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R. Schwengner

Publications and source records attributed to R. Schwengner.

At least 37 records · Page 2Linked to original sources

Completing the nuclear reaction puzzle of the nucleosynthesis of 92Mo

One of the greatest questions for modern physics to address is how elements heavier than iron are created in extreme, astrophysical environments. A particularly challenging part of that question is the creation of the so-called p-nuclei, which are believed to be mainly produced in some types of supernovae. The lack of needed nuclear data presents an obstacle in nailing down the precise site and astrophysical conditions. In this work, we present for the first time measurements on the nuclear level density and average strength function of $^{92}$Mo. State-of-the-art p-process calculations systematically underestimate the observed solar abundance of this isotope. Our data provide stringent constraints on the $^{91}$Nb$(p,γ)^{92}$Mo reaction rate, which is the last unmeasured reaction in the nucleosynthesis puzzle of $^{92}$Mo. Based on our results, we conclude that the $^{92}$Mo abundance anomaly is not due to the nuclear physics input to astrophysical model calculations.

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Experimentally constrained ($p,γ$)$^{89}$Y and ($n,γ$)$^{89}$Y reaction rates relevant to the $p$-process nucleosynthesis

The nuclear level density and the $γ$-ray strength function have been extracted for $^{89}$Y, using the Oslo Method on $^{89}$Y($p,p' γ$)$^{89}$Y coincidence data. The $γ$-ray strength function displays a low-energy enhancement consistent with previous observations in this mass region ($^{93-98}$Mo). Shell-model calculations give support that the observed enhancement is due to strong, low-energy $M1$ transitions at high excitation energies. The data were further used as input for calculations of the $^{88}$Sr($p,γ$)$^{89}$Y and $^{88}$Y($n,γ$)$^{89}$Y cross sections with the TALYS reaction code. Comparison with cross-section data, where available, as well as with values from the BRUSLIB library, shows a satisfying agreement.

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Magnetic dipole excitations of $^{50}$Cr

The low-lying $M1$-strength of the open-shell nucleus $^{50}$Cr has been studied with the method of nuclear resonance fluorescence up to 9.7 MeV, using bremsstrahlung at the superconducting Darmstadt linear electron accelerator S-DALINAC and Compton backscattered photons at the High Intensity $γ$-ray Source (HI$γ$S) facility between 6 and 9.7 MeV of the initial photon energy. Fifteen $1^{+}$ states have been observed between 3.6 and 9.7 MeV. Following our analysis, the lowest $1^{+}$ state at 3.6 MeV can be considered as an isovector orbital mode with some spin admixture. The obtained results generally match the estimations and trends typical for the scissors-like mode. Detailed calculations within the Skyrme Quasiparticle Random-Phase-Approximation method and the Large-Scale Shell Model justify our conclusions. The calculated distributions of the orbital current for the lowest $1^{+}$-state suggest the schematic view of Lipparini and Stringari (isovector rotation-like oscillations inside the rigid surface) rather than the scissors-like picture of Lo Iudice and Palumbo. The spin M1 resonance is shown to be mainly generated by spin-flip transitions between the orbitals of the $fp$-shell.

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Determination of gamma-ray widths in $^{15}$N using nuclear resonance fluorescence

The stable nucleus $^{15}$N is the mirror of $^{15}$O, the bottleneck in the hydrogen burning CNO cycle. Most of the $^{15}$N level widths below the proton emission threshold are known from just one nuclear resonance fluorescence (NRF) measurement, with limited precision in some cases. A recent experiment with the AGATA demonstrator array determined level lifetimes using the Doppler Shift Attenuation Method (DSAM) in $^{15}$O. As a reference and for testing the method, level lifetimes in $^{15}$N have also been determined in the same experiment. The latest compilation of $^{15}$N level properties dates back to 1991. The limited precision in some cases in the compilation calls for a new measurement in order to enable a comparison to the AGATA demonstrator data. The widths of several $^{15}$N levels have been studied with the NRF method. The solid nitrogen compounds enriched in $^{15}$N have been irradiated with bremsstrahlung. The $γ$-rays following the deexcitation of the excited nuclear levels were detected with four HPGe detectors. Integrated photon-scattering cross sections of ten levels below the proton emission threshold have been measured. Partial gamma-ray widths of ground-state transitions were deduced and compared to the literature. The photon scattering cross sections of two levels above the proton emission threshold, but still below other particle emission energies have also been measured, and proton resonance strengths and proton widths were deduced. Gamma and proton widths consistent with the literature values were obtained, but with greatly improved precision.

