arXiv subjects

R. S. Lubna

Publications and source records attributed to R. S. Lubna.

At least 19 recordsLinked to original sources

arXiv2025

Constraining the Synthesis of the Lightest p Nucleus 74Se

We provide the first experimental cross section of the $^{73}\text{As}(p,γ)^{74}\text{Se}$ reaction to constrain one of the main destruction mechanisms of the p nucleus $^{74}\text{Se}$ in explosive stellar environments. The measurement was done using a radioactive $^{73}\text{As}$ beam at effective center-of-mass energies of 2.9 and 2.3 MeV/nucleon. Along with the total cross-section measurement, statistical properties of the $^{74}\text{Se}$ compound nucleus were extracted, constraining the reaction cross section in the upper Gamow window of the $γ$ process. The impact of the experimentally constrained reaction rate on $^{74}\text{Se}$ production in Type II supernovae was investigated through Monte Carlo one-zone network simulations. The results indicate that the overproduction of $^{74}$Se by Type II supernova models cannot be resolved by nuclear physics alone and point toward the need for a more detailed understanding of the astrophysical conditions of relevance for the $γ$ process.

nucl-ex↗

arXiv2025

Beta-decay Half Lives beyond $^{54}$Ca: A Systematic Survey of Decay Properties approaching the Neutron Dripline

In an experiment performed at the Facility for Rare Isotope Beams (FRIB) using the FRIB Decay Station initiator (FDSi), 15 new half lives of isotopes near $^{54}$Ca were measured. A new method of extracting lifetimes from experimental data, taking into account the unknown $β$-delayed neutron emission branches of very neutron-rich nuclei, was developed to enable systematic uncertainty analysis. The experiment observed a dramatic change in the half-life systematics for the isotopes with neutron number N =34. Beyond N =34, the decline of nuclear lifetime is much slower, leading to longer than anticipated lifetimes for near-dripline nuclei. State-of-the-art shell-model calculations can explain the experimental results for Z$>$19 nuclei, revealing the imprint of shell effects and the need for modification of single-particle neutron states. The results from a newly developed QRPA model with potential for making global predictions were also tested against the experimental results and good agreement was found.

nucl-ex↗

arXiv2025

Intruder structures in $^{32}$Si and $^{29}$Al

We have studied $^{32}$Si and $^{29}$Al using $^{12}$C($^{22}$Ne,2p) and $^{12}$C($^{22}$Ne,$α$p) fusion-evaporation reactions. In both cases, we observed significant population of high-spin structures distinct from the ground-state yrast bands. In $^{32}$Si, most of the high-energy states feed into a $J^π = 5^-$ nanosecond isomer. In $^{29}$Al, we identified a rotor-like negative-parity band with a $J^π = 7/2^-$ band-head. Doppler shift lifetime measurements were performed for all observed states. These results were compared to shell model calculations and interpreted in terms of proton and neutron cross-shell excitation.

nucl-ex↗

arXiv2025

Universal Effective Charges in the $sd$ and $fp$ Shells

The 247-keV state in $^{54}$Sc, populated in the $β$ decay of $^{54}$Ca, is reported here as a nanosecond isomer with a half-life of 26.0(22) ns. The state is interpreted as the $1^+$ member of the $πf_{7/2}\otimesνf_{5/2}$ spin-coupled multiplet, which decays to the $3^+,πf_{7/2} \otimes νp_{1/2}$ ground state. The new half-life corresponds to a pure $E2$ transition with a strength of 1.93(16) W.u., providing the most precise, unambiguous $B(E2)$ value in the neutron-rich $fp$ region to date for a nucleus with valence protons above $Z=20$. Notably, it is roughly four times larger than the $B(E2; 1/2^{-} \rightarrow 5/2^{-})$ value in $^{55}$Ca. The results, as compared to semi-empirical and ab initio shell-model calculations, indicate (1) a weak $N=34$ sub-shell gap relative to $N = 32$, (2) a large $E2$ enhancement in Sc as compared to Ca due to $1p-1h$ proton excitations across $Z=28$, and (3) empirical effective proton and neutron charges, $e_π$ = 1.30(8)$e$ and $e_ν$ = 0.452(7)$e$, respectively, that are in contrast to reports of $e_π\approx 1.1-1.15e$ and $e_ν\approx 0.6-0.8e$ for $fp$-shell nuclei near $N = Z$. We demonstrate that these reports are erroneous and that, in fact, a universal set of effective charges can be used across the $sd$ and $fp$ shells.

