arXiv subjects

R. Winkler

Publications and source records attributed to R. Winkler.

At least 19 recordsLinked to original sources

arXiv2025

Even-denominator fractional quantum Hall states with spontaneously broken rotational symmetry

The interplay between the fractional quantum Hall effect and nematicity is intriguing as it links emerging topological order and spontaneous symmetry breaking. Anisotropic fractional quantum Hall states (FQHSs) have indeed been reported in GaAs quantum wells but only in tilted magnetic fields, where the in-plane field explicitly breaks the rotational symmetry. Here we report the observation of FQHSs with highly anisotropic longitudinal resistances in purely perpendicular magnetic fields at even-denominator Landau level (LL) fillings {\nu} = 5/2 and 7/2 in ultrahigh-quality GaAs two-dimensional hole systems. The coexistence of FQHSs and spontaneous symmetry breaking at half fillings signals the emergence of nematic FQHSs which also likely harbor non-Abelian quasiparticle excitations. By gate tuning the hole density, we observe a phase transition from an anisotropic, developing FQHS to an isotropic composite fermion Fermi sea at {\nu} = 7/2. Our calculations suggest that the mixed orbital components in the partially occupied LL play a key role in the competition and interplay between topological and nematic orders.

cond-mat.mes-hall↗

arXiv2025

Gauge-invariant absolute quantification of electric and magnetic multipole densities in crystals

Electric and magnetic multipole densities in crystalline solids, including the familiar electric dipole density in ferroelectrics and the magnetic dipole density in ferromagnets, are of central importance for our understanding of ordered phases in matter. However, determining the magnitude of these quantities has proven to be conceptually and technically difficult. Here we present a universally applicable approach, based on projection operators, that yields gauge-invariant absolute measures for all types of electric and magnetic order in crystals. We demonstrate the utility of the general theory using concrete examples of electric and magnetic multipole order in variants of lonsdaleite and diamond structures. Besides the magnetic dipole density in ferromagnets, we also consider, e.g., the magnetic octupole density in altermagnets. The robust method developed in this work lends itself to be incorporated into the suite of computational materials-science tools. The multipole densities can be used as thermodynamic state variables including Landau order parameters.

cond-mat.mtrl-sci↗

arXiv2025

Time inversion symmetry in the Dirac and Schr\"odinger-Pauli theories

The Schr\"odinger-Pauli theory is generally believed to give a faithful representation of the nonrelativistic and weakly relativistic limit of the Dirac theory. However, the Schr\"odinger-Pauli theory is fundamentally incomplete in its account of broken time inversion symmetry, e.g., in magnetically ordered systems. In the Dirac theory of the electron, magnetic order breaks time inversion symmetry even in the nonrelativistic limit, whereas time inversion symmetry is effectively preserved in the Schr\"odinger-Pauli theory in the absence of spin-orbit coupling. In the Dirac theory, the Berry curvature $1/(2m^2c^2)$ is thus an intrinsic property of nonrelativistic electrons similar to the well-known spin magnetic moment $e\hbar/(2m)$, while this result is missed by the nonrelativistic or weakly relativistic Schr\"odinger-Pauli equation. In ferromagnetically ordered systems, the intrinsic Berry curvature yields a contribution to the anomalous Hall conductivity independent of spin-orbit coupling.

cond-mat.mtrl-sci↗

arXiv2025

Competing Many-Body Phases at Small Fillings in Ultrahigh-Quality GaAs 2D Hole Systems: Role of Landau Level Mixing

The fractional quantum Hall state (FQHS), an incompressible liquid state hosting anyonic excitations with fractional charge and statistics, represents a compelling many-body phase observed in clean two-dimensional (2D) carrier systems. The expected non-Abelian nature of the FQHSs at even-denominator Landau level (LL) fillings has particularly sparked considerable recent interest. At sufficiently small fillings, another exotic phase, namely a quantum Wigner crystal (WC) state, dominates. Here we report magneto-transport measurements in an ultrahigh-quality GaAs 2D \textit{hole} system where the large hole effective mass leads to a significant LL mixing (LLM) even at very high magnetic fields and affects the many-body states at very small fillings. We observe numerous developing FQHSs at both even- and odd-denominator fillings, deep in the insulating regime at $\nu \lesssim$ 1/3 where WC states dominate. The FQHSs we observe at odd-denominator fillings on the flanks of $\nu=$ 1/4 and 1/6 are consistent with the Abelian Jain sequence of four-flux and six-flux composite fermions, while the ones at even-denominator fillings $\nu=$ 1/4 and 1/6 are likely non-Abelian states emerging from the pairing of these quasiparticles induced by severe LLM. Our results demonstrate that the competition between the FQHSs and WC phases is close at very small fillings even in the presence of severe LLM. We also measure activation energies of WC states near $\nu=$ 1/6, and find that they are substantially larger than what has been reported for ultrahigh-quality GaAs 2D electrons. A moderate LLM is believed to lower the activation energy associated to the formation of WC intrinsic defects. The surprisingly large activation energy for our 2DHS with significant LLM is therefore puzzling, and may suggest a different type of intrinsic WC defect compared to that in 2D electrons.

