arXiv subjects

R. Rodriguez-Guzman

Publications and source records attributed to R. Rodriguez-Guzman.

At least 19 recordsLinked to original sources

arXiv2026

Impact of perturbative tensor interactions on the spontaneous fission half-lives of superheavy nuclei

The standard microscopic description of fission, based on the mean-field Hartree-Fock-Bogoliubov approximation and a semi-classical description of tunneling through the fission barrier, has been used to analyse the impact of introducing a (perturbative) tensor term along with the well known Gogny-D1S force in the spontaneous fission half-lives. Calculations in a series of even-even isotopes of superheavy nuclei ranging from nobelium to darmstatium have been carried out. The results show that the tensor term only impacts the height of the first fission barrier and leaves mostly unaffected the pairing properties and therefore the collective inertias. As a consequence of the reduction in the barrier height, the spontaneous fission lifetimes obtained by including the tensor term are significantly smaller than the ones without it bringing the theoretical predictions in closer agreement with experimental data.

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arXiv2025

Quadrupole-hexadecapole coupling in the rare earth region with beyond mean field correlations

The roles of static hexadecapole deformation and beyond-mean-field quadrupole-hexadecapole configuration mixing are studied for a selected set of Yb, Hf, W and Os isotopes within the mass range $170 \le A \le 202$, using the Hartree-Fock-Bogoliubov (HFB) and the two-dimensional Generator Coordinate Method (2D-GCM) approaches, based on the Gogny energy density functional. The 2D-GCM ground and excited states of the lighter isotopes are associated with diamond-like shapes while, for each isotopic chain, a region where those states correspond to square-like shapes has been found below the neutron shell closure $N=126$. It is shown, that for the studied nuclei the quadrupole and hexadecapole degrees of freedom are interwoven in the ground and excited states up to the mass number $A=184-188$. This structural evolution, encoded in the 2D-GCM collective wave functions, is accompanied by an enhanced prolate-oblate shape coexistence around the neutron number $N=116$. In agreement with previous studies, it is also shown that for the considered Yb, Hf, W and Os isotopes the inclusion of hexadecapole deformation in the ground state dynamics leads to a non trivial additional correlation energy comparable to the quadrupole correlation energy itself.

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arXiv2025

Microscopic description of quadrupole-hexadecapole coupling in radium, thorium, uranium and plutonium isotopes with the Gogny energy density functional

The emergence and stability of static hexadecapole deformations as well as the impact in the development of dynamic deformation due to collective motion considering quadrupole-hexadecapole coupling are studied for a selected set of radium, thorium, uranium and plutonium isotopes, using the Gogny Hartree-Fock-Bogoliubov and Generator Coordinate Method frameworks. Sizable hexadecapole deformations are found to play a significant role in the ground and excited states of nuclei in the neighborhood of $^{238}$U. For each of the studied isotopic chains, it is shown that a region with small negative hexadecapole deformation, just below the neutron magic number $N =184$, remains stable once zero-point quadrupole-hexadecapole fluctuations are taken into account. A transition is predicted, with increasing mass number, from a regime in which the quadrupole and hexadecapole degrees of freedom are interwoven to a regime in which they are decoupled, accompanied by an enhanced shape coexistence in the more neutron-rich sectors of the isotopic chains. It is also shown, that quadrupole-hexadecapole configuration mixing brings a nontrivial additional correlation energy gain comparable to the quadrupole correlation energy itself.

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arXiv2023

Beyond-mean-field description of octupolarity in dysprosium isotopes with the Gogny-D1M energy density functional