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Low-energy enhancement in the γ-ray strength functions of $^{73,74}$Ge

The $γ$-ray strength functions and level densities of $^{73,74}$Ge have been extracted up to the neutron separation energy S$_n$ from particle-$γ$ coincidence data using the Oslo method. Moreover, the $γ$-ray strength function of $^{74}$Ge above S$_n$ has been determined from photo-neutron measurements, hence these two experiments cover the range of E$_γ\approx$ 1-13 MeV for $^{74}$Ge. The obtained data show that both $^{73,74}$Ge display an increase in strength at low $γ$ energies. The experimental $γ$-ray strength functions are compared with $M1$ strength functions deduced from average $B(M1)$ values calculated within the shell model for a large number of transitions. The observed low-energy enhancements in $^{73,74}$Ge are adopted in the calculations of the $^{72,73}$Ge(n,$γ$) cross sections, where there are no direct experimental data. Calculated reaction rates for more neutron-rich germanium isotopes are shown to be strongly dependent on the presence of the low-energy enhancement.

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Low-energy magnetic radiation: deviations from GOE

A pronounced spike at low energy in the strength function for magnetic radiation (LEMAR) is found by means of Shell Model calculations, which explains the experimentally observed enhancement of the dipole strength. LEMAR originates from statistical low-energy M1-transitions between many excited complex states. Re-coupling of the proton and neutron high-j orbitals generates the strong magnetic radiation. LEMAR is closely related to Magnetic Rotation. LEMAR is predicted for nuclides participating in the r-process of element synthesis and is expected to change the reaction rates. An exponential decrease of the strength function and a power law for the size distribution of the $B(M1)$ values are found, which strongly deviate from the ones of the GOE of random matrices, which is commonly used to represent complex compound states.

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Nuclear deformation and neutron excess as competing effects for pygmy dipole strength

The electromagnetic dipole strength below the neutron-separation energy has been studied for the xenon isotopes with mass numbers A = 124, 128, 132, and 134 in nuclear resonance fluorescence experiments using the ELBE bremsstrahlung facility at Helmholtz-Zentrum Dresden-Rossendorf and the HIgS facility at Triangle Universities Nuclear Laboratory Durham. The systematic study gained new information about the influence of the neutron excess as well as of nuclear deformation on the strength in the region of the pygmy dipole resonance. The results are compared with those obtained for the chain of molybdenum isotopes and with predictions of a random-phase approximation in a deformed basis. It turned out that the effect of nuclear deformation plays a minor role compared with the one caused by neutron excess. A global parametrization of the strength in terms of neutron and proton numbers allowed us to derive a formula capable of predicting the summed E1 strengths in the pygmy region for a wide mass range of nuclides.

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Low-energy enhancement of magnetic dipole radiation

Magnetic dipole strength functions have been deduced from averages of a large number of $M1$ transition strengths calculated within the shell model for the nuclides $^{90}$Zr, $^{94}$Mo, $^{95}$Mo, and $^{96}$Mo. An enhancement of $M1$ strength toward low transition energy has been found for all nuclides considered. Large $M1$ strengths appear for transitions between close-lying states with configurations including proton as well as neutron high-$j$ orbits that re-couple their spins and add up their magnetic moments coherently. The $M1$ strength function deduced from the calculated $M1$ transition strengths is compatible with the low-energy enhancement found in ($^3$He,$^3$He') and $(d,p)$ experiments. The present work presents for the first time an explanation of the experimental findings.

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Cross-Section Measurements of the 86Kr(g,n) Reaction to Probe the s-Process Branching at 85Kr

We have carried out photodisintegration cross-section measurements on 86Kr using monoenergetic photon beams ranging from the neutron separation energy, S_n = 9.86 MeV, to 13 MeV. We combine our experimental 86Kr(g,n)85Kr cross section with results from our recent 86Kr(g,g') measurement below the neutron separation energy to obtain the complete nuclear dipole response of 86Kr. The new experimental information is used to predict the neutron capture cross section of 85Kr, an important branching point nucleus on the abundance flow path during s-process nucleosynthesis. Our new and more precise 85Kr(n,g)86Kr cross section allows to produce more precise predictions of the 86Kr abundance from s-process models. In particular, we find that the models of the s-process in asymptotic giant branch stars of mass < 1.5 Msun, where the 13C neutron source burns convectively rather than radiatively, represent a possible solution for the highest 86Kr/82Kr ratios observed in meteoritic stardust SiC grains.

