arXiv subjects

R. V. F. Janssens

Publications and source records attributed to R. V. F. Janssens.

At least 19 recordsLinked to original sources

arXiv2026

Photonuclear Cross Sections for the $^{197}$Au($γ$,pn)$^{195m}$Pt Reaction Near Threshold

Platinum radioisotopes are of growing interest for targeted cancer therapy and diagnostic imaging because their decay delivers highly localized radiation doses in tissue, herewith enabling precise DNA damage through Auger-electron emission. Developing production technologies that provide platinum isotopes with high specific activity is therefore essential, and photonuclear reactions on stable nuclei offer a viable accelerator-based route when supported by reliable cross-section data. We report photonuclear cross-section measurements for the $^{197}$Au($γ$,pn)$^{195m}$Pt reaction at incident $γ$-ray energies of 27, 29, and 31 MeV using the activation method. The measurements were performed by irradiating a stack of concentric-ring gold targets with a quasi-monoenergetic $γ$-ray beam provided by the High Intensity Gamma-ray Source (HI$γ$S). The induced $^{195m}$Pt activity was quantified using off-line $γ$-ray spectroscopy. These data provide the first experimental constraints on the $^{197}$Au($γ$,pn)$^{195m}$Pt cross section in the near-threshold region. The measured excitation function is compared with PHITS and TALYS calculations and indicates that the reaction becomes measurable only near 30 MeV, with substantially higher bremsstrahlung end-point energies required for practically meaningful production.

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arXiv2026

Core Breaking at Low Spin in $^{68}$Zn from Nuclear Resonance Fluorescence

Low-spin excited states in $^{68}$Zn have been studied at the High Intensity Gamma-Ray Source (HI$γ$S) from the ground state up to the particle emission threshold using the nuclear resonance fluorescence technique (NRF) and the newly developed Clover Array. Low-spin levels were excited by linearly-polarized, $2.90 - 9.79$ MeV photon beams. Spin-parity quantum numbers as well as associated $M1$ and $E1$ decay strengths were determined for a large fraction of the 158 states observed. In addition, long-duration coincidence measurements at 9.46 and 9.79 MeV enabled the investigation of the level scheme near the ground state. The results have been interpreted with shell-model calculations using two different model spaces and several effective interactions often used to describe nuclei in this mass region. While the structure near the ground state can be understood in terms of excitations involving solely valence nucleons, core breaking is required to account for the evolution of the total $M1$ strength at excitation energies above $\sim5$ MeV.

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arXiv2026

Evolution of chirality from transverse wobbling in $^{135}$Pr

Chirality is a distinct signature that characterizes triaxial shapes in nuclei. We report the first observation of chirality in the nucleus $^{135}$Pr using a high-statistics Gammasphere experiment with the $^{123}$Sb($^{16}$O,4n)$^{135}$Pr reaction. Two chiral-partner bands with the configuration $π(1h_{11/2})^1\otimesν(1h_{11/2})^{-2}$ have been identified in this nucleus. Angular distribution analyses of the $ΔI = 1$ transitions connecting the two bands reveal a dominant dipole character, and quasiparticle triaxial rotor model calculations show good agreement with the data. Since the simultaneous observation of chirality and transverse wobbling in $^{135}$Pr relies critically on these angular distribution results, we also address and refute the experimental and theoretical criticisms raised in a recent work by Lv et al., presenting additional evidence that further strengthens our interpretation. This marks the first observation of both hallmarks of triaxiality-chirality and wobbling-in the same nucleus.

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arXiv2025

Extraction of ground-state nuclear deformations from ultra-relativistic heavy-ion collisions: Nuclear structure physics context

The collective-flow-assisted nuclear shape-imaging method in ultra-relativistic heavy-ion collisions has recently been used to characterize nuclear collective states. In this paper, we assess the foundations of the shape-imaging technique employed in these studies. We argue that some current UHIC nuclear imaging techniques neglect fundamental aspects of spontaneous symmetry-breaking and symmetry-restoration in colliding ions and incorrectly infer one-body multipole moments from studies of nucleonic correlations. Therefore, the impact of this approach on nuclear structure research has been overstated. Conversely, efforts to incorporate existing knowledge on nuclear shapes into analysis pipelines can be beneficial for benchmarking tools and calibrating models used to extract information from ultra-relativistic heavy-ion experiments.