cond-mat.mes-hall↗

arXiv2024

Standard model of electromagnetism and chirality in crystals

We present a general, quantitative theory of electromagnetism and chirality in crystals. Symmetry is its guiding principle, enabling us to consider macroscopic multipole densities without reference to specific microscopic configurations. We use a formal analogy between space inversion $i$ and time inversion $\theta$ to identify two complementary, comprehensive classifications of crystals, based on five categories of electric and magnetic multipole order---called polarizations---and five categories of chirality. The five categories of polarizations (parapolar, electropolar, magnetopolar, antimagnetopolar, and multipolar) embody the ways in which multipole order can be realized in solids, thus expanding the familiar notion of electric dipolarization in ferroelectrics and magnetization in ferromagnets to higher-rank multipole densities characterizing, e.g., altermagnets and alterelectrics. Group theory also permits the absolute, gauge-invariant quantification of these multipole densities. The five categories of chirality (parachiral, electrochiral, magnetochiral, antimagnetochiral, and multichiral) extend the notion of enantiomorphism---conventionally associated with the lack of spatial mirror symmetries---to include all possibilities for creating non-superposable images by applying the inversions $i$, $\theta$, and $i\theta$. In particular, multichiral systems lack all inversion symmetries and thus have four different enantiomorphs. Each category of chirality arises from particular superpositions of electric and magnetic multipole densities. Our theory has great predictive power by relating electric and magnetic multipolar order with, e.g., distinctive features in the crystal structure, the electronic band structure, and property tensors of quantum materials. These findings are critical for a large community working on fundamental and applied aspects of novel quantum materials.

cond-mat.mtrl-sci↗

arXiv2024

Origin of pinning disorder in magnetic-field-induced Wigner solids

At low Landau level filling factors ($ν$), Wigner solid phases of two-dimensional electron systems in GaAs are pinned by disorder, and exhibit a pinning mode, whose frequency is a measure of the disorder that pins the Wigner solid. Despite numerous studies spanning the last three decades, the origin of the disorder that causes the pinning and determines the pinning mode frequency remains unknown. Here we present a study of the pinning mode resonance in the low-$ν$ Wigner solid phases of a series of ultralow-disorder GaAs quantum wells which are similar except for their varying well widths, $d$. The pinning mode frequencies,$f_p$, decrease strongly as $d$ increases, with the widest well exhibiting $f_p$ as low as $\simeq$35 MHz. The amount of reduction of \fp\ with increasing $d$ can be explained remarkably well by tails of the wave function impinging into the alloy-disordered Al$_x$Ga$_{1-x}$As barriers that contain the electrons. However, it is imperative that the model for the confinement and wave function includes the Coulomb repulsion in the growth direction between the electrons as they occupy the quantum well.

cond-mat.mes-hall↗

arXiv2023

Ultraclean two-dimensional hole systems with mobilities exceeding 10$^7$ cm$^2$/Vs

Owing to their large effective mass, strong and tunable spin-orbit coupling, and complex band-structure, two-dimensional hole systems (2DHSs) in GaAs quantum wells provide rich platforms to probe exotic many-body physics, while also offering potential applications in ballistic and spintronics devices, and fault-tolerant topological quantum computing. We present here a systematic study of molecular-beam-epitaxy grown, modulation-doped, GaAs (001) 2DHSs where we explore the limits of low-temperature 2DHS mobility by optimizing two parameters, the GaAs quantum well width and the alloy fraction ($x$) of the flanking Al$_x$Ga$_{1-x}$As barriers. We obtain a breakthrough in 2DHS mobility, with a peak value $\simeq 18 \times 10^6$ cm$^2$/Vs at a density of 3.8 $\times$ 10$^{10}$ /cm$^{2}$, implying a mean-free-path of $\simeq 57 μ$m. Using transport calculations tailored to our structures, we analyze the operating scattering mechanisms to explain the non-monotonic evolution of mobility with density. We find it imperative to include the dependence of effective mass on 2DHS density, well width, and $x$. We observe concomitant improvement in quality as evinced by the appearance of delicate fractional quantum Hall states at very low density.

