arXiv subjects

R. Perry

Publications and source records attributed to R. Perry.

5 recordsLinked to original sources

arXiv2025

Magnetostriction as the origin of the magnetodielectric effect in La2CoMnO6

The La2CoMnO6 (LCMO) perovskite has received a lot of attention due to its near room temperature magnetodielectric effect. Despite the recent efforts, the mechanism ruling the correlation between its magnetic and dielectric properties is not yet fully understood. In order to address this issue, we conducted a detailed investigation of the coupling between the structural, electronic and magnetic properties of a polycrystalline LCMO sample. Using magnetic field-dependent x-ray powder diffraction and measurements with a capacitive dilatometer, we show that applying an external magnetic field decreases the unit cell volume, thereby modifying the octahedral distortions. Experiments involving temperature and field-dependent x-ray absorption spectroscopy at the Co-L2,3 edges provide further evidence that the spin-orbit interaction of outermost Co 3d-orbital and the field-induced enhancement of covalence effects are the key contributors to the magnetostrictive effects. From a detailed analysis using multiplet and density functional theory calculations, we propose that the field-induced modulations of the orbital hybridization and the ligand-to-metal charge transfer are responsible for the changes in the dielectric response of LCMO, thus enabling a direct coupling between magnetic, elastic and dielectric properties in this material.

cond-mat.mtrl-sci↗

arXiv2019

Commensurate to incommensurate magnetic phase transition in Honeycomb-lattice pyrovanadate Mn2V2O7

We have synthesized single crystalline sample of Mn$_2$V$_2$O$_7$ using floating zone technique and investigated the ground state using magnetic susceptibility, heat capacity and neutron diffraction. Our magnetic susceptibility and heat capacity reveal two successive magnetic transitions at $T_{N1} =$ 19 K and $T_{N2} =$ 11.8 K indicating two distinct magnetically ordered phases. The single crystal neutron diffraction study shows that in the temperature ($T$) range 11.8 K $\le T \le$ 19 K the magnetic structure is commensurate with propagation vector $k_1 = (0, 0.5, 0)$, while upon lowering temperature below $T_{N2} =$ 11.8 K an incommensurate magnetic order emerges with $k_2 = (0.38, 0.48, 0.5)$ and the magnetic structure can be represented by cycloidal modulation of the Mn spin in $ac-$plane. We are reporting this commensurate to incommensurate transition for the first time. We discuss the role of the magnetic exchange interactions and spin-orbital coupling on the stability of the observed magnetic phase transitions.

cond-mat.str-el↗

arXiv2018

Persistence of antiferromagnetic order upon La substitution in the $4d^4$ Mott insulator Ca$_2$RuO$_4$

The chemical and magnetic structures of the series of compounds Ca$_{2-x}$La$_x$RuO$_4$ [$x = 0$, $0.05(1)$, $0.07(1)$, $0.12(1)$] have been investigated using neutron diffraction and resonant elastic x-ray scattering. Upon La doping, the low temperature S-Pbca space group of the parent compound is retained in all insulating samples [$x\leq0.07(1)$], but with significant changes to the atomic positions within the unit cell. These changes can be characterised in terms of the local RuO$_6$ octahedral coordination: with increasing doping the structure, crudely speaking, evolves from an orthorhombic unit cell with compressed octahedra to a quasi-tetragonal unit cell with elongated ones. The magnetic structure on the other hand, is found to be robust, with the basic $k=(0,0,0)$, $b$-axis antiferromagnetic order of the parent compound preserved below the critical La doping concentration of $x\approx0.11$. The only effects of La doping on the magnetic structure are to suppress the A-centred mode, favouring the B mode instead, and to reduce the N\'{e}el temperature somewhat. Our results are discussed with reference to previous experimental reports on the effects of cation substitution on the $d^4$ Mott insulator Ca$_2$RuO$_4$, as well as with regard to theoretical studies on the evolution of its electronic and magnetic structure. In particular, our results rule out the presence of a proposed ferromagnetic phase, and suggest that the structural effects associated with La substitution play an important role in the physics of the system.

cond-mat.str-el↗

arXiv2018

A massive core for a cluster of galaxies at a redshift of 4.3

Massive galaxy clusters are now found as early as 3 billion years after the Big Bang, containing stars that formed at even earlier epochs. The high-redshift progenitors of these galaxy clusters, termed 'protoclusters', are identified in cosmological simulations with the highest dark matter overdensities. While their observational signatures are less well defined compared to virialized clusters with a substantial hot intra-cluster medium (ICM), protoclusters are expected to contain extremely massive galaxies that can be observed as luminous starbursts. Recent claimed detections of protoclusters hosting such starbursts do not support the kind of rapid cluster core formation expected in simulations because these structures contain only a handful of starbursting galaxies spread throughout a broad structure, with poor evidence for eventual collapse into a protocluster. Here we report that the source SPT2349-56 consists of at least 14 gas-rich galaxies all lying at z = 4.31 based on sensitive observations of carbon monoxide and ionized carbon. We demonstrate that each of these galaxies is forming stars between 50 and 1000 times faster than our own Milky Way, and all are located within a projected region only $\sim$ 130 kiloparsecs in diameter. This galaxy surface density is more than 10 times the average blank field value (integrated over all redshifts) and $>$1000 times the average field volume density. The velocity dispersion ($\sim$ 410 km s$^{-1}$) of these galaxies and enormous gas and star formation densities suggest that this system represents a galaxy cluster core at an advanced stage of formation when the Universe was only 1.4 billion years old. A comparison with other known protoclusters at high redshifts shows that SPT2349-56 is a uniquely massive and dense system that could be building one of the most massive structures in the Universe today.

astro-ph.GA↗

arXiv2011

New applications of the renormalization group method in physics -- a brief introduction

The renormalization group method developed by Ken Wilson more than four decades ago has revolutionized the way we think about problems involving a broad range of energy scales such as phase transitions, turbulence, continuum limits and bifurcations in dynamical systems. The theme issue provides articles reviewing recent progress made using the renormalization group method in atomic, condensed matter, nuclear and particle physics. In the following we introduce these articles in a way that emphasizes common themes and the universal aspects of the method.

hep-th↗