The emergence and stability of (static) octupole deformation effects in Dy isotopes from dripline to dripline ($72 \le N \le 142$) is analyzed in this paper using mean-field and beyond-mean-field techniques often used for this purpose. We find static octupole deformations at the Hartree-Fock-Bogoliubov (HFB) level with the Gogny D1M force for $N \approx 134$ isotopes, while nuclei with $N \approx 88$ exhibit reflection-symmetric ground states. It is shown that, given the softness found in the mean-field and parity-projected potential energy surfaces along the octupole direction, neither of these two levels of approximation is suficcient to extract conclusions about the (permanent and/or vibrational) nature of octupole dynamic in Dy isotopes. From the analysis of the collective wave functions as well as the excitation energies of the first negative-parity states and $B(E3)$ strengths, obtained within the framework of a two-dimensional symmetry-conserving generator coordinate method (2D-GCM), it is concluded that the increased octupole collectivity in Dy isotopes with $N \approx 88$ and $N \approx 134$ is a vibrational-like effect that is not directly related to permanent mean-field octupole deformation in the considered nuclei. A pronounced suppression of the $B(E1)$ strengths is predicted for isotopes with $N \approx 82$ and $N \approx 126$. The comparison of results obtained with other parametrizations, show the robustness of the predicted trends with respect to the underlying Gogny energy density functional.

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arXiv2023

Least action description of dynamic pairing correlations in the fission of Curium and Californium isotopes based on the Gogny energy density functional

The impact of dynamic pairing correlations and their interplay with Coulomb antipairing effects on the systematic of the spontaneous fission half-lives for the nuclei $^{240-250}$Cm and $^{240-250}$Cf is analyzed, using a hierarchy of approximations based on the parametrization D1M of the Gogny energy density functional (EDF). First, the constrained Hartree-Fock-Bogoliubov (HFB) approximation is used to compute deformed mean-field configurations, zero-point quantum corrections and collective inertias either by using the Slater approximation to Coulomb exchange and neglecting Coulomb antipairing or by fully considering the exchange and pairing channels of the Coulomb interaction. Next, the properties of the {\it{least action}} and {\it{least energy}} fission paths are compared. In the {\it{least action}} case, pairing is identified as the relevant degree of freedom in order to minimize the action entering the Wentzel-Kramers-Brillouin (WKB) approximation to the tunneling probability through the fission barrier. Irrespective of the treatment of Coulomb exchange and antipairing, it is shown that the {\it{least action}} path obtained taking into account the pairing degree of freedom leads to stronger pairing correlations that significantly reduce the spontaneous fission half-lives $t_{SF}$ improving thereby the comparison with the experiment by several orders of magnitude. It is also shown that the Coulomb antipairing effect is, to a large extent, washed out by the {\it{least action}} procedure and therefore the $t_{SF}$ values obtained by the two different treatments of the Coulomb exchange and pairing are of similar quality.

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arXiv2021

Microscopic description of quadrupole-octupole coupling in neutron-rich actinides and superheavy nuclei with the Gogny-D1M energy density functional

The interplay between quadrupole and octupole degrees of freedom is discussed in a series of neutron-rich actinides and superheavy nuclei with $92 \le$ Z $\le 110$ and $186 \le$ N $\le 202$. In addition to the static Hartree-Fock-Bogoliubov approach, dynamical beyond-mean-field correlations are taken into account via both parity restoration and symmetry-conserving Generator Coordinate Method calculations based on the Gogny-D1M energy density functional. Physical properties such as correlation energies, negative-parity excitation energies as well as reduced transition probabilities $B(E1)$ and $B(E3)$ are discussed in detail. It is shown that, for the studied nuclei, the quadrupole-octupole coupling is weak and to a large extent the properties of negative parity states can be reasonably well described in terms of the octupole degree of freedom alone.

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arXiv2018

Least action description of spontaneous fission in fermium and nobelium nuclei based on the Gogny energy density functional

The systematic of the spontaneous fission half-lives for the nuclei $^{242-262}$Fm and $^{250-260}$No is analyzed, within a least action scheme, with the parametrization D1M of the Gogny energy density functional. The properties of the dynamic (least action) fission paths are analyzed and compared to those of the static (minimal energy) ones. The constrained Hartree-Fock-Bogoliubov approximation is used to compute deformed mean-field configurations, zero-point quantum corrections and collective inertias. It is shown that a cumbersome full variational search of the least action fission path, within the space of HFB states, might not be required if the relevant degrees of freedom are taken into account in the minimization of the Wentzel-Kramers-Brillouin action. The action is minimized in terms of pairing fluctuations that explore the pairing content of the HFB states along the fission paths of the considered nuclei. It is found that, for a given shape, the minimum of the action in fermium and nobelium nuclei corresponds to a value of the pairing fluctuations larger than the one associated with the minimal energy solution for the same shape. The reduction of the action, via larger pairing correlations, has a significant impact on the predicted spontaneous fission half-lives improving their comparison with the experiment by several orders of magnitude.