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arXiv2025

Triaxiality and shape dynamics in $^{70}$Ge

The electromagnetic properties of low-lying states in $^{70}$Ge were investigated via multi-step Coulomb excitation of a $^{70}$Ge beam impinging on a $^{208}$Pb target at the ATLAS facility of the Argonne National Laboratory. A total of 27 transitional elements and six diagonal matrix elements coupling 11 low-lying states, were extracted from the measured cross sections. These were used to calculate reduced transition probabilities, spectroscopic quadrupole moments, and rotational invariant shape parameters, providing enhanced precision and expanding on previous studies. The experimental data were compared within several theoretical frameworks, including the generalized triaxial rotor model, configuration interaction shell-model calculations, and computations within the combined frameworks of relativistic density functional theory and the five-dimensional collective Hamiltonian. The results demonstrate a good agreement with the experimental data and, in conjunction with calculations using a two-state mixing model, support significant triaxiality and strong mixing between the $0^+_1$ and $0^+_2$ states. This results in the magnitudes of their respective quadrupole deformations $[β_\text{rms}(0^+_1) = 0.228\,(3),\,β_\text{rms}(0^+_2) = 0.273\,(1)]$ being more similar than previously observed. The implications of these results for understanding the complex shape coexistence phenomena, the role of triaxiality, and shape evolution along the Ge isotopic chain are discussed.

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arXiv2025

High-spin spectroscopy and the onset of quasicollective structures in $^{69}$Ga

The intermediate- and high-spin level structure of the odd-$A$ $^{69}$Ga nucleus was investigated via the $^{26}$Mg($^{48}$Ca, $p4nγ$) fusion evaporation reaction at a beam energy of 195 MeV. The experiment was performed using the Gammasphere multidetector array in conjunction with the Fragment Mass Analyzer (FMA), with mass and charge identification achieved via an ionization chamber placed at the focal plane of the spectrometer. Coincidence relationships between the $^{69}$Ga reaction products and emitted $γ$ rays were analyzed to establish the level sequences, while angular distribution and angular correlation measurements were used to propose spin and parity assignments. As a result, the level scheme of the nucleus has been considerably extended. Near the ground state, the structure of $^{69}$Ga is well described by single-particle excitations, with shell-model calculations using the JUN45 and jj44b effective interactions providing a satisfactory interpretation of the observed levels. At spins in excess of 21/2 $\hbar$, three sequences of $E2$ transitions have been delineated, suggesting the onset of collectivity. An interpretation within the framework of the tilted-axis-cranking covariant density functional theory is proposed which reveals the role of $g_{9/2}$ protons and neutrons in this angular momentum regime.

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arXiv2025

Deviations from the Porter-Thomas Distribution due to Nonstatistical $γ$ Decay below the $^{150}$Nd Neutron Separation Threshold

We introduce a new method for the study of fluctuations of partial transition widths based on nuclear resonance fluorescence experiments with quasimonochromatic linearly polarized photon beams below particle separation thresholds. It is based on the average branching of decays of $J=1$ states of an even-even nucleus to the $2^+_1$ state in comparison to the ground state. Between 5 and 7 MeV, a constant average branching ratio for $γ$ decays from $1^-$ states of 0.490(16) is observed for the nuclide $^{150}$Nd. Assuming $χ^2$-distributed partial transition widths, this average branching ratio is related to a degree of freedom of $ν= 1.93(12)$, rejecting the validity of the Porter-Thomas distribution, requiring $ν=1$. The observed deviation can be explained by nonstatistical effects in the $γ$-decay behavior with contributions in the range of 9.4(10)% up to 94(10)%.

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arXiv2025

Gamma decay of the $^{154}$Sm Isovector Giant Dipole Resonance: Smekal-Raman Scattering as a Novel Probe of Nuclear Ground-State Deformation

Gamma decays of the isovector giant dipole resonance (GDR) of the deformed nucleus $^{154}$Sm from $2^+_1$-Smekal-Raman and elastic scattering were measured using linearly polarized, quasimonochromatic photon beams. The two scattering processes were disentangled through their distinct angular distributions. Their branching ratio and cross sections were determined at six excitation energies covering the $^{154}$Sm GDR. Both agree with the predictions of the geometrical model for the GDR and establish $γ$ decay as an observable sensitive to the structure of the resonance. Consequently, the data place strong constraints on the nuclear shape, including the degree of triaxiality. The derived $^{154}$Sm shape parameters $β=0.2926(26)$ and $γ=5.0(14)$ agree well with other measurements and recent Monte Carlo Shell-Model calculations.

