arXiv subjects

R. R. P. Singh

Publications and source records attributed to R. R. P. Singh.

At least 19 recordsLinked to original sources

arXiv2025

Observation of a pronounced Hebel-Slichter peak in the spin-lattice relaxation rate and implications for gap and pairing symmetry in LaNiGa$_2$

We report a pronounced Hebel-Slichter coherence peak in the zero field nuclear quadrupolar resonance (NQR) spin-lattice relaxation rate of the topological crystalline superconductor LaNiGa$_2$ in the superconducting state. Previously, a two-band internally antisymmetric non-unitary triplet pairing (INT) state was proposed for this system, with equal spin-pairing and two distinct gaps associated with different spins. A detailed examination of the temperature dependence of the NQR data shows that the data best fit an INT model if the two gaps are equal and the model is unitary. Even a tiny non-unitarity with two unequal gaps causes the coherence peak to diminish rapidly and deviate from the data. On the other hand, the data are well-fit by a two-band singlet BCS-like pairing with two distinct gaps consistent with previous measurements. This raises doubts on the identification of non-unitary triplet-pairing with time-reversal symmetry breaking in this material.

cond-mat.supr-con↗

arXiv2024

Nuclear magnetic resonance studies in a model transverse field Ising system

The suppression of ferroquadrupolar order in TmVO$_4$ in a magnetic field is well-described by the transverse field Ising model, enabling detailed studies of critical dynamics near the quantum phase transition. We describe nuclear magnetic resonance measurements in pure and Y-doped single crystals. The non-Kramers nature of the ground state doublet leads to a unique form of the hyperfine coupling that exclusively probes the transverse field susceptibility. Our results show that this quantity diverges at the critical field, in contrast to the mean-field prediction. Furthermore, we find evidence for quantum critical fluctuations present near Tm-rich regions in Y-doped crystals at levels beyond which long-range order is suppressed, suggesting the presence of quantum Griffiths phases.

cond-mat.str-el↗

arXiv2023

Spin-echo and quantum versus classical critical fluctuations in TmVO$_4$

Using spin-echo Nuclear Magnetic Resonance in the model Transverse-Field Ising system TmVO$_4$, we show that low frequency quantum fluctuations at the quantum critical point have a very different effect on $^{51}$V nuclear-spins than classical low-frequency noise or fluctuations that arise at a finite temperature critical point. Spin-echos filter out the low frequency classical noise but not the quantum fluctuations. This allows us to directly visualize the quantum critical fan and demonstrate the persistence of quantum fluctuations at the critical coupling strength in TmVO$_4$ to high temperatures in an experiment that remains transparent to finite temperature classical phase transitions. These results show that while dynamical decoupling schemes can be quite effective in eliminating classical noise in a qubit, a quantum critical environment may lead to rapid entanglement and decoherence.

cond-mat.str-el↗

arXiv2018

Incipient and well-developed entropy plateaus in spin-S Kitaev models

We present results on entropy and heat-capacity of the spin-S honeycomb-lattice Kitaev models using high-temperature series expansions and thermal pure quantum (TPQ) state methods. We study models with anisotropic couplings $J_z=1\ge J_x=J_y$ for spin values 1/2, 1, 3/2, and 2. We show that for $S>1/2$, any anisotropy leads to well developed plateaus in the entropy function at an entropy value of $\frac{1}{2}\ln{2}$, independent of $S$. However, in the absence of anisotropy, there is an incipient entropy plateau at $S_{max}/2$, where $S_{max}$ is the infinite temperature entropy of the system. We discuss possible underlying microscopic reasons for the origin and implications of these entropy plateaus.

cond-mat.str-el↗

arXiv2017

Critical and Griffiths-McCoy singularities in quantum Ising spin-glasses on d-dimensional hypercubic lattices: A series expansion study

We study the $\pm J$ transverse-field Ising spin glass model at zero temperature on d-dimensional hypercubic lattices and in the Sherrington-Kirkpatrick (SK) model, by series expansions around the strong field limit. In the SK model and in high-dimensions our calculated critical properties are in excellent agreement with the exact mean-field results, surprisingly even down to dimension $d = 6$ which is below the upper critical dimension of $d=8$. In contrast, in lower dimensions we find a rich singular behavior consisting of critical and Griffiths-McCoy singularities. The divergence of the equal-time structure factor allows us to locate the critical coupling where the correlation length diverges, implying the onset of a thermodynamic phase transition. We find that the spin-glass susceptibility as well as various power-moments of the local susceptibility become singular in the paramagnetic phase $\textit{before}$ the critical point. Griffiths-McCoy singularities are very strong in two-dimensions but decrease rapidly as the dimension increases. We present evidence that high enough powers of the local susceptibility may become singular at the pure-system critical point.