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The first candidate for chiral nuclei in the $A\sim80$ mass region: $^{80}$Br

Excited states of $^{80}$Br have been investigated via the $^{76}$Ge($^{11}$B, $α$3n) and $^{76}$Ge($^{7}$Li, 3n) reactions and a new $ΔI$ = 1 band has been identified which resides $\sim$ 400 keV above the yrast band. Based on the experimental results and their comparison with the triaxial particle rotor model calculated ones, a chiral character of the two bands within the $πg_{9/2}\otimes νg_{9/2}$ configuration is proposed, which provides the first evidence for chirality in the $A\sim80$ region.

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Instantaneous Shape Sampling - a model for the $γ$-absorption cross section of transitional nuclei

The influence of the quadrupole shape fluctuations on the dipole vibrations in transitional nuclei is investigated in the framework of the Instantaneous Shape Sampling Model, which combines the Interacting Boson Model for the slow collective quadrupole motion with the Random Phase Approximation for the rapid dipole vibrations. Coupling to the complex background configurations is taken into account by folding the results with a Lorentzian with an energy dependent width. The low-energy energy portion of the $γ$- absorption cross section, which is important for photo-nuclear processes, is studied for the isotopic series of Kr, Xe, Ba, and Sm. The experimental cross sections are well reproduced. The low-energy cross section is determined by the Landau fragmentation of the dipole strength and its redistribution caused by the shape fluctuations. Collisional damping only wipes out fluctuations of the absorption cross section, generating the smooth energy dependence observed in experiment. In the case of semi-magic nuclei, shallow pygmy resonances are found in agreement with experiment.

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Experimental study of the electric dipole strength in the even Mo nuclei and its deformation dependence

Two methods based on bremsstrahlung were applied to the stable even Mo isotopes for the experimental determination of the photon strength function covering the high excitation energy range above 4 MeV with its increasing level density. Photon scattering was used up to the neutron separation energies Sn and data up to the maximum of the isovector giant resonance(GDR) were obtained by photo-activation. After a proper correction for multi-step processes the observed quasi-continuous spectra of scattered photons show a remarkably good match to the photon strengths derived from nuclear photo effect data obtained previously by neutron detection and corrected in absolute scale using the new activation results. The combined data form an excellent basis to derive a shape dependence of the E1 strength in the even Mo isotopes with increasing deviation from the N = 50 neutron shell, i.e. with the impact of quadrupole deformation and triaxiality. The wide energy coverage of the data allows for a stringent assessment of the dipole sum-rule, and a test of a novel parameterization developed previously which is based upon. This parameterization for the electric dipole strength function in nuclei with A>80 deviates significantly from prescriptions generally used previously. In astrophysical network calculations it may help to quantify the role the p-process plays in the cosmic nucleosynthesis. It also has impact on the accurate analysis of neutron capture data of importance for future nuclear energy systems and waste transmutation.

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Solving the stellar 62Ni problem with AMS

An accurate knowledge of the neutron capture cross sections of 62,63Ni is crucial since both isotopes take key positions which affect the whole reaction flow in the weak s process up to A=90. No experimental value for the 63Ni(n,gamma) cross section exists so far, and until recently the experimental values for 62Ni(n,gamma) at stellar temperatures (kT=30 keV) ranged between 12 and 37 mb. This latter discrepancy could now be solved by two activations with following AMS using the GAMS setup at the Munich tandem accelerator which are also in perfect agreement with a recent time-of-flight measurement. The resulting (preliminary) Maxwellian cross section at kT=30 keV was determined to be 30keV = 23.4 +/- 4.6 mb. Additionally, we have measured the 64Ni(gamma,n)63Ni cross section close to threshold. Photoactivations at 13.5 MeV, 11.4 MeV and 10.3 MeV were carried out with the ELBE accelerator at Forschungszentrum Dresden-Rossendorf. A first AMS measurement of the sample activated at 13.5 MeV revealed a cross section smaller by more than a factor of 2 compared to NON-SMOKER predictions.