cond-mat.mes-hall↗

arXiv2023

Fractional Quantum Hall State at Filling Factor $ν=1/4$ in Ultra-High-Quality GaAs 2D Hole Systems

Single-component fractional quantum Hall states (FQHSs) at even-denominator filling factors may host non-Abelian quasiparticles that are considered to be building blocks of topological quantum computers. Such states, however, are rarely observed in the lowest-energy Landau level, namely at filling factors $ν<1$. Here we report evidence for an even-denominator FQHS at $ν=1/4$ in ultra-high-quality two-dimensional hole systems confined to modulation-doped GaAs quantum wells. We observe a deep minimum in the longitudinal resistance at $ν=1/4$, superimposed on a highly insulating background, suggesting a close competition between the $ν=1/4$ FQHS and the magnetic-field-induced, pinned Wigner solid states. Our experimental observations are consistent with the very recent theoretical calculations which predict that substantial Landau level mixing, caused by the large hole effective mass, can induce composite fermion pairing and lead to a non-Abelian FQHS at $ν=1/4$. Our results demonstrate that Landau level mixing can provide a very potent means for tuning the interaction between composite fermions and creating new non-Abelian FQHSs.

cond-mat.mes-hall↗

arXiv2023

Highly-Anisotropic Even-Denominator Fractional Quantum Hall State in an Orbitally-Coupled Half-Filled Landau Level

The even-denominator fractional quantum Hall states (FQHSs) in half-filled Landau levels are generally believed to host non-Abelian quasiparticles and be of potential use in topological quantum computing. Of particular interest is the competition and interplay between the even-denominator FQHSs and other ground states, such as anisotropic phases and composite fermion Fermi seas. Here we report the observation of an even-denominator fractional quantum Hall state with highly-anisotropic in-plane transport coefficients at Landau level filling factor $ν=3/2$. We observe this state in an ultra-high-quality GaAs two-dimensional hole system when a large in-plane magnetic field is applied. By increasing the in-plane field, we observe a sharp transition from an isotropic composite fermion Fermi sea to an anisotropic even-denominator FQHS. Our data and calculations suggest that a unique feature of two-dimensional holes, namely the coupling between heavy-hole and light-hole states, combines different orbital components in the wavefunction of one Landau level, and leads to the emergence of a highly-anisotropic even-denominator fractional quantum Hall state. Our results demonstrate that the GaAs two-dimensional hole system is a unique platform for the exploration of exotic, many-body ground states.

cond-mat.mes-hall↗

arXiv2023

Coherent control of orbital wavefunctions in the quantum spin liquid $Tb_{2}Ti_{2}O_{7}$

Resonant driving of electronic transitions with coherent laser sources creates quantum coherent superpositions of the involved electronic states. Most time-resolved studies have focused on gases or isolated subsystems embedded in insulating solids, aiming for applications in quantum information. Here, we demonstrate coherent control of orbital wavefunctions in pyrochlore $Tb_{2}Ti_{2}O_{7}$, which forms an interacting spin liquid ground state. We show that resonant excitation with a strong THz pulse creates a coherent superposition of the lowest energy Tb 4f states before the magnetic interactions eventually dephase them. The coherence manifests itself as a macroscopic oscillating magnetic dipole, which is detected by ultrafast resonant x-ray diffraction. The induced quantum coherence demonstrates coherent control of orbital wave functions, a new tool for the ultrafast manipulation and investigation of quantum materials.

cond-mat.str-el↗

arXiv2023

Theory of electric, magnetic, and toroidal polarizations in crystalline solids with applications to hexagonal lonsdaleite and cubic diamond

Multipolar order in bulk crystalline solids is characterized by multipole densities -- denoted as polarizations in this work -- that cannot be cleanly defined using the concepts of classical electromagnetism. Here we use group theory to overcome this difficulty and present a systematic study of electric, magnetic and toroidal multipolar order in crystalline solids. Based on our symmetry analysis, we identify five categories of polarized matter, each of which is characterized by distinct features in the electronic band structure. For example, Rashba spin splitting in electropolar bulk materials like wurtzite represents the electric dipolarization in these materials. We also develop a general formalism of indicators for individual multipole densities that provide a physical interpretation and quantification of multipolar order. Our work clarifies the relation between patterns of localized multipoles and macroscopic multipole densities they give rise to. To illustrate the general theory, we discuss its application to polarized variants of hexagonal lonsdaleite and cubic diamond structures. Our work provides a general framework for classifying and expanding current understanding of multipolar order in complex materials.