cond-mat.stat-mech↗

arXiv2017

Tricriticality in Crossed Ising Chains

We explore the phase diagram of Ising spins on one-dimensional chains which criss-cross in two perpendicular directions and which are connected by interchain couplings. This system is of interest as a simpler, classical analog of a quantum Hamiltonian which has been proposed as a model of magnetic behavior in Nb$_{12}$O$_{29}$ and also, conceptually, as a geometry which is intermediate between one and two dimensions. Using mean field theory as well as Metropolis Monte Carlo and Wang-Landau simulations, we locate quantitatively the boundaries of four ordered phases. Each becomes an effective Ising model with unique effective couplings at large interchain coupling. Away from this limit we demonstrate non-trivial critical behavior, including tricritical points which separate first and second order phase transitions. Finally, we present evidence that this model belongs to the 2D Ising universality class.

cond-mat.stat-mech↗

arXiv2017

Efficient generation of series expansions for $\pm J$ Ising spin-glasses in a classical or a quantum (transverse) field

We discuss generation of series expansions for Ising spin-glasses with a symmetric $\pm J$ (i.e. bimodal) distribution on d-dimensional hypercubic lattices using linked-cluster methods. Simplifications for the bimodal distribution allow us to go to higher order than for a general distribution. We discuss two types of problem, one classical and one quantum. The classical problem is that of the Ising spin glass in a longitudinal magnetic field, $h$, for which we obtain high temperature series expansions in variables $\tanh(J/T)$ and $\tanh(h/T)$. The quantum problem is a $T=0$ study of the Ising spin glass in a transverse magnetic field $h_T$ for which we obtain a perturbation theory in powers of $J/h_T$. These methods require (i) enumeration and counting of \textit{all} connected clusters that can be embedded in the lattice up to some order $n$, and (ii) an evaluation of the contribution of each cluster for the quantity being calculated, known as the weight. We discuss a general method that takes the much smaller list (and count) of all no free-end (NFE) clusters on a lattice up to some order $n$, and automatically generates all other clusters and their counts up to the same order. The weights for finite clusters in both cases have a simple graphical interpretation that allows us to proceed efficiently for a general configuration of the $\pm J$ bonds, and at the end perform suitable disorder averaging. The order of our computations is limited by the weight calculations for the high-temperature expansions of the classical model, while they are limited by graph counting for the $T=0$ quantum system. Details of the calculational methods are presented.

cond-mat.dis-nn↗

arXiv2017

de Almeida-Thouless instability in short-range Ising spin-glasses

We use high temperature series expansions to study the $\pm J$ Ising spin-glass in a magnetic field in $d$-dimensional hypercubic lattices for $d=5, 6, 7$ and $8$, and in the infinite-range Sherrington-Kirkpatrick (SK) model. The expansions are obtained in the variable $w=\tanh^2{J/T}$ for arbitrary values of $u=\tanh^2{h/T}$ complete to order $w^{10}$. We find that the scaling dimension $Δ$ associated with the ordering-field $h^2$ equals $2$ in the SK model and for $d\ge 6$. However, in agreement with the work of Fisher and Sompolinsky, there is a violation of scaling in a finite field, leading to an anomalous $h$-$T$ dependence of the Almeida-Thouless (AT) line in high dimensions, while scaling is restored as $d \to 6$. Within the convergence of our series analysis, we present evidence supporting an AT line in $d\ge 6$. In $d=5$, the exponents $γ$ and $Δ$ are substantially larger than mean-field values, but we do not see clear evidence for the AT line in $d=5$.

cond-mat.dis-nn↗

arXiv2016

Magnetic excitations and electronic interactions in Sr$_2$CuTeO$_6$: a spin-1/2 square lattice Heisenberg antiferromagnet

Sr$_2$CuTeO$_6$ presents an opportunity for exploring low-dimensional magnetism on a square lattice of $S=1/2$ Cu$^{2+}$ ions. We employ ab initio multi-reference configuration interaction calculations to unravel the Cu$^{2+}$ electronic structure and to evaluate exchange interactions in Sr$_2$CuTeO$_6$. The latter results are validated by inelastic neutron scattering using linear spin-wave theory and series-expansion corrections for quantum effects to extract true coupling parameters. Using this methodology, which is quite general, we demonstrate that Sr$_2$CuTeO$_6$ is an almost realization of a nearest-neighbor Heisenberg antiferromagnet but with relatively weak coupling of 7.18(5) meV.

cond-mat.str-el↗

arXiv2015

Are multiphase competition & order-by-disorder the keys to understanding Yb2Ti2O7?