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arXiv2016

Microscopic description of fission in nobelium isotopes with the Gogny-D1M energy density functional

Constrained mean-field calculations, based on the Gogny-D1M energy density functional, have been carried out to describe fission in the isotopes $^{250-260}$No. The even-even isotopes have been considered within the standard Hartree-Fock-Bogoliobov (HFB) framework while for the odd-mass ones the Equal Filling Approximation (HFB-EFA) has been employed. Ground state quantum numbers and deformations, pairing energies, one-neutron separation energies, inner and outer barrier heights as well as fission isomer excitation energies are given. Fission paths, collective masses and zero-point quantum vibrational and rotational corrections are used to compute the systematic of the spontaneous fission half-lives t$_\mathrm{SF}$ both for even-even and odd-mass nuclei. Though there exists a strong variance of the predicted fission rates with respect to the details involved in their computation, it is shown that both the specialization energy and the pairing quenching effects, taken into account within the self-consistent HFB-EFA blocking procedure, lead to larger t$_\mathrm{SF}$ values in odd-mass nuclei as compared with their even-even neighbors. Alpha decay lifetimes have also been computed using a parametrization of the Viola-Seaborg formula. The high quality of the Gogny-D1M functional regarding nuclear masses leads to a very good reproduction of $Q_α$ values and consequently of lifetimes.

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arXiv2014

Microscopic description of quadrupole collectivity in neutron-rich nuclei across the N=126 shell closure

The quadrupole collectivity in Nd, Sm, Gd, Dy, Er, Yb, Hf and W nuclei with neutron numbers 122 $\le$ N $\le$ 156 is studied, both at the mean field level and beyond, using the Gogny energy density functional. Besides the robustness of the N=126 neutron shell closure, it is shown that the onset of static deformations in those isotopic chains with increasing neutron number leads to an enhanced stability and further extends the corresponding two-neutron driplines far beyond what could be expected from spherical calculations. Independence of the mean field predictions with respect to the particular version of the Gogny energy density functional employed is demonstrated by comparing results based on the D1S and D1M parameter sets. Correlations beyond mean field are taken into account in the framework of the angular momentum projected generator coordinate method calculation. It is shown that N=126 remains a robust neutron magic number when dynamical effects are included. The analysis of the collective wave functions, average deformations and excitation energies indicate that, with increasing neutron number, the zero-point quantum corrections lead to dominant prolate configurations in the 0$_{1}^{+}$, 0$_{2}^{+}$, 2$_{1}^{+}$ and 2$_{2}^{+}$ states of the studied nuclei. Moreover, those dynamical deformation effects provide an enhanced stability that further supports the mean field predictions, corroborating a shift of the r-process path to higher neutron numbers. Beyond mean field calculations provide a smaller shell gap at N=126 than the mean field one in good agreement with previous theoretical studies. However, the shell gap still remains strong enough in the two-neutron driplines.

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arXiv2014

Dynamic versus static fission paths with realistic interactions

The properties of dynamic (least action) fission paths are analyzed and compared to the ones of the more traditional static (least energy) paths. Both the BCPM and Gogny D1M energy density functionals are used in the calculation of the HFB constrained configurations providing the potential energy and collective inertias. The action is computed as in the WKB method. A full variational search of the least-action path over the complete variational space of HFB wave functions is cumbersome and probably unnecessary if the relevant degrees of freedom are identified. In this paper, we consider the particle number fluctuation degree of freedom that explores the amount of pairing correlations in the wave function. For a given shape, the minimum action can be up a factor of three smaller than the action computed for the minimum energy state with the same shape. The impact of this reduction on the lifetimes is enormous and dramatically improves the agreement with experimental data in the few examples considered.