cond-mat.mtrl-sci↗

arXiv2023

Valley-tunable, even-denominator fractional quantum Hall state in the lowest Landau level of an anisotropic system

Fractional quantum Hall states (FQHSs) at even-denominator Landau level filling factors ($ν$) are of prime interest as they are predicted to host exotic, topological states of matter. We report here the observation of a FQHS at $ν=1/2$ in a two-dimensional electron system of exceptionally high quality, confined to a wide AlAs quantum well, where the electrons can occupy multiple conduction-band valleys with an anisotropic effective mass. The anisotropy and multi-valley degree of freedom offer an unprecedented tunability of the $ν=1/2$ FQHS as we can control both the valley occupancy via the application of in-plane strain, and the ratio between the strengths of the short- and long-range Coulomb interaction by tilting the sample in the magnetic field to change the electron charge distribution. Thanks to this tunability, we observe phase transitions from a compressible Fermi liquid to an incompressible FQHS and then to an insulating phase as a function of tilt angle. We find that this evolution and the energy gap of the $ν=1/2$ FQHS depend strongly on valley occupancy.

cond-mat.mes-hall↗

arXiv2022

Fractional quantum Hall valley ferromagnetism in the extreme quantum limit

Electrons' multiple quantum degrees of freedom can lead to rich physics, including a competition between various exotic ground states, as well as novel applications such as spintronics and valleytronics. Here we report magneto-transport experiments demonstrating how the valley degree of freedom impacts the fractional quantum states (FQHSs), and the related magnetic-flux-electron composite fermions (CFs), at very high magnetic fields in the extreme quantum limit when only the lowest Landau level is occupied. Unlike in other multivalley two-dimensional electron systems such as Si or monolayer graphene and transition-metal dichalcogenides, in our AlAs sample we can continuously tune the valley polarization via the application of in-situ strain. We find that the FQHSs remain exceptionally strong even as they make valley polarization transitions, revealing a surprisingly robust ferromagnetism of the FQHSs and the underlying CFs. Our observation implies that the CFs are strongly interacting in our system. We are also able to obtain a phase diagram for the FQHS and CF valley polarization in the extreme quantum limit as we monitor transitions of the FHQSs with different valley polarizations.

cond-mat.mes-hall↗

arXiv2022

Robust Quantum Hall Ferromagnetism near a Gate-Tuned ν = 1 Landau Level Crossing

In a low-disorder two-dimensional electron system, when two Landau levels of opposite spin or pseudospin cross at the Fermi level, the dominance of the exchange energy can lead to a ferromagnetic, quantum Hall ground state whose gap is determined by the exchange energy and has skyrmions as its excitations. This is normally achieved via applying either hydrostatic pressure or uniaxial strain. We study here a very high-quality, low-density, two-dimensional hole system, confined to a 30-nm-wide (001) GaAs quantum well, in which the two lowest-energy Landau levels can be gate tuned to cross at and near filling factor $ν=1$. As we tune the field position of the crossing from one side of $ν=1$ to the other by changing the hole density, the energy gap for the quantum Hall state at $ν=1$ remains exceptionally large, and only shows a small dip near the crossing. The gap overall follows a $\sqrt{B}$ dependence, expected for the exchange energy. Our data are consistent with a robust quantum Hall ferromagnet as the ground state.

cond-mat.mes-hall↗

arXiv2022

Even-Denominator Fractional Quantum Hall State at Filling Factor ν = 3/4

Fractional quantum Hall states (FQHSs) exemplify exotic phases of low-disorder two-dimensional (2D) electron systems when electron-electron interaction dominates over the thermal and kinetic energies. Particularly intriguing among the FQHSs are those observed at even-denominator Landau level filling factors, as their quasi-particles are generally believed to obey non-Abelian statistics and be of potential use in topological quantum computing. Such states, however, are very rare and fragile, and are typically observed in the excited Landau level of 2D electron systems with the lowest amount of disorder. Here we report the observation of a new and unexpected even-denominator FQHS at filling factor ν = 3/4 in a GaAs 2D hole system with an exceptionally high quality (mobility). Our magneto-transport measurements reveal a strong minimum in the longitudinal resistance at ν = 3/4, accompanied by a developing Hall plateau centered at (h/e2)/(3/4). This even-denominator FQHS is very unusual as it is observed in the lowest Landau level and in a 2D hole system. While its origin is unclear, it is likely a non-Abelian state, emerging from the residual interaction between composite fermions.

