and the constraints on the near-neighbour XYZ Hamiltonian suggest that Ce$_2$Zr$_2$O$_7$ realizes a U(1)$_π$ QSL state at low temperatures, and one that likely resides near the boundary between dipolar and octupolar character.

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arXiv2021

Fingerprinting Triangular-Lattice Antiferromagnet by Excitation Gaps

CeCd$_3$As$_3$ is a rare-earth triangular-lattice antiferromagnet with large inter-layer separation. Our field-dependent heat capacity measurements at dilution fridge temperatures allow us to trace the field-evolution of the spin-excitation gaps throughout the antiferromagnetic and paramagnetic regions. The distinct gap evolution places strong constraints on the microscopic pseudo-spin model, which, in return, yields a close {\it quantitative} description of the gap behavior. This analysis provides crucial insights into the nature of the magnetic state of CeCd$_3$As$_3$, with a certainty regarding its stripe order and low-energy model parameters that sets a compelling paradigm for exploring and understanding the rapidly growing family of the rare-earth-based triangular-lattice systems.

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arXiv2017

Domain engineering of the metastable domains in the 4f-uniaxial-ferromagnet CeRu$_2$Ga$_2$B

In search of novel, improved materials for magnetic data storage and spintronic devices, compounds that allow a tailoring of magnetic domain shapes and sizes are essential. Good candidates are materials with intrinsic anisotropies or competing interactions, as they are prone to host various domain phases that can be easily and precisely selected by external tuning parameters such as temperature and magnetic field. Here, we utilize vector magnetic fields to visualize directly the magnetic anisotropy in the uniaxial ferromagnet CeRu$_2$Ga$_2$B. We demonstrate a feasible control both globally and locally of domain shapes and sizes by the external field as well as a smooth transition from single stripe to bubble domains, which opens the door to future applications based on magnetic domain tailoring.

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arXiv2015

Spin liquid ground state in the frustrated J1-J2 zigzag chain system BaTb2O4

We have investigated polycrystalline samples of the zigzag chain system BaTb$_2$O$_4$ with a combination of magnetic susceptibility, heat capacity, neutron powder diffraction, and muon spin relaxation measurements. Despite the onset of Tb$^{3+}$ short-range antiferromagnetic correlations at $|θ_{CW}|$ $=$ 18.5 K and a very large effective moment, our combined measurements indicate that BaTb$_2$O$_4$ remains paramagnetic down to 0.095 K. The magnetic properties of this material show striking similarities to the pyrochlore antiferromagnet Tb$_2$Ti$_2$O$_7$, and therefore we propose that BaTb$_2$O$_4$ is a new large moment spin liquid candidate.

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arXiv2014

Short-range magnetic correlations in the highly-correlated electron compound CeCu$_{4}Ga

We present experimental results for the heavy-electron compound CeCu$_{4}$Ga which show that it possesses short-range magnetic correlations down to a temperature of $T = 0.1$ K. Our neutron scattering data show no evidence of long-range magnetic order occurring despite a peak in the specific heat at $T^{*} =1.2$ K. Rather, magnetic diffuse scattering occurs which corresponds to short-range magnetic correlations occurring across two unit cells. The specific heat remains large as $T\sim0$ K resulting in a Sommerfeld coefficient of $γ_{0} = 1.44(2)$ J/mol-K$^{2}$, and, below $T^{*}$, the resistivity follows $T^{2}$ behavior and the ac magnetic susceptibility becomes temperature independent. A magnetic peak centered at an energy transfer of $E_{\rm{c}}=0.24(1)$ meV is seen in inelastic neutron scattering data which shifts to higher energies and broadens under a magnetic field. We discuss the coexistence of large specific heat, magnetic fluctuations, and short-range magnetic correlations at low temperatures and compare our results to those for materials possessing spin-liquid behavior.

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arXiv2014

Magnetic ordering in the frustrated J1-J2 Ising chain candidate BaNd2O4

The AR$_2$O$_4$ family (R = rare earth) have recently been attracting interest as a new series of frustrated magnets, with the magnetic R atoms forming zigzag chains running along the $c$-axis. We have investigated polycrystalline BaNd$_2$O$_4$ with a combination of magnetization, heat capacity, and neutron powder diffraction (NPD) measurements. Magnetic Bragg peaks are observed below $T_N$ $=$ 1.7 K, and they can be indexed with a propagation vector of $\vec{k}$ $=$ (0 1/2 1/2). The signal from magnetic diffraction is well described by long-range ordering from only one of the two types of Nd zigzag chains, with collinear up-up-down-down intrachain spin configurations. Furthermore, low temperature magnetization and heat capacity measurements reveal two field-induced spin transitions at 2.5 T and 4 T for $T$ $=$ 0.46 K. The high field phase is paramagnetic, while the intermediate field state may arise from a spin transition of the long-range ordered Nd chains, resulting in an up-up-down intrachain spin configuration. The proposed intermediate field state is consistent with the magnetic structure determined in zero field for these chains by NPD, as both phases are predicted for the classical Ising chain model with nearest neighbor and next nearest neighbor interactions.

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