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arXiv2024

Photo-nuclear cross sections on $^{197}$Au, an update on the gold standard

A method was developed for measuring photonuclear reactions concurrently at several discrete photon beam energies on a stack of different target materials via a single irradiation. Concentric ring targets of the materials (in order from front to back targets: Au, TiO$_2$, Zn, Os, and Au) were irradiated at the High Intensity Gamma-ray Source (HI$γ$S). As a proof of principle, we report the result of the cross section measurements from the front Au target. The excitation functions of the $^{197}$Au($γ$,n)$^{196}$Au and $^{197}$Au($γ$,3n)$^{194}$Au reactions were determined in the incident photon energy range of 13-31 MeV using quasi-monoenergetic photon beams provided at HI$γ$S. The cross sections of the combined ground state (2$^{-}$) and short-lived first isomeric state (m1, 5$^{+}$), and of the second isomeric state (m2, 12$^{-}$) in the $^{196}$Au production are obtained separately by subtracting the $γ$ rays from the internal conversion of the second isomeric state. The excitation function of the second isomeric state via the photon-induced reaction $^{197}$Au($γ$,n)$^{196m2}$Au was measured for the first time. By using the activation method rather than direct neutron counting, the exclusive cross sections for the ($γ$,n) and ($γ$,3n) reactions were determined. Comparing the yields from the front and back gold targets validates our ability to simulate the effect of photon scattering in the target stack and provides a method for assessing the systematic uncertainty of our technique.

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arXiv2024

Determination of the spins and parities for the 0$_{4}^{+}$ and 0$_{5}^{+}$ states in $^{100}$Zr

Two 0$^{+}$ states at 1294.5 and 1774.0 keV, together with three 2$^{+}$ and one 4$^{+}$ levels, were identified or unambiguously spin-parity assigned for the first time in $^{100}$Zr utilizing $γ$-ray spectroscopy and $γ$-$γ$ angular correlation techniques with the Gammasphere spectrometer, following the $β^{-}$ decay of neutron-rich, mass separated $^{100,100m}$Y isotopes. Comparisons with recent Monte Carlo Shell-Model (MCSM) calculations indicate that these two states are candidates for the bandhead of a sequence in a shape-coexisting spherical minimum predicted to be located around $\approx$1500 keV. According to the measured relative B(E2)$_{relative}$ transition probabilities, the 0$_{5}^{+}$ state exhibits decay properties which more closely align with those predicted for a spherical shape, while the 0$_{4}^{+}$ level is suggested to be associated with a weakly-deformed shape similar to one related to the 0$_{2}^{+}$ state.

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arXiv2022

Model-independent determination of the dipole response of $^{66}$Zn using quasi-monoenergetic and linearly-polarized photon beams

[Background] Photon strength functions are an important ingredient in calculations relevant for the nucleosynthesis of heavy elements. The relation to the photoabsorption cross section allows to experimentally constrain photon strength functions by investigating the photo-response of atomic nuclei. [Purpose] We determine the photoresponse of $^{66}$Zn in the energy region of 5.6 MeV to 9.9 MeV and analyze the contribution of the "elastic" decay channel back to the ground state. In addition, for the elastic channel electric and magnetic dipole transitions were separated. [Methods] Nuclear resonance fluorescence experiments were performed using a linearly-polarized quasi-monoenergetic photon beam at the High Intensity $γ$-ray Source. Photon beam energies from 5.6 to 9.9 MeV with an energy spread of about 3% were selected in steps of 200-300 keV. Two High Purity Germanium detectors were used for the subsequent $γ$-ray spectroscopy. [Results] Full photoabsorption cross sections are extracted from the data making use of the monoenergetic character of the photon beam. For the ground-state decay channel, the average contribution of electric and magnetic dipole strengths is disentangled. The average branching ratio back to the ground state is determined as well. [Conclusions] The new results indicate lower cross sections when compared to the values extracted from a former experiment using bremsstrahlung on $^{66}$Zn. In the latter, the average branching ratio to the ground state is estimated from statistical-model calculations in order to analyze the data. Corresponding estimates from statistical-model calculations underestimate this branching ratio compared to the values extracted from the present analysis, which would partly explain the high cross sections determined from the bremsstrahlung data.

