arXiv subjects

R. Sachser

Publications and source records attributed to R. Sachser.

18 recordsLinked to original sources

arXiv2023

Cherenkov radiation of spin waves by ultra-fast moving magnetic flux quanta

Despite theoretical predictions for a Cherenkov-type radiation of spin waves (magnons) by various propagating magnetic perturbations, fast-enough moving magnetic field stimuli have not been available so far. Here, we experimentally realize the Cherenkov radiation of spin waves in a Co-Fe magnonic conduit by fast-moving (>1 km/s) magnetic flux quanta (Abrikosov vortices) in an adjacent Nb-C superconducting strip. The radiation is evidenced by the microwave detection of spin waves propagating a distance of 2 micrometers from the superconductor and it is accompanied by a magnon Shapiro step in its current-voltage curve. The spin-wave excitation is unidirectional and monochromatic, with sub-40 nm wavelengths determined by the period of the vortex lattice. The phase-locking of the vortex lattice with the excited spin wave limits the vortex velocity and reduces the dissipation in the superconductor.

cond-mat.other↗

arXiv2021

Spin-wave eigenmodes in direct-write 3D nanovolcanoes

Extending nanostructures into the third dimension has become a major research avenue in modern magnetism, superconductivity and spintronics, because of geometry-, curvature- and topology-induced phenomena. Here, we introduce Co-Fe nanovolcanoes-nanodisks overlaid by nanorings-as purpose-engineered 3D architectures for nanomagnonics, fabricated by focused electron beam induced deposition. We use both perpendicular spin-wave resonance measurements and micromagnetic simulations to demonstrate that the rings encircling the volcano craters harbor the highest-frequency eigenmodes, while the lower-frequency eigenmodes are concentrated within the volcano crater, due to the non-uniformity of the internal magnetic field. By varying the crater diameter, we demonstrate the deliberate tuning of higher-frequency eigenmodes without affecting the lowest-frequency mode. Thereby, the extension of 2D nanodisks into the third dimension allows one to engineer their lowest eigenfrequency by using 3D nanovolcanoes with 30% smaller footprints. The presented nanovolcanoes can be viewed as multi-mode microwave resonators and 3D building blocks for nanomagnonics.

cond-mat.mes-hall↗

arXiv2020

Engineered magnetization and exchange stiffness in direct-write Co-Fe nanoelements

Media with engineered magnetization are essential building blocks in superconductivity, magnetism and magnon spintronics. However, the established thin-film and lithographic techniques insufficiently suit the realization of planar components with on-demand-tailored magnetization in the lateral dimension. Here, we demonstrate the engineering of the magnetic properties of CoFe-based nanodisks fabricated by the mask-less technique of focused electron beam induced deposition (FEBID). The material composition in the nanodisks is tuned \emph{in-situ} via the e-beam waiting time in the FEBID process and their post-growth irradiation with Ga ions. The magnetization $M_s$ and exchange stiffness $A$ of the disks are deduced from perpendicular ferromagnetic resonance measurements. The achieved $M_s$ variation in the broad range from $720$ emu/cm$^3$ to $1430$ emu/cm$^3$ continuously bridges the gap between the $M_s$ values of such widely used magnonic materials as permalloy and CoFeB. The presented approach paves a way towards nanoscale 2D and 3D systems with controllable and space-varied magnetic properties.

cond-mat.mes-hall↗

arXiv2020

Spin-wave spectroscopy of individual ferromagnetic nanodisks

The increasing demand for ultrahigh data storage densities requires development of 3D magnetic nanostructures. In this regard, focused electron beam induced deposition (FEBID) is a technique of choice for direct-writing of various complex nano-architectures. However, intrinsic properties of nanomagnets are often poorly known and can hardly be assessed by local optical probe techniques. Here, we demonstrate spatially resolved spin-wave spectroscopy of individual circular magnetic elements with radii down to 100 nm. The key component of the setup is a microwave antenna whose microsized central part is placed over a movable substrate with well-separated CoFe-FEBID nanodisks. The circular symmetry of the disks gives rise to standing spin-wave resonances and allows for the deduction of the saturation magnetization and the exchange stiffness of the material using an analytical theory. The presented approach is especially valuable for the characterization of direct-write elements opening new horizons for 3D nanomagnetism and magnonics.

