arXiv subjects

R. Redmer

Publications and source records attributed to R. Redmer.

At least 19 recordsLinked to original sources

arXiv2026

Volume Collapse Without a Structural Transition in Shock-Compressed FeO

We report x-ray diffraction and emission spectroscopy of FeO under laser-driven shock compression between 31-199 GPa. FeO retains the B1 (rocksalt) structure along the Hugoniot to the melt boundary at 191 GPa. While the phase and volume are broadly consistent with results from static compression, we observe an anomalous 7-10% volume collapse around 60 GPa absent in static experiments. We identify this as an isostructural high-spin to low-spin metallic transition in FeO. The low-spin state is directly evidenced by x-ray emission spectroscopy at 180 GPa.

cond-mat.mtrl-sci↗

arXiv2025

Probing the atomic dynamics of ultrafast melting with femtosecond electron diffraction

Melting is an everyday phase transition that is determined by thermodynamic parameters like temperature and pressure. In contrast, ultrafast melting is governed by the microscopic response to a rapid energy input and, thus, can reveal the strength and dynamics of atomic bonds as well as the energy flow rate to the lattice. Accurately describing these processes remains challenging and requires detailed insights into transient states encountered. Here, we present data from femtosecond electron diffraction measurements that capture the structural evolution of copper during the ultrafast solid to liquid phase transformations. At absorbed energy densities 2 to 4 times the melting threshold, melting begins at the surface slightly below the nominal melting point followed by rapid homogeneous melting throughout the volume. Molecular dynamics simulations reproduce these observations and reveal a weak electron lattice energy transfer rate for the given experimental conditions. Both simulations and experiments show no indications of rapid lattice collapse when its temperature surpasses proposed limits of superheating, providing evidence that inherent dynamics limits the speed of disordering in ultrafast melting of metals.

cond-mat.mtrl-sci↗

arXiv2025

Scaling of thin wire cylindrical compression after 100 fs Joule surface heating with material, diameter and laser energy

We present the first systematic experimental validation of return-current-driven implosion scaling in micrometer-sized wires irradiated by femtosecond laser pulses. Employing XFEL-based imaging with sub-micrometer spatial and femtosecond temporal resolution, supported by hydrodynamic and particle-in-cell simulations, we reveal how return current density depends precisely on wire diameter, material properties, and incident laser energy. We identify deviations from simple theoretical predictions due to geometrically influenced electron escape dynamics. These results refine and confirm the scaling laws essential for predictive modeling in high-energy-density physics and inertial fusion research.

physics.plasm-ph↗

arXiv2025

Femtosecond temperature measurements of laser-shocked copper deduced from the intensity of the x-ray thermal diffuse scattering

We present 50-fs, single-shot measurements of the x-ray thermal diffuse scattering (TDS) from copper foils that have been shocked via nanosecond laser-ablation up to pressures above 135~GPa. We hence deduce the x-ray Debye-Waller (DW) factor, providing a temperature measurement. The targets were laser-shocked with the DiPOLE 100-X laser at the High Energy Density (HED) endstation of the European X-ray Free-Electron Laser (EuXFEL). Single x-ray pulses, with a photon energy of 18 keV, were scattered from the samples and recorded on Varex detectors. Despite the targets being highly textured (as evinced by large variations in the elastic scattering), and with such texture changing upon compression, the absolute intensity of the azimuthally averaged inelastic TDS between the Bragg peaks is largely insensitive to these changes, and, allowing for both Compton scattering and the low-level scattering from a sacrificial ablator layer, provides a reliable measurement of $T/\Theta_D^2$, where $\Theta_D$ is the Debye temperature. We compare our results with the predictions of the SESAME 3336 and LEOS 290 equations of state for copper, and find good agreement within experimental errors. We thus demonstrate that single-shot temperature measurements of dynamically compressed materials can be made via thermal diffuse scattering of XFEL radation.

cond-mat.mtrl-sci↗

arXiv2023

Platform for Probing Radiation Transport Properties of Hydrogen at Conditions Found in the Deep Interiors of Red Dwarfs