cond-mat.mes-hall↗

arXiv2022

Record-quality GaAs two-dimensional hole systems

The complex band structure, large spin-orbit induced band splitting, and heavy effective mass of two-dimensional (2D) hole systems hosted in GaAs quantum wells render them rich platforms to study many-body physics and ballistic transport phenomena. Here we report ultra-high-quality (001) GaAs 2D hole systems, fabricated using molecular beam epitaxy and modulation doping, with mobility values as high as $5.8\times10^6$ cm$^2$/Vs at a hole density of $p=1.3\times10^{11}$ /cm$^2$, implying a mean-free path of $\simeq27$ $μ$m. In the low-temperature magnetoresistance trace of this sample, we observe high-order fractional quantum Hall states up to the Landau level filling $ν=12/25$ near $ν=1/2$. Furthermore, we see a deep minimum develop at $ν=1/5$ in the magnetoresistance of a sample with a much lower hole density of $p=4.0\times10^{10}$ /cm$^2$ where we measure a mobility of $3.6\times10^6$ cm$^2$/Vs. These improvements in sample quality were achieved by reduction of residual impurities both in the GaAs channel and the AlGaAs barrier material, as well as optimization in design of the sample structure.

cond-mat.mes-hall↗

arXiv2020

Thermal and quantum melting phase diagrams for a magnetic-field-induced Wigner solid

A sufficiently large perpendicular magnetic field quenches the kinetic (Fermi) energy of an interacting two-dimensional (2D) system of fermions, making them susceptible to the formation of a Wigner solid (WS) phase in which the charged carriers organize themselves in a periodic array in order to minimize their Coulomb repulsion energy. In low-disorder 2D electron systems confined to modulation-doped GaAs heterostructures, signatures of a magnetic-field-induced WS appear at low temperatures and very small Landau level filling factors ($ν\simeq1/5$). In dilute GaAs 2D \textit{hole} systems, on the other hand, thanks to the larger hole effective mass and the ensuing Landau level mixing, the WS forms at relatively higher fillings ($ν\simeq1/3$). Here we report our measurements of the fundamental temperature vs. filling phase diagram for the 2D holes' WS-liquid \textit{thermal melting}. Moreover, via changing the 2D hole density, we also probe their Landau level mixing vs. filling WS-liquid \textit{quantum melting} phase diagram. We find our data to be in good agreement with the results of very recent calculations, although intriguing subtleties remain.

cond-mat.mes-hall↗

arXiv2020

Collinear Orbital Antiferromagnetic Order and Magnetoelectricity in Quasi-2D Itinerant-Electron Paramagnets, Ferromagnets and Antiferromagnets

We develop a comprehensive theory for magnetoelectricity in magnetically ordered quasi-2D systems whereby in thermal equilibrium an electric field can induce a magnetization $m$ and a magnetic field can induce a polarization. This effect requires that both space-inversion and time-reversal symmetry are broken. Antiferromagnetic (AFM) order plays a central role in this theory. We define a Néel operator $τ$ such that a nonzero expectation value $\langle τ\rangle$ signals AFM order, in the same way $m$ signals ferromagnetic (FM) order. While $m$ is even under space inversion and odd under time reversal, $τ$ describes a toroidal moment that is odd under both symmetries. Thus $m$ and $\langle τ\rangle$ quantify complementary aspects of magnetic order in solids. In quasi-2D systems FM order can be attributed to dipolar equilibrium currents that give rise to $m$. In the same way, AFM order arises from quadrupolar currents that generate the moment $\langle τ\rangle$. The electric-field-induced magnetization can then be attributed to the electric manipulation of the quadrupolar currents. We develop a $k \cdot p$ envelope-function theory for AFM diamond structures that allows us to derive explicit expressions for the operator $τ$. Considering FM zincblende and AFM diamond, we derive quantitative expressions for the magnetoelectric responses due to electric and magnetic fields that reveal explicitly the inherent duality of these responses required by thermodynamics. Magnetoelectricity is found to be small in realistic calculations for quasi-2D electron systems. The magnetoelectric response of quasi-2D hole systems turns out to be sizable, however, with moderate electric fields being able to induce a magnetic moment of one Bohr magneton per charge carrier. Our theory provides a broad framework for the manipulation of magnetic order by means of external fields.

cond-mat.mes-hall↗