If magnetic frustration is most commonly known for undermining long-range order, as famously illustrated by spin liquids, the ability of matter to develop new collective mechanisms in order to fight frustration is no less fascinating, providing an avenue for the exploration and discovery of unconventional properties of matter. Here we study an ideal minimal model of such mechanisms which, incidentally, pertains to the perplexing quantum spin ice candidate Yb2Ti2O7. Specifically, we explain how thermal and quantum fluctuations, optimized by order-by-disorder selection, conspire to expand the stability region of an accidentally degenerate continuous symmetry U(1) manifold against the classical splayed ferromagnetic ground state that is displayed by the sister compound Yb2Sn2O7. The resulting competition gives rise to multiple phase transitions, in striking similitude with recent experiments on Yb2Ti2O7 [Lhotel et al., Phys. Rev. B 89 224419 (2014)]. Considering the effective Hamiltonian determined for Yb2Ti2O7, we provide, by combining a gamut of numerical techniques, compelling evidence that such multiphase competition is the long-sought missing key to understanding the intrinsic properties of this material. As a corollary, our work offers a pertinent illustration of the influence of chemical pressure in rare-earth pyrochlores.

cond-mat.str-el↗

arXiv2015

Magnons and Excitation Continuum in XXZ triangular antiferromagnetic model: Application to $Ba_3CoSb_2O_9$

We investigate the excitation spectrum of the triangular-lattice antiferromagnetic $XXZ$ model using series expansions and mean field Schwinger bosons approaches. The single-magnon spectrum computed with series expansions exhibits rotonic minima at the middle points of the edges of the Brillouin zone, for all values of the anisotropy parameter in the range $0\leq J^z/J\leq1$. Based on the good agreement with series expansions for the single-magnon spectrum, we compute the full dynamical magnetic structure factor within the mean field Schwinger boson approach to investigate the relevance of the $XXZ$ model for the description of the unusual spectrum found recently in $Ba_3CoSb_2O_9$. In particular, we obtain an extended continuum above the spin wave excitations, which is further enhanced and brought closer to those observed in $Ba_3CoSb_2O_9$ with the addition of a second neighbor exchange interaction approximately 15% of the nearest-neighbor value. Our results support the idea that excitation continuum with substantial spectral-weight are generically present in two-dimensional frustrated spin systems and fractionalization in terms of {\it bosonic} spinons presents an efficient way to describe them.

cond-mat.str-el↗

arXiv2013

Phase Transition and Thermal Order-by-Disorder in the Pyrochlore Quantum Antiferromagnet Er2Ti2O7: a High-Temperature Series Expansion Study

Several rare earth magnetic pyrochlore materials are well modeled by a spin-1/2 quantum Hamiltonian with anisotropic exchange parameters Js. For the Er2Ti2O7 material, the Js were recently determined from high-field inelastic neutron scattering measurements. Here, we perform high-temperature (T) series expansions to compute the thermodynamic properties of this material using these Js. Comparison with experimental data show that the model describes the material very well including the finite temperature phase transition to an ordered phase at Tc~1.2 K. We show that high temperature expansions give identical results for different q=0 xy order parameter susceptibilities up to 8th order in β=1/T (presumably to all orders in β). Conversely, a non-linear susceptibility related to the 6th power of the order parameter reveals a thermal order-by-disorder selection of the same non-colinear ψ_2 state as found in Er2Ti2O7.

cond-mat.str-el↗

arXiv2013

Disorder Line and Incommensurate Floating Phases in the Quantum Ising Model on an Anisotropic Triangular Lattice

We present a Quantum Monte Carlo study of the Ising model in a transverse field on a square lattice with nearest-neighbor antiferromagnetic exchange interaction J and one diagonal second-neighbor interaction $J'$, interpolating between square-lattice ($J'=0$) and triangular-lattice ($J'=J$) limits. At a transverse-field of $B_x=J$, the disorder-line first introduced by Stephenson, where the correlations go from Neel to incommensurate, meets the zero temperature axis at $J'\approx 0.7 J$. Strong evidence is provided that the incommensurate phase at larger $J'$, at finite temperatures, is a floating phase with power-law decaying correlations. We sketch a general phase-diagram for such a system and discuss how our work connects with the previous Quantum Monte Carlo work by Isakov and Moessner for the isotropic triangular lattice ($J'=J$). For the isotropic triangular-lattice, we also obtain the entropy function and constant entropy contours using a mix of Quantum Monte Carlo, high-temperature series expansions and high-field expansion methods and show that phase transitions in the model in presence of a transverse field occur at very low entropy.

cond-mat.str-el↗

arXiv2012

Low temperature properties of the triangular-lattice antiferromagnet: a bosonic spinon theory

We study the low temperature properties of the triangular-lattice Heisenberg antiferromagnet with a mean field Schwinger spin-1/2 boson scheme that reproduces quantitatively the zero temperature energy spectrum derived previously using series expansions. By analyzing the spin-spin and the boson density-density dynamical structure factors, we identify the unphysical spin excitations that come from the relaxation of the local constraint on bosons. This allows us to reconstruct a free energy based on the physical excitations only, whose predictions for entropy and uniform susceptibility seem to be reliable within the temperature range $0< T <0.3J, which is difficult to access by other methods. The high values of entropy, also found in high temperature expansions studies, can be attributed to the roton-like narrowed dispersion at finite temperatures.

cond-mat.str-el↗

arXiv2012

Is the Yb2Ti2O7 pyrochlore a quantum spin ice?