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arXiv2022

E2 Rotational Invariants of $0^+_1$ and $2^+_1$ states for $^{106}$Cd: the Emergence of Collective Rotation

The collective structure of $^{106}$Cd is elucidated by multi-step Coulomb excitation of a 3.849 MeV/$A$ beam of $^{106}$Cd on a 1.1 mg/cm$^2$ $^{208}$Pb target using GRETINA-CHICO2 at ATLAS. Fourteen $E2$ matrix elements were obtained. The nucleus $^{106}$Cd is a prime example of emergent collectivity that possesses a simple structure: it is free of complexity caused by shape coexistence and has a small, but collectively active number of valence nucleons. This work follows in a long and currently active quest to answer the fundamental question of the origin of nuclear collectivity and deformation, notably in the cadmium isotopes. The results are discussed in terms of phenomenological models, the shell model, and Kumar-Cline sums of $E2$ matrix elements. The ${\langle 0_2^+ ||E2||2_1^+ \rangle}$ matrix element is determined for the first time, providing a total, converged measure of the electric quadrupole strength, $\langle Q^2 \rangle$, of the first-excited $2_1^+$ level relative to the $0_1^+$ ground state, which does not show an increase as expected of harmonic and anharmonic vibrations. Strong evidence for triaxial shapes in weakly collective nuclei is indicated; collective vibrations are excluded. This is contrary to the only other cadmium result of this kind in $^{114}$Cd by C. Fahlander et al., Nucl. Phys. A485, 327 (1988), which is complicated by low-lying shape coexistence near midshell.

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arXiv2022

The Core of $^{25}$F studied by the $^{25}$F(-1p)$^{24}$O reaction

The $^{25}$F($5/2^+) (-1p) ^{24}$O reaction was studied at the NSCL using the S800 spectrometer. The experimental spectroscopic factor for the ground-state to ground-state transition indicates a substantial depletion of the proton $d_{5/2}$ strength compared to shell-model expectations. Our result supports the findings reported by Tang \textit{et al.}, from their study of the $(p,2p)$ reaction at RIBF. The overlap between the $^{25}$F and $^{24}$O ground-states is considerably less than anticipated if $^{24}$O acted as a robust and rigid doubly-magic core in $^{25}$F. We interpret the results within the framework of the Particle-Vibration Coupling (PVC) of a $d_{5/2}$ proton coupled to a quadrupole phonon of an effective core. This approach provides a good description of the experimental data by requiring an effective $^{24}$O* core with a phonon energy of $\hbarω_2$= 3.2 MeV, and a $B(E2) ~ 2.7$ W.u., softer and more collective than a bare $^{24}$O. Both the Nilsson deformed mean field and the PVC models appear to capture the properties of the effective core of $^{25}$F, suggesting that the additional proton tends to polarize the free, doubly magic $^{24}$O in such a way that it becomes either slightly deformed or a quadrupole vibrator.

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arXiv2022

Investigation of $^{11}$B and $^{40}$Ca levels at 8-9 MeV by Nuclear Resonance Fluorescence

We report on the measurement of $^{11}$B and $^{40}$Ca levels between excitation energies of 8 and 9 MeV using nuclear resonance fluorescence (NRF). The experiment was carried out with nearly-monoenergetic and linearly polarized photon beams provided by the High-Intensity $γ$-ray Source (HI$γ$S) facility at the Triangle Universities Nuclear Laboratory (TUNL). States in $^{11}$B are important for calibrations of NRF measurements, while the properties of $^{40}$Ca levels impact potassium nucleosynthesis in globular clusters. For $^{40}$Ca, we report on improved excitation energies and an unambiguous $2^-$ assignment for the state at 8425 keV. For $^{11}$B, we obtained improved values for $γ$-ray multipolarity mixing ratios and branching ratios of the 8920 keV level.