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arXiv2014

Microscopic description of fission in neutron-rich plutonium isotopes with the Gogny-D1M energy density functional

The most recent parametrization D1M of the Gogny energy density functional is used to describe fission in the isotopes $^{232-280}$ Pu. We resort to the methodology introduced in our previous studies [Phys. Rev. C \textbf{88}, 054325 (2013) and Phys. Rev. C \textbf {89}, 054310 (2014)] to compute the fission paths, collective masses and zero point quantum corrections within the Hartree-Fock-Bogoliubov framework. The systematics of the spontaneous fission half-lives t$_{SF}$, masses and charges of the fragments in Plutonium isotopes is analyzed and compared with available experimental data. We also pay attention to isomeric states, the deformation properties of the fragments as well as to the competition between the spontaneous fission and $α$-decay modes. The impact of pairing correlations on the predicted t$_{SF}$ values is demonstrated with the help of calculations for $^{232-280}$Pu in which the pairing strengths of the Gogny-D1M energy density functional are modified by 5 $\%$ and 10 $\%$, respectively. We further validate the use of the D1M parametrization through the discussion of the half-lives in $^{242-262}$Fm. Our calculations corroborate that, though the uncertainties in the absolute values of physical observables are large, the Gogny-D1M Hartree-Fock-Bogoliubov framework still reproduces the trends with mass and/or neutron numbers and therefore represents a reasonable starting point to describe fission in heavy nuclear systems from a microscopic point of view.

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arXiv2014

Microscopic description of fission in Uranium isotopes with the Gogny energy density functional

The most recent parametrizations D1S, D1N and D1M of the Gogny energy density functional are used to describe fission in the isotopes $^{232-280}$ U. Fission paths, collective masses and zero point quantum corrections, obtained within the constrained Hartree-Fock-Bogoliubov approximation, are used to compute the systematics of the spontaneous fission half-lives $t_\mathrm{SF}$, the masses and charges of the fission fragments as well as their intrinsic shapes. The Gogny-D1M parametrization has been benchmarked against available experimental data on inner and second barrier heights, excitation energies of the fission isomers and half-lives in a selected set of Pu, Cm, Cf, Fm, No, Rf, Sg, Hs and Fl nuclei. It is concluded that D1M represents a reasonable starting point to describe fission in heavy and superheavy nuclei. Special attention is also paid to understand the uncertainties in the predicted $t_\mathrm{SF}$ values arising from the different building blocks entering the standard semi-classical Wentzel-Kramers-Brillouin formula. Although the uncertainties are large, the trend with mass or neutron numbers are well reproduced and therefore the theory still has predictive power. In this respect, it is also shown that modifications of a few per cent in the pairing strength can have a significant impact on the collective masses leading to uncertainties in the $t_\mathrm{SF}$ values of several orders of magnitude.

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arXiv2014

Shape evolution and shape coexistence in Pt isotopes: comparing interacting boson model configuration mixing and Gogny mean-field energy surfaces

The evolution of the total energy surface and the nuclear shape in the isotopic chain $^{172-194}$Pt are studied in the framework of the interacting boson model, including configuration mixing. The results are compared with a self-consistent Hartree-Fock-Bogoliubov calculation using the Gogny-D1S interaction and a good agreement between both approaches shows up. The evolution of the deformation parameters points towards the presence of two different coexisting configurations in the region 176 $\leq$ A $\leq$ 186.

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arXiv2013

Shape evolution and the role of intruder configurations in Hg isotopes within the interacting boson model based on a Gogny energy density functional

The interacting boson model with configuration mixing, with parameters derived from the self-consistent mean-field calculation employing the microscopic Gogny energy density functional, is applied to the systematic analysis of the low-lying structure in Hg isotopes. Excitation energies, electromagnetic transition rates, deformation properties, and ground-state properties of the $^{172-204}$Hg nuclei are obtained by mapping the microscopic deformation energy surface onto the equivalent IBM Hamiltonian in the boson condensate. These results point to the overall systematic trend of the transition from the near spherical vibrational state in lower-mass Hg nuclei close to $^{172}$Hg, onset of intruder prolate configuration as well as the manifest prolate-oblate shape coexistence around the mid-shell nucleus $^{184}$Hg, weakly oblate deformed structure beyond $^{190}$Hg up to the spherical vibrational structure toward the near semi-magic nucleus $^{204}$Hg, as observed experimentally. The quality of the present method in the description of the complex shape dynamics in Hg isotopes is examined.