nucl-ex↗

arXiv2025

Investigation of the Excited States of $^{114}\mathrm{Sn}$ Using the GRIFFIN Spectrometer at TRIUMF

The semi-magic $^{110-122}\mathrm{Sn}$ isotopes display signs of shape coexistence in their excited $0^+$ states, which, in contrast to the spherical $0^+$ ground states, are deformed. This paper investigates the nuclear structure of $^{114}\mathrm{Sn}$ using the competing $β^+$ decay and electron capture of a radioactive beam of $^{114}\mathrm{Sb}$ produced at the TRIUMF-ISAC facility using the GRIFFIN spectrometer. This study will allow for an in-depth understanding of the excited $0^+$ states in $^{114}\mathrm{Sn}$, by focusing on their decay patterns. In the present experiment, transitions at 856.2-keV and 1405.0-keV, which were observed in an earlier $β^+$ decay study but not placed in the $^{114}\mathrm{Sn}$ level scheme, have been assigned to the level scheme in connection to the $0^+_3$ level at 2156.0-keV. Properly assigning these transitions refines the level scheme and enhances our understanding of the nuclear structure in $^{114}\mathrm{Sn}$.

nucl-ex↗

arXiv2024

The evidence of $N=16$ shell closure and $β$-delayed neutron emission from $^{25}$F

We measured the $β$-delayed neutron emission from $^{25}$F for the first time at the Facility for Rare Isotope Beams (FRIB). Using combined neutron and $γ$-ray detector systems of the FRIB Decay Station Initiator (FDSi), we observed $β$-decay transitions populating neutron unbound states between 4.2 and 8 MeV in $^{25}$Ne. The experimental results led to the revision of the $β$-decay half-life and $β$-delayed neutron-emission probability of $^{25}$F. The $β$-decay strength distribution of $^{25}$F extracted from the data agrees with the shell-model predictions using the USDB and SDPF-M effective interactions. This result indicates that the spherical neutron $N = 16$ shell gap persists in $^{25}$F and $^{25}$Ne.

nucl-ex↗

arXiv2024

Evolution of the nuclear spin-orbit splitting explored via the $^{32}$Si($d$,$p$)$^{33}$Si reaction using SOLARIS

The spin-orbit splitting between neutron 1$p$ orbitals at $^{33}$Si has been deduced using the single-neutron-adding ($d$,$p$) reaction in inverse kinematics with a beam of $^{32}$Si, a long-lived radioisotope. Reaction products were analyzed by the newly implemented SOLARIS spectrometer at the reaccelerated-beam facility at the National Superconducting Cyclotron Laboratory. The measurements show reasonable agreement with shell-model calculations that incorporate modern cross-shell interactions, but they contradict the prediction of proton density depletion based on relativistic mean-field theory. The evolution of the neutron 1$p$-shell orbitals is systematically studied using the present and existing data in the isotonic chains of $N=17$, 19, and 21. In each case, a smooth decrease in the separation of the $1p_{3/2}$-$1p_{1/2}$ orbitals is seen as the respective $p$-orbitals approach zero binding, suggesting that the finite nuclear potential strongly influences the evolution of nuclear structure in this region.

nucl-ex↗

arXiv2024

Cross-shell excited configurations in the structure of 34Si

The cross-shell excited states of $^{34}$Si have been investigated via $β$-decays of the $4^-$ ground state and the $1^+$ isomeric state of $^{34}$Al. Since the valence protons and valence neutrons occupy different major shells in the ground state as well as the intruder $1^+$ isomeric state of $^{34}$Al, intruder levels of $^{34}$Si are populated via allowed $β$ decays. Spin assignments to such intruder levels of $^{34}$Si were established through $γ$-$γ$ angular correlation analysis for the negative parity states with dominant configurations $(νd_{3/2})^{-1} \otimes (νf_{7/2})^{1}$ as well as the positive parity states with dominant configurations $(νsd)^{-2} \otimes (νf_{7/2}p_{3/2})^2$. The configurations of such intruder states play crucial roles in our understanding of the $N=20$ shell gap evolution. A configuration interaction model derived from the FSU Hamiltonian was utilized in order to interpret the intruder states in $^{34}$Si. Shell model interaction derived from a more fundamental theory with the Valence Space In Medium Similarity Renormalization Group (VS-IMSRG) method was also employed to interpret the structure of $^{34}$Si.