We use numerical linked cluster (NLC) expansions to compute the specific heat, C(T), and entropy, S(T), of a quantum spin ice model of Yb2Ti2O7 using anisotropic exchange interactions recently determined from inelastic neutron scattering measurements and find good agreement with experimental calorimetric data. In the perturbative weak quantum regime, this model has a ferrimagnetic ordered ground state, with two peaks in C(T): a Schottky anomaly signalling the paramagnetic to spin ice crossover followed at lower temperature by a sharp peak accompanying a first order phase transition to the ferrimagnetic state. We suggest that the two C(T) features observed in Yb2Ti2O7 are associated with the same physics. Spin excitations in this regime consist of weakly confined spinon-antispinon pairs. We suggest that conventional ground state with exotic quantum dynamics will prove a prevalent characteristic of many real quantum spin ice materials.

cond-mat.str-el↗

arXiv2011

High temperature series expansion study of the Heisenberg antiferromagnet on the hyperkagome lattice: Comparison with Na$_4$Ir$_3$O$_8$

We develop high temperature series expansions for $\ln{Z}$ and the uniform structure factor of the spin-half Heisenberg model on the hyperkagome lattice to order $β^{16}$. These expansions are used to calculate the uniform susceptibility ($χ$), the entropy ($S$), and the heat capacity ($C$) of the model as a function of temperature. Series extrapolations of the expansions converge well down to a temperature of approximately $J/4$. A comparison with the experimental data for Na$_4$Ir$_3$O$_8$ shows that its magnetic susceptibility is reasonably well described by the model with an exchange constant $J\approx 300 K$, but there are also additional smaller terms present in the system. The specific heat of the model has two peaks. The lower temperature peak, which is just below our range of convergence contains about 40 percent of the total entropy. Despite being a 3-dimensional lattice, this model shares many features with the kagome lattice Heisenberg model and the material must be considered a strong candidate for a quantum spin-liquid.

cond-mat.str-el↗

arXiv2011

Ground state properties, excitation spectra and phase transitions in the $S=1/2$ and $S=3/2$ bilayer Heisenberg models on the honeycomb Lattice

Motivated by the observation of a disordered spin ground state in the $S=3/2$ material Bi$_3$Mn$_4$O$_{12}$NO$_3$, we study the ground state properties and excitation spectra of the $S=3/2$ (and for comparison $S=1/2$) bilayer Heisenberg model on the honeycomb lattice, with and without frustrating further neighbor interactions. We use series expansions around the Néel state to calculate properties of the magnetically ordered phase. Furthermore, series expansions in $1/λ=J_1/J_{\perp}$, where $J_1$ is an in-plane exchange constant and $J_\perp$ is the exchange constant between the layers are used to study properties of the spin singlet phase. For the unfrustrated case, our results for the phase transitions are in very good agreement with recent Quantum Monte Carlo studies. We also obtain the excitation spectra in the disordered phase and study the change in the critical $λ$ when frustrating exchange interactions are added to the $S=3/2$ system and find a rapid suppression of the ordered phase with frustration. Implications for the material Bi$_3$Mn$_4$O$_{12}$NO$_3$ are discussed.

cond-mat.str-el↗

arXiv2011

Phase Diagram of the J1, J2, J3 Heisenberg Models on the Honeycomb Lattice: A Series Expansion Study

We study magnetically ordered phases and their phase boundaries in the $J_1-J_2-J_3$ Heisenberg models on the honeycomb lattice using series expansions around Néel and different colinear and non-colinear magnetic states. An Ising anisotropy ($λ=J_{\perp}/J_z\ne 1$) is introduced and ground state energy and magnetization order parameter are calculated as a power seies expansion in $λ$. Series extrapolation methods are used to study properties for the Heisenberg model ($λ=1$). We find that at large $J_3$ ($>0.6$) there is a first order transition between Néel and columnar states, in agreement with the classical answer. For $J_3=0$, we find that the Néel phase extends beyond the region of classical stability. We also find that spiral phases are stabilized over large parameter regions, although their spiral angles can be substantially renormalized with respect to the classical values. Our study also shows a magnetically disordered region at intermedaite $J_2/J_1$ and $J_3/J_1$ values.

cond-mat.str-el↗