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arXiv2022

Emergence of an island of extreme nuclear isomerism at high excitation near $^{208}$Pb

Metastable states with T$_{1/2}$ = 8(2) ms in $^{205}$Bi and T$_{1/2}$ = 0.22(2) ms in $^{204}$Pb, with $\approx $ 8 MeV excitation energy and angular momentum $\ge $ 22 $\hbar $, have been established. These represent, by up to two orders of magnitude, the longest-lived nuclear states above an excitation energy of 7 MeV, ever identified in the nuclear chart. Additionally, the half-life of the 10.17 MeV state in $^{206}$Bi has been determined to be 0.027(2) ms, the next highest value in this highly excited regime. These observations indicate the emergence of an island of extreme nuclear isomerism arising from core-excited configurations at high excitation in the vicinity of the doubly closed-shell nucleus $^{208}$Pb. These results are expected to provide discriminating tests of the effective interactions used in current large-scale shell-model calculations.

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arXiv2021

Shapes, Softness and Non-Yrast Collectivity in 186W

Non-yrast, excited states in neutron-rich $^{186}$W were populated via inelastic-scattering reactions using beams of $^{136}$Xe nuclei accelerated to 725 and 800 MeV. Levels populated in the reactions were investigated via particle-$ γ$ coincidence techniques using the Gammasphere array of High-Purity Germanium detectors and the compact heavy-ion counter, CHICO2. The $ K^π = 2 ^{+} $ ($γ$), $ K^π = 0^{+}$ and $ K^π = 2^{-} $ (octupole) rotational side bands were extended to spins $ 14\hbar $, $ 12\hbar $, and $ 13\hbar $, respectively. A staggering pattern observed in the energies of levels in the $ K^π = 2^{+} $ band was found to be consistent with a potential that gets softer to vibration in the $ γ$ degree of freedom with increasing spin. The odd-even staggering of states in the $ K^π = 2^{-}$ band was found to exhibit a phase opposite to that seen in the $ γ$ band; an effect most probably associated with Coriolis coupling to other, unobserved octupole vibrational bands in $^{186}$W.

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arXiv2021

Isomers in 203Tl and core excitations built on a five-nucleon-hole structure

Isomers with three- and five-nucleon-hole configurations have been established in $^{203}$Tl. These include newly identified levels with a three-nucleon structure: {\it I}$^{π}$ = (15/2$^{-}$) with {\it T}$_{1/2}$ = 7.9(5) ns, and {\it I}$^{π}$ = (35/2$^{-}$) with {\it T}$_{1/2}$ = 4.0(5) ns. In addition, five-quasiparticle states: {\it I}$^{π}$ = (39/2$^{-}$) with {\it T}$_{1/2}$ = 1.9(2) ns, and {\it I}$^{π}$ = (49/2$^{+}$) with {\it T}$_{1/2}$ = 3.4(4) ns have also been established. The previously determined long-lived decay [{\it T}$_{1/2}$ = 6.6(3) $μ$s from this work] is associated with isomerism of the {\it I}$^{π}$ = (29/2$^{+}$) state. Levels above this long-lived isomer have been identified through a delayed-prompt coincidence measurement. Five-nucleon-hole states with excitation energies {\it E}$_{x}$ $\approx $ 7 MeV have been established as well as possible octupole excitations of the $^{208}$Pb core built on these levels. The level scheme of $^{203}$Tl is extended up to {\it E}$_{x}$ $\approx $ 11 MeV with the inclusion of 25 new transitions. Empirical and shell-model calculations have been performed to aid in the description of the observed states which are found to be predominantly of intrinsic character.

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arXiv2021

Ground-state and decay properties of neutron-rich 106Nb

The ground-state properties of neutron-rich 106Nb and its beta decay into 106Mo have been studied using the CARIBU radioactive-ion-beam facility at Argonne National Laboratory. Niobium-106 ions were extracted from a 252Cf fission source and mass separated before being delivered as low-energy beams to the Canadian Penning Trap, as well as the X-Array and SATURN beta-decay-spectroscopy station. The measured 106Nb ground-state mass excess of -66202.0(13) keV is consistent with a recent measurement but has three times better precision; this work also rules out the existence of a second long-lived, beta-decaying state in 106Nb above 5 keV in excitation energy. The decay half-life of 106Nb was measured to be 1.097(21) s, which is 8% longer than the adopted value. The level scheme of the decay progeny, 106Mo, has been expanded up to approximately 4 MeV. The distribution of decay strength and considerable population of excited states in 106Mo of J >= 3 emphasises the need to revise the adopted Jpi = 1- ground-state spin-parity assignment of 106Nb; it is more likely to be J => 3.

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