nucl-ex↗

arXiv2023

Understanding Excitations in $^{59,61}$Co, $^{59}$Ni

High spin states in $^{59}$Co ($Z=27$), $^{59}$Ni ($Z=28$) and $^{61}$Co have been populated by the fusion evaporation reactions, $^{48}$Ti($^{14}$C, p2n)$^{59}$Co, $^{48}$Ti($^{14}$C, 3n)$^{59}$Ni, and $^{50}$Ti($^{14}$C, p2n)$^{61}$Co. The 9 MV tandem accelerator at the John D Fox Laboratory, Florida State University (FSU) was used to accelerate the $^{14}$C beam and the de-exciting $γ$ rays were detected by the FSU detector array consisting of six High Purity Germanium (HPGe) clover detectors, and three single crystals. Directional correlation of the $γ$ rays de-exciting oriented states (DCO ratios) and polarization asymmetry measurements helped to establish spin and parities of the excited states whenever possible. The level scheme of $^{59}$Co has been expanded with the inclusion of positive parity states up to 31/2$^+$ at around 11 MeV. The $^{59}$Ni positive parity states known from previous study were verified with modifications to some of the spins and parities. On the other hand, the negative parity states were extended to 31/2 at an excitation energy of 12 MeV. No new transition was observed for $^{61}$Co, but one of the major bands has been reassigned as consisting of positive parity states by reason of this study which is a candidate for magnetic rotation band. Cross shell excitations were observed in the three nuclei studied and the prominent role of excitation to g$_{9/2}$ orbital crossing the $N=40$ shell gap was established in relation to collective excitation in these nuclei by comparison with large-scale shell model calculations.

nucl-ex↗

arXiv2023

Identifying the spin trapped character of the $^{32}$Si isomeric state

The properties of a nanosecond isomer in $^{32}$Si, disputed in previous studies, depend on the evolution of proton and neutron shell gaps near the `island of inversion'. We have placed the isomer at 5505.2(2) keV with $J^π = 5^-$, decaying primarily via an $E3$ transition to the $2^+_1$ state. The $E3$ strength of 0.0841(10) W.u. is unusually small and suggests that this isomer is dominated by the $(νd_{3/2})^{-1} \otimes (νf_{7/2})^{1}$ configuration, which is sensitive to the $N=20$ shell gap. A newly observed $4^+_1$ state is placed at 5881.4(13) keV; its energy is enhanced by the $Z=14$ subshell closure. This indicates that the isomer is located in a `yrast trap', a feature rarely seen at low mass numbers.

nucl-ex↗

arXiv2023

Experimental Study of the $^{\textbf{38}}$S Excited Level Scheme

Information on the $^{38}$S level scheme was expanded through experimental work utilizing a fusion-evaporation reaction and in-beam $γ$-ray spectroscopy. Prompt $γ$-ray transitions were detected by the Gamma-Ray Energy Tracking Array (GRETINA) and recoiling $^{38}$S residues were selected by the Fragment Mass Analayzer (FMA). Tools based on machine-learning techniques were developed and deployed for the first time in order to enhance the unique selection of $^{38}$S residues and identify any associated $γ$-ray transitions. The new level information, including the extension of the even-spin yrast sequence through $J^π = 8^{(+)}$, was interpreted in terms of a basic single-particle picture as well shell-model calculations which incorporated the empirically derived FSU interaction. A comparison between the properties of the yrast states in the even-$Z$ $N=22$ isotones from $Z=14$ to $20$, and for $^{36}$Si-$^{38}$S in particular, was also presented with an emphasis on the role and influence of the neutron $1p_{3/2}$ orbital on the structure in the region.