We describe an experimental concept at the National Ignition Facility for specifically tailored spherical implosions to compress hydrogen to extreme densities (up to $\sim$800$\times$ solid density, electron number density n$_e$$\sim$4$\times$10$^{25}$ cm$^{-3}$ ) at moderate temperatures (T$\sim$200 eV), i.e., to conditions, which are relevant to the interiors of red dwarf stars. The dense plasma will be probed by laser-generated x-ray radiation of different photon energy to determine the plasma opacity due to collisional (free-free) absorption and Thomson scattering. The obtained results will benchmark radiation transport models, which in the case for free-free absorption show strong deviations at conditions relevant to red dwarfs. This very first experimental test of free-free opacity models at these extreme states will help to constrain where inside those celestial objects energy transport is dominated by radiation or convection. Moreover, our study will inform models for other important processes in dense plasmas, which are based on electron-ion collisions, e.g., stopping of swift ions or electron-ion temperature relaxation.

physics.plasm-ph↗

arXiv2021

Metallization of Shock-Compressed Liquid Ammonia

Ammonia is predicted to be one of the major components in the depths of the ice giant planets Uranus and Neptune. Their dynamics, evolution, and interior structure are insufficiently understood and models rely imperatively on data for equation of state and transport properties. Despite its great significance, the experimentally accessed region of the ammonia phase diagram today is still very limited in pressure and temperature. Here we push the probed regime to unprecedented conditions, up to $\sim$350 GPa and $\sim$40000 K. Along the Hugoniot, the temperature measured as a function of pressure shows a subtle change in slope at $\sim$7000 K and $\sim$90 GPa, in agreement with ab initio simulations we have performed. This feature coincides with the gradual transition from a molecular liquid to a plasma state. Additionally, we performed reflectivity measurements, providing the first experimental evidence of electronic conduction in high-pressure ammonia. Shock reflectance continuously rises with pressure above 50 GPa and reaches saturation values above 120 GPa. Corresponding electrical conductivity values are up to 1 order of magnitude higher than in water in the 100 GPa regime, with possible significant contributions of the predicted ammonia-rich layers to the generation of magnetic dynamos in ice giant interiors.

astro-ph.EP↗

arXiv2019

Thermodynamics of the insulator-metal transition in dense liquid deuterium

Recent dynamic compression experiments [M. D. Knudson et al., Science 348, 1455 (2015); P. M. Celliers et al., Science 361, 677 (2018)] have observed the insulator-metal transition in dense liquid deuterium, but with an approximately 95 GPa difference in the quoted pressures for the transition at comparable estimated temperatures. It was claimed in the latter of these two papers that a very large latent heat effect on the temperature was overlooked in the first, requiring correction of those temperatures downward by a factor of two, thereby putting both experiments on the same theoretical phase boundary and reconciling the pressure discrepancy. We have performed extensive path-integral molecular dynamics calculations with density functional theory to directly calculate the isentropic temperature drop due to latent heat in the insulator-metal transition for dense liquid deuterium and show that this large temperature drop is not consistent with the underlying thermodynamics.

cond-mat.mtrl-sci↗

arXiv2019

The structure in warm dense carbon

The structure of the fluid carbon phase in the pressure region of the graphite, diamond, and BC8 solid phase is investigated. We find increasing coordination numbers with an increase in density. From zero to $30$ GPa, the liquid shows a decrease of packing efficiency with increasing temperature. However, for higher pressures, the coordination number increases with increasing temperature. Up to $1.5$ eV and independent of the pressure up to $1000$ GPa, a double-peak structure in the ion structure factors exists, indicating persisting covalent bonds. Over the whole pressure range from zero to $1000$ GPa, the fluid structure and properties are strongly determined by such covalent bonds.

physics.plasm-ph↗

arXiv2017

The interaction of intense femtosecond laser pulses with argon microdroplets studied near the soft x-ray emission threshold

The extreme ultraviolet plasma emission from liquid microsized argon droplets exposed to intense near-infrared laser pulses has been investigated. Emission from the warm dense matter targets is recorded in a spectral range in between 16 and 30 nm at laser intensities of 10^14 W/cm^2. Above the emission threshold, soft x-ray radiation exponentially increases with the pulse energy whereby a strong dependence of the yields on the pulse duration is observed, which points at an effective electron collisional heating of the microplasma by inverse bremsstrahlung. Accompanying hydrodynamic simulations reveal the temporal and spatial development of the microplasma conditions. The good agreement in between the measured and calculated emission spectra as well as the extracted electron temperatures confirm that hydrodynamic simulations can be applied in the analysis of strongly excited droplets.