cond-mat.mes-hall↗

arXiv2020

Moving flux quanta cool superconductors by a microwave breath

Almost any use of a superconductor implies a nonequilibrium state. Remarkably, the non-equilibrium states induced by a microwave stimulus and the dynamics of magnetic flux quanta (Abrikosov vortices) can give rise to strikingly contrary effects: A sufficiently high-power electromagnetic field of GHz frequency can stimulate superconductivity, whereas fast vortex motion can trigger an instability abruptly quenching the superconducting state. Here, we advance or delay such dynamical quenching of the vortex state in Nb thin films by tuning the power and frequency of the microwave ac stimulus added to a dc bias current. The experimental findings are supported by time-dependent Ginzburg-Landau simulations and they can be explained qualitatively based on a model of "breathing mobile hot spots", implying a competition of heating and cooling of quasiparticles along the trajectories of moving fluxons whose core sizes vary in time. In addition, we demonstrate universality of the stimulation effect on the thermodynamic and transport properties of type II superconductors.

cond-mat.supr-con↗

arXiv2020

Ultra-fast vortex motion in dirty Nb-C superconductor with a close-to-perfect edge barrier

The ultra-fast dynamics of superconducting vortices harbors rich physics generic to nonequilibrium collective systems. The phenomenon of flux-flow instability (FFI), however, prevents its exploration and sets practical limits for the use of vortices in various applications. To suppress the FFI, a superconductor should exhibit a rarely achieved combination of properties: weak volume pinning, close-to-depairing critical current, and fast heat removal from heated electrons. Here, we demonstrate experimentally ultra-fast vortex motion at velocities of 10-15 km/s in a directly written Nb-C superconductor in which a close-to-perfect edge barrier orders the vortex motion at large current values. The spatial evolution of the FFI is described using the edge-controlled FFI model, implying a chain of FFI nucleation points along the sample edge and their development into self-organized Josephson-like junctions (vortex rivers). In addition, our results offer insights into the applicability of widely used FFI models and suggest Nb-C to be a good candidate material for fast single-photon detectors.

cond-mat.supr-con↗

arXiv2020

Upper frequency limits for vortex guiding and ratchet effects

Guided and rectified motion of magnetic flux quanta are important effects governing the magneto-resistive response of nanostructured superconductors. While at low ac frequencies these effects are rather well understood, their manifestation at higher ac frequencies remains poorly investigated. Here, we explore the upper frequency limits for guided and rectified net motion of superconducting vortices in epitaxial Nb films decorated with ferromagnetic nanostripes. By combining broadband electrical spectroscopy with resistance measurements we reveal that the rectified voltage vanishes at a geometrically defined frequency of about 700 MHz. By contrast, vortex guiding-related low-ac-loss response persists up to about 2 GHz. This value corresponds to the depinning frequency $f_\mathrm{d}^\mathrm{s}$ associated with the washboard pinning potential induced by the nanostripes and exhibiting peaks for the commensurate vortex lattice configurations. Applying a sum of dc and microwave ac currents at an angle $α$ with respect to the nanostripes, the angle dependence of $f_\mathrm{d}^\mathrm{s}(α)$ has been found to correlate with the angle dependence of the depinning current. In all, our findings suggest that superconductors with higher $f_\mathrm{d}^\mathrm{s}$ should be favored for an efficient vortex manipulation in the GHz ac frequency range.