nucl-ex↗

arXiv2023

$β^-$ decay of neutron-rich $^{45}$Cl at magic number N=28

Results from the study of $β^-$-decay of $^{45}$Cl, produced in the fragmentation of a 140-MeV/u $^{48}$Ca beam, are presented. The half-life for $^{45}$Cl $β$-decay is measured to be 513(36) ms. The $β^-$ and $β^- 1n$ decay of $^{45}$Cl populated excited states in $^{45,44}$Ar, respectively. On the basis of $γ$-ray singles and $γ$-$γ$ coincidence data, decay schemes for the two daughter nuclei have been established. They are compared with shell model calculations using the FSU interaction. The low-lying negative parity states for $^{45}$Ar are well described by a single particle (neutron) occupying orbitals near the Fermi surface, whereas neutron excitations across the $N = 20$ shell gap are needed to explain the positive-parity states which are expected to be populated in allowed Gamow-Teller $β$-decay of $^{45}$Cl. The highest $β$-feeding to the 5/2$^+$ state in $^{45}$Ar from the ground state of $^{45}$Cl points towards a 3/2$^+$ spin-parity assignment of the ground state of the parent over the other possibility of 1/2$^+$. The high Q$_{β^-}$ value of $^{45}$Cl decay allows for the population of $1p1h$ states above the neutron separation energy in $^{45}$Ar leading to positive parity states of $^{44}$Ar being populated by removal of one neutron from the $sd$ shell. The spin-parities of the excited levels in $^{44}$Ar are tentatively assigned for the first time by comparison with the shell model calculations. The 2978~keV level of $^{44}$Ar is identified as the excited 0$^+$ level which could correspond to a different configuration from the ground state.

nucl-ex↗

arXiv2023

Microsecond Isomer at the N=20 Island of Shape Inversion Observed at FRIB

Excited-state spectroscopy from the first Facility for Rare Isotope Beams (FRIB) experiment is reported. A 24(2)-$μ$s isomer was observed with the FRIB Decay Station initiator (FDSi) through a cascade of 224- and 401-keV $γ$ rays in coincidence with $^{32}\textrm{Na}$ nuclei. This is the only known microsecond isomer ($1{\text{ }μ\text{s}}\leq T_{1/2} < 1\text{ ms}$) in the region. This nucleus is at the heart of the $N=20$ island of shape inversion and is at the crossroads of spherical shell-model, deformed shell-model, and ab initio theories. It can be represented as the coupling of a proton hole and neutron particle to $^{32}\textrm{Mg}$, $^{32}\textrm{Mg}+π^{-1} + ν^{+1}$. This odd-odd coupling and isomer formation provides a sensitive measure of the underlying shape degrees of freedom of $^{32}\textrm{Mg}$, where the onset of spherical-to-deformed shape inversion begins with a low-lying deformed $2^+$ state at 885 keV and a low-lying shape-coexisting $0_2^+$ state at 1058 keV. We suggest two possible explanations for the 625-keV isomer in $^{32}$Na: a $6^-$ spherical shape isomer that decays by $E2$ or a $0^+$ deformed spin isomer that decays by $M2$. The present results and calculations are most consistent with the latter, indicating that the low-lying states are dominated by deformation.

nucl-ex↗

arXiv2023

Coexistence of single particle and collective excitation in $^{61}$Ni

The high spin states in 61 Ni have been studied using the fusion evaporation reaction, Ti( $^{14}$C,3n) $^{61}$Ni at an incident beam energy of 40 MeV. A Compton suppressed multi-HPGe detector setup, consisting of six Clover detectors and three single crystal HPGe detectors was used to detect the de-exciting $γ$ rays from the excited states. The level scheme has been extended up to an excitation energy of 12.8 MeV and a tentative J$_π$ = 35/2$^+$ . The low-lying negative parity levels are found to be generated by single particle excitation within the f p shell and also excitations to the g$_{9/2}$ orbitals as explained well with shell model calculations using the GXPF1Br+V M U (modified) interaction. Two rotational structure of regular E2 sequences with small to moderate axial deformation have been established at higher excitation energy. Most interestingly, two sequences of M1 transitions are reported for the first time and described as magnetic rotational bands. The shears mechanism for both the bands can be described satisfactorily by the geometrical model. The shell model calculation involving the cross shell excitation beyond the fp shell well reproduce the M1 and E2 sequences. The shell model predicted B(M1) values for the magnetic rotational band B1 show the decreasing trend with spin as expected with closing of the shears.

nucl-ex↗

arXiv2023

First Evidence of Axial Shape Asymmetry and Configuration Coexistence in $^{74}$Zn: Suggestion for a Northern Extension of the $N=40$ Island of Inversion