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Photon data shed new light upon the GDR spreading width in heavy nuclei

A global study of the electric dipole strength in and below the isovector giant dipole resonance (GDR) is presented for mass numbers A>80. It relies on the recently established remarkably good match between data for the nuclear photo effect to novel photon scattering data covering the region below the neutron emission threshold as well as by average resonance neutron capture (ARC). From the wide energy coverage of these data the correlation of the GDR spreading width with energy can be studied with remarkable accuracy. A clear sensitivity to details of the nuclear shape, i.e. the beta- and gamma-deformations, is demonstrated. Based hereon a new parameterization of the energy dependence of the nuclear electric-dipole strength is proposed which - with only two new parameters - allows to describe the dipole strength in all heavy nuclei with A>80. Although it differs significantly from previous parameterizations it holds for spherical, transitional, triaxial and well deformed nuclei. The GDR spreading width depends in a regular way on the respective resonance energy, but it is independent of the photon energy.

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Photoactivation experiment on 197Au and its implications for the dipole strength in heavy nuclei

The 197Au(gamma,n) reaction is used as an activation standard for photodisintegration studies on astrophysically relevant nuclei. At the bremsstrahlung facility of the superconducting electron accelerator ELBE (Electron Linear accelerator of high Brilliance and low Emittance) of Forschungszentrum Dresden-Rossendorf, photoactivation measurements on 197Au have been performed with bremsstrahlung endpoint energies from 8.0 to 15.5 MeV. The measured activation yield is compared with previous experiments as well as with calculations using Hauser-Feshbach statistical models. It is shown that the experimental data are best described by a two-Lorentzian parametrization with taking the axial deformation of 197Au into account. The experimental 197Au(gamma,n) reaction yield measured at ELBE via the photoactivation method is found to be consistent with previous experimental data using photon scattering or neutron detection methods.

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Pygmy dipole strength in 90Zr

The dipole response of the N=50 nucleus 90Zr was studied in photon-scattering experiments at the electron linear accelerator ELBE with bremsstrahlung produced at kinetic electron energies of 7.9, 9.0, and 13.2 MeV. We identified 189 levels up to an excitation energy of 12.9 MeV. Statistical methods were applied to estimate intensities of inelastic transitions and to correct the intensities of the ground-state transitions for their branching ratios. In this way we derived the photoabsorption cross section up to the neutron-separation energy. This cross section matches well the photoabsorption cross section obtained from (gamma,n) data and thus provides information about the extension of the dipole-strength distribution toward energies below the neutron-separation energy. An enhancement of E1 strength has been found in the range of 6 MeV to 11 MeV. Calculations within the framework of the quasiparticle-phonon model ascribe this strength to a vibration of the excessive neutrons against the N = Z neutron-proton core, giving rise to a pygmy dipole resonance.

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Electromagnetic Dipole Strength in Transitional Nuclei

Electromagnetic dipole absorption cross-sections of transitional nuclei with large-amplitude shape fluctuations are calculated in a microscopic way by introducing the concept of Instantaneous Shape Sampling. The concept bases on the slow shape dynamics as compared to the fast dipole vibrations. The elctromagnetic dipole strength is calculated by means of RPA for the instantaneous shapes, the probability of which is obtained by means of IBA. Very good agreement with the experimental absorption cross sections near the nucleon emission threshold is obtained.

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Photodisintegration studies on p-nuclei: The case of Mo and Sm isotopes

In explosive stellar environments like supernovae, the temperatures are high enough for the production of heavy neutron-deficient nuclei, the socalled p-nuclei. Up to now, the knowledge of the reaction rates of p-nuclei is based on theoretical parameterizations using statistical model calculations. At the bremsstrahlung facility of the superconducting electron accelerator ELBE of FZ Dresden-Rossendorf, we aim to measure the photodisintegration rates of heavy nuclei experimentally. Photoactivation measurements on the astrophysically relevant p-nuclei 92Mo and 144Sm have been performed with bremsstrahlung end-point energies from 10.0 to 16.5 MeV. First experiments on the short-lived decays following the reaction 144Sm(gamma,n) are carried out using a pneumatic delivery system for rapid transport of activated samples. The activation yields are compared with calculations using cross sections from recent Hauser-Feshbach models.

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