physics.atm-clus↗

arXiv2016

The interaction of intense ultrashort laser pulses with cryogenic He jets

We study the interaction of intense ultrashort laser pulses with cryogenic He jets using 2d/3v relativistic Particle-in-Cell simulations (XOOPIC). Of particular interest are laser intensities $(10^{15}-10^{20})$ W/cm$^2$, pulse lengths $\le 100$ fs, and the frequency regime $\sim 800$ nm for which the jets are initially transparent and subsequently not homogeneously ionized. Pulses $\ge 10^{16}$ W/cm$^2$ are found to drive ionization along the jet and outside the laser spot, the ionization-front propagates along the jet at a fraction of the speed of light. Within the ionized region, there is a highly transient field, which may be interpreted as two-surface wave decay and as a result of the charge-neutralizing disturbance at the jet-vacuum interface. The ionized region has solid-like densities and temperatures of few to hundreds of eV, i.e., warm and hot dense matter regimes. Such extreme conditions are relevant for high-energy densities as found, e.g., in shock-wave experiments and inertial confinement fusion studies. The temporal evolution of the ionization is studied considering theoretically a pump-probe x-ray Thomson scattering (XRTS) scheme. We observe plasmon and non-collective modes that are generated in the jet, and their amplitude is proportional to the ionized volume. Our theoretical findings could be tested at free-electron laser facilities such as FLASH and the European XFEL (Hamburg) and the LCLS (Stanford).

physics.plasm-ph↗

arXiv2016

Uranus evolution models with simple thermal boundary layers

The strikingly low luminosity of Uranus (Teff ~ Teq) constitutes a long-standing challenge to our understanding of Ice Giant planets. Here we present the first Uranus structure and evolution models that are constructed to agree with both the observed low luminosity and the gravity field data. Our models make use of modern ab initio equations of state at high pressures for the icy components water, methane, and ammonia. Proceeding step by step, we confirm that adiabatic models yield cooling times that are too long, even when uncertainties in the ice:rock ratio (I:R) are taken into account. We then argue that the transition between the ice/rock-rich interior and the H/He-rich outer envelope should be stably stratified. Therefore, we introduce a simple thermal boundary and adjust it to reproduce the low luminosity. Due to this thermal boundary, the deep interior of the Uranus models are up to 2--3 warmer than adiabatic models, necessitating the presence of rocks in the deep interior with a possible I:R of $1\times$ solar. Finally, we allow for an equilibrium evolution (Teff ~ Teq) that begun prior to the present day, which would therefore no longer require the current era to be a "special time" in Uranus' evolution. In this scenario, the thermal boundary leads to more rapid cooling of the outer envelope. When Teff ~ Teq is reached, a shallow, subadiabatic zone in the atmosphere begins to develop. Its depth is adjusted to meet the luminosity constraint. This work provides a simple foundation for future Ice Giant structure and evolution models, that can be improved by properly treating the heat and particle fluxes in the diffusive zones.

astro-ph.EP↗

arXiv2014

Warm dense matter conductivity including electron-electron collisions

The controversy with respect to the role of electron-electron collisions in the dynamic conductivity of dense plasmas is resolved. In particular, the dc conductivity is analyzed in the low-density, non-degenerate limit where the Spitzer theory is valid and electron-electron collisions lead to the well-known reduction of the result for a Lorentz plasma. With increasing degeneracy, the contribution of electron-electron collisions to the dc conductivity is decreasing and can be neglected for the liquid metal domain where the Ziman-Faber theory is applicable. We show how electron-electron collisions have to be implemented in calculations based on the Kubo-Greenwood formula which is prevalently applied in simulations for the frequency-dependent conductivity in the warm dense matter region, i.e. for arbitrary degeneracy.