The excited states of $N=44$ $^{74}$Zn were investigated via $γ$-ray spectroscopy following $^{74}$Cu $β$ decay. By exploiting $γ$-$γ$ angular correlation analysis, the $2_2^+$, $3_1^+$, $0_2^+$ and $2_3^+$ states in $^{74}$Zn were firmly established. The $γ$-ray branching and $E2/M1$ mixing ratios for transitions de-exciting the $2_2^+$, $3_1^+$ and $2_3^+$ states were measured, allowing for the extraction of relative $B(E2)$ values. In particular, the $2_3^+ \to 0_2^+$ and $2_3^+ \to 4_1^+$ transitions were observed for the first time. The results show excellent agreement with new microscopic large-scale shell-model calculations, and are discussed in terms of underlying shapes, as well as the role of neutron excitations across the $N=40$ gap. Enhanced axial shape asymmetry (triaxiality) is suggested to characterize $^{74}$Zn in its ground state. Furthermore, an excited $K=0$ band with a significantly larger softness in its shape is identified. A shore of the $N=40$ ``island of inversion'' appears to manifest above $Z=26$, previously thought as its northern limit in the chart of the nuclides.

nucl-ex↗

arXiv2022

Multiparticle-hole excitations in nuclei near N = Z = 20: $^{41}$K

This experimental study of high-spin structure near N = Z = 20 nuclei was focused on $^{41}$K, but will also mention three newly observed $γ$ transitions in $^{41}$Ca observed in the same reaction. High-spin states were populated using the $^{26}$Mg($^{18}$O, $p2nγ$)$^{41}$K and $^{26}$Mg($^{18}$O, $3nγ$)$^{41}$Ca reactions. The experiment was carried out at an incident beam energy of 50 MeV at the Florida State University (FSU) John D. Fox Superconducting Linear Accelerator Laboratory and used the FSU high-purity germanium detector array. The $^{41}$K level scheme was extended to 12325 keV, possibly with J$^π$ = 25/2$^-$ or 27/2$^+$, by means of 25 new transitions and that of $^{41}$Ca to 9916 keV. Linear polarization and a measure of angular distribution results are also reported and used to provide information on the spins and parities of several states in the $^{41}$K decay scheme. The results have been compared to the $spsdpf$ cross-shell FSU shell model interaction calculations. The theoretical results from configurations involving no or one additional nucleon promoted from the $sd$ to the $fp$ shell agree relatively well with the energies of known states, while those that involve multi-particle excitations paint an interesting and complex picture of interplay between single-particle excitations, collective pairing, and deformation. This presents an interesting challenge for future theory.

nucl-ex↗

arXiv2021

First Direct Measurement of an Astrophysical p-Process Reaction Cross Section Using a Radioactive Ion Beam

We have performed the first direct measurement of the 83Rb(p,g) radiative capture reaction cross section in inverse kinematics using a radioactive beam of 83Rb at incident energies of 2.4 and 2.7 A MeV. The measured cross section at an effective relative kinetic energy of Ecm = 2.393 MeV, which lies within the relevant energy window for core collapse supernovae, is smaller than the prediction of statistical model calculations. This leads to the abundance of 84Sr produced in the astrophysical p process being higher than previously calculated. Moreover, the discrepancy of the present data with theoretical predictions indicates that further experimental investigation of p-process reactions involving unstable projectiles is clearly warranted.

nucl-ex↗

arXiv2020

Evolution of the N=20 and 28 Shell Gaps and 2-particle-2-hole states in the FSU Interaction

The FSU $spsdfp$ cross-shell interaction for the shell model was successfully fitted to a wide range of mostly intruder negative parity states of the $sd$ shell nuclei. This paper reports the application of the FSU interaction to systematically trace out the relative positions of the effective single-particle energies of the $0f_{7/2}$ and $1p_{3/2}$ orbitals, the evolution from normally ordered low-lying states to the "Island of Inversion" (IoI), and the behavior of a wide range of excited states with a $0f_{7/2}$ proton and neutron coupled to maximum spin of $7 \hbar$. Above a proton number of about 13 the $0f_{7/2}$ orbital lies below that of $1p_{3/2}$, which is considered normal ordering, but systematically at $Z = 10$ to $12$ the orbitals cross. The calculations reproduce well the 2p2h - 0p0h inversion in the configurations of nuclei inside the IoI, they reproduce the absolute binding energies and the transition to normal ordering as the proton number approaches that of the neutrons. The important role of $1p_{3/2}$ neutron pairs in the IoI is also demonstrated. The calculations account well for the energies of the fully aligned states with 0, 1, or 2 individual $sd$ nucleon aligned in spin with the aligned $π0f_{7/2}$ - $ν0f_{7/2}$ pair and reproduce well their systematic variation with $A$ and number of aligned $sd$ nucleons. The results presented in this paper give hope for the predictive power of the FSU interaction for more exotic nuclei to be explored in near future.

nucl-ex↗