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arXiv2012

Microscopic description of quadrupole-octupole coupling in Sm and Gd isotopes with the Gogny Energy Density Functional

The interplay between the collective dynamics of the quadrupole and octupole deformation degree of freedom is discussed in a series of Sm and Gd isotopes both at the mean field level and beyond, including parity symmetry restoration and configuration mixing. Physical properties like negative parity excitation energies, E1 and E3 transition probabilities are discussed and compared to experimental data. Other relevant intrinsic quantities like dipole moments, ground state quadrupole moments or correlation energies associated to symmetry restoration and configuration mixing are discussed. For the considered isotopes, the quadrupole-octupole coupling is found to be weak and most of the properties of negative parity states can be described in terms of the octupole degree of freedom alone.

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arXiv2012

Shape coexistence in Lead isotopes in the interacting boson model with Gogny energy density functional

We investigate the emergence and evolution of shape coexistence in the neutron-deficient Lead isotopes within the interacting boson model (IBM) plus configuration mixing with microscopic input based on the Gogny energy density functional (EDF). The microscopic potential energy surface obtained from the constrained self-consistent Hartree-Fock-Bogoliubov method employing the Gogny-D1M EDF is mapped onto the coherent-state expectation value of the configuration-mixing IBM Hamiltonian. In this way, the parameters of the IBM Hamiltonian are fixed for each of the three relevant configurations (spherical, prolate and oblate) associated to the mean field minima. Subsequent diagonalization of the Hamiltonian provides the excitation energy of the low-lying states and transition strengths among them. The model predictions for the $0^{+}$ level energies and evolving shape coexistence in the considered Lead chain are consistent both with experiment and with the indications of the Gogny-EDF energy surfaces.

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arXiv2012

N-electron Slater determinants from non-unitary canonical transformations of fermion operators

Mean-field methods such as Hartree-Fock (HF) or Hartree-Fock-Bogoliubov (HFB) constitute the building blocks upon which more elaborate many-body theories are based on. The HF and HFB wavefunctions are built out of independent quasi-particles resulting from a unitary linear canonical transformation of the elementary fermion operators. Here, we discuss the possibility of allowing the HF transformation to become non-unitary. The properties of such HF vacua are discussed, as well as the evaluation of matrix elements among such states. We use a simple ansatz to demonstrate that a non-unitary transformation brings additional flexibility that can be exploited in variational approximations to many-fermion wavefunctions. The action of projection operators on non-unitary based HF states is also discussed and applied to the one-dimensional Hubbard model with periodic boundary conditions.

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arXiv2011

Collective structural evolution in neutron-rich Yb, Hf, W, Os and Pt isotopes

An interacting boson model Hamiltonian determined from Hartree-Fock-Bogoliubov calculations with the new microscopic Gogny energy density functional D1M, is applied to the spectroscopic analysis of neutron-rich Yb, Hf, W, Os and Pt isotopes with mass $A\sim 180-200$. Excitation energies and transition rates for the relevant low-lying quadrupole collective states are calculated by this method. Transitions from prolate to oblate ground-state shapes are analyzed as a function of neutron number $N$ in a given isotopic chain by calculating excitation energies, $B$(E2) ratios, and correlation energies in the ground state. It is shown that such transitions tend to occur more rapidly for the isotopes with lower proton number $Z$, when departing from the proton shell closure Z=82. The triaxial degrees of freedom turn out to play an important role in describing the considered mass region. Predicted low-lying spectra for the neutron-rich exotic Hf and Yb isotopes are presented. The approximations used in the model and the possibilities to refine its predictive power are addressed.

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