physics.plasm-ph↗

arXiv2013

Saturn layered structure and homogeneous evolution models with different EOSs

The core mass of Saturn is commonly assumed to be 10-25 ME as predicted by interior models with various equations of state (EOSs) and the Voyager gravity data, and hence larger than that of Jupiter (0-10 ME). We here re-analyze Saturn's internal structure and evolution by using more recent gravity data from the Cassini mission and different physical equations of state: the ab initio LM-REOS which is rather soft in Saturn's outer regions but stiff at high pressures, the standard Sesame-EOS which shows the opposite behavior, and the commonly used SCvH-i EOS. For all three EOS we find similar core mass ranges, i.e. of 0-20 ME for SCvH-i and Sesame EOS and of 0-17 ME for LM-REOS. Assuming an atmospheric helium mass abundance of 18%, we find maximum atmospheric metallicities, Zatm of 7x solar for SCvH-i and Sesame-based models and a total mass of heavy elements, MZ of 25-30 ME. Some models are Jupiter-like. With LM-REOS, we find MZ=16-20 ME, less than for Jupiter, and Zatm less than 3x solar. For Saturn, we compute moment of inertia values lambda=0.2355(5). Furthermore, we confirm that homogeneous evolution leads to cooling times of only about 2.5 Gyr, independent on the applied EOS. Our results demonstrate the need for accurately measured atmospheric helium and oxygen abundances, and of the moment of inertia for a better understanding of Saturn's structure and evolution.

astro-ph.EP↗

arXiv2012

New indication for a dichotomy in the interior structure of Uranus and Neptune from the application of modified shape and rotation data

Since the Voyager fly-bys of Uranus and Neptune, improved gravity field data have been derived from long-term observations of the planets' satellite motions, and modified shape and solid-body rotation periods were suggested. A faster rotation period (-40 min) for Uranus and a slower rotation period (+1h20) of Neptune compared to the Voyager data were found to minimize the dynamical heights and wind speeds. We apply the improved gravity data, the modified shape and rotation data, and the physical LM-R equation of state to compute adiabatic three-layer structure models, where rocks are confined to the core, and homogeneous thermal evolution models of Uranus and Neptune. We present the full range of structure models for both the Voyager and the modified shape and rotation data. In contrast to previous studies based solely on the Voyager data or on empirical EOS, we find that Uranus and Neptune may differ to an observationally significant level in their atmospheric heavy element mass fraction Z1 and nondimensional moment of inertia, nI. For Uranus, we find Z1 < 8% and nI=0.2224(1), while for Neptune Z1 < 65% and nI=0.2555(2) when applying the modified shape and rotation data, while for the unmodified data we compute Z1 < 17% and nI=0.230(1) for Uranus and Z1 < 54% and nI=0.2410(8) for Neptune. In each of these cases, solar metallicity models (Z1=0.015) are still possible. The cooling times obtained for each planet are similar to recent calculations with the Voyager rotation periods: Neptune's luminosity can be explained by assuming an adiabatic interior while Uranus cools far too slowly. More accurate determinations of these planets' gravity fields, shapes, rotation periods, atmospheric heavy element abundances, and intrinsic luminosities are essential for improving our understanding of the internal structure and evolution of icy planets.

astro-ph.EP↗

arXiv2012

Probing the interiors of the ice giants: Shock compression of water to 700 GPa and 3.8 g/ccm

Recently there has been tremendous increase in the number of identified extra-solar planetary systems. Our understanding of their formation is tied to exoplanet internal structure models, which rely upon equations of state of light elements and compounds like water. Here we present shock compression data for water with unprecedented accuracy that shows water equations of state commonly used in planetary modeling significantly overestimate the compressibility at conditions relevant to planetary interiors. Furthermore, we show its behavior at these conditions, including reflectivity and isentropic response, is well described by a recent first-principles based equation of state. These findings advocate this water model be used as the standard for modeling Neptune, Uranus, and "hot Neptune" exoplanets, and should improve our understanding of these types of planets.

astro-ph.EP↗

arXiv2011

Constraining the interior of extrasolar giant planets with the tidal Love number k_2 using the example of HAT-P-13b