cond-mat.supr-con↗

arXiv2019

Spin-wave phase inverter upon a single nanodefect

Local modification of magnetic properties of nanoelements is a key to design future-generation magnonic devices, in which information is carried and processed via spin waves. One of the biggest challenges here is to fabricate simple and miniature phase-controlling elements with broad tunability. Here, we successfully realize such spin-wave phase shifter upon a single nanogroove milled by focused ion beam in a Co-Fe microsized magnonic waveguide. By varying the groove depth and the in-plane bias magnetic field we continuously tune the spin-wave phase and experimentally evidence a complete phase inversion. The microscopic mechanism of the phase shift is based on the combined action of the nanogroove as a geometrical defect and the lower spin-wave group velocity in the waveguide under the groove where the magnetization is reduced due to the incorporation of Ga ions during the ion-beam milling. The proposed phase shifter can easily be on-chip integrated with spin-wave logic gates and other magnonic devices. Our findings are crucial for designing nano-magnonic circuits and for the development of spin-wave nano-optics.

cond-mat.mes-hall↗

arXiv2019

Supersonic dynamics of guided magnetic flux quanta

The dynamics of Abrikosov vortices in superconductors is usually limited to vortex velocities $v\simeq1$ km/s above which samples abruptly transit into the normal state. In the Larkin-Ovchinnikov framework, near the critical temperature this is because of a flux-flow instability triggered by the reduction of the viscous drag coefficient due to the quasiparticles leaving the vortex cores. While the existing instability theories rely upon a uniform spatial distribution of vortex velocities, the measured (mean) value of $v$ is always smaller than the maximal possible one, since the distribution of $v$ never reaches the $δ$-functional shape. Here, by guiding magnetic flux quanta at a tilt angle of $15^\circ$ with respect to a Co nanostripe array, we speed up vortices to supersonic velocities. These exceed $v$ in the reference as-grown Nb films by almost an order of magnitude and are only a factor of two smaller than the maximal vortex velocities observed in superconductors so far. We argue that such high $v$ values appear in consequence of a collective dynamic ordering when all vortices move in the channels with the same pinning strength and exhibit a very narrow distribution of $v$. Our findings render the well-known vortex guiding effect to open prospects for investigations of ultrafast vortex dynamics.

cond-mat.supr-con↗

arXiv2019

Zero-bias Shapiro steps in asymmetric pinning nanolandscapes

The coherent nonlinear dynamics of Abrikosov vortices in asymmetric pinning nanolandscapes is studied by theoretical modeling and combined microwave and dc electrical resistance measurements. The problem is considered on the basis of a single-vortex Langevin equation within the framework of a stochastic model of anisotropic pinning. When the distance over which Abrikosov vortices are driven during one half ac cycle coincides with one or a multiple of the nanostructure period, Shapiro steps appear in the current-voltage curves (CVCs) as a general feature of systems whose evolution in time can be described in terms of a particle moving in a periodic potential under combined dc and ac stimuli. While a dc voltage appears in response to the ac drive, the addition of a dc bias allows one to diminish the rectified voltage and eventually to change its sign when the extrinsic dc bias-induced asymmetry of the pinning potential starts to dominate the intrinsic one. This rectified negative voltage in the CVCs becomes apparent as \emph{zero-bias} Shapiro steps, which are theoretically predicted and experimentally observed for the first time.

cond-mat.supr-con↗

arXiv2019

Magnon-Fluxon interaction in a ferromagnet/superconductor heterostructure

Ferromagnetism and superconductivity are most fundamental phenomena in condensed matter physics. Entailing opposite spin orders, they share an important conceptual similarity: Disturbances in magnetic ordering in magnetic materials can propagate in the form of spin waves (magnons) while magnetic fields penetrate superconductors as a lattice of magnetic flux quanta (fluxons). Despite a rich choice of wave and quantum phenomena predicted, magnon-fluxon coupling has not been observed experimentally so far. Here, we clearly evidence the interaction of spin waves with a flux lattice in ferromagnet/superconductor Py/Nb bilayers. We demonstrate that, in this system, the magnon frequency spectrum exhibits a Bloch-like band structure which can be tuned by the biasing magnetic field. Furthermore, we observe Doppler shifts in the frequency spectra of spin waves scattered on a flux lattice moving under the action of a transport current in the superconductor.