Transit and radial velocity observations continuously discover an increasing number of exoplanets. However, when it comes to the composition of the observed planets the data are compatible with several interior structure models. Thus, a planetary parameter sensitive to the planet's density distribution could help constrain this large number of possible models even further. We aim to investigate to what extent an exoplanet's interior can be constrained in terms of core mass and envelope metallicity by taking the tidal Love number k_2 into account as an additional possibly observable parameter. Because it is the only planet with an observationally determined k_2, we constructed interior models for the Hot Jupiter exoplanet HAT-P-13b by solving the equations of hydrostatic equilibrium and mass conservation for different boundary conditions. In particular, we varied the surface temperature and the outer temperature profile, as well as the envelope metallicity within the widest possible parameter range. We also considered atmospheric conditions that are consistent with nongray atmosphere models. For all these models we calculated the Love number k_2 and compared it to the allowed range of k_2 values that could be obtained from eccentricity measurements of HAT-P-13b. We use the example of HAT-P-13b to show the general relationships between the quantities temperature, envelope metallicity, core mass, and Love number of a planet. For any given k_2 value a maximum possible core mass can be determined. For HAT-P-13b we find Mcore < 27 ME, based on the latest eccentricity measurement. We are able to constrain both the envelope and bulk metallicity of HAT-P-13b to 1 -- 11 times stellar metallicity and the extension of the isothermal layer in the planet's atmosphere to 3 -- 44 bar. Assuming equilibrium tidal theory, we find lower limits on the tidal Q consistent with 10^3 - 10^5.

astro-ph.EP↗

arXiv2011

Young Exoplanet Transit Initiative (YETI)

We present the Young Exoplanet Transit Initiative (YETI), in which we use several 0.2 to 2.6m telescopes around the world to monitor continuously young (< 100 Myr), nearby (< 1 kpc) stellar clusters mainly to detect young transiting planets (and to study other variability phenomena on time-scales from minutes to years). The telescope network enables us to observe the targets continuously for several days in order not to miss any transit. The runs are typically one to two weeks long, about three runs per year per cluster in two or three subsequent years for about ten clusters. There are thousands of stars detectable in each field with several hundred known cluster members, e.g. in the first cluster observed, Tr-37, a typical cluster for the YETI survey, there are at least 469 known young stars detected in YETI data down to R=16.5 mag with sufficient precision of 50 milli-mag rms (5 mmag rms down to R=14.5 mag) to detect transits, so that we can expect at least about one young transiting object in this cluster. If we observe 10 similar clusters, we can expect to detect approximately 10 young transiting planets with radius determinations. The precision given above is for a typical telescope of the YETI network, namely the 60/90-cm Jena telescope (similar brightness limit, namely within +/-1 mag, for the others) so that planetary transits can be detected. For planets with mass and radius determinations, we can calculate the mean density and probe the internal structure. We aim to constrain planet formation models and their time-scales by discovering planets younger than 100 Myr and determining not only their orbital parameters, but also measuring their true masses and radii, which is possible so far only by the transit method. Here, we present an overview and first results. (Abstract shortened)

astro-ph.SR↗

arXiv2011

On the degeneracy of the tidal Love number k2 in multi-layer planetary models: application to Saturn and GJ436b

In order to accurately model giant planets, a whole set of observational constraints is needed. As the conventional constraints for extrasolar planets like mass, radius, and temperature allow for a large number of acceptable models, a new planetary parameter is desirable in order to further constrain planetary models. Such a parameter may be the tidal Love number k2. In this paper we aim to study the capability of k2 to reveal further information about the interior structure of a planet. With theoretical planetary models we investigate how the tidal Love number k2 responds to the internal density distribution of a planet. In particular, we demonstrate the effect of the degeneracy of k2 due to a density discontinuity in the envelope of a three-layer planetary model. The effect of a possible outer density discontinuity masks the effect of the core mass on the Love number k2. Hence, there is no unique relationship between the Love number k2 and the core mass of a planet. We show that the degeneracy of k2 with respect to a layer boundary in the envelope also occurs in existing planets, e.g. Saturn and the Hot Neptune GJ436b. As a result of the degeneracy, the planetary parameter k2 cannot be used to further constrain Saturnian models and for GJ436b only a maximum possible core mass can be derived from a given k2. To significantly narrow the uncertainty about the core mass of GJ436b the combined knowledge of k2 and atmospheric metallicity and temperature profile is necessary.

astro-ph.EP↗