cond-mat.supr-con↗

arXiv2018

Reduction of microwave loss by mobile fluxons in grooved Nb films

In the mixed state of type II superconductors penetrated by an external magnetic field in the form of a lattice of Abrikosov vortices the dc resistance is known to increase with increasing velocity of the vortex lattice. Accordingly, vortex pinning sites impeding the vortex motion are widely used to preserve the low-dissipative response of the system. Here, while subjecting superconducting Nb films with nanogrooves to a combination of dc and ac current stimuli and tuning the number of mobile and pinned vortices by varying the magnetic field around the so-called matching values, we observe a completely opposite effect. Namely, the vortex-related microwave excess loss for mobile vortices becomes smaller than for pinned vortices in a certain range of power levels at ac current frequencies above 100\,MHz. While a theoretical description of the observed effect is yet to be elaborated we interpret our findings in terms of a competition of the effective cooling of the system by the quasiparticles leaving the vortex cores with the conventional Joule heating caused by the current flow.

cond-mat.supr-con↗

arXiv2018

Microwave emission from superconducting vortices in Mo/Si superlattices

Most of superconductors in a magnetic field are penetrated by a lattice of quantized flux vortices. In the presence of a transport current causing the vortices to cross sample edges, emission of electromagnetic waves is expected due to the continuity of tangential components of the fields at the surface. Yet, such a radiation has not been observed so far due to low radiated power levels and lacking coherence in the vortex motion. Here, we report emission of electromagnetic waves from vortices crossing the layers of a superconductor/insulator Mo/Si superlattice. The emission spectra consist of narrow harmonically related peaks which can be finely tuned in the GHz range by the dc bias current and, coarsely, by the in-plane magnetic field value. Our findings show that superconductor/insulator superlattices can act as dc-tunable microwave generators bridging the frequency gap between conventional radiofrequency oscillators and (sub-)terahertz generators relying upon the Josephson effect.

cond-mat.supr-con↗

arXiv2016

dc and ac magnetic properties of thin-walled Nb cylinders with and without a row of antidots

dc and ac magnetic properties of two thin-walled superconducting Nb cylinders with a rectangular cross-section are reported. Magnetization curves and the ac response were studied on as-prepared and patterned samples in magnetic fields parallel to the cylinder axis. A row of micron-sized antidots (holes) was made in the film along the cylinder axis. Avalanche-like jumps of the magnetization are observed for both samples at low temperatures for magnetic fields not only above $H_{c1}$, but in fields lower than $H_{c1}$ in the vortex-free region. The positions of the jumps are not reproducible and they change from one experiment to another, resembling vortex lattice instabilities usually observed for magnetic fields larger than $H_{c1}$. At temperatures above $0.66T_c$ and $0.78T_c$ the magnetization curves become smooth for the patterned and the as-prepared samples, respectively. The magnetization curve of a reference planar Nb film in the parallel field geometry does not exhibit jumps in the entire range of accessible temperatures. The ac response was measured in constant and swept dc magnetic field modes. Experiment shows that ac losses at low magnetic fields in a swept field mode are smaller for the patterned sample. For both samples the shapes of the field dependences of losses and the amplitude of the third harmonic are the same in constant and swept field near $H_{c3}$. This similarity does not exist at low fields in a swept mode.

cond-mat.supr-con↗

arXiv2016

Fabrication of FeSi and Fe3Si compounds by electron beam induced mixing of [Fe/Si]2 and [Fe3/Si]2 multilayers grown by focused electron beam induced deposition

Fe-Si binary compounds have been fabricated by focused electron beam induced deposition by the alternating use of iron pentacarbonyl, Fe(CO)5, and neopentasilane, Si5H12 as precursor gases. The fabrication procedure consisted in preparing multilayer structures which were treated by low-energy electron irradiation and annealing to induce atomic species intermixing. In this way we are able to fabricate FeSi and Fe3Si binary compounds from [Fe=Si]2 and [Fe3=Si]2 multilayers, as shown by transmission electron microscopy investigations. This fabrication procedure is useful to obtain nanostructured binary alloys from precursors which compete for adsorption sites during growth and, therefore, cannot be used simultaneously.

cond-mat.mes-hall↗

arXiv2011

Magnetotransport properties of iron microwires fabricated by focused electron beam induced autocatalytic growth

We have prepared iron microwires in a combination of focused electron beam induced deposition (FEBID) and autocatalytic growth from the iron pentacarbonyl, Fe(CO)5, precursor gas under UHV conditions. The electrical transport properties of the microwires were investigated and it was found that the temperature dependence of the longitudinal resistivity (rhoxx) shows a typical metallic behaviour with a room temperature value of about 88 microΩ cm. In order to investigate the magnetotransport properties we have measured the isothermal Hall-resistivities in the range between 4.2 K and 260 K. From these measurements positive values for the ordinary and the anomalous Hall coefficients were derived. The relation between anomalous Hall resistivity (rhoAN) and longitudinal resistivity is quadratic, rhoAN rho^2 xx, revealing an intrinsic origin of the anomalous Hall effect. Finally, at low temperature in the transversal geometry a negative magnetoresistance of about 0.2 % was measured.

cond-mat.mtrl-sci↗

arXiv2011

Tuning the electrical conductivity of Pt-containing granular metals by postgrowth electron irradiation

We have fabricated Pt-containing granular metals by focused electron beam induced deposition from the $(CH_3)_3CH_3C_5H_4Pt$ precursor gas. The granular metals are made of platinum nanocrystallites embedded in a carbonaceous matrix. We have exposed the as-grown nanocomposites to low energy electron beam irradiation and we have measured the electrical conductivity as a function of the irradiation dose. Postgrowth electron beam irradiation transforms the matrix microstructure and thus the strength of the tunneling coupling between Pt nanocrystallites. For as-grown samples (weak tunnel coupling regime) we find that the temperature dependence of the electrical conductivity follows the stretched exponential behavior characteristic of the correlated variable-range hopping transport regime. For briefly irradiated samples (strong tunnel coupling regime) the electrical conductivity is tuned across the metal-insulator transition. For long-time irradiated samples the electrical conductivity behaves like that of a metal. In order to further analyze changes of the microstructure as a function of the electron irradiation dose we have carried out transmission electron microscope (TEM), micro-Raman and atomic force microscopy (AFM) investigations. TEM pictures reveal that the crystallites' size of long-time irradiated samples is larger than that of as-grown samples. Furthermore we do not have evidence of microstructural changes in briefly irradiated samples. By means of micro-Raman we find that by increasing the irradiation dose the matrix changes following a graphitization trajectory between amorphous carbon and nanocrystalline graphite. Finally, by means of AFM measurements we observe a reduction of the volume of the samples with increasing irradiation time which we attribute to the removal of carbon molecules.

cond-mat.mtrl-sci↗

arXiv2009

Transient electrical conductivity of W-based electron beam induced deposits during growth, irradiation and exposure to air

W-based granular metals have been prepared by electron beam induced deposition from the tungsten-hexacarbonyl W(CO)6 precursor. In situ electrical conductivity measurements have been performed to monitor the growth process and to investigate the behavior of the deposit under electron beam post irradiation and by exposure to air. During the first part of the growth process, the electrical conductivity grows non-linearly, independent of the electron beam parameters. This behavior is interpreted as the result of the increase of the W-particles diameter. Once the growth process is terminated, the electrical conductivity decreases with the logarithm of time, sigma ln(t). Temperature-dependent conductivity measurements of the deposits reveal that the electrical transport takes place by means of electron tunneling either between W-metal grains or between grains and trap sites in the matrix. After venting the electron microscope the electrical conductivity of the deposits shows a degradation behavior, which depends on the composition. Electron post-irradiation increases the electrical conductivity of the deposits.

cond-mat.mtrl-sci↗